Calculation of stratosphere–troposphere exchange in East Asia cut-off lows:cases from the Lagrangian perspective

In this study,the authors focus on the cut-off low pressure systems（COLs）lingering over East Asia in late spring and early summer and quantify the two-way stratosphere–troposphere exchange（STE）by 3D trajectory integrations,achieved using a revised version of the UK Universities Global Atmospheric Modelling Programme Offline Trajectory Code（Version 3）.By selecting 10 typical COLs and calculating the cross-tropopause air mass fluxes,it is found that stratosphere-to-troposphere transport（STT）fluxes exist in the center of COLs;and in the periphery of the COL center,troposphereto-stratosphere transport（TST）fluxes and STT fluxes are distributed alternately.Net transport fluxes in COLs are from stratosphere to troposphere,and the magnitude is about 10-4 kg m-2 s-1.The ratio between the area-averaged STT and TST fluxes increases with increasing strength of the COLs.By adopting appropriate residence time,the spurious transports are effectively excluded.Finally,the authors compare the results with previous studies,and find that the cross-tropopause fluxes（CTFs）induced by COLs are about one to two orders of magnitude larger than global CTFs.COLs play a significant role in local,rapid air mass exchanges,although they may only be responsible for a fraction of the total STE.

Gravity Wave Activity and Stratosphere-Troposphere Exchange During Typhoon Molave(2020)

To investigate the stratosphere-troposphere exchange(STE)process induced by the gravity waves(GWs)caused by Typhoon Molave(2020)in the upper troposphere and lower stratosphere,we analyzed the ERA5 reanalysis data provided by the European Centre for Medium-Range Weather Forecasts and the CMA Tropical Cyclone Best Track Dataset.We also adopted the mesoscale forecast model Weather Research and Forecasting model V4.3 for numerical simulation.Most of the previous studies were about typhoon-induced STE and typhoon-induced GWs,while our research focused on the STE caused by typhoon-induced gravity waves.Our analysis shows that most of the time,the gravity wave signal of Typhoon Molave appeared below the tropopause.It was stronger on the east side of the typhoon center(10°-20°N,110°-120°E)than on the west side,suggesting an eastward tilted structure with height increase.When the GWs in the upper troposphere and lower stratosphere region on the west side of the typhoon center broke up,it produced strong turbulence,resulting in stratosphere-troposphere exchange.At this time,the average potential vorticity vertical flux increased with the average ozone mass mixing ratio.The gravity wave events and STE process simulated by the WRF model were basically consistent with the results of ERA5 reanalysis data,but the time of gravity wave breaking was different.This study indicates that after the breaking of the GWs induced by typhoons,turbulent mixing will also be generated,and thus the STE.

A multi-location joint field observation of the stratosphere and troposphere over the Tibetan Plateau

The unique geographical location and high altitude of the Tibetan Plateau can greatly influence regional weather and climate.In particular, the Asian summer monsoon(ASM) anticyclone circulation system over the Tibetan Plateau is recognized to be a significant transport pathway for water vapor and pollutants to enter the stratosphere. To improve understanding of these physical processes, a multi-location joint atmospheric experiment was performed over the Tibetan Plateau from late July to August in 2018, funded by the fiveyear(2018–2022) STEAM(stratosphere and troposphere exchange experiment during ASM) project, during which multiple platforms/instruments—including long-duration stratospheric balloons, dropsondes, unmanned aerial vehicles, special sounding systems, and ground-based and satellite-borne instruments—will be deployed. These complementary methods of data acquisition are expected to provide comprehensive atmospheric parameters(aerosol, ozone, water vapor, CO_2, CH_4, CO, temperature, pressure,turbulence, radiation, lightning and wind); the richness of this approach is expected to advance our comprehension of key mechanisms associated with thermal, dynamical, radiative, and chemical transports over the Tibetan Plateau during ASM activity.

