The problem of bound polarons in quantum dot quantum well (QDQW) structures is studied theoretically. The eigenfrequencies of bulk longitudinal optical (LO) and surface optical (SO) modes are derived in the fram...The problem of bound polarons in quantum dot quantum well (QDQW) structures is studied theoretically. The eigenfrequencies of bulk longitudinal optical (LO) and surface optical (SO) modes are derived in the framework of the dielectric continuum approximation. The electron-phonon interaction Hamiltonian for QDQW structures is obtained and the exchange interaction between impurity and LO-phonons is discussed. The binding energy and the trapping energy of the bound polaron in CdS/HgS QDQW structures are calculated. The numerical results reveal that there exist three branches of eigenfrequencies of surface optical vibration in the CdS/HgS QDQW structure. It is also shown that the binding energy and the trapping energy increase as the inner radius of the QDQW structure decreases, with the outer radius fixed, and the trapping energy takes a major part of the binding energy when the inner radius is very small.展开更多
We investigated the properties of polarons in a wurtzite ZnO/MgxZn1-xO quantum well by adopting a modified Lee–Low–Pines variational method, giving the ground state energy, transition energy, and phonon contribution...We investigated the properties of polarons in a wurtzite ZnO/MgxZn1-xO quantum well by adopting a modified Lee–Low–Pines variational method, giving the ground state energy, transition energy, and phonon contributions from various optical-phonon modes to the ground state energy as functions of the well width and Mg composition. In our calculations, we considered the effects of confined optical phonon modes, interface-optical phonon modes, and half-space phonon modes, as well as the anisotropy of the electron effective band mass, phonon frequency, and dielectric constant. Our numerical results indicate that the electron–optical phonon interactions importantly affect the polaronic energies in the ZnO/MgxZn1-xO quantum well. The electron–optical phonon interactions decrease the polaron energies. For quantum wells with narrower wells, the interface optical phonon and half-space phonon modes contribute more to the polaronic energies than the confined phonon modes. However, for wider quantum wells, the total contribution to the polaronic energy mainly comes from the confined modes. The contributions of the various phonon modes to the transition energy change differently with increasing well width. The contribution of the half-space phonons decreases slowly as the QW width increases, whereas the contributions of the confined and interface phonons reach a maximum at d ≈ 5.0 nm and then decrease slowly. However,the total contribution of phonon modes to the transition energy is negative and increases gradually with the QW width of d.As the composition x increases, the total contribution of phonons to the ground state energies increases slowly, but the total contributions of phonons to the transition energies decrease gradually. We analyze the physical reasons for these behaviors in detail.展开更多
The vibrational frequency(VF), the ground state(GS) energy and the GS binding energy of the weak electron-phonon coupling polaron in a quantum well(QW) with asymmetrical Gaussian confinement potential are calculated. ...The vibrational frequency(VF), the ground state(GS) energy and the GS binding energy of the weak electron-phonon coupling polaron in a quantum well(QW) with asymmetrical Gaussian confinement potential are calculated. First we introduce the linear combination operator to express the momentum and coordinates in the Hamilton and then operate the system Hamilton using unitary transformation. The results indicate the relations of the quantities(the VF, the absolute value of GS energy and the GS binding energy) and the parameters(the QW barrier height and the range of Gaussian confinement potential in the growth direction of the QW).展开更多
With hydrogen-like impurity(HLI) located in the center of Cs I quantum pseudodot(QPD) and by using the variational method of Pekar type(VMPT), we investigate the first-excited state energy(FESE), excitation en...With hydrogen-like impurity(HLI) located in the center of Cs I quantum pseudodot(QPD) and by using the variational method of Pekar type(VMPT), we investigate the first-excited state energy(FESE), excitation energy and transition frequency of the strongly-coupled bound polaron in the present paper. Temperature effects on bound polaron properties are calculated by employing the quantum statistical theory(QST). According to the present work's numerical results, the FESE, excitation energy and transition frequency decay(amplify) with raising temperature in the regime of lower(higher)temperature. They are decreasing functions of Coulomb impurity potential strength.展开更多
The temperature and the size dependences of the self-trapping energy of a polaron in a GaAs parabolic quantum dot are investigated by the second order Rayleigh-Schrodinger perturbation method using the framework of th...The temperature and the size dependences of the self-trapping energy of a polaron in a GaAs parabolic quantum dot are investigated by the second order Rayleigh-Schrodinger perturbation method using the framework of the effective mass approximation. The numerical results show that the self-trapping energies of polaron in GaAs parabolic quantum dots shrink with the enhancement of temperature and the size of the quantum dot. The results also indicate that the temperature effect becomes obvious in small quantum dots展开更多
