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Mineral and Sea-Salt Aerosol Fluxes over the Last 340 kyr Reconstructed from the Total Concentration of Al and Na in the Dome Fuji Ice Core 被引量:1
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作者 Hironori Sato Toshitaka Suzuki +3 位作者 Motohiro Hirabayashi Yoshinori Iizuka Hideaki Motoyama Yoshiyuki Fujii 《Atmospheric and Climate Sciences》 2013年第2期186-192,共7页
A quantitative analysis of the total concentrations of Al and Na in the Antarctic ice sheet during the past 340 kyr was performed by applying the acid digestion method to the Dome Fuji ice core. Atmospheric fluxes of ... A quantitative analysis of the total concentrations of Al and Na in the Antarctic ice sheet during the past 340 kyr was performed by applying the acid digestion method to the Dome Fuji ice core. Atmospheric fluxes of mineral and sea-salt aerosol to Dome Fuji were calculated from the total concentration. The average fluxes of mineral aerosol to Dome Fuji in the periods of glacial maximum, 18.6 ± 10.1 mg·m–2·yr–1, were larger than the value in the interglacial periods, 3.77 ± 2.20 mg·m–2·yr–1. Conversely, the fluxes of sea-salt have no significant difference between the average value of glacial maximum, 130 ± 55 mg·m–2·yr–1, and that of interglacial, 111 ± 54 mg·m–2·yr–1. The results obtained in this study suggest that the variation of mineral aerosol flux in Dome Fuji, together with climate change, was much larger than that of sea-salt aerosol flux. This result may have occurred because the variety in the intensity of the source and transport during the glacial-interglacial cycle is more significant for mineral aerosol than that for sea-salt aerosol. 展开更多
关键词 Ice Core ANTARCTICA DOME FUJI Climate Change aerosol Flux Full DIGESTION
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Simulation of the Ecosystem Productivity Responses to Aerosol Diffuse Radiation Fertilization Effects over the Pan-Arctic during 2001–19 被引量:1
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作者 Zhiding ZHANG Xu YUE +3 位作者 Hao ZHOU Jun ZHU Yadong LEI Chenguang TIAN 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第1期84-96,共13页
The pan-Arctic is confronted with air pollution transported from lower latitudes.Observations have shown that aerosols help increase plant photosynthesis through the diffuse radiation fertilization effects(DRFEs).Whil... The pan-Arctic is confronted with air pollution transported from lower latitudes.Observations have shown that aerosols help increase plant photosynthesis through the diffuse radiation fertilization effects(DRFEs).While such DRFEs have been explored at low to middle latitudes,the aerosol impacts on pan-Arctic ecosystems and the contributions by anthropogenic and natural emission sources remain less quantified.Here,we perform regional simulations at 0.2o×0.2ousing a well-validated vegetation model(Yale Interactive terrestrial Biosphere,YIBs)in combination with multi-source of observations to quantify the impacts of aerosol DRFEs on the net primary productivity(NPP)in the pan-Arctic during 2001-19.Results show that aerosol DRFEs increase pan-Arctic NPP by 2.19 Pg C(12.8%)yr^(-1)under clear-sky conditions,in which natural and anthropogenic sources contribute to 8.9% and 3.9%,respectively.Under all-sky conditions,such DRFEs are largely dampened by cloud to only 0.26 Pg C(1.24%)yr^(-1),with contributions of 0.65% by natural and 0.59% by anthropogenic species.Natural aerosols cause a positive NPP trend of 0.022% yr^(-1)following the increased fire activities in the pan-Arctic.In contrast,anthropogenic aerosols induce a negative trend of-0.01% yr^(-1)due to reduced emissions from the middle latitudes.Such trends in aerosol DRFEs show a turning point in the year of 2007 with more positive NPP trends by natural aerosols but negative NPP trends by anthropogenic aerosols thereafter.Though affected by modeling uncertainties,this study suggests a likely increasing impact of aerosols on terrestrial ecosystems in the pan-Arctic under global warming. 展开更多
关键词 diffuse radiation fertilization effects anthropogenic aerosols natural aerosols pan-Arctic net primary productivity
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Electric field and force characteristic of dust aerosol particles on the surface of high-voltage transmission line
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作者 刘滢格 李兴财 +2 位作者 王娟 马鑫 孙文海 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第1期368-378,共11页