The Impact of Cut-off Lows on Ozone in the Upper Troposphere and Lower Stratosphere over Changchun from Ozonesonde Observations

In situ measurements of the vertical structure of ozone were made in Changchun （43.53°N, 125.13°E）, China, by the Institute of Atmosphere Physics, in the summers of 2010-13. Analysis of the 89 validated ozone profiles shows the vari- ation of ozone concentration in the upper troposphere and lower stratosphere （UTLS） caused by cut-off lows （COLs） over Changchun. During the COL events, an increase of the ozone concentration and a lower height of the tropopause are observed. Backward simulations with a trajectory model show that the ozone-rich airmass brought by the COL is from Siberia. A case study proves that stratosphere-troposphere exchange （STE） occurs in the COL. The ozone-rich air mass transported from the stratosphere to the troposphere first becomes unstable, then loses its high ozone concentration. This process usually happens during the decay stage of COLs. In order to understand the influence of COLs on the ozone in the UTLS, statistical analysis of the ozone profiles within COLs, and other profiles, are employed. The results indicate that the ozone concentrations of the in-COL profiles are significantly higher than those of the other profiles between ±4 km around the tropopause. The COLs induce an increase in UTLS column ozone by 32% on average. Meanwhile, the COLs depress the lapse-rate tropopause （LRT）/dynamical tropopause height by 1.4/1.7 km and cause the atmosphere above the tropopause to be less stable. The influence of COLs is durable because the increased ozone concentration lasts at least one day after the COL has passed over Changchun. Furthermore, the relative coefficient between LRT height and lower stratosphere （LS） column ozone is -0.62, which implies a positive correlation between COL strength and LS ozone concentration.

Study on Horizontal Relative Diffusion in theTroposphere and Lower Stratosphere

The behaviour of relative diffusion theory and Gifford’s random-force theory for long-range atmospheric diffusion is examined. When a puff scale is smaller than the Lagrangian length scale, √2KTL, an accelerative relative diffusion region exists, i.e., σy∝ t 3/2. While the puff diffusion enters a two-dimensional turbulence region, in which the diffusion scale is larger than 500 km, or time scale is larger than 1 day, divergence and convergence are main cause of horizontal diffusion. Between the two above-mentioned regimes, diffusion deviation is given by σy = √2KT. The large-scale horizontal relative diffusion parameters were obtained by analyzing the data of radioactive cloud width collected in air nuclear tests. Key words Tropospheric and lower stratospheric diffusion - Relative diffusion - Large scale turbulence - Nuclear explosion clouds This work is sponsored by the National Natural Science Foundation of China under Grant No. 49505064.The author would like to thank Prof. Chen Jiayi Department of Geophysics of Peking University and Dr. Cai Xiaoming School of Geography and Environmental Sciences of Birmingham University for their helpful discussions.

A Two-way Stratosphere–Troposphere Coupling of Submonthly Zonal-Mean Circulations in the Arctic

This paper examines the dominant submonthly variability of zonally symmetrical atmospheric circula- tion in the Northern Hemisphere （NH） winter within the context of the Northern Annular Mode （NAM）, with particular emphasis on interactive stratosphere-troposphere processes. The submonthly variability is identified and measured using a daily NAM index, which concentrates primarily on zonally symmetrical circulation. A schematic lifecycle of submonthly variability is developed that reveals a two-way coupling pro- cess between the stratosphere and troposphere in the NH polar region. Specifically, anomalous tropospheric zonal winds in the Atlantic and Pacific sectors of the Arctic propagate upwards to the low stratosphere, disturbing the polar vortex, and resulting in an anomalous stratospheric geopotential height （HGT） that subsequently propagates down into the troposphere and changes the sign of the surface circulations. From the standpoint of planetary-scale wave activities, a feedback loop is also evident when the anoma- lous planetary-scale waves （with wavenumbers 2 and 3） propagate upwards, which disturbs the anomalous zonally symmetrical flow in the low stratosphere, and induces the anomalous HGT to move poleward in the low stratosphere, and then propagates down into the troposphere. This increases the energy of waves at wavenumbers 2 and 3 in the low troposphere in middle latitudes by enhancing the land-sea contrast of the anomalous HGT field. Thus, this study supports the viewpoint that the downward propagation of stratospheric NAM signals may not originate in the stratosphere.