We study the two-dimensional weak-coupling Frohlich polaron in a completely anisotropic quantum dot in a perpendicular magnetic field. By performing a unitary transformation, we first transform the Hamiltonian into a ...We study the two-dimensional weak-coupling Frohlich polaron in a completely anisotropic quantum dot in a perpendicular magnetic field. By performing a unitary transformation, we first transform the Hamiltonian into a new one which describes an anisotropic harmonic oscillator with new mass and trapping frequencies interacting with the same phonon bath but with different interaction form and strength. Then employing the second-order Rayleigh–Schrodinger perturbation theory, we obtain the polaron correction to the ground-state energy. The magnetic field and anisotropic effects on the polaron correction to the ground-state energy are discussed.展开更多
The properties ofpolarons in zinc-blende and wurtzite GaN/AIN quantum wells with Frohlich interaction Hamiltonians are compared in detail. The energy shifts of polarons at ground state due to the interface (IF), con...The properties ofpolarons in zinc-blende and wurtzite GaN/AIN quantum wells with Frohlich interaction Hamiltonians are compared in detail. The energy shifts of polarons at ground state due to the interface (IF), confined (CO) and half-space phonon modes are calculated by a finite-difference computation combined with a modified LLP variational method. It is found that the two Frohlich interaction Hamiltonians are consistent with each other when the anisotropic effect from the z-direction and the x-y plane is neglected. The influence of the anisotropy on the polaron energy shifts due to the IF phonon modes for a smaller well width or due to the CO phonon modes for a moderate well width is obvious. In addition, the built-in electric field has a remarkable effect on the polaron energy shifts contributed by the various phonon modes.展开更多
: The effects of a magnetic field on the vibrational frequency, the ground state energy and the ground state binding energy of a weak-coupling polaron in asymmetrical Gaussian confinement potential quantum well (AGC...: The effects of a magnetic field on the vibrational frequency, the ground state energy and the ground state binding energy of a weak-coupling polaron in asymmetrical Gaussian confinement potential quantum well (AGCPQW) are investigated by using linear combination operator and unitary transformation methods. Our cal- culated results show that the vibrational frequency increases with increasing cyclotron frequency of the magnetic field; meanwhile, the absolute value of the ground state energy and the ground state binding energy decrease. The vibrational frequency, the absolute value of the ground state energy and the ground state binding energy are in- creasing functions of the barrier height of the AGCPQW. It is shown that the barrier height of the AGCPQW and the magnetic field are important factors that influence the properties of the magnetopolaron in AGCPQW.展开更多
基金supported by Universities Program of Inner Mongol of China(Grant No NJZZ07008)the Natural Science Foundation of Inner Mongol of China(Grant No 200607010105)
文摘The problem of bound polarons in quantum dot quantum well (QDQW) structures is studied theoretically. The eigenfrequencies of bulk longitudinal optical (LO) and surface optical (SO) modes are derived in the framework of the dielectric continuum approximation. The electron-phonon interaction Hamiltonian for QDQW structures is obtained and the exchange interaction between impurity and LO-phonons is discussed. The binding energy and the trapping energy of the bound polaron in CdS/HgS QDQW structures are calculated. The numerical results reveal that there exist three branches of eigenfrequencies of surface optical vibration in the CdS/HgS QDQW structure. It is also shown that the binding energy and the trapping energy increase as the inner radius of the QDQW structure decreases, with the outer radius fixed, and the trapping energy takes a major part of the binding energy when the inner radius is very small.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11264027 and 11364030)the Project of Prairie Excellent Specialist of Inner Mongolia,Chinathe "Thousand,Hundred and Ten" Talent Training Project Foundation of Inner Mongolia Normal University,China(Grant No.RCPY-2-2012-K-039)
文摘We investigated the properties of polarons in a wurtzite ZnO/MgxZn1-xO quantum well by adopting a modified Lee–Low–Pines variational method, giving the ground state energy, transition energy, and phonon contributions from various optical-phonon modes to the ground state energy as functions of the well width and Mg composition. In our calculations, we considered the effects of confined optical phonon modes, interface-optical phonon modes, and half-space phonon modes, as well as the anisotropy of the electron effective band mass, phonon frequency, and dielectric constant. Our numerical results indicate that the electron–optical phonon interactions importantly affect the polaronic energies in the ZnO/MgxZn1-xO quantum well. The electron–optical phonon interactions decrease the polaron energies. For quantum wells with narrower wells, the interface optical phonon and half-space phonon modes contribute more to the polaronic energies than the confined phonon modes. However, for wider quantum wells, the total contribution to the polaronic energy mainly comes from the confined modes. The contributions of the various phonon modes to the transition energy change differently with increasing well width. The contribution of the half-space phonons decreases slowly as the QW width increases, whereas the contributions of the confined and interface phonons reach a maximum at d ≈ 5.0 nm and then decrease slowly. However,the total contribution of phonon modes to the transition energy is negative and increases gradually with the QW width of d.As the composition x increases, the total contribution of phonons to the ground state energies increases slowly, but the total contributions of phonons to the transition energies decrease gradually. We analyze the physical reasons for these behaviors in detail.
