Observations of a quasi-90-day oscillation in the mesosphere and lower thermosphere(MLT) region from April 2011 to December 2014 are presented in this study. There is clear evidence of a quasi-90-day oscillation in te...Observations of a quasi-90-day oscillation in the mesosphere and lower thermosphere(MLT) region from April 2011 to December 2014 are presented in this study. There is clear evidence of a quasi-90-day oscillation in temperatures obtained from the Kunming meteor radar(25.6°N, 103.8°E) and Sounding of the Atmosphere using Broadband Emission Radiometry(SABER), as well as in wind observed by the Kunming meteor radar. The quasi-90-day oscillation appears to be a prominent feature in the temperatures and meridional wind tides and presents quite regular cycles that occur approximately twice per year. The amplitudes and phases of the quasi-90-day oscillation in the SABER temperature show a feature similar to that of upward-propagated diurnal tides, which have a vertical wavelength of ~20 km above 70 km. In the lower atmosphere, a similar 90-day variability is presented in the surface latent heat flux and correlates with the temperature in the MLT region. Similar to the quasi-90-day oscillation in temperature, a 90-day variability of ozone(O3) is also present in the MLT region and is considered to be driven by a similar variability in the upwardly-propagated diurnal tides generated in the lower atmosphere. Moreover, the 90-day variability in the absorption of ultraviolet(UV) radiation by daytime O3 in the MLT region is an in situ source of the quasi-90-day oscillation in the MLT temperature.展开更多
This study presents an analysis of the quasi-16-day wave(Q16DW)at three stations in the middle latitudes by using a meteor radar chain in conjunction with Aura Microwave Limb Sounder temperature data and MERRA2(Modern...This study presents an analysis of the quasi-16-day wave(Q16DW)at three stations in the middle latitudes by using a meteor radar chain in conjunction with Aura Microwave Limb Sounder temperature data and MERRA2(Modern-Era Retrospective Analysis for Research and Applications,Version 2)reanalysis data from 2008 to 2017.The radar chain consists of three meteor radar stations located at Mohe(MH,53.5°N,122.3°E),Beijing(BJ,40.3°N,116.2°E),and Wuhan(WH,30.5°N,114.6°E).The Q16DW wave exhibits similar seasonal variation in the neutral wind and temperature,and the Q16DW amplitude is generally strong during winter and weak around summer.The Q16DW at BJ was found to have secondary enhancement around September in the zonal wind,which is rarely reported at similar latitudes.The latitudinal variations of the Q16DW in the neutral wind and temperature are quite different.The Q16DW at BJ is the most prominent in both neutral wind components among the three stations and the Q16DW amplitudes at MH and WH are comparable,whereas the wave amplitude in temperature decreases with decreasing latitude.The quasi-geostrophic refractive index squared at the three stations in the period from 2008 to 2017 was revealed.The results indicate that the Q16DW in the mesosphere and lower thermosphere(MLT)at MH has a limited contribution from the lower atmosphere.Around March and October,the Q16DW in the troposphere at BJ can propagate upward into the MLT region,whereas at WH,the contribution to the Q16DW in the MLT region is largely from the mesosphere.展开更多
By using atmospheric wind data in the mesopause and lower thermosphere(MLT)region,features of seasonal variations in the quasi-6-day wave(6DW)at different latitudes are analyzed,and modulation of the 6DW by the diurna...By using atmospheric wind data in the mesopause and lower thermosphere(MLT)region,features of seasonal variations in the quasi-6-day wave(6DW)at different latitudes are analyzed,and modulation of the 6DW by the diurnal tide and solar 27-day period is discussed.The data used in the analysis are extracted from a wind dataset collected by a meteor radar chain from December 2008 to November 2017.The meteor radar chain includes four stations,in Mohe,Beijing,Wuhan,and Sanya.Features of seasonal variations in the 6DW indicate that in summer the 6DW is usually strongest during July and August,followed by stronger variations in January and April.At certain altitudes over Wuhan and Sanya,the 6DW is slightly different in different years and altitudes.In our analysis of seasonal variations in the 6DW,we find that it is generally affected by annual oscillations and semiannual oscillations.The annual oscillations of the 6DW in the mid-low latitudes are modulated by the quasibiennial oscillation in the diurnal tide,resulting in seasonal features that are different from those at other latitudes.In addition,the 6DW amplitude at mid-high latitudes has a significant 27-day solar rotation variation,which was prominent in 2016.展开更多