High-voltage transmission lines play a crucial role in facilitating the utilization of renewable energy in regions prone to desertification. The accumulation of atmospheric particles on the surface of these lines can ... High-voltage transmission lines play a crucial role in facilitating the utilization of renewable energy in regions prone to desertification. The accumulation of atmospheric particles on the surface of these lines can significantly impact corona discharge and wind-induced conductor displacement. Accurately quantifying the force exerted by particles adhering to conductor surfaces is essential for evaluating fouling conditions and making informed decisions. Therefore, this study investigates the changes in electric field intensity along branched conductors caused by various fouling layers and their resulting influence on the adhesion of dust particles. The findings indicate that as individual particle size increases, the field strength at the top of the particle gradually decreases and eventually stabilizes at approximately 49.22 k V/cm, which corresponds to a field strength approximately 1.96 times higher than that of an unpolluted transmission line. Furthermore,when particle spacing exceeds 15 times the particle size, the field strength around the transmission line gradually decreases and approaches the level observed on non-adhering surface. The electric field remains relatively stable. In a triangular arrangement of three particles, the maximum field strength at the tip of the fouling layer is approximately 1.44 times higher than that of double particles and 1.5 times higher compared to single particles. These results suggest that particles adhering to the transmission line have a greater affinity for adsorbing charged particles. Additionally, relevant numerical calculations demonstrate that in dry environments, the primary adhesion forces between particles and transmission lines follow an order of electrostatic force and van der Waals force. Specifically, at the minimum field strength, these forces are approximately74.73 times and 19.43 times stronger than the gravitational force acting on the particles. 展开更多
关键词 high-voltage current electric field aerosol particles force characteristic
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Composition optimization and performance prediction for ultra-stable water-based aerosol based on thermodynamic entropy theory
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作者 Tingting Kang Canjun Yan +6 位作者 Xinying Zhao Jingru Zhao Zixin Liu Chenggong Ju Xinyue Zhang Yun Zhang Yan Wu 《Defence Technology(防务技术)》 SCIE EI CAS CSCD 2024年第3期437-446,共10页
Water-based aerosol is widely used as an effective strategy in electro-optical countermeasure on the battlefield used to the preponderance of high efficiency,low cost and eco-friendly.Unfortunately,the stability of th... Water-based aerosol is widely used as an effective strategy in electro-optical countermeasure on the battlefield used to the preponderance of high efficiency,low cost and eco-friendly.Unfortunately,the stability of the water-based aerosol is always unsatisfactory due to the rapid evaporation and sedimentation of the aerosol droplets.Great efforts have been devoted to improve the stability of water-based aerosol by using additives with different composition and proportion.However,the lack of the criterion and principle for screening the effective additives results in excessive experimental time consumption and cost.And the stabilization time of the aerosol is still only 30 min,which could not meet the requirements of the perdurable interference.Herein,to improve the stability of water-based aerosol and optimize the complex formulation efficiently,a theoretical calculation method based on thermodynamic entropy theory is proposed.All the factors that influence the shielding effect,including polyol,stabilizer,propellant,water and cosolvent,are considered within calculation.An ultra-stable water-based aerosol with long duration over 120 min is obtained with the optimal fogging agent composition,providing enough time for fighting the electro-optic weapon.Theoretical design guideline for choosing the additives with high phase transition temperature and low phase transition enthalpy is also proposed,which greatly improves the total entropy change and reduce the absolute entropy change of the aerosol cooling process,and gives rise to an enhanced stability of the water-based aerosol.The theoretical calculation methodology contributes to an abstemious time and space for sieving the water-based aerosol with desirable performance and stability,and provides the powerful guarantee to the homeland security. 展开更多
关键词 Ultra-stable Water-based aerosol Thermodynamic entropy Composition optimization Performance prediction
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Optical Modeling of Sea Salt Aerosols Using in situ Measured Size Distributions and the Impact of Larger Size Particles
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作者 Wushao LIN Lei BI 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第10期1917-1935,共19页