On the Temporal and Spatial Structure of Troposphere-toStratosphere Transport in the Lowermost Stratosphere over the Asian Monsoon Region during Boreal Summer

This study produced a novel characterization of the troposphere-to-stratosphere transport （TST） over the Asian monsoon region during boreal summer, using a comprehensive analysis of 60-day backward trajectories initialized in the stratosphere. The trajectory datasets were derived from the high-resolution Lagrangian particle dispersion model （FLEXPART） simulation driven by the wind fields acquired from the National Center for Environmental Prediction （NCEP）. The results indicate that the distribution of residence time （tTST） of tropopause-crossing trajectories in the lowermost stratosphere represents a horizontal signature of the Asian summer monsoon. Vertically, the distribution of tTST can be roughly separated into two layers： a consistent lower layer with tTST 〈5 days forming a narrow band, corresponding to a layer-3 km thick following the location of the tropopause, and an upper layer at a larger distance from the local tropopause. The maximum residence time was -20 days, especially within the Asian high anticyclone consistent with its confinement effects. In general, the overall geographical distribution of dehydration points was not coincident with the location of tropopause crossing. TST trajectories, which were initialized in the stratosphere, underwent their Lagrangian cold points mostly in the tropics and subtropics 1 4 days after the TST event; they were characterized by a wide range of temperature differences, with a mean value of 3-12 K. The vertical extent of the influence of tropospheric intrusion on the Asian monsoon region in the stratosphere exhibited a peak at -16.5-18.5 km, and the uppermost height was -21 km.

Variation of Zonal Winds in the Upper Troposphere and Lower Stratosphere in Association with Deficient and Excess Indian Summer Monsoon Scenario

The Indian summer monsoon is one of the most dominant tropical circulation systems in the general circulation of the atmosphere. The country receives more than 80% of the annual rainfall during a short span of four months (June to September) of the southwest monsoon season. Variability in the quantum of rainfall during the monsoon season has profound impacts on water resources, power generation, agriculture, economics and ecosystems in the country. The inter annual variability of Indian Summer Monsoon Rainfall (ISMR) depends on atmospheric and oceanic conditions prevailed during the season. In this study we have made an attempt to understand the variation of the of zonal winds in the tropical Upper Troposphere and Lower Stratosphere (UT/LS) region during deficient and Excess rainfall years of Indian summer monsoon and its relation to Indian Summer Monsoon Rainfall (ISMR). It is found that in the equatorial Upper Troposphere zonal winds have westerly anomalies during deficient rainfall year’s and easterly anomaly during excess rainfall years of Indian summer monsoon and opposite zonal wind anomaly is noted in the equatorial Lower Stratosphere during the deficient and excess rainfall years of Indian summer monsoon. It is also found that the June to September upper troposphere zonal winds averaged between 15°N and 15°S latitudes have a long-term trend during 1960 to 1998. Over this period the tropical easterlies and the tropical jet stream have weakened with time.

Recent Enhanced Deep Troposphere-to-Stratosphere Air Mass Transport Accompanying the Weakening Asian Monsoon

The Asian monsoon(AM) region is a well-known region with prevailing stratosphere–troposphere exchange(STE).However,how the STE across this region changes with the weakening AM remains unclear.Here,we particularly diagnose the air mass transport between the planetary boundary layer(PBL) and the stratosphere over the AM region during 1992–2017 using the Lagrangian particle dispersion model FLEXPART based on the ERA-Interim reanalysis data.The results show that both the downward and upward deep STEs exhibit a detectable increasing trend,while the latter,namely,the deep troposphere-to-stratosphere transport(DTST),is relatively more significant.Further analysis reveals that the long-term trend of DTST over the AM region could be partly attributed to changes in the Pacific Walker circulation and the air temperature(especially at upper levels).Additionally,it is found that DTST increases markedly over the tropical oceanic regions,while the increasing DTST into the stratosphere can be attributed to the enhanced air masses originated from the PBL over the terrestrial regions,where large amounts of pollutant emissions occur.The results imply that the influence of the DTST on the chemical composition and the climate of the stratosphere over the AM region is expected to become increasingly important,and is thereby of relevance to climate projection in an evolving climate.