The two-dimensional(2 D) Ruddlesden–Popper-type perovskites, possessing tunable bandgap, narrow light emission,strong quantum confinement effect, as well as a simple preparation method, are identified as a new genera...The two-dimensional(2 D) Ruddlesden–Popper-type perovskites, possessing tunable bandgap, narrow light emission,strong quantum confinement effect, as well as a simple preparation method, are identified as a new generation of candidate materials for efficient light-emitting diodes. However, the preparation of high-quality quasi-2 D perovskite films is still a challenge currently, such as the severe mixing of phases and a high density of defects within the films, impeding the further promotion of device performance. Here, we prepared the quasi-2 D PEA_(2) MA_(n-1) Pbn Br_(3 n+1) perovskite films by a modified spin-coating method, and the phases with large bandgap were effectively suppressed by the vacuum evaporation treatment. We systematically investigated the optical properties and stability of the optimized films, and the photoluminescence(PL) quantum yield of the treated films was enhanced from 23% to 45%. We also studied the emission mechanisms by temperature-dependent PL spectra. Moreover, the stability of films against moisture, ultraviolet light, and heat was also greatly improved.展开更多
In order to improve the efficiency and stability of inverted three-dimensional(3D) or quasi-2D perovskite solar cells(PSCs) for future commercialization, exploring high efficient dopant-free polymer holetransporting m...In order to improve the efficiency and stability of inverted three-dimensional(3D) or quasi-2D perovskite solar cells(PSCs) for future commercialization, exploring high efficient dopant-free polymer holetransporting materials(HTMs) is still desired and meaningful. One simple and efficient way to achieve high performance dopant-free HTMs is to synthesize novel non-conjugated side-chain polymers via rational molecular design. In this work, N-(4-methoxyphenyl)-9,9-dimethyl-9H-fluoren-2-amine(FMeNPh) groups are introduced into the poly(N-vinylcarbazole)(PVK) side chains to afford two nonconjugated polymers PVCz-DFMeNPh and PVCz-FMeNPh as dopant-free HTMs in inverted quasi-2D PSCs. Benefited from the flexible properties of polyethylene backbone and excellent optoelectronic natures of FMeNPh side-chain groups, PVCz-DFMeNPh with more FMeNPh units exhibited excellent thermal stability, well-matched energy levels and improved charge mobility as compared to PTAA and PVCzFMeNPh. Moreover, the morphologies investigation of quasi-2D perovskite on PVCz-DFMeNPh shows more compact and homogeneous perovskite films than those on PTAA and PVCz-FMeNPh. As a result,the dopant-free PVCz-DFMeNPh based inverted quasi-2D PSCs deliver power conversion efficiency(PCE) up to 18.44% as well as negligible hysteresis and favorable long-term stability, which represents as excellent performance reported to date for inverted quasi-2D PSCs. The results demonstrate the great potentials of constructing non-conjugated side-chain polymer HTMs based on phenylfluorenamine-func tionalized PVK for the development of high efficient and stable inverted 3D or quasi-2D PSCs.展开更多
The in-plane anisotropy of transition metal trichalcogenides(MX_(3))has a significant impact on the molding of materi-als and MX_(3) is a perfect choice for polarized photodetectors.In this study,the crystal structure...The in-plane anisotropy of transition metal trichalcogenides(MX_(3))has a significant impact on the molding of materi-als and MX_(3) is a perfect choice for polarized photodetectors.In this study,the crystal structure,optical and optoelectronic aniso-tropy of one kind of quasi-one-dimensional(1D)semiconductors,ZrSe_(3),are systematically investigated through experiments and theoretical studies.The ZrSe_(3)-based photodetector shows impressive wide spectral response from ultraviolet(UV)to near in-frared(NIR)and exhibits great optoelectrical properties with photoresponsivity of 11.9 mA·W^(-1) and detectivity of~106 at 532 nm.Moreover,the dichroic ratio of ZrSe_(3)-based polarized photodetector is around 1.1 at 808 nm.This study suggests that ZrSe_(3) has potential in optoelectronic applications and polarization detectors.展开更多
