The nature of resistive transition of high-quality crystalline thin films of YBa2Cu3O7-δhas been studied under magnetic fields(H) applied along the c direction over a wide range of doped holes, p, in the Cu O2 plan...The nature of resistive transition of high-quality crystalline thin films of YBa2Cu3O7-δhas been studied under magnetic fields(H) applied along the c direction over a wide range of doped holes, p, in the Cu O2 planes. The field- and temperature-dependent in-plane resistivity, ρab(T, H), has been analyzed within the thermally assisted flux-flow(TAFF)formalism. The flux activation energy, U(T, H), has been extracted from this analysis. The low-T part of the ρab(T, H)data can be described by an activation energy having the functional form of U(T, H) =(1- t)m(H-0/H)β, where t = T /Tc(reduced temperature), and H0 is a field scale that primarily determines the magnitude of U(T, H). The temperature exponent, m, shows a systematic variation with p, whereas the field exponent, β, is insensitive to the p values and is close to unity. The H0, on the other hand, changes rapidly as p is varied. U(T, H) is linked to the pinning potential and consequently on the superconducting condensation energy. Since the normal state pseudogap directly affects superconducting condensation energy, a clear correspondence between H0 and the PG energy scale, ε g, is found. Possible implications of these results are discussed.展开更多
This paper deduces that the particular electronic structure of cuprate superconductors confines Cooper pairs to be first formed in the antinodal region which is far from the Fermi surface, and these pairs are incohere...This paper deduces that the particular electronic structure of cuprate superconductors confines Cooper pairs to be first formed in the antinodal region which is far from the Fermi surface, and these pairs are incoherent and result in the pseudogap state. With the change of doping or temperature, some pairs are formed in the nodal region which locates the Fermi surface, and these pairs are coherent and lead to superconductivity. Thus the coexistence of the pseudogap and the superconducting gap is explained when the two kinds of gaps are not all on the Fermi surface. It also shows that the symmetry of the pseudogap and the superconducting gap are determined by the electronic structure, and non-s wave symmetry gap favours the high-temperature superconductivity. Why the high-temperature superconductivity occurs in the metal region near the Mott metal-insulator transition is also explained.展开更多
A mean-field spin-density wave (SDW) analysis of pseudogap in the underdoped cuprates is proposed on the dependence of the energy gap which mimics the pseudogap near (π, 0) point at least. It implies that the pseudog...A mean-field spin-density wave (SDW) analysis of pseudogap in the underdoped cuprates is proposed on the dependence of the energy gap which mimics the pseudogap near (π, 0) point at least. It implies that the pseudogap structure near (π, 0) is not sensitive to the long-range order and will survive leading to the pseudogap phenomenon in the underdoped metallic phase. On the other hand, in the long-range ordering antiferromagnetic region, the mean-field SDW theory holds and the pseudogap structure predicated by the theory should be observable experimentallyv. Then one prediction is that the pseudogap would smoothly extrapolate between itinerant antiferromagnetic phase and underdoped metallic phase.展开更多
The pseudogap state is one of the most enigmatic characteristics in the anomalous normal state properties of the high temperature cuprate superconductors. A central issue is to reveal whether there is a symmetry break...The pseudogap state is one of the most enigmatic characteristics in the anomalous normal state properties of the high temperature cuprate superconductors. A central issue is to reveal whether there is a symmetry breaking and which symmetries are broken across the pseudogap transition. By performing high resolution laser-based angle-resolved photoemission measurements on the optimally-doped Bi_(2)Sr_(1.6)La_(0.4)CuO_(6+δ) superconductor, we report the observations of the particle-hole symmetry conservation in both the superconducting state and the pseudogap state along the entire Fermi surface. These results provide key insights in understanding the nature of the pseudogap and its relation with high temperature superconductivity.展开更多
