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Reversible solid-liquid conversion enabled by self-capture effect for stable non-flow zinc-bromine batteries 被引量:1
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作者 Xixi Zhang Xiaoke Wang +7 位作者 Guangmeng Qu Tairan Wang Xiliang Zhao Jun Fan Cuiping Han Xijin Xu Chunyi Zhi Hongfei Li 《Green Energy & Environment》 SCIE EI CAS CSCD 2024年第6期1035-1044,共10页
Non-flow aqueous zinc-bromine batteries without auxiliary components(e.g.,pumps,pipes,storage tanks)and ion-selective membranes represent a cost-effective and promising technology for large-scale energy storage.Unfort... Non-flow aqueous zinc-bromine batteries without auxiliary components(e.g.,pumps,pipes,storage tanks)and ion-selective membranes represent a cost-effective and promising technology for large-scale energy storage.Unfortunately,they generally suffer from serious diffusion and shuttle of polybromide(Br^(-),Br^(3-))due to the weak physical adsorption between soluble polybromide and host carbon materials,which results in low energy efficiency and poor cycling stability.Here,we develop a novel self-capture organic bromine material(1,10-bis[3-(trimethylammonio)propyl]-4,4'-bipyridinium bromine,NVBr4)to successfully realize reversible solid complexation of bromide components for stable non-flow zinc-bromine battery applications.The quaternary ammonium groups(NV^(4+)ions)can effectively capture the soluble polybromide species based on strong chemical interaction and realize reversible solid complexation confined within the porous electrodes,which transforms the conventional“liquid-liquid”conversion of soluble bromide components into“liquid-solid”model and effectively suppresses the shuttle effect.Thereby,the developed non-flow zinc-bromide battery provides an outstanding voltage platform at 1.7 V with a notable specific capacity of 325 mAh g^(-1)NVBr4(1 A g^(-1)),excellent rate capability(200 mAh g^(-1)NVBr4 at 20 A g^(-1)),outstanding energy density of 469.6 Wh kg^(-1)and super-stable cycle life(20,000 cycles with 100%Coulombic efficiency),which outperforms most of reported zinc-halogen batteries.Further mechanism analysis and DFT calculations demonstrate that the chemical interaction of quaternary ammonium groups and bromide species is the main reason for suppressing the shuttle effect.The developed strategy can be extended to other halogen batteries to obtain stable charge storage. 展开更多
关键词 Solid-liquid conversion self-capture Non-flow zinc-bromine batteries Quaternary ammonium
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Self-separation ionic liquid catalyst for the highly effective conversion of H_(2)S by α,β-unsaturated carboxylate esters under mild conditions
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作者 Wenjie Xiong Xiaomin Zhang +1 位作者 Xingbang Hu Youting Wu 《Green Energy & Environment》 SCIE EI CAS CSCD 2024年第9期1440-1448,共9页
The deep-processing utility of pure hydrogen sulfide (H_(2)S) is a significant direction in natural gas chemical industry.Herein,a brand-new strategy of H_(2)S conversion by a,β-unsaturated carboxylate esters into th... The deep-processing utility of pure hydrogen sulfide (H_(2)S) is a significant direction in natural gas chemical industry.Herein,a brand-new strategy of H_(2)S conversion by a,β-unsaturated carboxylate esters into thiols or thioethers using task-specific carboxylate ionic liquids (ILs) as catalyst has been developed,firstly accomplishing the phase separation of product and catalyst without introducing the third component.It can be considered as a cascade reaction in which the product selectivity can be controlled by adjusting the molar ratio of H_(2)S to a,β-unsaturated carboxylate esters.Also,the effects of ILs with different anions and cations,intermittent feeding operations,as well as pressure-time kinetic behaviors on cascade reaction were investigated.Furthermore,the proposed interaction mechanism of H_(2)S conversion using butyl acrylate catalyzed by[Emim][Ac]was revealed by DFT-based theoretical calculation.The approach enables the self-phase separation promotion of catalyst and product and achieves 99%quantitative conversion under mild conditions in the absence of solvent,making the entire process ecologically benign.High-efficiency reaction activity can still be maintained after ten cycles of the catalyst.Therefore,the good results,combined with its simplicity of operation and the high recyclability of the catalyst,make this green method environmentally friendly and cost-effective.It is anticipated that this self-separation method mediated by task-specific ILs will provide a feasible strategy for H_(2)S utilization,which will guide its application on an industrial scale. 展开更多