Based on the 2D horizontal plane numerical model, a quasi-3D numerical model is established for coastal regions of shallow water. The characteristics of this model are that the velocity profiles;can be obtained at the...Based on the 2D horizontal plane numerical model, a quasi-3D numerical model is established for coastal regions of shallow water. The characteristics of this model are that the velocity profiles;can be obtained at the same time when the equations of the value of difference between the horizontal current velocity and its depth-averaged velocity in the vertical direction are solved and the results obtained are consistent with the results of the 2D, model. The circulating flow in the rectangular area induced by wind is simulated and applied to the tidal flow field of the radial sandbanks in the South Yellow Sea. The computational results from this quasi-3D model are in good agreement with analytical results and observed data. The solution of the finite difference equations has been found to be stable, and the model is simple, effective and practical.展开更多
The purpose of this article is to discuss a modified Halpern-type iteration algorithm for a countable family of uniformly totally quasi- ? -asymptotically nonexpansive multi-valued mappings and establish some strong c...The purpose of this article is to discuss a modified Halpern-type iteration algorithm for a countable family of uniformly totally quasi- ? -asymptotically nonexpansive multi-valued mappings and establish some strong convergence theorems under certain conditions. We utilize the theorems to study a modified Halpern-type iterative algorithm for a system of equilibrium problems. The results improve and extend the corresponding results of Chang et al. (Applied Mathematics and Computation, 218, 6489-6497).展开更多
The purpose of this article is to introduce a class of total quasi-Ф- asymptotically nonexpansive nonself mappings. Strong convergence theorems for common fixed points of a countable family of total quasi-Ф-asymptot...The purpose of this article is to introduce a class of total quasi-Ф- asymptotically nonexpansive nonself mappings. Strong convergence theorems for common fixed points of a countable family of total quasi-Ф-asymptotically nonexpan- sive mappings are established in the framework of Banach spaces based on modified Halpern and Mann-type iteration algorithm. The main results presented in this article extend and improve the corresponding results of many authors.展开更多
A study is made of the distribution of the diagnostic quantity vector E and the teleconnection structure of 30-50 (quasi-40) day oscillation, together with the dependence on the conversion of barotropic unstable energ...A study is made of the distribution of the diagnostic quantity vector E and the teleconnection structure of 30-50 (quasi-40) day oscillation, together with the dependence on the conversion of barotropic unstable energy of mean flow in terms of ECWMF daily 500 hPa grid data in winter, indicating that the energy transportation is closely associated with the westerly jet position, with zonal (meridional) propagation in the strong (weak) wind region, that considerable conversion of barotropic energy occurs at the jet exit region where low-frequency oscillation gains energy from the mean flow, leading to maximum kinetic energy for the oscillation observed there, which is marked by evident barotropy in striking contrast to the baroclinicity at low latitudes and that the teleconnection core is related to the center of action in the atmosphere and bound up with the pattern of the west wind.展开更多
Several theorems on the finiteness of energy for quasi- harmonic spheres are proved, some counter- examples which state thatthe energy of quasi- harmonic sphere may be infinite are given.The results support some con...Several theorems on the finiteness of energy for quasi- harmonic spheres are proved, some counter- examples which state thatthe energy of quasi- harmonic sphere may be infinite are given.The results support some conditions of a question posed by Lin Fanghua and Wang Changyou.展开更多
Two-dimensional(2D)/quasi-2D perovskite solar cells(PSCs)incorporating organic spacer cations exhibit appealing ambient stability in comparison with their 3D analogs.Most reported organic spacer cations are based on a...Two-dimensional(2D)/quasi-2D perovskite solar cells(PSCs)incorporating organic spacer cations exhibit appealing ambient stability in comparison with their 3D analogs.Most reported organic spacer cations are based on ammonium,whereas formamidinium(FA^(+))has been seldom applied despite that FA has been extensively used in high-efficiency 3D PSCs.Herein,a novel FA-based organic spacer cation,4-chloro-phenylformamidinium(CPFA^(+)),is applied in quasi-2D Ruddlesden-Popper(RP)PSCs for the first time,and methylammonium chloride(MACl)is employed to promote crystal growth and orientation of perovskite film,resulting in high power conversion