基金supported by the National Science Foundation of China(Nos.11464033,11464034)
文摘The vibrational frequency(VF), the ground state(GS) energy and the GS binding energy of the weak electron-phonon coupling polaron in a quantum well(QW) with asymmetrical Gaussian confinement potential are calculated. First we introduce the linear combination operator to express the momentum and coordinates in the Hamilton and then operate the system Hamilton using unitary transformation. The results indicate the relations of the quantities(the VF, the absolute value of GS energy and the GS binding energy) and the parameters(the QW barrier height and the range of Gaussian confinement potential in the growth direction of the QW).
基金Project supported by the National Natural Science Foundation of China(Grant No.11464033)
文摘With hydrogen-like impurity(HLI) located in the center of Cs I quantum pseudodot(QPD) and by using the variational method of Pekar type(VMPT), we investigate the first-excited state energy(FESE), excitation energy and transition frequency of the strongly-coupled bound polaron in the present paper. Temperature effects on bound polaron properties are calculated by employing the quantum statistical theory(QST). According to the present work's numerical results, the FESE, excitation energy and transition frequency decay(amplify) with raising temperature in the regime of lower(higher)temperature. They are decreasing functions of Coulomb impurity potential strength.
文摘The temperature and the size dependences of the self-trapping energy of a polaron in a GaAs parabolic quantum dot are investigated by the second order Rayleigh-Schrodinger perturbation method using the framework of the effective mass approximation. The numerical results show that the self-trapping energies of polaron in GaAs parabolic quantum dots shrink with the enhancement of temperature and the size of the quantum dot. The results also indicate that the temperature effect becomes obvious in small quantum dots
基金Project supported by the National Natural Science Foundation of China(Grant No.11375090)the K.C.Wong Magna Foundation in Ningbo University,China
文摘We study the two-dimensional weak-coupling Frohlich polaron in a completely anisotropic quantum dot in a perpendicular magnetic field. By performing a unitary transformation, we first transform the Hamiltonian into a new one which describes an anisotropic harmonic oscillator with new mass and trapping frequencies interacting with the same phonon bath but with different interaction form and strength. Then employing the second-order Rayleigh–Schrodinger perturbation theory, we obtain the polaron correction to the ground-state energy. The magnetic field and anisotropic effects on the polaron correction to the ground-state energy are discussed.
基金supported by the National Natural Science Foundation of China(No.60966001)the Specialized Research Fund for the Doctoral Program of Higher Education of China(No.20070126001 )+1 种基金the Key Project of Natural Science Foundation of Inner Mongolia Autonomous Region(No.20080404Zd02)the Natural Science Doctoral Foundation of Inner Mongolia Autonomous Region(No.2010BS0102)
文摘The properties ofpolarons in zinc-blende and wurtzite GaN/AIN quantum wells with Frohlich interaction Hamiltonians are compared in detail. The energy shifts of polarons at ground state due to the interface (IF), confined (CO) and half-space phonon modes are calculated by a finite-difference computation combined with a modified LLP variational method. It is found that the two Frohlich interaction Hamiltonians are consistent with each other when the anisotropic effect from the z-direction and the x-y plane is neglected. The influence of the anisotropy on the polaron energy shifts due to the IF phonon modes for a smaller well width or due to the CO phonon modes for a moderate well width is obvious. In addition, the built-in electric field has a remarkable effect on the polaron energy shifts contributed by the various phonon modes.
基金Project supported by the National Natural Science Foundation of China(Nos.11464033,11464034)
文摘: The effects of a magnetic field on the vibrational frequency, the ground state energy and the ground state binding energy of a weak-coupling polaron in asymmetrical Gaussian confinement potential quantum well (AGCPQW) are investigated by using linear combination operator and unitary transformation methods. Our cal- culated results show that the vibrational frequency increases with increasing cyclotron frequency of the magnetic field; meanwhile, the absolute value of the ground state energy and the ground state binding energy decrease. The vibrational frequency, the absolute value of the ground state energy and the ground state binding energy are in- creasing functions of the barrier height of the AGCPQW. It is shown that the barrier height of the AGCPQW and the magnetic field are important factors that influence the properties of the magnetopolaron in AGCPQW.