Unusual quantum phenomena usually emerge upon doping Mott insulators.Using a molecular beam epitaxy system integrated with cryogenic sc√annin√g tunneling microscope,we investigate the electronic structure of a modul...Unusual quantum phenomena usually emerge upon doping Mott insulators.Using a molecular beam epitaxy system integrated with cryogenic sc√annin√g tunneling microscope,we investigate the electronic structure of a modulation-doped Mott insulator Sn/Si(111)-(√3×√3)R30°.In underdoped regions,we observe a universal pseudogap opening around the Fermi level,which changes little with the applied magnetic field and the occurrence of Sn vacancies.The pseudogap gets smeared out at elevated temperatures and alters in size with the spatial confinement of the Mott insulating phase.Our findings,along with the previously observed superconductivity at a higher doping level,are highly reminiscent of the electronic phase diagram in the doped copper oxide compounds.展开更多
We carry out detailed momentum-dependent and temperature-dependent measurements on Bi_2Sr_2CaCu_2O_(8+δ)(Bi2212) superconductor in the superconducting and pseudogap states by super-high resolution laser-based an...We carry out detailed momentum-dependent and temperature-dependent measurements on Bi_2Sr_2CaCu_2O_(8+δ)(Bi2212) superconductor in the superconducting and pseudogap states by super-high resolution laser-based angleresolved photoemission spectroscopy. The precise determination of the superconducting gap for the nearly optimally doped Bi2212(T_c= 91 K) at low temperature indicates that the momentum-dependence of the superconducting gap deviates from the standard d-wave form(cos(2Φ)). It can be alternatively fitted by including a high-order term(cos(6Φ)) in which the next nearest-neighbor interaction is considered. We find that the band structure near the antinodal region smoothly evolves across the pseudogap temperature without a signature of band reorganization which is distinct from that found in Bi_2Sr_2CuO_(6+δ) superconductors. This indicates that the band reorganization across the pseudogap temperature is not a universal behavior in cuprate superconductors.These results provide new insights in understanding the nature of the superconducting gap and pseudogap in high-temperature cuprate superconductors.展开更多
The influence of pseudogap on the inelastic neutron scattering spectra of the underdoped lanthanum cuprate is studied on the basis of the model which incorporates both the superconducting state and pscudogap state.It ...The influence of pseudogap on the inelastic neutron scattering spectra of the underdoped lanthanum cuprate is studied on the basis of the model which incorporates both the superconducting state and pscudogap state.It is found that the striking effects of the influence of the pseudogap on the incommensurability of the spin excitation spectrum are that in the superconducting state the pseudogap makes the intensity of the incommensurate peak increase,in the normal state the pseudogap not only makes the intensity of the incommensurate peak increase,but also sharpens the incommensurate peak and increases incommensurability.展开更多
The pairing and superfluid phenomena in a two-component ultracold atomic Fermi gas is an analogue of Cooper pairing and superconductivity in an electron system, in particular, the high Tc superconductors. Owing to the...The pairing and superfluid phenomena in a two-component ultracold atomic Fermi gas is an analogue of Cooper pairing and superconductivity in an electron system, in particular, the high Tc superconductors. Owing to the various tunable parameters that have been made accessible experimentally in recent years, atomic Fermi gases can be explored as a prototype or quantum sinmlator of superconductors. It is hoped that, utilizing such an analogy, the study of atomic Fermi gases may shed light to the mysteries of high Tc superconductivity. One obstacle to the ultimate understand- ing of high Tc superconductivity, from day one of its discovery, is the anomalous yet widespread pseudogap phenomena, for which a consensus is yet to be reached within the physics comnnmity, after over 27 years of intensive research efforts. In this article, we shall review the progress in the study of pseudogap phenomena in atomic Fermi gases in terms of both theoretical understanding and experimental observations. We show that there is strong, unambiguous evidence for the existence of a pseudogap in strongly interacting Fermi gases. In this context, we shall present a pairing fuctuation theory of the pseudogap physics and show that it is indeed a strong candidate theory for high Tc superconductivity.展开更多