efficiency(PCE)with improved stability.Upon incorporating CPFA+organic spacer cation and MACl additive,high-quality quasi-2D CPFA_(2)MA_(n-1)Pb_(n)(I_(0.857)Cl_(0.143))_(3n+1)(n=9)perovskite film forms,exhibiting improved crystal orientation,reduced trap state density,prolonged carrier lifetime and optimized energy level alignment.Consequently,the CPFA_(2)MA_(n-1)Pb_(n)(I_(0.857)Cl_(0.143))_(3n+1)(n=9)quasi-2D RP PSC devices deliver a highest PCE of 14.78%.Moreover,the un-encapsulated CPFA-based quasi-2D RP PSC devices maintain~80%of its original PCE after exceeding 2000 h storage under ambient condition,whereas the 3D MAPb I3counterparts retain only~45%of its original PCE.Thus,the ambient stability of quasi-2D RP PSC devices is improved obviously relative to its 3D MAPb I3counterpart.展开更多
In this paper,we study the hyperstability for the general linear equation f(ax+by)=Af(x)+Bf(y)in the setting of complete quasi-2-Banach spaces.We first extend the main fixed point result of Brzdek and Ciepliński(Acta...In this paper,we study the hyperstability for the general linear equation f(ax+by)=Af(x)+Bf(y)in the setting of complete quasi-2-Banach spaces.We first extend the main fixed point result of Brzdek and Ciepliński(Acta Mathematica Scientia,2018,38 B(2):377-390)to quasi-2-Banach spaces by defining an equivalent quasi-2-Banach space.Then we use this result to generalize the main results on the hyperstability for the general linear equation in quasi-2-Banach spaces.Our results improve and generalize many results of literature.展开更多
We shall generalize the results of [9] about characterization of isomorphisms on quasi-Banach algebras by providing integral type conditions. Also, we shall give some new results in this way and finally, give a result...We shall generalize the results of [9] about characterization of isomorphisms on quasi-Banach algebras by providing integral type conditions. Also, we shall give some new results in this way and finally, give a result about hybrid fixed point of two homomorphisms on quasi-Banach algebras.展开更多
We characterize V modules by relative (quasi )continuity of left R modules in this paper. It is shown that a left R module M is a V module if and only if every finitely cogenerated left R ...We characterize V modules by relative (quasi )continuity of left R modules in this paper. It is shown that a left R module M is a V module if and only if every finitely cogenerated left R module in σ[M] is S ( quasi )continuous if and only if every left R module in σ[M] is S continuous, where S is the set of all simple left R modules. We also show that a left R module M is a locally noetherian V module if and only if every semisimple left R module (in σ[M]) is M injective if and only if every essential extension in σ[M] of every semisimple left R module in σ[M] is S ? 2 (quasi )continuous, where S ? 2 is the set of all semisimple left R modules.展开更多
Recent years has seen increasing interest in building artificial synaptic devices to emulate the computation performed by biological synapses.Biological synapses are functional links between neurons,through which info...Recent years has seen increasing interest in building artificial synaptic devices to emulate the computation performed by biological synapses.Biological synapses are functional links between neurons,through which information is transmitted in the neuron network.The information can be stored and processed simultaneously in the same synapse through tuning synaptic weight,which is defined as the strength of the correlation between展开更多
The dynamic behaviors of water contained in calcium-silicate-hydrate(C-S-H) gel with different water content values from 10%to 30%(by weight),are studied by using an empirical diffusion model(EDM) to analyze the...The dynamic behaviors of water contained in calcium-silicate-hydrate(C-S-H) gel with different water content values from 10%to 30%(by weight),are studied by using an empirical diffusion model(EDM) to analyze the experimental data of quasi-elastic neutron scattering(QENS) spectra at measured temperatures ranging from 230 K to 280 K.In the study,the experimental QENS spectra with the whole Q-range are considered.Several important parameters including the bound/immobile water elastic coefficient A,the bound water index BWI,the Lorentzian with a half-width at half-maximum(HWHM) Γ;(Q) and Γ;(Q),the self-diffusion coefficients D;and D;of water molecules,the average residence times τ;and τ;,and the proton mean squared displacement(MSD)(u;) are obtained.The results show that the QENS spectra can be fitted very well not only for small Q(≤1 A;) but also for large Q.The bound/immobile water fraction in a C-S-H gel sample can be shown by the fitted BWI.The distinction between bound/immobile and mobile water,which includes confined water and ultra-confined water,can be seen by the fitted MSD.All the MSD tend to be the smallest value below 0.25 A;(the MSD of bound/immobile water) as the Q increases to 1.9 A;no matter what the temperature and water content are.Furthermore,by the abrupt changes of the fitted values of D;,τ;,and Γ;(Q),a crossover temperature at 250 K,namely the liquid-to-crystal-like transition temperature,can be identified for confined water in large gel pores(LGPs) and/or small gel pores(SGPs) contained in the C-S-H gel sample with 30% water content.展开更多