关键词 Ionic liquid Cascade reaction self-separation H_(2)S conversion Catalysis
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Characteristic changes in astrocyte properties during astrocyte-to-neuron conversion induced by NeuroD1/Ascl1/Dlx2
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作者 Qing He Zhen Wang +5 位作者 Yuchen Wang Mengjie Zhu Zhile Liang Kanghong Zhang Yuge Xu Gong Chen 《Neural Regeneration Research》 SCIE CAS 2025年第6期1801-1815,共15页
Direct in vivo conversion of astrocytes into functional new neurons induced by neural transcription factors has been recognized as a potential new therapeutic intervention for neural injury and degenerative disorders.... Direct in vivo conversion of astrocytes into functional new neurons induced by neural transcription factors has been recognized as a potential new therapeutic intervention for neural injury and degenerative disorders. However, a few recent studies have claimed that neural transcription factors cannot convert astrocytes into neurons, attributing the converted neurons to pre-existing neurons mis-expressing transgenes. In this study, we overexpressed three distinct neural transcription factors––NeuroD1, Ascl1, and Dlx2––in reactive astrocytes in mouse cortices subjected to stab injury, resulting in a series of significant changes in astrocyte properties. Initially, the three neural transcription factors were exclusively expressed in the nuclei of astrocytes. Over time, however, these astrocytes gradually adopted neuronal morphology, and the neural transcription factors was gradually observed in the nuclei of neuron-like cells instead of astrocytes. Furthermore,we noted that transcription factor-infected astrocytes showed a progressive decrease in the expression of astrocytic markers AQP4(astrocyte endfeet signal), CX43(gap junction signal), and S100β. Importantly, none of these changes could be attributed to transgene leakage into preexisting neurons. Therefore, our findings suggest that neural transcription factors such as NeuroD1, Ascl1, and Dlx2 can effectively convert reactive astrocytes into neurons in the adult mammalian brain. 展开更多
关键词 AQUAPORIN-4 Ascl1 ASTROCYTE cortex Dlx2 gap junction glia-to-neuron conversion neural regeneration NeuroD1 REPROGRAMMING
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基于改进Converse断裂点模型和加权Voronoi图的区域城镇体系结构研究——以天水市为例 被引量:11
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作者 郭晓东 李莺飞 马利邦 《地域研究与开发》 CSSCI CSCD 北大核心 2017年第6期70-75,共6页
在对Converse断裂点模型进行改进的基础上,通过构建评价指标体系和计算城镇中心性强度,对天水市城镇体系等级结构进行了划分;通过运用加权Voronoi图,划分了城镇影响范围和城镇经济区。研究表明:1)天水市城镇体系等级分化非常明显,可按... 在对Converse断裂点模型进行改进的基础上,通过构建评价指标体系和计算城镇中心性强度,对天水市城镇体系等级结构进行了划分;通过运用加权Voronoi图,划分了城镇影响范围和城镇经济区。研究表明:1)天水市城镇体系等级分化非常明显,可按中心性值的大小分为3个等级,其中一级城镇主要为天水各县区政府所在地;2)基于加权Voronoi图的城镇经济区打破了行政区划界线,更符合区域"城镇-腹地"相互联系和作用的实际;3)城镇影响空间既受城镇综合实力和区位交通条件的影响,也与地形、资源分布以及历史文化等因素密切相关。在天水市东部和南部,城镇空间影响范围明显大于中部和北部地区。 展开更多
关键词 城镇中心性 城镇等级结构 converse断裂点模型 城镇影响空间 天水市
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应用Converse3D设计和实现虚拟校园 被引量:5
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作者 陶健林 王广军 +1 位作者 章健 苏本跃 《安庆师范学院学报(自然科学版)》 2013年第1期62-65,共4页
高等院校合理运用虚拟校园系统,不仅立体展示校园实景信息和校园文化,而且可以更有效地进行学校的组织管理,同时能够提高学校的知名度、增强学校的竞争力。本文以安庆职业技术学院校园为基础,建立三维实景模型,利用Converse3D虚拟漫游平... 高等院校合理运用虚拟校园系统,不仅立体展示校园实景信息和校园文化,而且可以更有效地进行学校的组织管理,同时能够提高学校的知名度、增强学校的竞争力。本文以安庆职业技术学院校园为基础,建立三维实景模型,利用Converse3D虚拟漫游平台,建立虚拟校园系统,实现实时交互式漫游。 展开更多
关键词 虚拟校园 漫游 三维实景模型 converse3D 实时交互式
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Strong Converse Inequalities for Certain Mixed Szász-Beta Operators 被引量:2
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作者 QI Qiu-lan ZHANG Yu-ping 《Chinese Quarterly Journal of Mathematics》 CSCD 2011年第1期152-158,共7页