Understanding the nature of the mysterious pseudogap phenomenon is one of the most important issues associated with cuprate high-T_(c) superconductors.Here,we report 17O nuclear magnetic resonance(NMR) studies on two ...Understanding the nature of the mysterious pseudogap phenomenon is one of the most important issues associated with cuprate high-T_(c) superconductors.Here,we report 17O nuclear magnetic resonance(NMR) studies on two planar oxygen sites in stoichio?metric cuprate YBa_(2)Cu_(4)O_(8) to investigate the symmetry breaking inside the pseudogap phase.We observe that the Knight shifts of the two oxygen sites are identical at high temperatures but different below T_(nem) ~185 K,which is close to the pseudogap temperature T^(*).Our result provides a microscopic evidence for intra-unit-cell electronic nematicity.The difference in quadrupole resonance frequency between the two oxygen sites is unchanged below T_(nem),which suggests that the observed nematicity does not directly stem from the local charge density modulation.Furthermore,a short-range charge density wave(CDW) order is observed below T=150 K.The additional broadening in the 17O-NMR spectra because of this CDW order is determined to be inequivalent for the two oxygen sites,which is similar to that observed in case of nematicity.These results suggest a possible connection between nematicity,CDW order,and pseudogap.展开更多
One of important challenges in condensed-matter physics is to realize new quantum states of matter by manipulating the dimensionality of materials,as represented by the discovery of high-temperature superconductivity ...One of important challenges in condensed-matter physics is to realize new quantum states of matter by manipulating the dimensionality of materials,as represented by the discovery of high-temperature superconductivity in atomic-layer pnictides and room-temperature quantum Hall effect in graphene.Tran sition-metal dichalcogenides(TMDs)provide a fertile platform for exploring novel quantum phenomena accompanied by the dimensionality change,since they exhibit a variety of electronic/magnetic states owing to quantum confinement.Here we report an anomalous metal-i nsulator transition in duced by three-dimensional(3D)-two-dimensional(2D)crossover in mono layer 1T-VSe2 grown on bilayer graphene.We observed a complete insulating state with a finite energy gap on the entire Fermi surface in monolayer 1T-VSe2 at low temperatures,in sharp contrast to metallic nature of bulk.More surprisingly,monolayer 1T-VSe2 exhibits a pseudogap with Fermi arc at temperatures above the charge-density-wave temperature,showing a close resemblanee to high-temperature cuprates.This similarity suggests a common underlying physics between two apparently different systems,pointing to the importance of charge/spin fluctuations to create the novel electronic states,such as pseudogap and Fermi arc,in these materials.展开更多
Looking back on the experiments about the normal state of thehigh temperature superconductor (HTS), the authors point out nine important experimental results. On the basis of these results, the authors have argued tha...Looking back on the experiments about the normal state of thehigh temperature superconductor (HTS), the authors point out nine important experimental results. On the basis of these results, the authors have argued that the two-dimension, two-subsystem Hamiltonian is the appropriate starting point for describing the normal state of HTS. By this Hamiltonian, using the decoupling approximation of Green's function method by Kaga through numerical calculations, the authors have obtained the temperature dependent pseudogap in the density of states (DOS), which is consistent qualitatively with the experimental results by angle-resolved photoemission spectroscopy (ARPES). Theoretically, this Hamiltonian has the superconducting order parameter of d+s symmetry with d-wave as the main component, which is consistent with experiments. Further, the quantum electronic liquid in HTS is a near Fermi liquid in which there is coexistence of the delocalized states and nearly localized states, and there is finite probability for the nearly localized carriers to form the nearly localized carrier pairs at any finite temperature.展开更多
