Radiative Effects on Torrential Rainfall during the Landfall of Typhoon Fitow(2013)

Cloud microphysical and rainfall responses to radiative processes are examined through analysis of cloud-resolving model sensitivity experiments of Typhoon Fitow（2013） during landfall.The budget analysis shows that the increase in the mean rainfall caused by the exclusion of radiative effects of water clouds corresponds to the decrease in accretion of raindrops by cloud ice in the presence of radiative effects of ice clouds,but the rainfall is insensitive to radiative effects of water clouds in the absence of radiative effects of ice clouds.The increases in the mean rainfall resulting from the removal of radiative effects of ice clouds correspond to the enhanced net condensation.The increases（decreases） in maximum rainfall caused by the exclusion of radiative effects of water clouds in the presence（absence） of radiative effects of ice clouds,or the removal of radiative effects of ice clouds in the presence（absence） of radiative effects of water clouds,correspond mainly to the enhancements（reductions） in net condensation.The mean rain rate is a product of rain intensity and fractional rainfall coverage.The radiation-induced difference in the mean rain rate is related to the difference in rain intensity.The radiation-induced difference in the maximum rain rate is associated with the difference in the fractional coverage of maximum rainfall.

Impact of COVID-19 lockdown on the optical properties and radiative effects of urban brown carbon aerosol

Intensive measurements were conducted in Xi’an,China before and during a COVID-19 lockdown period to investigate how changes in anthropogenic emissions affected the optical properties and radiative effects of brown carbon(BrC)aerosol.The contribution of BrC to total aerosol light absorption during the lockdown(13%-49%)was higher compared with the normal period(4%-29%).Mass absorption cross-sections(MACs)of specific organic aerosol(OA)factors were calculated from a ridge regression model.Of the primary OA(POA),coal combustion OA(CCOA)had the largest MACs at all tested wave-lengths during both periods due to high molecular-weight BrC chromophores;that was followed by biomass burning OA(BBOA)and hydrocarbon-like OA(HOA).For secondary OA(SOA),the MACs of the lessoxidized oxygenated OA(OOA)species(LO-OOA)atλ=370-590 nm were higher than those of more-oxidized OOA(MO-OOA)during both periods,presumably due to chromophore bleaching.The largest contributor to BrC absorption at the short wavelengths was CCOA during both periods,but BrC absorption by LO-OOA and MO-OOA became dominant at longer wavelengths during the lockdown.The estimated radiation forcing efficiency of BrC over 370-600 nm increased from 37.5 W·gduring the normal period to 50.2 W·gduring the lockdown,and that enhancement was mainly caused by higher MACs for both LO-OOA and MO-OOA.This study provides insights into the optical properties and radiative effects of source-specific BrC aerosol when pollution emissions are reduced.

A Preliminary Evaluation of Global and East Asian Cloud Radiative Effects in Reanalyses

Cloud radiative effects （CREs） at the top of the atmosphere （TOA） in three reanalysis datasets （the Eur- opean Center for Medium-Range Weather Forecasts In- terim Reanalysis （ERA-Interim）, the Japanese 55-yr Re- analysis Project （JRA-55）, and the Modem-Era Retro- spective Analysis for Research and Applications （MERRA）） are evaluated using recent satellite-based observations. The reanalyses can basically capture the spatial pattern of the annual mean shortwave CRE, but the global mean longwave CRE in ERA-interim and JRA55 is weaker than observed, leading to overestimations of the net CRE. Moreover, distinct CRE biases of the reanalyses occur in the Intertropical Convergence Zone （ITCZ）, coastal Pa- cific and Atlantic regions, and East Asia. Quantitative examination further indicates that the spatial correlations of CREs and TOA upward radiation fluxes with corre- sponding observations in ERA-Interim are better than in the other two reanalyses. Although MERRA has certain abilities in producing the magnitudes of global mean CREs, its performance in terms of spatial correlations in winter and summer are worse than for the other two re- analyses. The ability of JRA55 in reflecting CREs lies between the other two datasets. Compared to the global mean results, the spatial correlations of shortwave CRE in East Asia decrease and the biases of regional mean CREs increase in the three reanalyses. This implies that, cur- rently, it is still difficult to reproduce East Asian CREs based on these reanalyses. Relatively, ERA-Interim de- scribes the seasonal variation of East Asian CREs well, albeit weaker than observed. The present study also sug- gests that in-depth exploration of the ability of reanalysis data to describe aspects relating to cloud properties and rad- iation is needed usin~ more comprehensive observations.