基金supported by Project(KJCX2-EW-J01,KZZD-EW-0101)of the Chinese Academy of Sciencesthe National Natural Science Foundation of China(41322029,41474129,41421063 and41804147)+5 种基金the National Basic Research Program of China(2012CB825605)the Youth Innovation Promotion Association of the Chinese Academy of Sciences(2011324)the Fundamental Research Funds for the Central Universitiesthe open research project of Chinese Academy of Sciences Large Research Infrastructuresthe Chinese Meridian Projectthe Open Research Program of National Key Laboratory of Electromagnetic Environment of the China Research Institute of Radiowave Propagation
文摘Observations of a quasi-90-day oscillation in the mesosphere and lower thermosphere(MLT) region from April 2011 to December 2014 are presented in this study. There is clear evidence of a quasi-90-day oscillation in temperatures obtained from the Kunming meteor radar(25.6°N, 103.8°E) and Sounding of the Atmosphere using Broadband Emission Radiometry(SABER), as well as in wind observed by the Kunming meteor radar. The quasi-90-day oscillation appears to be a prominent feature in the temperatures and meridional wind tides and presents quite regular cycles that occur approximately twice per year. The amplitudes and phases of the quasi-90-day oscillation in the SABER temperature show a feature similar to that of upward-propagated diurnal tides, which have a vertical wavelength of ~20 km above 70 km. In the lower atmosphere, a similar 90-day variability is presented in the surface latent heat flux and correlates with the temperature in the MLT region. Similar to the quasi-90-day oscillation in temperature, a 90-day variability of ozone(O3) is also present in the MLT region and is considered to be driven by a similar variability in the upwardly-propagated diurnal tides generated in the lower atmosphere. Moreover, the 90-day variability in the absorption of ultraviolet(UV) radiation by daytime O3 in the MLT region is an in situ source of the quasi-90-day oscillation in the MLT temperature.
基金the National Natural Science Foundation of China(through grants 41574142 and 41531070)the National Science Foundation(through grant AGS-1744033).
文摘This study presents an analysis of the quasi-16-day wave(Q16DW)at three stations in the middle latitudes by using a meteor radar chain in conjunction with Aura Microwave Limb Sounder temperature data and MERRA2(Modern-Era Retrospective Analysis for Research and Applications,Version 2)reanalysis data from 2008 to 2017.The radar chain consists of three meteor radar stations located at Mohe(MH,53.5°N,122.3°E),Beijing(BJ,40.3°N,116.2°E),and Wuhan(WH,30.5°N,114.6°E).The Q16DW wave exhibits similar seasonal variation in the neutral wind and temperature,and the Q16DW amplitude is generally strong during winter and weak around summer.The Q16DW at BJ was found to have secondary enhancement around September in the zonal wind,which is rarely reported at similar latitudes.The latitudinal variations of the Q16DW in the neutral wind and temperature are quite different.The Q16DW at BJ is the most prominent in both neutral wind components among the three stations and the Q16DW amplitudes at MH and WH are comparable,whereas the wave amplitude in temperature decreases with decreasing latitude.The quasi-geostrophic refractive index squared at the three stations in the period from 2008 to 2017 was revealed.The results indicate that the Q16DW in the mesosphere and lower thermosphere(MLT)at MH has a limited contribution from the lower atmosphere.Around March and October,the Q16DW in the troposphere at BJ can propagate upward into the MLT region,whereas at WH,the contribution to the Q16DW in the MLT region is largely from the mesosphere.
基金the National Natural Science Foundation of China(41774158,41974174,41674150,41831071 and 41904135)the Open Research Project of Large Research Infrastructures of CAS—“Study on the interaction between low/mid-latitude atmosphere and ionosphere based on the Chinese Meridian Project”.
