Aggregate dust model to study the polarization properties of comet C/1996 B2 Hyakutake

The observed linear polarization data of comet Hyakutake are studied at wavelengths λ=0.365 μm,λ=0.485 μm and 0.684μm through simulations using Ballistic Particle-Cluster Aggregate and Ballistic Cluster-Cluster Aggregate aggregates of 128 spherical monomers.We first found that the size parameter of the monomer,x ～ 1.56-1.70,turned out to be the most suitable which provides the best fits to the observed dust scattering properties at three wavelengths：λ=0.365 μm,0.485μm and 0.684μm.Thus,the effective radius of the aggregate （r） lies in the range 0.45 μm ≤ r ≤ 0.49 μm at λ=0.365 μm;0.60 μm ≤ r ≤ 0.66 μm at λ=0.485 μm and 0.88 μm ≤ r ≤ 0.94 μm at λ=0.684 μm.Now using superposition T-MATRIX code and the power-law size distribution,n（r） ～ r-3,the best-fitting values of complex refractive indices are calculated for the observed polarization data at the above three wavelengths.The best-fitting complex refractive indices （n,k） are found to be （1.745,0.095） at λ=0.365 μm,（1.743,0.100） at λ=0.485 μm and （1.695,0.100） at λ=0.684 μm.The refractive indices derived from the present analysis correspond to a mixture of both silicates and organics,which are in good agreement with the in situ measurement of comets by different spacecraft.

Changes in visibility with PM_(2.5) composition and relative humidity at a background site in the Pearl River Delta region

In fall–winter, 2007–2013, visibility and light scattering coefficients（b sp） were measured along with PM_（2.5）mass concentrations and chemical compositions at a background site in the Pearl River Delta（PRD） region. The daily average visibility increased significantly（p 〈 0.01） at a rate of 1.1 km/year, yet its median stabilized at ~13 km. No haze days occurred when the 24-hr mean PM_（2.5）mass concentration was below 75 μg/m^3. By multiple linear regression on the chemical budget of particle scattering coefficient（b sp）, we obtained site-specific mass scattering efficiency（MSE） values of 6.5 ± 0.2, 2.6 ± 0.3, 2.4 ± 0.7 and 7.3 ± 1.2 m2/g,respectively, for organic matter（OM）, ammonium sulfate（AS）, ammonium nitrate（AN） and sea salt（SS）. The reconstructed light extinction coefficient（b ext） based on the Interagency Monitoring of Protected Visual Environments（IMPROVE） algorithm with our site-specific MSE revealed that OM, AS, AN, SS and light-absorbing carbon（LAC） on average contributed 45.9% ± 1.6%,25.6% ± 1.2%, 12.0% ± 0.7%, 11.2% ± 0.9% and 5.4% ± 0.3% to light extinction, respectively.Averaged b ext displayed a significant reduction rate of 14.1/Mm·year（p 〈 0.05）; this rate would be 82% higher if it were not counteracted by increasing relative humidity（RH） and hygroscopic growth factor（f（RH）） at rates of 2.5% and 0.16/year-1（p 〈 0.01）, respectively, during the fall–winter, 2007–2013. This growth of RH and f（RH） partly offsets the positive effects of lowered AS in improving visibility, and aggravated the negative effects of increasing AN to impair visibility.