Impacts of the stratospheric quasi-biennial oscillation on the tropospheric circulation and climate in the Northeast Asia-North Pacific region in early summer

本文研究了平流层准两年振荡(QBO)对东北亚-北太平洋地区初夏对流层环流和地表气温的影响.在QBO西风位相年,东北亚至北太平洋地区存在一支由QBO引发的平均经向环流异常,该经向环流异常可在东北亚至北太平洋地区激发正涡度,并形成异常气旋式环流.气旋左侧出现的异常偏北风导致6月东北亚地表气温下降.QBO东风位相年的结果与西风位相年大致相反.这些结果为QBO对热带外地区天气,气候的影响提供了新的证据,并为东北亚初夏地表气温的预测提供了新的线索。

Cross-Tropopause Mass Exchange Associated with a Tropopause Fold Event over the Northeastern Tibetan Plateau

A springtime tropopause fold event, found to be related to a cold trough intrusion from the north, was detected in the northeastern Tibetan Plateau （TP） based on various observations. A nested high-resolution mesoscale model was employed to investigate the effect of orography on the stratosphere-troposphere exchange. The model was found to be able to capture plausible tropopause fold properties. The propagation of the tropopause fold changed significantly when the terrain height in the model was altered. However, decreasing the terrain height had no significant effect on the morphology of folds. When a fold passed over an elevated surface, a leeside jet stream and a layer of humid air in the middle troposphere tended to develop. This strong leeside descent of air masses and high mid-level potential instability （PI） could give rise to deep upward motions in the leeside and inject tropospheric air into the lower stratosphere. Besides, when the flow encounters an elevated surface, forced lifting together with mid-level PI can trigger deep convective motions on the windward slope. The troposphere to stratosphere transport was found to be persistent and almost stationary over the windward slope of the TP during the evolution of the fold.

An estimation of ozone flux in a stratosphere-troposphere exchange event

A new method based on mass fluxes and observed ozone profiles was developed to estimate crosstropopause ozone flux. Using this method, we estimated the cross-tropopause ozone flux in a stratospheric-tropospheric exchange event that occurred over East Asia in March 2001.The result revealed that the ozone flux across the tropopause in this event was an order of magnitude higher than the global and hemispheric average. Compared to the traditional method using a linear relationship between ozone mixing ratio and potential vorticity near the tropopause, the cross-tropopause ozone flux evaluated with ozonesonde data was somewhat higher, although the orders of the two values were the same.

北疆冬季持续性极端低温事件延伸期的环流异常特征

本文利用1951~2019年国家气象信息中心逐日站点数据和NCEP/NCAR再分析资料,分析了冬季北疆(新疆北部)持续性极端低温事件(PECE)频次的时空分布特征,并探讨了平流层与对流层在事件发生发展过程中的作用。分析表明:年代际尺度上,北疆PECE在20世纪60年代发生频次最多,此后逐渐减少,表明北疆区域发生该事件的概率在降低。空间分布上,无论是极端低温频次还是冷空气强度,极值中心皆在额尔齐斯河流域一线。北疆PECE发展过程中,平流层和对流层环流皆发生了阶段性的调整。延伸期阶段,距事件爆发前25日时,平流层I区(30°E~120°E)极涡首先开始了由强到弱的转变(欧亚弱极涡型)。行星波向下游频散,东南支波列携带能量影响北疆。至事件爆发前20日,对流层极涡也表现出强度减弱,冷空气分裂南下。此后进入短期阶段,来自北冰洋的冷空气在乌拉尔山高压脊前堆积,使得高压脊加强维持至事件爆发前3日,西伯利亚高压携带冷空气向东南方向扩展,随后对流层大型横槽斜脊引导冷空气南下,地面西伯利亚高压发展强盛向南爆发,3日后冷空气影响北疆地区。