文摘By using atmospheric wind data in the mesopause and lower thermosphere(MLT)region,features of seasonal variations in the quasi-6-day wave(6DW)at different latitudes are analyzed,and modulation of the 6DW by the diurnal tide and solar 27-day period is discussed.The data used in the analysis are extracted from a wind dataset collected by a meteor radar chain from December 2008 to November 2017.The meteor radar chain includes four stations,in Mohe,Beijing,Wuhan,and Sanya.Features of seasonal variations in the 6DW indicate that in summer the 6DW is usually strongest during July and August,followed by stronger variations in January and April.At certain altitudes over Wuhan and Sanya,the 6DW is slightly different in different years and altitudes.In our analysis of seasonal variations in the 6DW,we find that it is generally affected by annual oscillations and semiannual oscillations.The annual oscillations of the 6DW in the mid-low latitudes are modulated by the quasibiennial oscillation in the diurnal tide,resulting in seasonal features that are different from those at other latitudes.In addition,the 6DW amplitude at mid-high latitudes has a significant 27-day solar rotation variation,which was prominent in 2016.
基金supported by the National Natural Science Foundation of China (Grant Nos. 11774318, 12074347, 12004346, and 61935009)the Open Fund of State Key Laboratory of Integrated Optoelectronics (Grant No. IOSKL2020KF04)。
文摘The two-dimensional(2 D) Ruddlesden–Popper-type perovskites, possessing tunable bandgap, narrow light emission,strong quantum confinement effect, as well as a simple preparation method, are identified as a new generation of candidate materials for efficient light-emitting diodes. However, the preparation of high-quality quasi-2 D perovskite films is still a challenge currently, such as the severe mixing of phases and a high density of defects within the films, impeding the further promotion of device performance. Here, we prepared the quasi-2 D PEA_(2) MA_(n-1) Pbn Br_(3 n+1) perovskite films by a modified spin-coating method, and the phases with large bandgap were effectively suppressed by the vacuum evaporation treatment. We systematically investigated the optical properties and stability of the optimized films, and the photoluminescence(PL) quantum yield of the treated films was enhanced from 23% to 45%. We also studied the emission mechanisms by temperature-dependent PL spectra. Moreover, the stability of films against moisture, ultraviolet light, and heat was also greatly improved.
基金financially supported by the National Key Research and Development Program of China (2018YFB0406704)the National Natural Science Foundation of China (61974066, 61725502, 61634001)+3 种基金the Major Research Plan of the National Natural Science Foundation of China (91733302)the fund for Talented of Nanjing Tech University (201983)the Major Program of Natural Science Research of Jiangsu Higher Education Institutions of China (18KJA510002)the Synergetic Innovation Center for Organic Electronics and Information Displays。
文摘In order to improve the efficiency and stability of inverted three-dimensional(3D) or quasi-2D perovskite solar cells(PSCs) for future commercialization, exploring high efficient dopant-free polymer holetransporting materials(HTMs) is still desired and meaningful. One simple and efficient way to achieve high performance dopant-free HTMs is to synthesize novel non-conjugated side-chain polymers via rational molecular design. In this work, N-(4-methoxyphenyl)-9,9-dimethyl-9H-fluoren-2-amine(FMeNPh) groups are introduced into the poly(N-vinylcarbazole)(PVK) side chains to afford two nonconjugated polymers PVCz-DFMeNPh and PVCz-FMeNPh as dopant-free HTMs in inverted quasi-2D PSCs. Benefited from the flexible properties of polyethylene backbone and excellent optoelectronic natures of FMeNPh side-chain groups, PVCz-DFMeNPh with more FMeNPh units exhibited excellent thermal stability, well-matched energy levels and improved charge mobility as compared to PTAA and PVCzFMeNPh. Moreover, the morphologies investigation of quasi-2D perovskite on PVCz-DFMeNPh shows more compact and homogeneous perovskite films than those on PTAA and PVCz-FMeNPh. As a result,the dopant-free PVCz-DFMeNPh based inverted quasi-2D PSCs deliver power conversion efficiency(PCE) up to 18.44% as well as negligible hysteresis and favorable long-term stability, which represents as excellent performance reported to date for inverted quasi-2D PSCs. The results demonstrate the great potentials of constructing non-conjugated side-chain polymer HTMs based on phenylfluorenamine-func tionalized PVK for the development of high efficient and stable inverted 3D or quasi-2D PSCs.