In this paper,a strong converse inequality of type B in terms of a new Kfunctional Kλα f,t2(0 < α < 2,0 ≤λ≤ 1) for certain mixed Szász-Beta operators is given.By this inequality,the converse theorem c... In this paper,a strong converse inequality of type B in terms of a new Kfunctional Kλα f,t2(0 < α < 2,0 ≤λ≤ 1) for certain mixed Szász-Beta operators is given.By this inequality,the converse theorem can be obtained for the operators. 展开更多
关键词 Szász-Beta operators K-FUNCTIONAL strong converse inequality Hlder inequality
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Strong Converse Inequalities for Szasz-Mirakjan Operators with Weights 被引量:5
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作者 LIU Guo-jun XUE Yin-chuan SUN Wei-bin 《Chinese Quarterly Journal of Mathematics》 CSCD 北大核心 2008年第3期384-389,共6页
In this paper, we give the strong converse inequalities of type B with the new K-functional Kλα(f,t2)w(0 ≤λ≤ 1, 0 < α < 2) on weighted approximation for Sz′asz-Mirakjan operators, which extend the previou... In this paper, we give the strong converse inequalities of type B with the new K-functional Kλα(f,t2)w(0 ≤λ≤ 1, 0 < α < 2) on weighted approximation for Sz′asz-Mirakjan operators, which extend the previous results. 展开更多
关键词 Szasz-Mirakjan operators strong converse inequalities APPROXIMATION
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A Self-supported Graphene/Carbon Nanotube Hollow Fiber for Integrated Energy Conversion and Storage 被引量:3
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作者 Kai Liu Zilin Chen +4 位作者 Tian Lv Yao Yao Ning Li Huili Li Tao Chen 《Nano-Micro Letters》 SCIE EI CAS CSCD 2020年第5期95-105,共11页
Wearable fiber-shaped integrated energy conversion and storage devices have attracted increasing attention,but it remains a big challenge to achieve a common fiber electrode for both energy conversion and storage with... Wearable fiber-shaped integrated energy conversion and storage devices have attracted increasing attention,but it remains a big challenge to achieve a common fiber electrode for both energy conversion and storage with high performance.Here,we grow aligned carbon nanotubes(CNTs)array on continuous graphene(G)tube,and their seamlessly connected structure provides the obtained G/CNTs composite fiber with a unique self-supported hollow structure.Taking advantage of the hollow structure,other active materials(e.g.,polyaniline,PANI)could be easily functionalized on both inner and outer surfaces of the tube,and the obtained G/CNTs/PANI composite hollow fibers achieve a high mass loading(90%)of PANI.The G/CNTs/PANI composite hollow fibers can not only be used for high-performance fiber-shaped supercapacitor with large specific capacitance of 472 mF cm^-2,but also can replace platinum wire to build fiber-shaped dye-sensitized solar cell(DSSC)with a high power conversion efficiency of 4.20%.As desired,the integrated device of DSSC and supercapacitor with the G/CNTs/PANI composite hollow fiber used as the common electrode exhibits a total power conversion and storage efficiency as high as 2.1%.Furthermore,the self-supported G/CNTs hollow fiber could be further functionalized with other active materials for building other flexible and wearable electronics. 展开更多
关键词 Carbon NANOTUBE GRAPHENE INTEGRATED ENERGY conversion ENERGY STORAGE
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Chloromycetin resistance of clinically isolated E coli is conversed by using EGS technique to repress the Chloromycetin acetyl transferase 被引量:3
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作者 Mei-Ying Gao Chuan-Rui Xu +2 位作者 RU Chen Shou-Gui Liu Jiang-Nan Feng 《World Journal of Gastroenterology》 SCIE CAS CSCD 2005年第46期7368-7373,共6页
AIM: To explore the possibility of repression of chloromycetin (Cm) acyl transferase by using external guided sequence (EGS) in order to converse the clinical E coli isolates from Cm- resistant to Cm- sensitive. ... AIM: To explore the possibility of repression of chloromycetin (Cm) acyl transferase by using external guided sequence (EGS) in order to converse the clinical E coli isolates from Cm- resistant to Cm- sensitive. METHODS: EGS directed against chloromycetin acetyl transferase gene (cat) was cloned to vector pEGFP-C1 which contains the kanamycin (Kin) resistance gene. The recombinant plasmid pEGFP-C1+EGScatl+cat2 was constructed and the blank vector without EGS fragment was used as control plasmids. By using the CaCl2 transformation method, the recombinant plasmids were introduced into the