Sea salt aerosols play a critical role in regulating the global climate through their interactions with solar radiation.The size distribution of these particles is crucial in determining their bulk optical properties.... Sea salt aerosols play a critical role in regulating the global climate through their interactions with solar radiation.The size distribution of these particles is crucial in determining their bulk optical properties.In this study,we analyzed in situ measured size distributions of sea salt aerosols from four field campaigns and used multi-mode lognormal size distributions to fit the data.We employed super-spheroids and coated super-spheroids to account for the particles’non-sphericity,inhomogeneity,and hysteresis effect during the deliquescence and crystallization processes.To compute the singlescattering properties of sea salt aerosols,we used the state-of-the-art invariant imbedding T-matrix method,which allows us to obtain accurate optical properties for sea salt aerosols with a maximum volume-equivalent diameter of 12μm at a wavelength of 532 nm.Our results demonstrated that the particle models developed in this study were successful in replicating both the measured depolarization and lidar ratios at various relative humidity(RH)levels.Importantly,we observed that large-size particles with diameters larger than 4μm had a substantial impact on the optical properties of sea salt aerosols,which has not been accounted for in previous studies.Specifically,excluding particles with diameters larger than 4μm led to underestimating the scattering and backscattering coefficients by 27%−38%and 43%−60%,respectively,for the ACE-Asia field campaign.Additionally,the depolarization ratios were underestimated by 0.15 within the 50%−70%RH range.These findings emphasize the necessity of considering large particle sizes for optical modeling of sea salt aerosols. 展开更多
关键词 sea salt aerosol particle size distribution LIDAR optical property
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Contrast in Secondary Organic Aerosols between the Present Day and the Preindustrial Period:The Importance of Nontraditional Sources and the Changed Atmospheric Oxidation Capability
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作者 Yingchuan YANG Wenyi YANG +13 位作者 Xueshun CHEN Jiawen ZHU Huansheng CHEN Yuanlin WANG Wending WANG Lianfang WEI Ying WEI Qian YE Huiyun DU Zichen WU Zhe WANG Jie LI Xiaodong ZENG Zifa WANG 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第10期1936-1952,I0002-I0010,共26页
Quantifying differences in secondary organic aerosols(SOAs)between the preindustrial period and the present day is crucial to assess climate forcing and environmental effects resulting from anthropogenic activities.Th... Quantifying differences in secondary organic aerosols(SOAs)between the preindustrial period and the present day is crucial to assess climate forcing and environmental effects resulting from anthropogenic activities.The lack of vegetation information for the preindustrial period and the uncertainties in describing SOA formation are two leading factors preventing simulation of SOA.This study calculated the online emissions of biogenic volatile organic compounds(VOCs)in the Aerosol and Atmospheric Chemistry Model of the Institute of Atmospheric Physics(IAP-AACM)by coupling the Model of Emissions of Gases and Aerosols from Nature(MEGAN),where the input vegetation parameters were simulated by the IAP Dynamic Global Vegetation Model(IAP-DGVM).The volatility basis set(VBS)approach was adopted to simulate SOA formation from the nontraditional pathways,i.e.,the oxidation of intermediate VOCs and aging of primary organic aerosol.Although biogenic SOAs(BSOAs)were dominant in SOAs globally in the preindustrial period,the contribution of nontraditional anthropogenic SOAs(ASOAs)to the total SOAs was up to 35.7%.In the present day,the contribution of ASOAs was 2.8 times larger than that in the preindustrial period.The contribution of nontraditional sources of SOAs to SOA was as high as 53.1%.The influence of increased anthropogenic emissions in the present day on BSOA concentrations was greater than that of increased biogenic emission changes.The response of BSOA concentrations to anthropogenic emission changes in the present day was more sensitive than that in the preindustrial period.The nontraditional sources and the atmospheric oxidation capability greatly affect the global SOA change. 展开更多
关键词 IAP-AACM VBS MEGAN secondary organic aerosol anthropogenic and biogenic emissions
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Experimental investigation on effective aerosol scavenging using different spray configurations with pre-injection of water mist for Fukushima Daiichi decommissioning
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作者 Rui-Cong Xu Avadhesh Kumar Sharma +2 位作者 Erdal Ozdemir Shuichiro Miwa Shunichi Suzuki 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2024年第5期154-172,共19页