基金financially supported by the National Key Research and Development Program of China (Grant No.2017YFA0207500)the National Natural Science Foundation of China (Grant No. 62125404, 12004375, 62004193,62174155)+1 种基金the CAS-JSPS Cooperative Research Project (No.GJHZ2021131)the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB43000000)
文摘The in-plane anisotropy of transition metal trichalcogenides(MX_(3))has a significant impact on the molding of materi-als and MX_(3) is a perfect choice for polarized photodetectors.In this study,the crystal structure,optical and optoelectronic aniso-tropy of one kind of quasi-one-dimensional(1D)semiconductors,ZrSe_(3),are systematically investigated through experiments and theoretical studies.The ZrSe_(3)-based photodetector shows impressive wide spectral response from ultraviolet(UV)to near in-frared(NIR)and exhibits great optoelectrical properties with photoresponsivity of 11.9 mA·W^(-1) and detectivity of~106 at 532 nm.Moreover,the dichroic ratio of ZrSe_(3)-based polarized photodetector is around 1.1 at 808 nm.This study suggests that ZrSe_(3) has potential in optoelectronic applications and polarization detectors.
基金National Natural Science Foundation of China(Grant No.49236120)
文摘Based on the 2D horizontal plane numerical model, a quasi-3D numerical model is established for coastal regions of shallow water. The characteristics of this model are that the velocity profiles;can be obtained at the same time when the equations of the value of difference between the horizontal current velocity and its depth-averaged velocity in the vertical direction are solved and the results obtained are consistent with the results of the 2D, model. The circulating flow in the rectangular area induced by wind is simulated and applied to the tidal flow field of the radial sandbanks in the South Yellow Sea. The computational results from this quasi-3D model are in good agreement with analytical results and observed data. The solution of the finite difference equations has been found to be stable, and the model is simple, effective and practical.
文摘The purpose of this article is to discuss a modified Halpern-type iteration algorithm for a countable family of uniformly totally quasi- ? -asymptotically nonexpansive multi-valued mappings and establish some strong convergence theorems under certain conditions. We utilize the theorems to study a modified Halpern-type iterative algorithm for a system of equilibrium problems. The results improve and extend the corresponding results of Chang et al. (Applied Mathematics and Computation, 218, 6489-6497).
基金Scientific Research Fund(2011JYZ010)of Science Technology Department of Sichuan ProvinceScientific Research Fund(11ZA172 and 12ZB345)of Sichuan Provincial Education Department
文摘The purpose of this article is to introduce a class of total quasi-Ф- asymptotically nonexpansive nonself mappings. Strong convergence theorems for common fixed points of a countable family of total quasi-Ф-asymptotically nonexpan- sive mappings are established in the framework of Banach spaces based on modified Halpern and Mann-type iteration algorithm. The main results presented in this article extend and improve the corresponding results of many authors.
基金This work is supported by National Natural Science Foundation of China.
文摘A study is made of the distribution of the diagnostic quantity vector E and the teleconnection structure of 30-50 (quasi-40) day oscillation, together with the dependence on the conversion of barotropic unstable energy of mean flow in terms of ECWMF daily 500 hPa grid data in winter, indicating that the energy transportation is closely associated with the westerly jet position, with zonal (meridional) propagation in the strong (weak) wind region, that considerable conversion of barotropic energy occurs at the jet exit region where low-frequency oscillation gains energy from the mean flow, leading to maximum kinetic energy for the oscillation observed there, which is marked by evident barotropy in striking contrast to the baroclinicity at low latitudes and that the teleconnection core is related to the center of action in the atmosphere and bound up with the pattern of the west wind.
文摘Several theorems on the finiteness of energy for quasi- harmonic spheres are proved, some counter- examples which state thatthe energy of quasi- harmonic sphere may be infinite are given.The results support some conditions of a question posed by Lin Fanghua and Wang Changyou.