clinically isolated Cm resistant but Km sensitive E coli strains. Transformants were screened on LB agar plates containing Kin. Extraction of plasmids and PCR were applied to identify the positive clones. The growth curve of EGS transformed bacteria cultured in broth with Cm resistance was determined by using spectrophotometer at A600. Drug sensitivity was tested in solid culture containing Cm by using KB method. RESULTS: Transformation studies were carried out on 16 clinically isolated Cm-resistant (250 μg/mL of Cm) E colistrains by using pEGFP-C1-EGScatlcat2 recombinant plasmid. Transformants were screened on LB-agar plates containing Km after the transformation using EGS. Of the 16 tested strains, 4 strains were transformed successfully. Transformants with EGS plasmid showed growth inhibition when grown in liquid broth culture containing 200 μg/mL of Cm. In drug sensitivity test, these strains were sensitive to Cm on LB-agar plates containing 200 μg/mL of Cm. Extraction of plasmids and PCR amplification showed the existence of EGS plasmids in these four transformed strains. These results indicated that the Cat of the four clinical isolates had been suppressed and the four strains were converted to Cm sensitive ones. CONCLUSION: The EGS directed against Cat is able to inhibit the expression of Cat, and hence convert Cm- resistant bacteria to Cm-sensitive ones. Thus, the EGS has the capability of converting the phenotype of clinical drug-resistant isolates strains to drug-sensitive ones. 展开更多
关键词 External guide sequence Drug-resistant bacteria conversion of drug resistance
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Conversion factor analysis of self-balanced loading test of cast-in-situ piles based on analogue test method 被引量:3
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作者 Li Jianhang Li Xiaojuan +2 位作者 Gao Luchao Dai Guoliang Wu Weiguo 《Journal of Southeast University(English Edition)》 EI CAS 2019年第2期185-190,共6页
Based on the characteristics of pile-soil interaction and the Mohr-Coulomb strength theory,a new method of determining the side friction at a pile-soil interaction is proposed.Combined with the actual engineering case... Based on the characteristics of pile-soil interaction and the Mohr-Coulomb strength theory,a new method of determining the side friction at a pile-soil interaction is proposed.Combined with the actual engineering cases,the effectiveness of the analogue test method is verified by comparing it with the traditional anchor pile method and self-balanced method.Taking the self-balanced test of the bridge pile foundation in the Songhua River as an example,the conversion factor of sandy soil and weathered mudstone are confirmed by the analogue test method.The results show that the conversion factor of sandy soil and weathered mudstone in the Songhua River area should consider the geological conditions and the construction technology,etc.The standard values are relatively conservative.It is suggested that the engineering application should be properly revised.The recommended range of the conversion factor of sandy soil in this area is 0.65 to 0.85,and that of weathered mudstone is 1.0. 展开更多
关键词 cast-in-situ piles self-balanced method analogue test method Mohr-Coulomb strength theory conversion factor
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Oxidative Molecular Layer Deposition Tailoring Eco-Mimetic Nanoarchitecture to Manipulate Electromagnetic Attenuation and Self-Powered Energy Conversion 被引量:3
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作者 Jin-Cheng Shu Yan-Lan Zhang +1 位作者 Yong Qin Mao-Sheng Cao 《Nano-Micro Letters》 SCIE EI CAS CSCD 2023年第9期224-237,共14页