Superconducting metal dichalcogenides(MDCs)present several similarities to the other layered SI1-perconductors like cuprates.The superconductivity in atomically thin MDCs has been demonstrated by recent experiments,ho...Superconducting metal dichalcogenides(MDCs)present several similarities to the other layered SI1-perconductors like cuprates.The superconductivity in atomically thin MDCs has been demonstrated by recent experiments,however,the investigation of the superconductivity intertwined with other or-ders are scarce.Investigating the pseudogap in atomic layers of MDCs may help to understand the superconducting mechanism for these true two dimensional(2D)superconducting systemns.Herein we report a pseudogap opening in the tunneling spectra of thin layers of SnSe2 epitaxially grown on highly oriented pyrolytic graphite(HOPG)with scanning tunneling microscopy/spectroscopy(STM/STS).A significant V-shaped pseudogap was observed to open near the Fermi level(Er)in the sTS.And at elevated temperatures,the gap gradually evolves to a shallow dip.Our experimental observations provide direct evidence of a pseudogap state in the electron-doped SnSe2 atomic layers on the HOPG surface,which may stimulate further exploration of the mechanism of superconductivity at 2D limit in MDCs.展开更多
By using scanning tunneling microscopy(STM)/spectroscopy(STS), we systematically characterize the electronic structure of lightly doped 1 T-TiSe_2, and demonstrate the existence of the electronic inhomogeneity and the...By using scanning tunneling microscopy(STM)/spectroscopy(STS), we systematically characterize the electronic structure of lightly doped 1 T-TiSe_2, and demonstrate the existence of the electronic inhomogeneity and the pseudogap state. It is found that the intercalation induced lattice distortion impacts the local band structure and reduce the size of the charge density wave(CDW) gap with the persisted 2 × 2 spatial modulation. On the other hand, the delocalized doping electrons promote the formation of pseudogap. Domination by either of the two effects results in the separation of two characteristic regions in real space, exhibiting rather different electronic structures. Further doping electrons to the surface confirms that the pseudogap may be the precursor for the superconducting gap. This study suggests that the competition of local lattice distortion and the delocalized doping effect contribute to the complicated relationship between charge density wave and superconductivity for intercalated 1 T-TiSe_2.展开更多
基金the Mac Diarmid Institute for Advanced Materials and Nanotechnology, New Zealand, and the IRC in Superconductivity, University of Cambridge, UK, for funding this research
文摘The nature of resistive transition of high-quality crystalline thin films of YBa2Cu3O7-δhas been studied under magnetic fields(H) applied along the c direction over a wide range of doped holes, p, in the Cu O2 planes. The field- and temperature-dependent in-plane resistivity, ρab(T, H), has been analyzed within the thermally assisted flux-flow(TAFF)formalism. The flux activation energy, U(T, H), has been extracted from this analysis. The low-T part of the ρab(T, H)data can be described by an activation energy having the functional form of U(T, H) =(1- t)m(H-0/H)β, where t = T /Tc(reduced temperature), and H0 is a field scale that primarily determines the magnitude of U(T, H). The temperature exponent, m, shows a systematic variation with p, whereas the field exponent, β, is insensitive to the p values and is close to unity. The H0, on the other hand, changes rapidly as p is varied. U(T, H) is linked to the pinning potential and consequently on the superconducting condensation energy. Since the normal state pseudogap directly affects superconducting condensation energy, a clear correspondence between H0 and the PG energy scale, ε g, is found. Possible implications of these results are discussed.
文摘This paper deduces that the particular electronic structure of cuprate superconductors confines Cooper pairs to be first formed in the antinodal region which is far from the Fermi surface, and these pairs are incoherent and result in the pseudogap state. With the change of doping or temperature, some pairs are formed in the nodal region which locates the Fermi surface, and these pairs are coherent and lead to superconductivity. Thus the coexistence of the pseudogap and the superconducting gap is explained when the two kinds of gaps are not all on the Fermi surface. It also shows that the symmetry of the pseudogap and the superconducting gap are determined by the electronic structure, and non-s wave symmetry gap favours the high-temperature superconductivity. Why the high-temperature superconductivity occurs in the metal region near the Mott metal-insulator transition is also explained.
