Positive corona burst pulses are an unstable pulse mode.They appear in a small range of the onset stage,and their current pulses result from the collective movement of charged species.This paper focused on the connect...Positive corona burst pulses are an unstable pulse mode.They appear in a small range of the onset stage,and their current pulses result from the collective movement of charged species.This paper focused on the connections between these pulses and the collective movement of charged species.The movement of species is divided into four parts with respect to time:the(1)initial growth of species,(2)formation and development of the streamer region and negative ion sheath,(3)dead time(the time interval between the pulses),and(4)rapid re-growth of species.The movement of the species in the four parts and the correspondence with the current pulse were analyzed.The numerical results indicated the following:the rapid rising of the species matched the rising edge of the pulses,the streamer region,and negative ion sheath appeared in the falling edge of the primary pulse,and the rapid re-growth of species matched the re-ignition of the pulses.The results were in qualitative agreement with deductions and experimental observations in the literature.展开更多
The emission spectra of excited radicals(OH(A^2E),O(3p^3 P),Hα(3P)) and emissive species(N2^+(B^2∑u^+),N2(C3Πu)) produced by positive pulsed high-voltage needle-plane corona discharges in atmospheri...The emission spectra of excited radicals(OH(A^2E),O(3p^3 P),Hα(3P)) and emissive species(N2^+(B^2∑u^+),N2(C3Πu)) produced by positive pulsed high-voltage needle-plane corona discharges in atmospheric N2 and O2 flows wetted with 10%H2O at 80 ℃ are used to investigate the relative concentrations of the produced radicals.The results indicate that the tendencies of the concentrations of radicals with discharge conditions are similar to each other due to their similar excitation processes by electron collision.The influence of oxygen flow mixed with the nitrogen flow on the emission intensities of O(3p^5P → 3s^5S2^0.),Hα(3P → 2S),N2+(B^2∑u^+ → X^2∑g+0-0),and N2(C^3Πu → B^3Πg 1-0) is presented.When the flow rate of oxygen addition is varied from 0-30 ml min^-1,the emission intensities of O(3p^5P → 3s^5S2^0.),Hα(3P → 2s),and N2^+(B^2∑u^+ →X^2∑g 0-0) increase and reach a maximum.Then,if the oxygen flow rate increases further,the emission intensities tend to decrease.However,the intensity of N2(C^3Πu → B^3Πg1-0) decreases monotonously with the increasing oxygen flow,which indicates that the electron density decreases with the increasing oxygen flow.By the tendencies of the relative intensities to N2(C^3Πu → B^3Πg 1-0),the concentrations of the total produced O,H,and N2^+ are shown to increase with the oxygen flow.Based on the reactions for the production of H and O without and with the addition of O2,the analytic solutions for H and O production are derived in accordance with the experimental results.展开更多
This study investigated the treatment of textile-dyeing wastewater by using an electrical discharge technique (positive pulsed corona discharge). The high-voltage electrode was placed above the surface Of the wastew...This study investigated the treatment of textile-dyeing wastewater by using an electrical discharge technique (positive pulsed corona discharge). The high-voltage electrode was placed above the surface Of the wastewater while the ground electrode was submerged in the wastewater. The electrical discharge starting at the tip of the high voltage electrode propagated toward the surface of the wastewater, producing various oxidative radicals and ozone. Oxygen was used as the working gas instead of air to prevent nitrogen oxides from forming. The simulated wastewater was made up with amaranth, which is a kind of azo dye. The results obtained showed that the chromaticity of the wastewater was almost completely removed within an hour. The ultraviolet/visible spectra of the wastewater treated by the electrical discharge revealed that the total hydrocarbon level also decreased significantly.展开更多
The corona current pulses generated by corona discharge are the sources of the radio interference from transmission lines and the detailed characteristics of the corona current pulses from conductor should be investig...The corona current pulses generated by corona discharge are the sources of the radio interference from transmission lines and the detailed characteristics of the corona current pulses from conductor should be investigated in order to reveal their generation mechanism.In this paper,the line-to-plane electrodes are designed to measure and analyze the characteristics of corona current pulses from positive corona discharges.The influences of inter-electrode gap and line diameters on the detail characteristics of corona current pulses,such as pulse amplitude,rise time,duration time and repetition frequency,are carefully analyzed.The obtained results show that the pulse amplitude and the repetition frequency increase with the diameter of line electrode when the electric fields on the surface of line electrodes are same.With the increase of inter-electrode gap,the pulse amplitude and the repetition frequency first decrease and then turn to be stable,while the rise time first increases and finally turns to be stable.The distributions of electric field and space charges under the line electrodes are calculated,and the influences of inter-electrode gap and line electrode diameter on the experimental results are qualitatively explained.展开更多
基金supported by National Natural Science Foundation of China(No.51907145)。
文摘Positive corona burst pulses are an unstable pulse mode.They appear in a small range of the onset stage,and their current pulses result from the collective movement of charged species.This paper focused on the connections between these pulses and the collective movement of charged species.The movement of species is divided into four parts with respect to time:the(1)initial growth of species,(2)formation and development of the streamer region and negative ion sheath,(3)dead time(the time interval between the pulses),and(4)rapid re-growth of species.The movement of the species in the four parts and the correspondence with the current pulse were analyzed.The numerical results indicated the following:the rapid rising of the species matched the rising edge of the pulses,the streamer region,and negative ion sheath appeared in the falling edge of the primary pulse,and the rapid re-growth of species matched the re-ignition of the pulses.The results were in qualitative agreement with deductions and experimental observations in the literature.