THE RADIATIVE EFFECTS OF ANTHROPOGENIC AEROSOLS OVER CHINA AND THEIR SENSITIVITY TO SOURCE EMISSION

In this paper,the RIEMS 2.0 model,source emission in 2006 and 2010 are used to simulate the distributions and radiative effects of different anthropogenic aerosols over China.The comparison between the results forced by source emissions in 2006 and 2010 also reveals the sensitivity of the radiative effects to source emission.The results are shown as follows:(1) Compared with those in 2006,the annual average surface concentration of sulfate in 2010 decreased over central and eastern China with a range of-5 to 0 μg/m^3;the decrease of annual average aerosol optical depth of sulfate over East China varied from 0.04 to 0.08;the annual average surface concentrations of BC,OC and nitrate increased over central and eastern China with maximums of 10.90,11.52 and 12.50μg/m^3,respectively;the annual aerosol optical depths of BC,OC and nitrate increased over some areas of East China with extremes of 0.006,0.007 and 0.008,respectively.(2)For the regional average results in 2010,the radiative forcings of sulfate,BC,OC,nitrate and their total net radiative forcing at the top of the atmosphere over central and eastern China were-0.64,0.29,-0.41,-0.33 and-1.1 W/m^2,respectively.Compared with those in 2006,the radiative forcings of BC and OC in 2010 were both enhanced,while that of sulfate and the net radiative forcing were both weakened over East China mostly.(3)The reduction of the cooling effect of sulfate in 2010 produced a warmer surface air temperature over central and eastern China;the maximum value was 0.25 K.The cooling effect of nitrate was also slightly weakened.The warming effect of BC was enhanced over most of the areas in China,while the cooling effect of OC was enhanced over the similar area,particularly the area between Yangtze and Huanghe Rivers.The net radiative effect of the four anthropogenic aerosols generated the annual average reduction and the maximum reduction were-0.096 and-0.285 K,respectively,for the surface temperature in 2006,while in 2010 they were-0.063 and-0.256 K,respectively.In summary,the change in source emission lowered the cooling effect of anthropogenic aerosols,mainly because of the enhanced warming effect of BC and weakened cooling effect of scattering aerosols.

Simulating Aerosol Optical Depth and Direct Radiative Effects over the Tibetan Plateau with a High-Resolution CAS FGOALS-f3 Model

Current global climate models cannot resolve the complex topography over the Tibetan Plateau(TP)due to their coarse resolution.This study investigates the impacts of horizontal resolution on simulating aerosol and its direct radiative effect(DRE)over the TP by applying two horizontal resolutions of about 100 km and 25 km to the Chinese Academy of Sciences Flexible Global Ocean-Atmosphere Land System(CAS FGOALS-f3)over a 10-year period.Compared to the AErosol RObotic NETwork observations,a high-resolution model(HRM)can better reproduce the spatial distribution and seasonal cycles of aerosol optical depth(AOD)compared to a low-resolution model(LRM).The HRM bias and RMSE of AOD decreased by 0.08 and 0.12,and the correlation coefficient increased by 0.22 compared to the LRM.An LRM is not sufficient to reproduce the aerosol variations associated with fine-scale topographic forcing,such as in the eastern marginal region of the TP.The difference between hydrophilic aerosols in an HRM and LRM is caused by the divergence of the simulated relative humidity(RH).More reasonable distributions and variations of RH are conducive to simulating hydrophilic aerosols.An increase of the 10-m wind speed in winter by an HRM leads to increased dust emissions.The simulated aerosol DREs at the top of the atmosphere(TOA)and at the surface by the HRM are–0.76 W m^(–2)and–8.72 W m^(–2)over the TP,respectively.Both resolution models can capture the key feature that dust TOA DRE transitions from positive in spring to negative in the other seasons.