文摘A mean-field spin-density wave (SDW) analysis of pseudogap in the underdoped cuprates is proposed on the dependence of the energy gap which mimics the pseudogap near (π, 0) point at least. It implies that the pseudogap structure near (π, 0) is not sensitive to the long-range order and will survive leading to the pseudogap phenomenon in the underdoped metallic phase. On the other hand, in the long-range ordering antiferromagnetic region, the mean-field SDW theory holds and the pseudogap structure predicated by the theory should be observable experimentallyv. Then one prediction is that the pseudogap would smoothly extrapolate between itinerant antiferromagnetic phase and underdoped metallic phase.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 11888101, 11922414 and 11974404)the National Key Research and Development Program of China (Grant Nos. 2021YFA1401800, 2017YFA0302900, 2018YFA0305602, and 2018YFA0704200)+3 种基金the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (Grant Nos. XDB25000000 and XDB33000000)the Youth Innovation Promotion Association of the Chinese Academy of Sciences (Grant No. 2021006)the Synergetic Extreme Condition User Facility (SECUF)the Research Program of Beijing Academy of Quantum Information Sciences (Grant No. Y18G06)。
文摘The pseudogap state is one of the most enigmatic characteristics in the anomalous normal state properties of the high temperature cuprate superconductors. A central issue is to reveal whether there is a symmetry breaking and which symmetries are broken across the pseudogap transition. By performing high resolution laser-based angle-resolved photoemission measurements on the optimally-doped Bi_(2)Sr_(1.6)La_(0.4)CuO_(6+δ) superconductor, we report the observations of the particle-hole symmetry conservation in both the superconducting state and the pseudogap state along the entire Fermi surface. These results provide key insights in understanding the nature of the pseudogap and its relation with high temperature superconductivity.
基金by the National Natural Science Foundation of China(Grant Nos.62074092 and 11604366)the National Key R&D Program of China(Grant No.2018YFA0305603)。
文摘Unusual quantum phenomena usually emerge upon doping Mott insulators.Using a molecular beam epitaxy system integrated with cryogenic sc√annin√g tunneling microscope,we investigate the electronic structure of a modulation-doped Mott insulator Sn/Si(111)-(√3×√3)R30°.In underdoped regions,we observe a universal pseudogap opening around the Fermi level,which changes little with the applied magnetic field and the occurrence of Sn vacancies.The pseudogap gets smeared out at elevated temperatures and alters in size with the spatial confinement of the Mott insulating phase.Our findings,along with the previously observed superconductivity at a higher doping level,are highly reminiscent of the electronic phase diagram in the doped copper oxide compounds.
基金Supported by the National Key Research and Development Program of China under Grant No 2016YFA0300300the National Natural Science Foundation of China under Grant No 11334010+1 种基金the National Basic Research Program of China under Grant No2015CB921300the Strategic Priority Research Program(B)of the Chinese Academy of Sciences under Grant No XDB07020300
文摘We carry out detailed momentum-dependent and temperature-dependent measurements on Bi_2Sr_2CaCu_2O_(8+δ)(Bi2212) superconductor in the superconducting and pseudogap states by super-high resolution laser-based angleresolved photoemission spectroscopy. The precise determination of the superconducting gap for the nearly optimally doped Bi2212(T_c= 91 K) at low temperature indicates that the momentum-dependence of the superconducting gap deviates from the standard d-wave form(cos(2Φ)). It can be alternatively fitted by including a high-order term(cos(6Φ)) in which the next nearest-neighbor interaction is considered. We find that the band structure near the antinodal region smoothly evolves across the pseudogap temperature without a signature of band reorganization which is distinct from that found in Bi_2Sr_2CuO_(6+δ) superconductors. This indicates that the band reorganization across the pseudogap temperature is not a universal behavior in cuprate superconductors.These results provide new insights in understanding the nature of the superconducting gap and pseudogap in high-temperature cuprate superconductors.