During the decommissioning of the Fukushima Daiichi nuclear power plant,it is important to consider the retrieval of resolidified debris both in air and underwater configurations.For the subsequent retrieval of debris... During the decommissioning of the Fukushima Daiichi nuclear power plant,it is important to consider the retrieval of resolidified debris both in air and underwater configurations.For the subsequent retrieval of debris from the reactor building,the resolidified debris must be cut into smaller pieces using various cutting methods.During the cutting process,aerosol particles are expected to be generated at the submicron scale.It has been noted that such aerosols sizing within the Greenfield gap(0.1-1μm)are difficult to remove effectively using traditional spraying methods.Therefore,to improve the aerosol removal efficiency of the spray system,a new aerosol agglomeration method was recently proposed,which involves injecting water mist to enlarge the sizes of the aerosol particles before removing them using water sprays.In this study,a series of experiments were performed to clarify the proper spray configurations for effective aerosol scavenging and to improve the performance of the water mist.The experimental results showed that the spray flow rate and droplet characteristics are important factors for the aerosol-scavenging efficiency and performance of the water mist.The results obtained from this study will be helpful for the optimization of the spray system design for effective aerosol scavenging during the decommissioning of the Fukushima Daiichi plant. 展开更多
关键词 Fukushima Daiichi decommissioning aerosol scavenging Multiphase flow Spray system aerosol-mist agglomeration
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A Deep-Learning and Transfer-Learning Hybrid Aerosol Retrieval Algorithm for FY4-AGRI:Development and Verification over Asia
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作者 Disong Fu Hongrong Shi +9 位作者 Christian AGueymard Dazhi Yang Yu Zheng Huizheng Che Xuehua Fan Xinlei Han Lin Gao Jianchun Bian Minzheng Duan Xiangao Xia 《Engineering》 SCIE EI CAS CSCD 2024年第7期164-174,共11页
The Advanced Geosynchronous Radiation Imager(AGRI)is a mission-critical instrument for the Fengyun series of satellites.AGRI acquires full-disk images every 15 min and views East Asia every 5 min through 14 spectral b... The Advanced Geosynchronous Radiation Imager(AGRI)is a mission-critical instrument for the Fengyun series of satellites.AGRI acquires full-disk images every 15 min and views East Asia every 5 min through 14 spectral bands,enabling the detection of highly variable aerosol optical depth(AOD).Quantitative retrieval of AOD has hitherto been challenging,especially over land.In this study,an AOD retrieval algorithm is proposed that combines deep learning and transfer learning.The algorithm uses core concepts from both the Dark Target(DT)and Deep Blue(DB)algorithms to select features for the machinelearning(ML)algorithm,allowing for AOD retrieval at 550 nm over both dark and bright surfaces.The algorithm consists of two steps:①A baseline deep neural network(DNN)with skip connections is developed using 10 min Advanced Himawari Imager(AHI)AODs as the target variable,and②sunphotometer AODs from 89 ground-based stations are used to fine-tune the DNN parameters.Out-of-station validation shows that the retrieved AOD attains high accuracy,characterized by a coefficient of determination(R2)of 0.70,a mean bias error(MBE)of 0.03,and a percentage of data within the expected error(EE)of 70.7%.A sensitivity study reveals that the top-of-atmosphere reflectance at 650 and 470 nm,as well as the surface reflectance at 650 nm,are the two largest sources of uncertainty impacting the retrieval.In a case study of monitoring an extreme aerosol event,the AGRI AOD is found to be able to capture the detailed temporal evolution of the event.This work demonstrates the superiority of the transfer-learning technique in satellite AOD retrievals and the applicability of the retrieved AGRI AOD in monitoring extreme pollution events. 展开更多
关键词 aerosol optical depth Retrieval algorithm Deep learning Transfer learning Advanced Geosynchronous Radiation IMAGER
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Aerosol deposition technology and its applications in batteries
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作者 Xinyu Wang Ramon Alberto Paredes Camacho +6 位作者 Xiaoyu Xu Yumei Wang Yi Qiang Hans Kungl Ruediger-AEichel Yunfeng Zhang Li Lu 《Nano Materials Science》 EI CAS CSCD 2024年第1期24-37,共14页
Aerosol deposition(AD)method is a kind of additive manufacturing technology for fabricating dense films such as metals and ceramics at room temperature.It resolves the challenge of integrating ceramic films onto tempe... Aerosol deposition(AD)method is a kind of additive manufacturing technology for fabricating dense films such as metals and ceramics at room temperature.It resolves the challenge of integrating ceramic films onto temperaturesensitive substrates,including metals,glasses,and polymers.It should be emphasized that the AD is a spray coating technology that uses powder without thermal assistance to generate films with high density.Compared to the traditional sputter-based approach,the AD shows several advantages in efficiency,convenience,better interfacial bonding and so on.Therefore,it opens some possibilities to the field of batteries,especially all-solidstate batteries(ASSBs)and draws much attention not only for research but also for large scale applications.The purpose of this work is to provide a critical review on the science and technology of AD as well as its applications in the field of batteries.The process,mechanism and effective parameters of AD,and recent developments in AD applications in the field of batteries will be systematically reviewed so that a trend for AD will be finally provided. 展开更多