Advanced electromagnetic devices,as the pillars of the intelligent age,are setting off a grand transformation,redefining the structure of society to present pluralism and diversity.However,the bombardment of electroma... Advanced electromagnetic devices,as the pillars of the intelligent age,are setting off a grand transformation,redefining the structure of society to present pluralism and diversity.However,the bombardment of electromagnetic radiation on society is also increasingly serious along with the growing popularity of"Big Data".Herein,drawing wisdom and inspiration from nature,an eco-mimetic nanoarchitecture is constructed for the first time,highly integrating the advantages of multiple components and structures to exhibit excellent electromagnetic response.Its electromagnetic properties and internal energy conversion can be flexibly regulated by tailoring microstructure with oxidative molecular layer deposition(oMLD),providing a new cognition to frequency-selective microwave absorption.The optimal reflection loss reaches≈−58 dB,and the absorption frequency can be shifted from high frequency to low frequency by increasing the number of oMLD cycles.Meanwhile,a novel electromagnetic absorption surface is designed to enable ultra-wideband absorption,covering almost the entire K and Ka bands.More importantly,an ingenious self-powered device is constructed using the eco-mimetic nanoarchitecture,which can convert electromagnetic radiation into electric energy for recycling.This work offers a new insight into electromagnetic protection and waste energy recycling,presenting a broad application prospect in radar stealth,information communication,aerospace engineering,etc. 展开更多
关键词 Oxidative molecular layer deposition Eco-mimetic nanoarchitecture Microwave absorption Electromagnetic attenuation self-powered energy conversion device
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STRONG CONVERSE INEQUALITY FOR SZASZ-DURRMEYER OPERATORS 被引量:1
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作者 LI SONG(Department of Applied Mathematics,Zhejiang University, Hangzhou 310027.) 《Applied Mathematics(A Journal of Chinese Universities)》 SCIE CSCD 1996年第3期361-368,共8页
For Szasz-Durrmeyer operators L.(f,x),1<p ∞ we prove that, forsome m,where(x)2=x,M>0,is Ditzian-Totik modulus of smoothness.
关键词 Szasz-Durrmeyer operators strong converse inequality Ditzian-Totik modulus of smoothness.
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Enabling heterogeneous catalysis to achieve carbon neutrality: Directional catalytic conversion of CO_(2) into carboxylic acids 被引量:7
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作者 Xiaofei Zhang Wenhuan Huang +4 位作者 Le Yu Max García-Melchor Dingsheng Wang Linjie Zhi Huabin Zhang 《Carbon Energy》 SCIE EI CAS CSCD 2024年第3期1-35,共35页
The increase in anthropogenic carbon dioxide(CO_(2))emissions has exacerbated the deterioration of the global environment,which should be controlled to achieve carbon neutrality.Central to the core goal of achieving c... The increase in anthropogenic carbon dioxide(CO_(2))emissions has exacerbated the deterioration of the global environment,which should be controlled to achieve carbon neutrality.Central to the core goal of achieving carbon neutrality is the utilization of CO_(2) under economic and sustainable conditions.Recently,the strong need for carbon neutrality has led to a proliferation of studies on the direct conversion of CO_(2) into carboxylic acids,which can effectively alleviate CO_(2) emissions and create high-value chemicals.The purpose of this review is to present the application prospects of carboxylic acids and the basic principles of CO_(2) conversion into carboxylic acids through photo-,electric-,and thermal catalysis.Special attention is focused on the regulation strategy of the activity of abundant catalysts at the molecular level,inspiring the preparation of high-performance catalysts.In addition,theoretical calculations,advanced technologies,and numerous typical examples are introduced to elaborate on the corresponding process and influencing factors of catalytic activity.Finally,challenges and prospects are provided for the future development of this field.It is hoped that this review will contribute to a deeper understanding of the conversion of CO_(2) into carboxylic acids and inspire more innovative breakthroughs. 展开更多
关键词 carbon neutrality carboxylic acids CO_(2)conversion heterogeneous catalyst in situ technology
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A New Self-Assembled Monolayer of Fullerene Derivative and ItsPhotoelectric Conversion Property
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作者 Jin ZHAI Tian Xin WEI +2 位作者 Jun Hao GE Liang Bing GAN Chun Hui HUANG(State Key Laboratory of Rare Earth Materials Chemistry and Applications. Peking University.Beijng 100871) 《Chinese Chemical Letters》 SCIE CAS CSCD 1999年第5期421-424,共4页