青藏高原地区一次深对流活动对平流层——对流层物质交换影响的模拟研究

利用WRF-Chem模式分析了2010年8月12日发生在青藏高原东南部的一次深对流过程中的平流层—对流层物质交换(STE)过程及其影响机制。结果表明,此次深对流系统具备穿透性对流特征,强上升气流能够直接将近地面含高浓度CO和低浓度O_(3)的空气输送至低平流层,使低平流层CO浓度升高、O_(3)浓度降低。同时,深对流活动激发了较强的湍流混合过程,在深对流活动结束后的3~4小时内,湍流混合作用导致上对流层下平流层(UTLS)区域持续发生STE过程,将对流层的冰晶、CO和O_(3)输送至低平流层,但受凝结脱水作用影响,湍流过程向低平流层传输的水汽减少。

碳中和情景下人为排放对全球对流层臭氧的影响研究

本文采用地球系统模式,以未来碳中和排放清单和平流层示踪物O_(3)S为基础,揭示了未来对流层O_(3)及其前体物的变化特征及成因.研究结果表明:碳中和排放情景下,特别在冬春季节,全球范围内的NO_(x)人为排放和飞机排放量均显著降低,这使得近地面NO_(x)浓度随之降低.NO_(x)作为对流层O_(3)的重要前体物之一,其浓度的剧烈减少使得近地层O_(3)浓度显著降低,但在中国东部地区,由于NO对O_(3)滴定作用的减弱,最终使得冬季近地面O_(3)呈现增加趋势;垂直方向上O_(3)浓度减少最为显著的区域集中在对流层顶附近,减少量达26×10^(-9)以上,且夏季最为显著,这主要与飞机排放减少导致的平流层O_(3)浓度降低有关.碳中和排放情景下平流层入侵对全球近地面O_(3)的平均贡献减少量在冬季最高,为1.7×10^(-9),夏季最低,为0.9×10^(-9);北半球平流层入侵贡献减少量最显著区域集中在高纬地区,达4×10^(-9).垂直方向上,平流层入侵贡献减少量随高度增加,在对流层上层,平流层的贡献量降低高达24×10^(-9)以上,且冬季最强.总之,碳中和排放情景下地表人为排放及飞机排放的改变对全球O_(3)污染有很好的减轻作用,平流层贡献量的降低对未来O_(3)浓度的变化也有重要贡献.

模式垂直分辨率对模拟ENSO遥相关的影响

模式分辨率对气候模式的模拟效果具有重要影响。然而,当前模式开发对于垂直分辨率的重视不够。以ENSO(厄尔尼诺-南方涛动)遥相关为例,利用CESM(Community Earth System Model)模式,探究不同模式垂直分辨率设置下模式模拟的ENSO对平流层、对流层影响的差异,评估模式垂直分辨率在气候模拟中的重要性。结果表明,提高垂直分辨率可以显著改进模式对ENSO遥相关的模拟能力。以ECMWF(European Centre for Medium-Range Weather Forecasts)第五代再分析数据集(ERA5)为参照,ENSO对纬向平均温度的影响在北半球中高纬地区冬季呈现出“负正负”的三极子模态。CESM默认的垂直分辨率设置(L66)不能模拟出这一模态,而提高模式垂直分辨率(L103)后则可以较好地模拟出这个模态。对于水平分布而言,L66模拟的ENSO在对流层的信号与再分析资料相比明显偏强,L103则可以显著改善。同时,L103对ENSO影响平流层的模拟效果也比L66有所改善。进一步分析发现,L103模拟的行星波从对流层向平流层的传播更强,更接近再分析资料。提高垂直分辨率可以改善模式对大气波活动以及平流层-对流层动力耦合的模拟,重视模式的研发。

On the Differences and Climate Impacts of Early and Late Stratospheric Polar Vortex Breakup

The stratospheric polar vortex breakup （SPVB） is an important phenomenon closely related to the seasonal transition of stratospheric circulation. In this paper, 62-year NCEP/NCAR reanalysis data were employed to investigate the distinction between early and late SPVB. The results showed that the anomalous circulation signals extending from the stratosphere to the troposphere were reversed before and after early SPVB, while the stratospheric signals were consistent before and after the onset of late SPVB. Arctic Oscillation （AO） evolution during the life cycle of SPVB also demonstrated that the negative AO signal can propagate downward after early SPVB. Such downward AO signals could be identified in both geopotential height and temperature anomalies. After the AO signal reached the lower troposphere, it influenced the Aleutian Low and Siberian High in the troposphere, leading to a weak winter monsoon and large-scale warming at mid latitudes in Asia. Compared to early SPVB, downward propagation was not evident in late SPVB. The high-latitude tropospheric circulation in the Northern Hemisphere was affected by early SPVB, causing it to enter a summer circulation pattern earlier than in late SPVB years.