Assessment of Individual Direct Radiative Effects of Major Aerosol Species in East Asia

To assess individual direct radiative effects of diverse aerosol species on a regional scale, the air quality modeling system RAMS-CMAQ （Regional Atmospheric Modeling System and Community Multiscale Air Quality） coupled with an aerosol optical properties/radiative transfer module was used to simulate the temporal and spatial distributions of their optical and radiative properties over East Asia throughout 2005. Annual and seasonal averaged aerosol direct radiative forcing （ADRF） of all important aerosols and individual components, such as sulfate, nitrate, ammonium, black carbon （BC）, organic carbon （OC）, and dust at top-of-atmosphere （TOA） in clear sky are analyzed. Analysis of the model results shows that the annual average ADRF of all important aerosols was in the range of 0 to -18 W m-z, with the maximum values mainly distributed over the Sichuan Basin. The direct radiative effects of sulfate, nitrate, and ammonium make up most of the total ADRF in East Asia, being concentrated mainly over North and Southeast China. The model domain is also divided into seven regions based on different administrative regions or countries to investigate detailed information about regional ADRF variations over East Asia. The model results show that the ADRFs of sulfate, ammonium, BC, and OC were stronger in summer and weaker in winter over most regions of East Asia, except over Southeast Asia. The seasonal variation in the ADRF of nitrate exhibited the opposite trend. A strong ADRF of dust mainly appeared in spring over Northwest China and Mongolia.

Regional Characteristics of Cloud Radiative Effects before and after the South China Sea Summer Monsoon Onset

The South China Sea summer monsoon(SCSSM)onset is characterized by rapid thermodynamical changes in the atmosphere that are critical to regional weather and climate processes.So far,few studies have focused on the changes in the associated cloud and radiative features.This study investigates spatiotemporal characteristics of topof-atmosphere(TOA)cloud radiative effects(CREs)before and after the SCSSM onset over the South China Sea(SCS)and South China(SC),based on the 2001–2016 Clouds and the Earth’s Radiant Energy System(CERES)Energy Balanced and Filled(EBAF)satellite data and ERA-Interim reanalysis data.Before the SCSSM onset,strong net CRE(NCRE)dominated by its cooling shortwave component occurs over SC,while descending motion and weak NCRE prevail over the SCS.In the SCSSM onset pentad,convection,high clouds,and longwave and shortwave CREs(LWCRE and SWCRE)abruptly increase over the southern and central SCS,and their high-value centers subsequently move northeastward and are strongly affected by the western Pacific subtropical high.The strong offset between LWCRE and SWCRE enables the NCRE intensity(TOA radiation budget)to be quite small(large)between the SCS and the western North Pacific after the SCSSM onset.In contrast,low–middle-level clouds and strong cooling SWCRE remain over SC after the SCSSM onset,but the increasing high clouds and LWCRE weaken(intensify)the regional NCRE(TOA radiation budget)intensity.These marked latitudinal differences in CREs between the SCS and SC primarily arise from their respective dominant cloud types and circulation conditions,which manifest the differences between the tropical SCSSM and subtropical East Asian monsoon processes.The results indicate that regional cloud fractions and CREs before and after the SCSSM onset are strongly modulated by quickly changed largescale circulation over the East Asian monsoon regions,and the spatiotemporal variation of CREs is a response to the monsoonal circulation adjustment to a large extent.

Observational Characteristics of Cloud Radiative Effects over Three Arid Regions in the Northern Hemisphere