基金supported by the National Key Research and Development Program of China(2017YFA0402800)the National Natural Science Foundation of China(51925206,U1932214)。
文摘Two-dimensional(2D)/quasi-2D perovskite solar cells(PSCs)incorporating organic spacer cations exhibit appealing ambient stability in comparison with their 3D analogs.Most reported organic spacer cations are based on ammonium,whereas formamidinium(FA^(+))has been seldom applied despite that FA has been extensively used in high-efficiency 3D PSCs.Herein,a novel FA-based organic spacer cation,4-chloro-phenylformamidinium(CPFA^(+)),is applied in quasi-2D Ruddlesden-Popper(RP)PSCs for the first time,and methylammonium chloride(MACl)is employed to promote crystal growth and orientation of perovskite film,resulting in high power conversion efficiency(PCE)with improved stability.Upon incorporating CPFA+organic spacer cation and MACl additive,high-quality quasi-2D CPFA_(2)MA_(n-1)Pb_(n)(I_(0.857)Cl_(0.143))_(3n+1)(n=9)perovskite film forms,exhibiting improved crystal orientation,reduced trap state density,prolonged carrier lifetime and optimized energy level alignment.Consequently,the CPFA_(2)MA_(n-1)Pb_(n)(I_(0.857)Cl_(0.143))_(3n+1)(n=9)quasi-2D RP PSC devices deliver a highest PCE of 14.78%.Moreover,the un-encapsulated CPFA-based quasi-2D RP PSC devices maintain~80%of its original PCE after exceeding 2000 h storage under ambient condition,whereas the 3D MAPb I3counterparts retain only~45%of its original PCE.Thus,the ambient stability of quasi-2D RP PSC devices is improved obviously relative to its 3D MAPb I3counterpart.
基金AISTDF,DST India for the research grant vide project No.CRD/2018/000017。
文摘In this paper,we study the hyperstability for the general linear equation f(ax+by)=Af(x)+Bf(y)in the setting of complete quasi-2-Banach spaces.We first extend the main fixed point result of Brzdek and Ciepliński(Acta Mathematica Scientia,2018,38 B(2):377-390)to quasi-2-Banach spaces by defining an equivalent quasi-2-Banach space.Then we use this result to generalize the main results on the hyperstability for the general linear equation in quasi-2-Banach spaces.Our results improve and generalize many results of literature.
文摘We shall generalize the results of [9] about characterization of isomorphisms on quasi-Banach algebras by providing integral type conditions. Also, we shall give some new results in this way and finally, give a result about hybrid fixed point of two homomorphisms on quasi-Banach algebras.
文摘We characterize V modules by relative (quasi )continuity of left R modules in this paper. It is shown that a left R module M is a V module if and only if every finitely cogenerated left R module in σ[M] is S ( quasi )continuous if and only if every left R module in σ[M] is S continuous, where S is the set of all simple left R modules. We also show that a left R module M is a locally noetherian V module if and only if every semisimple left R module (in σ[M]) is M injective if and only if every essential extension in σ[M] of every semisimple left R module in σ[M] is S ? 2 (quasi )continuous, where S ? 2 is the set of all semisimple left R modules.
基金supported by the National Natural Science Foundation of Chinathe Ministry of Science and Technology of Chinathe Chinese Academy of Sciences
文摘Recent years has seen increasing interest in building artificial synaptic devices to emulate the computation performed by biological synapses.Biological synapses are functional links between neurons,through which information is transmitted in the neuron network.The information can be stored and processed simultaneously in the same synapse through tuning synaptic weight,which is defined as the strength of the correlation between
文摘The dynamic behaviors of water contained in calcium-silicate-hydrate(C-S-H) gel with different water content values from 10%to 30%(by weight),are studied by using an empirical diffusion model(EDM) to analyze the experimental data of quasi-elastic neutron scattering(QENS) spectra at measured temperatures ranging from 230 K to 280 K.In the study,the experimental QENS spectra with the whole Q-range are considered.Several important parameters including the bound/immobile water elastic coefficient A,the bound water index BWI,the Lorentzian with a half-width at half-maximum(HWHM) Γ;(Q) and Γ;(Q),the self-diffusion coefficients D;and D;of water molecules,the average residence times τ;and τ;,and the proton mean squared displacement(MSD)(u;) are obtained.The results show that the QENS spectra can be fitted very well not only for small Q(≤1 A;) but also for large Q.The bound/immobile water fraction in a C-S-H gel sample can be shown by the fitted BWI.The distinction between bound/immobile and mobile water,which includes confined water and ultra-confined water,can be seen by the fitted MSD.All the MSD tend to be the smallest value below 0.25 A;(the MSD of bound/immobile water) as the Q increases to 1.9 A;no matter what the temperature and water content are.Furthermore,by the abrupt changes of the fitted values of D;,τ;,and Γ;(Q),a crossover temperature at 250 K,namely the liquid-to-crystal-like transition temperature,can be identified for confined water in large gel pores(LGPs) and/or small gel pores(SGPs) contained in the C-S-H gel sample with 30% water content.