A new self-assembled monolayer (SAM) of fullerene derivative has been fabricated and their photoelectric conversion property has been observed. The SAM was fabricated on indium-tin-oxide (ITO) and quartz by amide bond... A new self-assembled monolayer (SAM) of fullerene derivative has been fabricated and their photoelectric conversion property has been observed. The SAM was fabricated on indium-tin-oxide (ITO) and quartz by amide bonding. It was characterized bq contact angle, UV spectrum. and cyclic voltammetry. The mild fabrication conditions and the stability of the SAM provides a way to build three-dimensional structure more easily. 展开更多
关键词 self-assembled monolayer C-60 DERIVATIVES photoelectric conversion
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The Application of Lights-Conversed Polyethylene Film for Agriculture
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作者 Zhang Ke\|li, Yuan Liang\|jie, Xi Mei\|yun, Yu You\|zu, Sun Ju\|tang College of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, Hubei, China 《Wuhan University Journal of Natural Sciences》 CAS 2002年第3期365-367,共3页
Lanthanum-rhodamine (6G and B) complexes were synthesized by Rheological Phase Reaction Method. Lanthanum-rhodamine (6G and B) complexes doped polyethylene films which have a function of lights-conversion were prepare... Lanthanum-rhodamine (6G and B) complexes were synthesized by Rheological Phase Reaction Method. Lanthanum-rhodamine (6G and B) complexes doped polyethylene films which have a function of lights-conversion were prepared. The emission and excitation spectra were measured. The experiments of growing seedling and culture were carried out in the shed built with doped and undoped polyethylene films. Lanthanum-rhodamine doped polyethylene films which have a function of lights-conversion can efficiently convert the green light in the sunlight to the red light for photosynthesis of crops, to promote the maturing of crops and raise the yield of crops. 展开更多
关键词 LANTHANUM lights conversION polyethylene film RHODAMINE rheological phase reaction
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Pathologically successful conversion hepatectomy for advanced giant hepatocellular carcinoma after multidisciplinary therapy:A case report and review of literature 被引量:3
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作者 Ju-Hang Chu Lu-Yao Huang +6 位作者 Ya-Ru Wang Jun Li Shi-Long Han Hao Xi Wen-Xue Gao Ying-Yu Cui Ming-Ping Qian 《World Journal of Gastrointestinal Oncology》 SCIE 2024年第4期1647-1659,共13页
BACKGROUND Hepatocellular carcinoma(HCC)is one of the leading causes of death due to its complexity,heterogeneity,rapid metastasis and easy recurrence after surgical resection.We demonstrated that combination therapy ... BACKGROUND Hepatocellular carcinoma(HCC)is one of the leading causes of death due to its complexity,heterogeneity,rapid metastasis and easy recurrence after surgical resection.We demonstrated that combination therapy with transcatheter arterial chemoembolization(TACE),hepatic arterial infusion chemotherapy(HAIC),Epclusa,Lenvatinib and Sintilimab is useful for patients with advanced HCC.CASE SUMMARY A 69-year-old man who was infected with hepatitis C virus(HCV)30 years previously was admitted to the hospital with abdominal pain.Enhanced computed tomography(CT)revealed a low-density mass in the right lobe of the liver,with a volume of 12.9 cm×9.4 cm×15 cm,and the mass exhibited a“fast-in/fast-out”pattern,with extensive filling defect areas in the right branch of the portal vein and an alpha-fetoprotein level as high as 657 ng/mL.Therefore,he was judged to have advanced HCC.During treatment,the patient received three months of Epclusa,three TACE treatments,two HAIC treatments,three courses of sintilimab,and twenty-one months of lenvatinib.In the third month of treatment,the patient developed severe side effects and had to stop immunotherapy,and the Lenvatinib dose had to be halved.Postoperative pathological diagnosis indicated a complete response.The patient recovered well after the operation,and no tumor recurrence was found.CONCLUSION Multidisciplinary conversion therapy for advanced enormous HCC caused by HCV infection has a significant effect.Individualized drug adjustments should be made during any treatment according to the patient's tolerance to treatment. 展开更多