关键词 aerosol deposition Room temperature impact consolidation Ceramic film All-solid-state battery Spray coating technology
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Contribution of Satellite Observations in the Optical and Microphysical Characterization of Aerosols in Burkina Faso, West Africa
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作者 Nébon Bado Serge Dimitri Bazyomo +4 位作者 Germain Wende Pouiré Ouedraogo Bruno Korgo Mamadou Simina Dramé Florent P. Kieno Sié Kam 《Atmospheric and Climate Sciences》 2024年第1期154-171,共18页
In this work, we proceed to an optical and microphysical analysis of the observations reversed by the MODIS, SeaWiFS, MISR and OMI sensors with the aim of proposing the best-adapted airborne sensor for better monitori... In this work, we proceed to an optical and microphysical analysis of the observations reversed by the MODIS, SeaWiFS, MISR and OMI sensors with the aim of proposing the best-adapted airborne sensor for better monitoring of aerosols in Burkina Faso. To this end, a comparison of AOD between satellite observations and in situ measurements at the Ouagadougou site reveals an underestimation of AERONET AOD except for OMI which overestimates them. Also, an inter-comparison done based on the linear regression line representation shows the correlation between the aerosol models incorporated in the airborne sensor inversion algorithms and the aerosol population probed. This can be seen through the correlation coefficients R which are 0.84, 0.64, 0.55 and 0.054 for MODIS, SeaWiFS, MISR and OMI respectively. Furthermore, an optical analysis of aerosols in Burkina Faso by the MODIS sensor from 2001 to 2016 indicates a large spatial and temporal variability of particles strongly dominated by desert dust. This is corroborated by the annual and seasonal cycles of the AOD at 550 nm and the Angström coefficient measured in the spectral range between 412 nm and 470 nm. A zoom on a few sites chosen according to the three climatic zones confirms the majority presence of mineral aerosols in Burkina Faso, whose maxima are observed in spring and summer. 展开更多
关键词 AERONET Airborne Sensors aerosol Optical and Microphysical Properties
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Some Features of Black Carbon Aerosols Connected with Regional Climate Over Pristine Environment
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作者 Saurabh Yadav Panuganti C.S.Devara +4 位作者 S.M.Sonbawne B.S.Murthy S.Tiwari S.Wadhwa A.Kumar 《Journal of Atmospheric Science Research》 2024年第1期1-18,共18页
The authors report the results of aethalometer black carbon(BC)aerosol measurements carried out over a rural(pristine)site,Panchgaon,Haryana State,India during the winter months of 2021-2022 and 2022-2023.They are com... The authors report the results of aethalometer black carbon(BC)aerosol measurements carried out over a rural(pristine)site,Panchgaon,Haryana State,India during the winter months of 2021-2022 and 2022-2023.They are compared with collocated and concurrent observations from the Air Quality Monitoring Station(AQMS),which provides synchronous air pollution and surface meteorological parameters.Secular variations in BC mass concentration are studied and explained with variations in local meteorological parameters.The biomass burning fire count retrievals from NASA-NOAA VIIRS satellite,and backward airmass trajectories from NOAA-ERL HYSPLIT Model analysis have also been utilized to explain the findings.They reveal that the north-west Indian region contributes maximum to the BC mass concentration over the study site during the study period.Moreover,the observed BC mass concentrations corroborate the synchronous fire count,primary and secondary pollutant concentrations.The results were found to aid the development of mitigation methods to achieve a sustainable climate system. 展开更多
关键词 Carbonaceous aerosols Dual-spot technique Temporal variations Primary and secondary pollutants Stubble burning Long-range transport Satellite products
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Sea-Salt Aerosol Effects on the Simulated Microphysics and Precipitation in a Tropical Cyclone 被引量:1
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作者 Baolin JIANG Wenshi LIN +1 位作者 Fangzhou LI Junwen CHEN 《Journal of Meteorological Research》 SCIE CSCD 2019年第1期115-125,共11页