Cloud–radiation processes play an important role in regional energy budgets and surface temperature changes over arid regions. Cloud radiative effects（CREs） are used to quantitatively measure the aforementioned climatic role. This study investigates the characteristics of CREs and their temporal variations over three arid regions in central Asia（CA）, East Asia（EA）, and North America（NA）, based on recent satellite datasets. Our results show that the annual mean shortwave（SW） and net CREs（SWCRE and NCRE） over the three arid regions are weaker than those in the same latitudinal zone of the Northern Hemisphere. In most cold months（November–March）, the longwave（LW）CRE is stronger than the SWCRE over the three arid regions, leading to a positive NCRE and radiative warming in the regional atmosphere–land surface system. The cold-season mean NCRE at the top of the atmosphere（TOA） averaged over EA is 4.1 W m^-2, with a positive NCRE from November to March, and the intensity and duration of the positive NCRE is larger than that over CA and NA. The CREs over the arid regions of EA exhibit remarkable annual cycles due to the influence of the monsoon in the south. The TOA LWCRE over arid regions is closely related to the high-cloud fraction, and the SWCRE relates well to the total cloud fraction. In addition, the relationship between the SWCRE and the low-cloud fraction is good over NA because of the considerable occurrence of low cloud. Further results show that the interannual variation of TOA CREs is small over the arid regions of CA and EA, but their surface LWCREs show certain decreasing trends that correspond well to their decreasing total cloud fraction. It is suggested that combined studies of more observational cloud properties and meteorological elements are needed for indepth understanding of cloud–radiation processes over arid regions of the Northern Hemisphere.

CLOUD RADIATIVE AND MICROPHYSICAL EFFECTS ON THE RELATION BETWEEN SPATIAL MEAN RAIN RATE, RAIN INTENSITY AND FRACTIONAL RAINFALL COVERAGE

Cloud radiative and microphysical effects on the relation between spatial mean rain rate, rain intensity and fractional rainfall coverage are investigated in this study by conducting and analyzing a series of two-dimensional cloud resolving model sensitivity experiments of pre-summer torrential rainfall in June 2008. The analysis of time-mean data shows that the exclusion of radiative effects of liquid clouds reduces domain mean rain rate by decreasing convective rain rate mainly through the reduced convective-rainfall area associated with the strengthened hydrometeor gain in the presence of radiative effects of ice clouds, whereas it increases domain mean rain rate by enhancing convective rain rate mainly via the intensified convective rain intensity associated with the enhanced net condensation in the absence of radiative effects of ice clouds. The removal of radiative effects of ice clouds decreases domain mean rain rate by reducing stratiform rain rate through the suppressed stratiform rain intensity related to the suppressed net condensation in the presence of radiative effects of liquid clouds, whereas it increases domain mean rain rate by strengthening convective rain rate mainly via the enhanced convective rain intensity in response to the enhanced net condensation in the absence of radiative effects of liquid clouds. The elimination of microphysical effects of ice clouds suppresses domain mean rain rate by reducing stratiform rain rate through the reduced stratiform-rainfall area associated with severely reduced hydrometeor loss.

Seasonal and Spatial Variation of Radiative Effects of Anthropogenic Sulfate Aerosol

On the basis of the emission data of the industrial sulphur dioxide (SO_2) and observed climate fields over East Asia, the distribution of anthropogenic sulfate aerosol(SO_4~2-) with seasonal variation in the troposphere is simulated and analyzed by a regional sulfur transport model, and the direct radiative effects of SO_4~2- under different weather conditions are also calculated using the discrete ordinate method. The results show that the concentration of SO_4~2- has significant seasonal and spatial variations resulting from the effects of SO_2 emission source and precipitation and wind fields. Both the concentration of SO_2 and its radiative forcing have the largest values in October and the lowest in July. SO_4~2- causes the decrease of the radiation flux absorbed by earth-atmosphere and the cooling of air temperature by scattering more solar radiation back into space. Besides, the radiative and climatic effects of SO_4~2- are related to the types and height and optical thickness, etc., of the clouds.

Radiative Effects on Mixed Convection in a Uniformly HeatedVertical Convergent Channel with an Unheated Moving Plate

Fluids engineering is extremely important in a wide variety of materials processing systems,such as soldering,welding,extrusion of plastics and other polymeric materials,Chemical Vapor Deposition(CVD),composite materials manufacturing.In particular,mixed convection due to moving surfaces is very important in these applications.Mixed convection in a channel,as a result of buoyancy and motion of one of its walls has received little research attention and few guidelines are available for choosing the best performing channel configuration,particularly when radiative effects are significant.In this study a numerical investigation of the effect of radiation on mixed convection in air due to the interaction between a buoyancy flow and an unheated moving plate induced flow in a uniformly heated convergent vertical channel is carried out.The moving plate has a constant velocity and moves in the buoyancy force direction.The principal walls of the channel are heated at uniform heat flux.The numerical analysis is accomplished by means of the commercial code Fluent.The effects of the wall emissivity,the minimum channel spacing,the converging angle and the moving plate velocity are investigated and results in terms of air velocity and temperature fields inside the channel and wall temperature profiles,both of the moving and the heated plates,are given.Nusselt numbers,both accounting and not for the radiative contribution to heat removal,are also presented.