关键词 Hepatocellular therapy conversion hepatectomy Interventional therapy Epclusa Lenvatinib Sintilimab Case report
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Two-photon live imaging of direct glia-to-neuron conversion in the mouse cortex 被引量:1
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作者 Zongqin Xiang Shu He +13 位作者 Rongjie Chen Shanggong Liu Minhui Liu Liang Xu Jiajun Zheng Zhouquan Jiang Long Ma Ying Sun Yongpeng Qin Yi Chen Wen Li Xiangyu Wang Gong Chen Wenliang Lei 《Neural Regeneration Research》 SCIE CAS CSCD 2024年第8期1781-1788,共8页
Over the past decade,a growing number of studies have reported transcription factor-based in situ reprogramming that can directly conve rt endogenous glial cells into functional neurons as an alternative approach for ... Over the past decade,a growing number of studies have reported transcription factor-based in situ reprogramming that can directly conve rt endogenous glial cells into functional neurons as an alternative approach for n euro regeneration in the adult mammalian central ne rvous system.Howeve r,many questions remain regarding how a terminally differentiated glial cell can transform into a delicate neuron that forms part of the intricate brain circuitry.In addition,concerns have recently been raised around the absence of astrocyte-to-neuron conversion in astrocytic lineage-tra cing mice.In this study,we employed repetitive two-photon imaging to continuously capture the in situ astrocyte-to-neuron conversion process following ecto pic expression of the neural transcription factor NeuroD1 in both prolife rating reactive astrocytes and lineage-tra ced astrocytes in the mouse cortex.Time-lapse imaging over several wee ks revealed the ste p-by-step transition from a typical astrocyte with numero us short,tapered branches to a typical neuro n with a few long neurites and dynamic growth cones that actively explored the local environment.In addition,these lineage-converting cells were able to migrate ra dially or to ngentially to relocate to suitable positions.Furthermore,two-photon Ca2+imaging and patch-clamp recordings confirmed that the newly generated neuro ns exhibited synchronous calcium signals,repetitive action potentials,and spontaneous synaptic responses,suggesting that they had made functional synaptic connections within local neural circuits.In conclusion,we directly visualized the step-by-step lineage conversion process from astrocytes to functional neurons in vivo and unambiguously demonstrated that adult mammalian brains are highly plastic with respect to their potential for neuro regeneration and neural circuit reconstruction. 展开更多
关键词 astrocyte-to-neuron conversion Ca2+imaging direct lineage conversion GLIA ASTROCYTE in vivo reprogramming lineage-tracing mice NeuroD1 NEURON two-photon imaging
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Dealuminated Hβ zeolite for selective conversion of fructose to furfural and formic acid 被引量:1
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作者 Rui Li Qixuan Lin +3 位作者 Junli Ren Xiaobao Yang Yingxiong Wang Lingzhao Kong 《Green Energy & Environment》 SCIE EI CAS CSCD 2024年第2期311-320,共10页
The fructose-to-furfural transformation is facing major challenges in the selectivity and high efficiency. Herein, we have developed a simple and effective approach for the selective conversion of fructose to furfural... The fructose-to-furfural transformation is facing major challenges in the selectivity and high efficiency. Herein, we have developed a simple and effective approach for the selective conversion of fructose to furfural using Hβ zeolite modified by organic acids for dealuminization to regulate its textural and acidic properties. It was found that citric acid-dealuminized Hβ zeolite possessed high specific surface areas, wide channels and high Brønsted acid amount, which facilitated the selective conversion of fructose to furfural with a maximum yield of 76.2% at433 K for 1 h in the γ-butyrolactone(GBL)-H_(2)O system, as well as the concomitant formation of 83.0% formic acid. The^(13)C-isotope labelling experiments and the mechanism revealed that the selective cleavage of C1–C2 or C5–C6 bond on fructose was firstly occurred to form pentose or C5 intermediate by weak Brønsted acid, which was then dehydrated to furfural by strong Brønsted acid. Also this dealuminized Hβ catalyst showed the great recycling performance and was active for the conversion of glucose and mannose. 展开更多