We investigate the effects of sea-salt aerosol(SSA) activated as cloud condensation nuclei on the microphysical processes, precipitation, and thermodynamics of a tropical cyclone(TC). The Weather Research and Forecast... We investigate the effects of sea-salt aerosol(SSA) activated as cloud condensation nuclei on the microphysical processes, precipitation, and thermodynamics of a tropical cyclone(TC). The Weather Research and Forecasting model coupled with Chemistry(WRF-Chem) was used together with a parameterization of SSA production. Three simulations, with different levels of SSA emission(CTL, LOW, HIGH), were conducted. The simulation results show that SSA contributes to the processes of autoconversion of cloud water and accretion of cloud water by rain,thereby promoting rain formation. The latent heat release increases with SSA emission, slightly increasing horizontal wind speeds of the TC. The presence of SSA also regulates the thermodynamic structure and precipitation of the TC.In the HIGH simulation, higher latent heat release gives rise to stronger updrafts in the TC eyewall area, leading to enhanced precipitation. In the LOW simulation, due to decreased latent heat release, the temperature in the TC eye is lower, enhancing the downdrafts in the region; and because of conservation of mass, updrafts in the eyewall also strengthen slightly; as a result, precipitation in the LOW experiment is a little higher than that in the CTL experiment.Overall, the relationship between the precipitation rate and SSA emission is nonlinear. 展开更多
关键词 sea-salt aerosol MICROPHYSICS tropical CYCLONE WRF-Chem cloud CONDENSATION NUCLEI
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Crystallization kinetics of sea-salt aerosols studied by high-speed photography 被引量:1
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作者 QIAN ZhengGang WANG Feng +2 位作者 ZHENG YuXia YU JunYing ZHANG YunHong 《Chinese Science Bulletin》 SCIE CAS 2012年第6期591-594,共4页
Morphological changes with decreasing relative humidity(RH) of supersaturated sea-salt aerosol droplets on a quartz substrate were observed using a high-speed video-camera.Stable gypsum(CaSO4·2H2O) or the metasta... Morphological changes with decreasing relative humidity(RH) of supersaturated sea-salt aerosol droplets on a quartz substrate were observed using a high-speed video-camera.Stable gypsum(CaSO4·2H2O) or the metastable hemihydrate(CaSO4·0.5H2O) were precipitated as the RH decreased.The dynamic process of crystal growth under steady-state humidity was studied by controlling the RH;the metastable hemihydrate was precipitated at 70.5%-77.1% RH,and the apparent crystal growth rate was between 1.42 and 2.33 μm3/s.Stable gypsum was formed at 80.7%-82.2% RH,and the apparent crystal growth rate was between 0.70 and 0.81 μm3/s. 展开更多
关键词 气溶胶 结晶动力学 高速摄影 海盐 晶体生长速率 相对湿度 稳定状态 形态学变化
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Sea-salt aerosol transport patterns over the Northern Hemisphere inferred from two subarctic ice core records
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作者 YAN Yuping1,2, KANG Shichang2,3,5, SUN Junying4,5, Paul A. Mayewski2 & QIN Dahe5 1. National Climate Center, China Meteorological Administration, Beijing 100081, China 2. Climate Change Institute, University of Maine, Orono, ME 04469, USA +2 位作者 3. Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing 100085, China 4. Chinese Academy of Meteorological Sciences, Beijing 100081, China 5. Key Laboratory of Ice Core and Cold Regions Environment, Cold and Arid Environmental and Engineering Research Institute, Chinese Academy of Sciences, Lanzhou 730000, China 《Science China Earth Sciences》 SCIE EI CAS 2005年第4期576-584,共9页
Atmospheric circulation reconstruction based on glaciochemical records requires knowledge of chemical concentration controls, such as source, transport pathway and strength. To gain insight into these processes, the r... Atmospheric circulation reconstruction based on glaciochemical records requires knowledge of chemical concentration controls, such as source, transport pathway and strength. To gain insight into these processes, the relationships between glaciochemical records from two Northern Hemisphere sites (Mt. Logan in Yukon Territory and 20D in southern Greenland) and instrumental sea level pressure (SLP) series are investigated. Calibrations between Mt. Logan sea-salt sodium (ssNa+) concentration and SLP series show that ssNa+ concentrations are closely correlated with the autumntime (SON) Aleutian Low and the summertime (JJA) North Pacific Subtropical High. Both the deepened Aleutian Low and enhanced North Pacific Sub- tropical High strengthen the transport of sea-salt aerosols from the North Pacific to the Mt. Logan region. Calibrations between 20D ssNa+ concentrations and SLP series indicate that ssNa+ concentrations are closely related to the wintertime (Jan.) Icelandic Low. A deepening of the Icelandic Low strengthens winter storms and frequent cyclogenesis over the North Atlantic and pushes more sea-salt laden air masses to the Greenland ice sheet. Therefore, ice core ssNa+ records from the Mt. Logan region can be considered as a proxy for reconstructing the au- tumntime Aleutian Low and summertime North Pacific Subtropical High, and the ssNa+ records from Greenland ice core (20D) may provide a proxy for reconstructing the wintertime Icelandic Low. 展开更多
关键词 sea-salt aerosol ICE core records sea level pressure SUBARCTIC regions.