Modeling radiative effects of haze on summer-time convective precipitation over North China： a case study

The impact of haze radiative effect on summertime 24-h convective precipitation over North China was investigated using WRF model （version 3.3） through model sensitivity studies between scenarios with and without aerosol radiative effects. The haze radiative effect was represented by incorporating an idealized aerosol optical profile, with AOD values around 1, derived from the aircraft measurement into the WRF shortwave scheme. We found that the shortwave heating induced by aerosol radiative effects would significantly reduce heavy rainfalls, although its effect on the post-frontal localized thunderstorm precipitation was more diverse. To capture the key factors that determine whether precipitation is enhanced or suppressed, model grids with 24-h precipitation difference between the ：two scenarios exceeding certain threshold （〉30 mm or〈 -30 mm） were separated into two sets. Analyses of key meteorological variables between the enhanced and suppressed regimes suggested that atmospheric convection was the most important factor that determined whether precipitation was enhanced or suppressed during summertime over North China. The convection was stronger over places with precipitation enhancement over 30 mm. Haze weakened the convection over places with precipitation suppression exceeding 30 mm and caused less water vapor to rise to a higher level and thus further suppressed precipitation. The suppression of precipitation was often accompanied with relatively high convective available potential energy （CAPE）, relative humidity （RH） and updraft velocities.

A Review of Aerosol Optical Properties and Radiative Effects

Atmospheric aerosols influence the earth＇s radiative balance directly through scattering and absorbing solar radiation,and indirectly through affecting cloud properties.An understanding of aerosol optical properties is fundamental to studies of aerosol effects on climate.Although many such studies have been undertaken,large uncertainties in describing aerosol optical characteristics remain,especially regarding the absorption properties of different aerosols.Aerosol radiative effects are considered as either positive or negative perturbations to the radiation balance,and they include direct,indirect（albedo effect and cloud lifetime effect）,and semi-direct effects.The total direct effect of anthropogenic aerosols is negative（cooling）,although some components may contribute a positive effect（warming）.Both the albedo effect and cloud lifetime effect cool the atmosphere by increasing cloud optical depth and cloud cover,respectively.Absorbing aerosols,such as carbonaceous aerosols and dust,exert a positive forcing at the top of atmosphere and a negative forcing at the surface,and they can directly warm the atmosphere.Internally mixed black carbon aerosols produce a stronger warming effect than externally mixed black carbon particles do.The semidirect effect of absorbing aerosols could amplify this warming effect.Based on observational（ground- and satellite-based） and simulation studies,this paper reviews current progress in research regarding the optical properties and radiative effects of aerosols and also discusses several important issues to be addressed in future studies.

Effects of sea surface temperature,cloud radiative and microphysical processes,and diurnal variations on rainfall in equilibrium cloud-resolving model simulations

The effects of sea surface temperature（SST）,cloud radiative and microphysical processes,and diurnal variations on rainfall statistics are documented with grid data from the two-dimensional equilibrium cloud-resolving model simulations.For a rain rate of higher than 3 mm.h 1,water vapor convergence prevails.The rainfall amount decreases with the decrease of SST from 29℃ to 27℃,the inclusion of diurnal variation of SST,or the exclusion of microphysical effects of ice clouds and radiative effects of water clouds,which are primarily associated with the decreases in water vapor convergence.However,the amount of rainfall increases with the increase of SST from 29℃ to 31℃,the exclusion of diurnal variation of solar zenith angle,and the exclusion of the radiative effects of ice clouds,which are primarily related to increases in water vapor convergence.For a rain rate of less than 3 mm.h 1,water vapor divergence prevails.Unlike rainfall statistics for rain rates of higher than 3 mm.h 1,the decrease of SST from 29℃ to 27℃ and the exclusion of radiative effects of water clouds in the presence of radiative effects of ice clouds increase the rainfall amount,which corresponds to the suppression in water vapor divergence.The exclusion of microphysical effects of ice clouds decreases the amount of rainfall,which corresponds to the enhancement in water vapor divergence.The amount of rainfall is less sensitive to the increase of SST from 29℃ to 31℃ and to the radiative effects of water clouds in the absence of the radiative effects of ice clouds.