基金supported by National Natural Science Foundation of China under Grant No.513377014
文摘The emission spectra of excited radicals(OH(A^2E),O(3p^3 P),Hα(3P)) and emissive species(N2^+(B^2∑u^+),N2(C3Πu)) produced by positive pulsed high-voltage needle-plane corona discharges in atmospheric N2 and O2 flows wetted with 10%H2O at 80 ℃ are used to investigate the relative concentrations of the produced radicals.The results indicate that the tendencies of the concentrations of radicals with discharge conditions are similar to each other due to their similar excitation processes by electron collision.The influence of oxygen flow mixed with the nitrogen flow on the emission intensities of O(3p^5P → 3s^5S2^0.),Hα(3P → 2S),N2+(B^2∑u^+ → X^2∑g+0-0),and N2(C^3Πu → B^3Πg 1-0) is presented.When the flow rate of oxygen addition is varied from 0-30 ml min^-1,the emission intensities of O(3p^5P → 3s^5S2^0.),Hα(3P → 2s),and N2^+(B^2∑u^+ →X^2∑g 0-0) increase and reach a maximum.Then,if the oxygen flow rate increases further,the emission intensities tend to decrease.However,the intensity of N2(C^3Πu → B^3Πg1-0) decreases monotonously with the increasing oxygen flow,which indicates that the electron density decreases with the increasing oxygen flow.By the tendencies of the relative intensities to N2(C^3Πu → B^3Πg 1-0),the concentrations of the total produced O,H,and N2^+ are shown to increase with the oxygen flow.Based on the reactions for the production of H and O without and with the addition of O2,the analytic solutions for H and O production are derived in accordance with the experimental results.
文摘This study investigated the treatment of textile-dyeing wastewater by using an electrical discharge technique (positive pulsed corona discharge). The high-voltage electrode was placed above the surface Of the wastewater while the ground electrode was submerged in the wastewater. The electrical discharge starting at the tip of the high voltage electrode propagated toward the surface of the wastewater, producing various oxidative radicals and ozone. Oxygen was used as the working gas instead of air to prevent nitrogen oxides from forming. The simulated wastewater was made up with amaranth, which is a kind of azo dye. The results obtained showed that the chromaticity of the wastewater was almost completely removed within an hour. The ultraviolet/visible spectra of the wastewater treated by the electrical discharge revealed that the total hydrocarbon level also decreased significantly.
基金supported by National Natural Science Foundation of China under Grant No.51707066by the Fundamental Research Funds for the Central Universities under Grant No.2017 MS004 and No.XCA17003-04
文摘The corona current pulses generated by corona discharge are the sources of the radio interference from transmission lines and the detailed characteristics of the corona current pulses from conductor should be investigated in order to reveal their generation mechanism.In this paper,the line-to-plane electrodes are designed to measure and analyze the characteristics of corona current pulses from positive corona discharges.The influences of inter-electrode gap and line diameters on the detail characteristics of corona current pulses,such as pulse amplitude,rise time,duration time and repetition frequency,are carefully analyzed.The obtained results show that the pulse amplitude and the repetition frequency increase with the diameter of line electrode when the electric fields on the surface of line electrodes are same.With the increase of inter-electrode gap,the pulse amplitude and the repetition frequency first decrease and then turn to be stable,while the rise time first increases and finally turns to be stable.The distributions of electric field and space charges under the line electrodes are calculated,and the influences of inter-electrode gap and line electrode diameter on the experimental results are qualitatively explained.