文摘The influence of pseudogap on the inelastic neutron scattering spectra of the underdoped lanthanum cuprate is studied on the basis of the model which incorporates both the superconducting state and pscudogap state.It is found that the striking effects of the influence of the pseudogap on the incommensurability of the spin excitation spectrum are that in the superconducting state the pseudogap makes the intensity of the incommensurate peak increase,in the normal state the pseudogap not only makes the intensity of the incommensurate peak increase,but also sharpens the incommensurate peak and increases incommensurability.
基金Acknowledgements This work was supported by the National Basic Research Program of China (Grant Nos. 2011CB921303 and 2012CB927404), the National Natural Science Foundation of China (Grant Nos. 10974173 and 11274267), and the Natural Science Foundation of Zhejiang Province (Grant No. LZ13A040001).
文摘The pairing and superfluid phenomena in a two-component ultracold atomic Fermi gas is an analogue of Cooper pairing and superconductivity in an electron system, in particular, the high Tc superconductors. Owing to the various tunable parameters that have been made accessible experimentally in recent years, atomic Fermi gases can be explored as a prototype or quantum sinmlator of superconductors. It is hoped that, utilizing such an analogy, the study of atomic Fermi gases may shed light to the mysteries of high Tc superconductivity. One obstacle to the ultimate understand- ing of high Tc superconductivity, from day one of its discovery, is the anomalous yet widespread pseudogap phenomena, for which a consensus is yet to be reached within the physics comnnmity, after over 27 years of intensive research efforts. In this article, we shall review the progress in the study of pseudogap phenomena in atomic Fermi gases in terms of both theoretical understanding and experimental observations. We show that there is strong, unambiguous evidence for the existence of a pseudogap in strongly interacting Fermi gases. In this context, we shall present a pairing fuctuation theory of the pseudogap physics and show that it is indeed a strong candidate theory for high Tc superconductivity.
基金supported by the National Natural Science Foundation of China (Grant Nos. 11974405, 11674377, and 11634015)the Ministry of Science and Technology of China (Grant Nos. 2016YFA0300502, and 2017YFA0302904)the Strategic Priority Research Program of the Chinese Academy of Sciences (Grant No. XDB33010100)。
文摘Understanding the nature of the mysterious pseudogap phenomenon is one of the most important issues associated with cuprate high-T_(c) superconductors.Here,we report 17O nuclear magnetic resonance(NMR) studies on two planar oxygen sites in stoichio?metric cuprate YBa_(2)Cu_(4)O_(8) to investigate the symmetry breaking inside the pseudogap phase.We observe that the Knight shifts of the two oxygen sites are identical at high temperatures but different below T_(nem) ~185 K,which is close to the pseudogap temperature T^(*).Our result provides a microscopic evidence for intra-unit-cell electronic nematicity.The difference in quadrupole resonance frequency between the two oxygen sites is unchanged below T_(nem),which suggests that the observed nematicity does not directly stem from the local charge density modulation.Furthermore,a short-range charge density wave(CDW) order is observed below T=150 K.The additional broadening in the 17O-NMR spectra because of this CDW order is determined to be inequivalent for the two oxygen sites,which is similar to that observed in case of nematicity.These results suggest a possible connection between nematicity,CDW order,and pseudogap.
文摘One of important challenges in condensed-matter physics is to realize new quantum states of matter by manipulating the dimensionality of materials,as represented by the discovery of high-temperature superconductivity in atomic-layer pnictides and room-temperature quantum Hall effect in graphene.Tran sition-metal dichalcogenides(TMDs)provide a fertile platform for exploring novel quantum phenomena accompanied by the dimensionality change,since they exhibit a variety of electronic/magnetic states owing to quantum confinement.Here we report an anomalous metal-i nsulator transition in duced by three-dimensional(3D)-two-dimensional(2D)crossover in mono layer 1T-VSe2 grown on bilayer graphene.We observed a complete insulating state with a finite energy gap on the entire Fermi surface in monolayer 1T-VSe2 at low temperatures,in sharp contrast to metallic nature of bulk.More surprisingly,monolayer 1T-VSe2 exhibits a pseudogap with Fermi arc at temperatures above the charge-density-wave temperature,showing a close resemblanee to high-temperature cuprates.This similarity suggests a common underlying physics between two apparently different systems,pointing to the importance of charge/spin fluctuations to create the novel electronic states,such as pseudogap and Fermi arc,in these materials.