Direct Radiative Effects of Dust Aerosols over Northwest China Revealed by Satellite-Derived Aerosol Three-Dimensional Distribution

Northwest China is recognized as a main source and a major transport channel of dust aerosols in East Asia.With a fragile ecological environment,this region is quite sensitive to global climate change.Based on the satellite-derived aerosol three-dimensional distribution,the direct radiative effects of dust aerosols over Northwest China are evaluated.Aerosols over Northwest China are mainly distributed in the Tarim Basin,Junggar Basin,Gobi Desert,and Loess Plateau.The aerosol extinction coefficients are greater than 0.36 km-1 over the Tarim Basin and 0.16 km^(-1) over the Gobi Desert and Loess Plateau,decreasing with height.Aerosols over Northwest China are mainly composed of pure dust and polluted dust.These dust aerosols can modify the horizontal temperature gradient,vertical thermodynamic structure,and diurnal temperature range by absorbing and scattering shortwave radiation and emitting longwave radiation.For the column atmosphere,the radiative effect of dust aerosols shows heating effect of approximately 0.3 K day^(-1) during the daytime and cooling effect of approximately-0.4 K day^(-1) at night.In the vertical direction,dust aerosols can heat up the lower atmosphere(0.5–1.5 K day^(-1))and cool down the upper atmosphere(about-1.0 K day^(-1))during the daytime,while they cool down the lower atmosphere(-3 to-1.5 K day^(-1))and heat up the upper atmosphere(1–1.5 K day^(-1))at night.There are also significant lateral and vertical variations in the dust radiative effects corresponding to their spatial distributions.This study provides some scientific basis for reducing uncertainty in the investigation of aerosol radiative effects and provides observation evidence for simulation studies.

RADIATIVE AND MICROPHYSICAL EFFECTS OF ICE CLOUDS ON A TORRENTIAL RAINFALL EVENT OVER HUNAN,CHINA

The radiative and microphysical effects of ice clouds on a torrential rainfall event over Hunan,China in June 2004 are investigated by analyzing the sensitivity of cloud-resolving model simulations.The model is initialized by zonally-uniform vertical velocity,zonal wind,horizontal temperature and vapor advection from National Centers for Environmental Prediction(NCEP) /National Center for Atmospheric Research(NCAR) reanalysis data.The exclusion of radiative effects of ice clouds increases model domain mean surface rain rates through the increase in the mean net condensation associated with the increase in the mean radiative cooling during the onset phase and the increases in the mean net condensation and the mean hydrometeor loss during the mature phase.The decrease in the mean rain rate corresponds to the decreased mean net condensation and associated mean latent heat release as the enhanced mean radiative cooling by the removal of radiative effects of ice clouds cools the mean local atmosphere during the decay phase.The removal of microphysical effects of ice clouds decreases the mean rain rates through the decrease in the mean net condensation during the onset phase,while the evolution of mean net condensation and the mean hydrometeor changes from decrease to increase during the mature phase.The reduction in the mean rain rate is primarily associated with the mean hydrometeor change in the absence of microphysical effects of ice clouds during the decay phase.

Simulation of the Radiative Effect of Black Carbon Aerosols and the Regional Climate Responses over China

As part of the development work of the Chinese new regional climate model (RIEMS), the radiative process of black carbon (BC) aerosols has been introduced into the original radiative procedures of RIEMS, and the transport model of BC aerosols has also been established and combined with the RIEMS model. Using the new model system, the distribution of black carbon aerosols and their radiative effect over the China region are investigated. The influences of BC aerosole on the atmospheric radiative transfer and on the air temperature, land surface temperature, and total rainfall are analyzed. It is found that BC aerosols induce a positive radiative forcing at the top of the atmosphere (TOA), which is dominated by shortwave radiative forcing. The maximum radiative forcing occurs in North China in July and in South China in April. At the same time, negative radiative forcing is observed on the surface. Based on the radiative forcing comparison between clear sky and cloudy sky, it is found that cloud can enforce the TOA positive radiative forcing and decrease the negative surface radiative forcing. The responses of the climate system in July to the radiative forcing due to BC aerosols are the decrease in the air temperature in the middle and lower reaches of the Changjiang River and Huaihe area and most areas of South China, and the weak increase or decrease in air temperature over North China. The total rainfall in the middle and lower reaches of the Changjiang River area is increased, but it decreased in North China in July.

