The radiation effect of neutrons in a reactor on polyurethane was studied.The gases produced by irradiated samples were analyzed by gas chromatography,and the dynamic mechanical and compression properties of the sampl...The radiation effect of neutrons in a reactor on polyurethane was studied.The gases produced by irradiated samples were analyzed by gas chromatography,and the dynamic mechanical and compression properties of the samples were also studied.The positron annihilation lifetime of irradiated samples was measured at room temperature in vacuum.The experimental results indicate that gas chromatography is a powerful tool to quantitatively analyze the gas products from neutron-irradiated polyurethane and characterizes the chemical changes in the sample.And the changes in microstructure determined from the PAL correlate well with the measurements of the mechanical properties by dynamic mechanical analysis(DMA).展开更多
Twenty five impurity elements in aluminium applied as reactor material are determined. Titanium and nickel are determined with epithermal neutron activation analysis (NAA), magnesium and silicon by inductance coupling...Twenty five impurity elements in aluminium applied as reactor material are determined. Titanium and nickel are determined with epithermal neutron activation analysis (NAA), magnesium and silicon by inductance coupling plasma emission spectra (ICP), other elements by thermal NAA. The fission coefficient of uraniumis given by an experiment, the interferences of uranium to Ce, Nd, Mo, Zr, La, Sin are subtracted. The detection limits of these methods to all of impurity elements in aluminium are calculated.展开更多
A perturbation method is proposed to obtain the effective delayed neutron fraction βeff of a cylindrical highly enriched uranium reactor. Based on reactivity measurements with and without a sample at a specified posi...A perturbation method is proposed to obtain the effective delayed neutron fraction βeff of a cylindrical highly enriched uranium reactor. Based on reactivity measurements with and without a sample at a specified position using the positive period technique, the reactor reactivity perturbation Ap of the sample in βeff units is measured. Simulations of the perturbation experiments are performed using the MCNP program. The PERT card is used to provide the difference dk of effective neutron multiplication factors with and without the sample inside the reactor. Based on the relationship between the effective multiplication factor and the reactivity, the equation βeff=dk/△ρ is derived. In this paper, the reactivity perturbations of 13 metal samples at the designable position of the reactor are measured and calculated. The average βeff value of the reactor is given as 0.00645, and the standard uncertainty is 3.0%. Additionally, the perturbation experiments for fleer can be used to evaluate the reliabilities of the delayed neutron parameters. This work shows that the delayed neutron data of 235U and 23SU froin G.R. Keepin's publication are more reliable than those from ENDF-B6.0, ENDF-B7.0, JENDL3.3 and CENDL2.2.展开更多
基金Funded by the Joint Foundation of the National Natural Science Foundation Committee and China Academy of Engineering Physics (No.10576029)
文摘The radiation effect of neutrons in a reactor on polyurethane was studied.The gases produced by irradiated samples were analyzed by gas chromatography,and the dynamic mechanical and compression properties of the samples were also studied.The positron annihilation lifetime of irradiated samples was measured at room temperature in vacuum.The experimental results indicate that gas chromatography is a powerful tool to quantitatively analyze the gas products from neutron-irradiated polyurethane and characterizes the chemical changes in the sample.And the changes in microstructure determined from the PAL correlate well with the measurements of the mechanical properties by dynamic mechanical analysis(DMA).
文摘Twenty five impurity elements in aluminium applied as reactor material are determined. Titanium and nickel are determined with epithermal neutron activation analysis (NAA), magnesium and silicon by inductance coupling plasma emission spectra (ICP), other elements by thermal NAA. The fission coefficient of uraniumis given by an experiment, the interferences of uranium to Ce, Nd, Mo, Zr, La, Sin are subtracted. The detection limits of these methods to all of impurity elements in aluminium are calculated.
基金Supported by Foundation of Key Laboratory of Neutron Physics,China Academy of Engineering Physics(2012AA01,2014AA01)National Natural Science Foundation(11375158,91326104)
文摘A perturbation method is proposed to obtain the effective delayed neutron fraction βeff of a cylindrical highly enriched uranium reactor. Based on reactivity measurements with and without a sample at a specified position using the positive period technique, the reactor reactivity perturbation Ap of the sample in βeff units is measured. Simulations of the perturbation experiments are performed using the MCNP program. The PERT card is used to provide the difference dk of effective neutron multiplication factors with and without the sample inside the reactor. Based on the relationship between the effective multiplication factor and the reactivity, the equation βeff=dk/△ρ is derived. In this paper, the reactivity perturbations of 13 metal samples at the designable position of the reactor are measured and calculated. The average βeff value of the reactor is given as 0.00645, and the standard uncertainty is 3.0%. Additionally, the perturbation experiments for fleer can be used to evaluate the reliabilities of the delayed neutron parameters. This work shows that the delayed neutron data of 235U and 23SU froin G.R. Keepin's publication are more reliable than those from ENDF-B6.0, ENDF-B7.0, JENDL3.3 and CENDL2.2.