Core-Excited Molecules by Resonant Intense X-Ray Pulses Involving Electron-Rotation Coupling

It has been reported that electron-rotation coupling plays a significant role in diatomic nuclear dynamics induced by intense VUV pulses [Phys. Rev. A 102(2020) 033114;Phys. Rev. Res. 2(2020) 043348]. As a further step, we present here investigations of the electron-rotation coupling effect in the presence of Auger decay channel for core-excited molecules, based on theoretical modeling of the total electron yield(TEY), resonant Auger scattering(RAS) and x-ray absorption spectra(XAS) for two showcases of CO and CH^(+) molecules excited by resonant intense x-ray pulses. The Wigner D-functions and the universal transition dipole operators are introduced to include the electron-rotation coupling for the core-excitation process. It is shown that with the pulse intensity up to 10^(16) W/cm^(2), no sufficient influence of the electron-rotation coupling on the TEY and RAS spectra can be observed. This can be explained by a suppression of the induced electron-rotation dynamics due to the fast Auger decay channel, which does not allow for effective Rabi cycling even at extreme field intensities,contrary to transitions in optical or VUV range. For the case of XAS, however, relative errors of about 10% and 30% are observed for the case of CO and CH^(+), respectively, when the electron-rotation coupling is neglected.It is concluded that conventional treatment of the photoexcitation, neglecting the electron-rotation coupling,can be safely and efficiently employed to study dynamics at the x-ray transitions by means of electron emission spectroscopy, yet the approximation breaks down for nonlinear processes as stimulated emission, especially for systems with light atoms.

Restructuring of plasmonic nanoparticle aggregates with arbitrary particle size distribution in pulsed laser fields

We have studied processes of interaction of pulsed laser radiation with resonant groups of plasmonic nanoparticles（resonant domains） in large colloidal nanoparticle aggregates having different interparticle gaps and particle size distributions.These processes are responsible for the origin of nonlinear optical effects and photochromic reactions in multiparticle aggregates.To describe photo-induced transformations in resonant domains and alterations in their absorption spectra remaining after the pulse action,we introduce the factor of spectral photomodification.Based on calculation of changes in thermodynamic,mechanical,and optical characteristics of the domains,the histograms of the spectrum photomodification factor have been obtained for various interparticle gaps,an average particle size,and the degree of polydispersity.Variations in spectra have been analyzed depending on the intensity of laser radiation and various combinations of size characteristics of domains.The obtained results can be used to predict manifestation of photochromic effects in composite materials containing different plasmonic nanoparticle aggregates in pulsed laser fields.

Harmonic dissipative soliton resonance pulses in a fiber ring laser at different values of anomalous dispersion

The pulse dynamics of harmonic mode-locking in a dissipative soliton resonance(DSR) region in an erbiumdoped fiber ring laser is investigated at different values of anomalous dispersion. The fiber laser is mode-locked by a nonlinear polarization rotation technique. By inserting 0–200 m anomalous dispersion single-mode fiber in the laser cavity, the cavity length is changed from 17.3 to 217.3 m, and the corresponding dispersion of the cavity ranges from -0.27 to-4.67 ps^2. The observed results show that the tuning range of repetition rate under a harmonic DSR condition is highly influenced by the cavity dispersion. Furthermore, it is found that, by automatically adjusting their harmonic orders, the lasers can work at certain values of repetition rate, which are independent of the cavity length and dispersion. The pulses at the same repetition rate in different laser configurations have similar properties, demonstrating that each achievable repetition rate represents an operation regime of harmonic DSR lasers.

Practical pulse engineering： Gradient ascent without matrix exponentiation

Since 2005, there has been a huge growth in the use of engineered control pulses to perform desired quantum operations in systems such as nuclear magnetic resonance quantum information processors. These approaches, which build on the original gradient ascent pulse engineering algorithm, remain computationally intensive because of the need to calculate matrix exponentials for each time step in the control pulse. In this study, we discuss how the propagators for each time step can be approximated using the Trotter-Suzuki formula, and a further speedup achieved by avoiding unnecessary operations. The resulting procedure can provide substantial speed gain with negligible costs in the propagator error, providing a more practical approach to pulse en-ineerinK.

Stopping and storing light pulses within a fiber optic ring resonator

A simple all optical system for stopping and storing light pulses is demonstrated. The system consists of an erbium-doped fiber amplifier （EDFA）, a semiconductor optical amplifier （SOA）, and a fiber ring resonator. The results show that the multisoliton generation with a free spectrum range of 2.4 nm and a pulse spectral width of 0.96 nm is achieved. The memory time of 15 min and the maximum soliton output power of 5.94 dBm are noted, respectively. This means that light pulses can be trapped, i.e., stopped optically within the fiber ring resonator.