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Modification of Sea-salt Aerosols over the Coastal Area in China
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作者 李放 段民征 吕达仁 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 1998年第4期101-110,共10页
Aerosol particles over the coastal area are subject to the modification of their chemical composition during their transport and diffusion. For examining the modification, the marine aerosol particles are collected at... Aerosol particles over the coastal area are subject to the modification of their chemical composition during their transport and diffusion. For examining the modification, the marine aerosol particles are collected at an island, East China Sea. Comparison of elemental composition of the marine aerosols with that of the samples collected at a coastal site, e.g. in Shanghai, was made. The results of chemical analysis show that the loss of chlorine component in aerosol particles is one of the main characteristics in the course of diffusion of marine aerosols into the coastal continent. Sulphur is a dominant component for fine particles in both marine and coastal aerosols. The relation of particle number concentration and particle size distribution to the meteorological conditions was discussed briefly. These results can be used as a reference in the estimation of equivalent refractive index of the aerosols for radiation transfer. 展开更多
关键词 Marine aerosol MODIFICATION Elemental component Coastal area
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A Statistical Algorithm for Retrieving Background Value of Absorbing Aerosol Index Based on TROPOMI Measurements
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作者 Fuying TANG Weihe WANG +4 位作者 Fuqi SI Haijin ZHOU Yuhan LUO Dongshang YANG Yuanyuan QIAN 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2023年第6期1104-1116,共13页
The ultraviolet aerosol index(UVAI) is essential for monitoring the absorbing aerosols during aerosol events. UVAI depends on the absorbing aerosol concentration, the viewing geometry, and the temporal drift of radiom... The ultraviolet aerosol index(UVAI) is essential for monitoring the absorbing aerosols during aerosol events. UVAI depends on the absorbing aerosol concentration, the viewing geometry, and the temporal drift of radiometric sensitivity. To efficiently detect absorbing aerosols with the highest precision and to improve the accuracy of long-term UVAI estimates,the background UVAI must be examined through the UVAI retrieval. This study presents a statistical method that calculates the background value of UVAI using TROPOspheric Monitoring Instrument(TROPOMI) observation data over the Pacific Ocean under clear-sky scenes. Radiative transfer calculations were performed to simulate the dependence of UVAI on aerosol type and viewing geometry. We firstly applied the background UVAI to reducing the effects of viewing geometry and the degradation of the TROPOMI irradiance measurements on the UVAI. The temporal variability of the background UVAI under the same viewing geometry and aerosol concentration was identified. Radiative transfer calculations were performed to study the changes in background UVAI using Aerosol Optical Depth from the Moderate Resolution Imaging Spectroradiometer(MODIS) and reflectance measurements from TROPOMI as input. The trends of the temporal variations in the background UVAI agreed with the simulations. Alterations in the background UVAI expressed the reflectance variations driven by the changes in satellite state. Decreasing trends in solar irradiance at 340 and 380 nm due to instrument degradation were identified. Our findings are valuable because they can be applied to future retrievals of UVAI from the Environmental Trace Gases Monitoring Instrument(EMI) onboard the Chinese GaoFen-5 satellite. 展开更多
关键词 ultraviolet aerosol index background UVAI TROPOMI reflectance DEGRADATION
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Changes in Aerosol Optical Depth over the Arctic Ocean as Seen by CALIOP, MAIAC, and MODIS C6.1
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作者 Nicole Mölders Mariel Friberg 《Journal of Environmental Protection》 2023年第6期419-440,共22页
Due to the recent increase in Arctic shipping, 2006-2020 June to October Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6.1 (C6.1), and Mult... Due to the recent increase in Arctic shipping, 2006-2020 June to October Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6.1 (C6.1), and Multi-Angle Implementation of Atmospheric Correction (MAIAC) retrieved aerosol optical depth (AOD) data were examined for changes in AOD from period 1 (P1, 2006-2012) to period 2 (P2, 2014-2020 (P2). Herein, AOD was statistically analyzed on a 0.25° × 0.25° grid and in the airsheds over the various ocean basins over the Arctic north of 59.75°N. According to heatmaps of the correlation between AOD and ship traffic, and AOD and fire emissions for the airsheds, all three AOD products captured the observed inter-annual variability in wildfire occurrence well, and showed wildfire emissions over Siberia were more severe in P2 than P1. Except for the Atlantic, North, and Baltic Seas, Beaufort Sea, and Barents Sea, all three AOD products indicated that AOD was higher over the various basins in P2 than P1, but disagreed on the magnitude. This fact suggests that the detection of changes in the typical low AOD over the Arctic Ocean might be rather qualitative than quantitative. While all products captured increases in AOD due to ships at berth, only MODIS C6.1 caught the elevated AOD due to shipping on the Siberian rivers. Obviously, sub-daily resolutions are required to capture increased AOD due to short-term events like a traveling ship or short-interval fire. 展开更多
关键词 Arctic aerosol Optical Depth Changes in aerosol Optical Depth Arctic Ship-Emissions Impacts on AOD Boreal Wildfire Impacts on AOD
