Developing an efficientmethod to improve the photocatalytic efficiency of graphitic carbon nitride(g-C3 N4)is of great significance for solar H2 production.Electronic structure modulation has been considered one of th...Developing an efficientmethod to improve the photocatalytic efficiency of graphitic carbon nitride(g-C3 N4)is of great significance for solar H2 production.Electronic structure modulation has been considered one of the most crucial strategies to improving the photocatalytic efficiency of g-C_(3)N_(4),but how to efficiently modulate its electronic structure remains a huge challenge.Herein,we,for the first time,report a facile and highly-efficient approach to modulating the electronic structure of g-C_(3)N_(4)through single Ag atom implantation with a Ag_(1)-N_(3)coordination configuration into the g-C_(3)N_(4)framework.展开更多
基金supported by National Natural Science Foundation of China(no.21978030),and also sponsored by the Chinese Ministry of Education via the Program for New Century Excellent Talents in University(no.NCET-12-0079).
文摘Developing an efficientmethod to improve the photocatalytic efficiency of graphitic carbon nitride(g-C3 N4)is of great significance for solar H2 production.Electronic structure modulation has been considered one of the most crucial strategies to improving the photocatalytic efficiency of g-C_(3)N_(4),but how to efficiently modulate its electronic structure remains a huge challenge.Herein,we,for the first time,report a facile and highly-efficient approach to modulating the electronic structure of g-C_(3)N_(4)through single Ag atom implantation with a Ag_(1)-N_(3)coordination configuration into the g-C_(3)N_(4)framework.