A Modeling Study of Effective Radiative Forcing and Climate Response Due to Tropospheric Ozone

This study simulates the effective radiative forcing （ERF） of tropospheric ozone from 1850 to 2013 and its effects on global climate using an aerosol-climate coupled model, BCC_AGCM2.0. I_CUACE/Aero, in combination with OMI （Ozone Monitoring Instrument） satellite ozone data. According to the OMI observations, the global annual mean tropospheric col- umn ozone （TCO） was 33.9 DU in 2013, and the largest TCO was distributed in the belts between 30°N and 45°N and at approximately 30°S; the annual mean TCO was higher in the Northern Hemisphere than that in the Southern Hemisphere; and in boreal summer and autumn, the global mean TCO was higher than in winter and spring. The simulated ERF due to the change in tropospheric ozone concentration from 1850 to 2013 was 0.46 W m-2, thereby causing an increase in the global annual mean surface temperature by 0.36°C, and precipitation by 0.02 mm d-1 （the increase of surface temperature had a significance level above 95%）. The surface temperature was increased more obviously over the high latitudes in both hemispheres, with the maximum exceeding 1.4°C in Siberia. There were opposite changes in precipitation near the equator, with an increase of 0.5 mm d- 1 near the Hawaiian Islands and a decrease of about -0.6 mm d- 1 near the middle of the Indian Ocean.

A modeling study of effective radiative forcing and climate response due to increased methane concentration

An atmospheric general circulation model BCC_AGCM2.0 and observation data from ARIS were used to calculate the effective radiative forcing（ERF） due to increased methane concentration since pre-industrial times and its impacts on climate. The ERF of methane from 1750 to2011 was 0.46 W m^-2 by taking it as a well-mixed greenhouse gas, and the inhomogeneity of methane increased its ERF by about 0.02 W m^-2.The change of methane concentration since pre-industrial led to an increase of 0.31 ℃ in global mean surface air temperature and 0.02 mm d 1in global mean precipitation. The warming was prominent over the middle and high latitudes of the Northern Hemisphere（with a maximum increase exceeding 1.4℃）. The precipitation notably increased（maximum increase of 1.8 mm d^-1） over the ocean between 10°N and 20° N and significantly decreased（maximum decrease 〉-0.6 mm d^-1） between 10° S and 10° N. These changes caused a northward movement of precipitation cell in the Intertropical Convergence Zone（ITCZ）. Cloud cover significantly increased（by approximately 4%） in the high latitudes in both hemispheres, and sharply decreased（by approximately 3%） in tropical areas.

Simulation of the Direct Radiative Effect of Mineral Dust and Sea Salt Aerosols in a Doubled Carbon Dioxide Climate

The authors examine the equilibrium climatic response to the direct radiative effect （DRE） of mineral dust and sea salt aerosols in a doubled-CO2 climate with two-way coupling of aerosol-climate interactions.In response to the drier and windier conditions,dust emissions increase by 26％ in the Sahara Desert and by 18％ on the global scale relative to present day.Sea salt emissions increase in high latitudes （＞60°） but decrease in middle latitudes （30°-60°） of both hemispheres due to the poleward shift of westerlies,leading to a 3％ decrease in global emissions.The burdens of dust and sea salt increase by 31％ and 7％ respectively,because reductions in rainfall over the tropical oceans increase the lifetime of particles in the warmer climate.The higher aerosol loading in the doubled-CO2 climate reinforces aerosol DRE by -0.2 W m-2,leading to an additional cooling of 0.1℃ at the surface compared with the climatic effects of aerosols in present day.The additional cooling from changes in natural aerosols compensates for up to 15％ of the regional warming induced by doubled CO2.