What Causes the Springtime Tropospheric Ozone Maximum over Northeast Asia?

Scientists have long debated the relative importance of tropospheric photochemical production versus stratospheric influx as causes of the springtime tropospheric ozone maximum over northern mid-latitudes. This paper investigates whether or not stratospheric intrusion and photochemistry play a significant role in the springtime ozone maximum over Northeast Asia, where ozone measurements are sparse. We examine how tropospheric ozone seasonalities over Naha （26°N, 128°E）, Kagoshima （31°N, 131°E）, and Pohang （36°N, 129°E）, which are located on the same meridional line, are related to the timing and location of the jet stream. The ozone seasonality shows a gradual increase from January to the maximum ozone month, which corresponds to April at Naha, May at Kagoshima, and June at Pohang. In order to examine the occurrence of stratospheric intrusion, we analyze a correlation between jet stream activity and tropospheric ozone seasonality. From these analyses, we did not find any favorable evidence supporting the hypothesis that the springtime enhancement may result from stratospheric intrusion. According to trajectory analysis for vertical and horizontal origins of the airmass, a gradual increasing tendency in ozone amounts from January until the onset of monsoon was similar to the increasing ozone formation tendency from winter to spring over China's Mainland, which has been observed during the build-up of tropospheric ozone over Central Europe in the winter-spring transition period due to photochemistry. Overall, the analyses suggest that photochemistry is the most important contributor to observed ozone seasonality over Northeast Asia.

^(10)Be/~7Be implies the contribution of stratosphere-troposphere transport to the winter-spring surface O_3 variation observed on the Tibetan Plateau

10Be/7Be is a stratospheric sensitive tracer.In this paper,measurements of 10Be/7Be and surface O3 from October 2005 to May 2006 at Mt.Waliguan (hereafter WLG,100.898°E,39.287°N,3810 m,a.s.l.),China global atmospheric watch (GAW) observatory,are introduced and used to investigate the stratosphere-troposphere transport (STT) and its impact on surface O3 on the Tibetan Plateau.The results show that the magnitude of STT is weak in winter,followed by strengthening from the end of winter to the middle of spring (from mid February to mid April) with large increases in 10Be,7Be,10Be/7Be and surface O3.At the end of spring (from the end of April to mid May in this paper),the STT weakened,and the continuous increase of surface O3 at WLG is produced by tropospheric photochemistry reactions.

Progress in Research of Stratosphere—Troposphere Interactions:Application of Isentropic Potential Vorticity Dynamics and the Effects of the Tibetan Plateau

This paper reviews recent progress in understanding isentropic potential vorticity （PV） dynamics during interactions between the stratosphere and troposphere, including the spatial and temporal propagation of circulation anomalies associated with the winter polar vortex oscillation and the mechanisms of stratosphere- troposphere coupling in the global mass circulation framework. The origins and mechanisms of interannual variability in the stratospheric circulation are also reviewed. Particular attention is paid to the role of the Tibetan Plateau as a PV source （via its thermal forcing） in the global and East Asian atmospheric circulation. Diagnosis of meridional isentropic PV advection over tile Tibetan Plateau and East Asia indicates that the distributions of potential temperature and PV over the east flank of the Tibetan Plateau and East Asia favor a downward and southward isentropic transport of high PV from the stratosphere to the troposphere. This transport manifests the possible influence of the Tibetan Plateau on the dynamic coupling between the stratosphere and troposphere during summer, and may provide a new framework for understanding the climatic effects of the Tibetan Plateau.