关键词 FRUCTOSE Dealuminated-Hb zeolite Selective conversion FURFURAL
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Oxygen functionalization-assisted anionic exchange toward unique construction of flower-like transition metal chalcogenide embedded carbon fabric for ultra-long life flexible energy storage and conversion 被引量:1
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作者 Roshan M.Bhattarai Kisan Chhetri +5 位作者 Nghia Le Debendra Acharya Shirjana Saud Mai Cao Hoang Phuong Lan Nguyen Sang Jae Kim Young Sun Mok 《Carbon Energy》 SCIE EI CAS CSCD 2024年第1期72-93,共22页
The metal-organic framework(MOF)derived Ni–Co–C–N composite alloys(NiCCZ)were“embedded”inside the carbon cloth(CC)strands as opposed to the popular idea of growing them upward to realize ultrastable energy storag... The metal-organic framework(MOF)derived Ni–Co–C–N composite alloys(NiCCZ)were“embedded”inside the carbon cloth(CC)strands as opposed to the popular idea of growing them upward to realize ultrastable energy storage and conversion application.The NiCCZ was then oxygen functionalized,facilitating the next step of stoichiometric sulfur anion diffusion during hydrothermal sulfurization,generating a flower-like metal hydroxysulfide structure(NiCCZOS)with strong partial implantation inside CC.Thus obtained NiCCZOS shows an excellent capacity when tested as a supercapacitor electrode in a three-electrode configuration.Moreover,when paired with the biomass-derived nitrogen-rich activated carbon,the asymmetric supercapacitor device shows almost 100%capacity retention even after 45,000 charge–discharge cycles with remarkable energy density(59.4 Wh kg^(-1)/263.8μWh cm^(–2))owing to a uniquely designed cathode.Furthermore,the same electrode performed as an excellent bifunctional water-splitting electrocatalyst with an overpotential of 271 mV for oxygen evolution reaction(OER)and 168.4 mV for hydrogen evolution reaction(HER)at 10 mA cm−2 current density along with 30 h of unhinged chronopotentiometric stability performance for both HER and OER.Hence,a unique metal chalcogenide composite electrode/substrate configuration has been proposed as a highly stable electrode material for flexible energy storage and conversion applications. 展开更多
关键词 carbon cloth energy conversion energy storage FLEXIBLE metal embedding ultra-stable
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Enhancing I^(0)/I^(-)Conversion Efficiency by Starch Confinement in Zinc-lodine Battery 被引量:1
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作者 Danyang Zhao Qiancheng Zhu +4 位作者 Qiancheng Zhou Wenming Zhang Ying Yu Shuo Chen Zhifeng Ren 《Energy & Environmental Materials》 SCIE EI CAS CSCD 2024年第1期114-120,共7页
The redox couple of I^(0)/I^(-)in aqueous rechargeable iodine–zinc(I^(2)-Zn)batteries is a promising energy storage resource since it is safe and cost-effective,and provides steady output voltage.However,the cycle li... The redox couple of I^(0)/I^(-)in aqueous rechargeable iodine–zinc(I^(2)-Zn)batteries is a promising energy storage resource since it is safe and cost-effective,and provides steady output voltage.However,the cycle life and efficiency of these batteries remain unsatisfactory due to the uncontrolled shuttling of polyiodide(I_(3)^(-)and I_(5)^(-))and side reactions on the Zn anode.Starch is a very low-cost and widely sourced food used daily around the world.“Starch turns blue when it encounters iodine”is a classic chemical reaction,which results from the unique structure of the helix starch molecule–iodine complex.Inspired by this,we employ starch to confine the shuttling of polyiodide,and thus,the I^(0)/I^(-)conversion efficiency of an I^(2)-Zn battery is clearly enhanced.According to the detailed characterizations and theoretical DFT calculation results,the enhancement of I^(0)/I^(-)conversion efficiency is mainly originated from the strong bonding between the charged products of I_(3)^(-)and I_(5)^(-)and the rich hydroxyl groups in starch.This work provides inspiration for the rational design of high-performance and low-cost I^(2)-Zn in AZIBs. 展开更多
关键词 aqueous battery conversion efficiency iodine-zinc battery starch confinement
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