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Current Status of Rn-220 Chamber Carrier Aerosol Modulation Research
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作者 Yanan Liu Yu Cheng 《Journal of Geoscience and Environment Protection》 2023年第4期30-36,共7页
Radon is the most important source of natural radiation to human beings and the second major causative agent of lung cancer other than smoking. In recent years, the hazards of human exposure to thoron (Rn-220), anothe... Radon is the most important source of natural radiation to human beings and the second major causative agent of lung cancer other than smoking. In recent years, the hazards of human exposure to thoron (Rn-220), another isotope of radon, and its progeny have gained consensus. To accurately evaluate the dose level and hazards of Rn-220 and its progeny, a standard Rn-220 chamber with strong regulation ability for Rn-220 and its progeny needs to be established for the scale or calibration of measurement instruments. This paper describes the hazards, sources, behavioral characteristics of Rn-220 and its progeny, and some representative Rn-220 chambers established in various countries. 展开更多
关键词 THORON Rn-220 Chamber aerosol Modulation
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Temporal and Spatial Distribution of SARS-CoV-2 Aerosols in a Large-Scale Fangcang Shelter Hospital in Shanghai,China
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作者 Jiafu Jiang Zhe Yin +23 位作者 Jing Li Leili Jia Rulin He Wenhui Yang Jihu Yang Hang Fan Sen Zhang Yunfei Wang Zengming Zhao Haoran Peng Lizhong Li Yi Yang Shi-Yong Fan Rong Xiang Jianshu Guo Jinjin Wang Juanning Wei Fengling Zhou Ding Liu Ping Zhao Yujun Cui Yunxi Liu Dongsheng Zhou Gang Dong 《Engineering》 SCIE EI CAS CSCD 2023年第9期222-233,共12页
The coronavirus disease 2019(COVID-19)pandemic caused by frequently mutating severe acute respiratory syndrome coronavirus 2(SARS-CoV-2)has had a worldwide impact.However,detailed data on the potential aerosol transmi... The coronavirus disease 2019(COVID-19)pandemic caused by frequently mutating severe acute respiratory syndrome coronavirus 2(SARS-CoV-2)has had a worldwide impact.However,detailed data on the potential aerosol transmission of SARS-CoV-2 in real-world and controlled laboratory settings remain sparse.During the COVID-19 pandemic in Shanghai,China in 2022,samples were collected in a Fangcang shelter hospital,a large-scale temporary hospital rapidly built by converting the existing National Exhibition and Convention Center(Shanghai)into a health care facility.Aerosol samples at different sites and intervals around patients and in public areas,surface samples,and pharyngeal swab samples from corresponding patients were included.Samples were tested for SARS-CoV-2 using real-time quantitative polymerase chain reaction(RT-qPCR)assays,followed by sequencing if the cycle threshold(Ct)value was<30.The positivity rate for SARS-CoV-2 in aerosol samples was high in contaminated zones(37.5%,104/277),especially around the bed(41.2%,68/165)and near ventilation inlets(45.2%,14/31).The prevalence of SARS-CoV-2 around the bed,public areas,and air inlets of exhaust vents fluctuated and was closely related to the positivity rate among patients at corresponding sampling sites.Some surface samples of different personal protective equipment from medical staff had high positivity rates.Sixty sequences of joined ORF1ab and spike genes obtained from sixty samples represented two main clusters of Omicron SARS-CoV-2.There was consistency in virus sequences from the same patient and their environment,and the detected virus sequences matched those of virus strains in circulation during the collection periods,which indicated a high likelihood of cross-contamination in the Fangcang shelter hospital.In summary,the results provide a quantitative and real landscape of the aerosol transmission of SARS-CoV-2 and a patient-centered view of contamination in large and enclosed spaces and offer a useful guide for taking targeted measures to avoid nosocomial infections during the management of SARS-CoV-2 or other respiratory virus diseases in a Fangcang shelter hospital. 展开更多
关键词 Coronavirus disease 2019 Severe acute respiratory syndrome coronavirus 2 aerosolS Fangcang shelter hospital China
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Design and Characterization of an Aerosol Test Chamber for Emergency Response Patient Contamination Control Simulation and Research
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作者 Megan L. Steele Emily M. Spatz +4 位作者 George P. Lemmer Jacob M. Denney Jeremy M. Slagley Casey W. Cooper Robert M. Eninger 《Occupational Diseases and Environmental Medicine》 2023年第1期78-96,共19页
Contaminated or infected patients present a risk of cross-contamination for emergency responders, attending medical personnel and medical facilities as they enter a treatment facility. The controlled conditions of an ... Contaminated or infected patients present a risk of cross-contamination for emergency responders, attending medical personnel and medical facilities as they enter a treatment facility. The controlled conditions of an aerosol test chamber are required to examine factors of contamination, decontamination, and cross-contamination. This study presents the design, construction, and a method for characterizing an aerosol test chamber for a full-sized manikin on a standard North Atlantic Treaty Organization litter. The methodology combined air velocity measurements, aerosol particle counts and size distributions, and computational fluid dynamics modeling to describe the chamber’s performance in three dimensions. This detailed characterization facilitates future experimental design by predicting chamber performance for a variety of patient-focused research. 展开更多
关键词 Test Chamber Characterization aerosol Generation Exposure Chamber Design Air Velocity Mapping Spatial Variability CFD Modeling Patient Decontamination
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