文摘Looking back on the experiments about the normal state of thehigh temperature superconductor (HTS), the authors point out nine important experimental results. On the basis of these results, the authors have argued that the two-dimension, two-subsystem Hamiltonian is the appropriate starting point for describing the normal state of HTS. By this Hamiltonian, using the decoupling approximation of Green's function method by Kaga through numerical calculations, the authors have obtained the temperature dependent pseudogap in the density of states (DOS), which is consistent qualitatively with the experimental results by angle-resolved photoemission spectroscopy (ARPES). Theoretically, this Hamiltonian has the superconducting order parameter of d+s symmetry with d-wave as the main component, which is consistent with experiments. Further, the quantum electronic liquid in HTS is a near Fermi liquid in which there is coexistence of the delocalized states and nearly localized states, and there is finite probability for the nearly localized carriers to form the nearly localized carrier pairs at any finite temperature.
基金We thank Prof.Tao Wu for helpful discus.sion.This work was supported by the National Key R&D Program of China(Grant Nos.2016YFA0200603 and 2017YFA0205004)the"Strategic Priority Research Program"of CAS(Grant No.XDB01020100)+2 种基金the National Natural Science Foundation of China(Grant Nos.91321309,21421063,and 21473174)the Funda-mental Research Funds for the Central Science Advances Universi-ties(Nos.WK2060190027 and WK2060190084)A.Z.acknowledges a fellowship from the Youth Innovation Promotion Association of CAS(No.2011322)。
文摘Superconducting metal dichalcogenides(MDCs)present several similarities to the other layered SI1-perconductors like cuprates.The superconductivity in atomically thin MDCs has been demonstrated by recent experiments,however,the investigation of the superconductivity intertwined with other or-ders are scarce.Investigating the pseudogap in atomic layers of MDCs may help to understand the superconducting mechanism for these true two dimensional(2D)superconducting systemns.Herein we report a pseudogap opening in the tunneling spectra of thin layers of SnSe2 epitaxially grown on highly oriented pyrolytic graphite(HOPG)with scanning tunneling microscopy/spectroscopy(STM/STS).A significant V-shaped pseudogap was observed to open near the Fermi level(Er)in the sTS.And at elevated temperatures,the gap gradually evolves to a shallow dip.Our experimental observations provide direct evidence of a pseudogap state in the electron-doped SnSe2 atomic layers on the HOPG surface,which may stimulate further exploration of the mechanism of superconductivity at 2D limit in MDCs.
基金supported by the Ministry of Science and Technology of China(2014CB921103,2013CB922103,2016YFA0300400,2015CB921202)the National Natural Science Foundation of China(11774149,11374140,11190023,11774152,51372112,11574133)+1 种基金NSF Jiangsu Province(BK20150012)the Open Research Fund Program of the State Key Laboratory of Low-Dimensional Quantum Physics
文摘By using scanning tunneling microscopy(STM)/spectroscopy(STS), we systematically characterize the electronic structure of lightly doped 1 T-TiSe_2, and demonstrate the existence of the electronic inhomogeneity and the pseudogap state. It is found that the intercalation induced lattice distortion impacts the local band structure and reduce the size of the charge density wave(CDW) gap with the persisted 2 × 2 spatial modulation. On the other hand, the delocalized doping electrons promote the formation of pseudogap. Domination by either of the two effects results in the separation of two characteristic regions in real space, exhibiting rather different electronic structures. Further doping electrons to the surface confirms that the pseudogap may be the precursor for the superconducting gap. This study suggests that the competition of local lattice distortion and the delocalized doping effect contribute to the complicated relationship between charge density wave and superconductivity for intercalated 1 T-TiSe_2.