Based on the finite difference time domain method, we investigated theoretically the optical properties and the plasmonic interactions between a gold film perforated with periodic sub-wavelength holes and a thin gold ...Based on the finite difference time domain method, we investigated theoretically the optical properties and the plasmonic interactions between a gold film perforated with periodic sub-wavelength holes and a thin gold film. We showed that the plasmon resonant energies and intensities depend strongly on the thicknesses of the two films and the lattice constant. Based on the distributions of normal electric field component Ez, tangential electric field component Ey and total energy, we showed that the optical transmission is due to the collaboration of the localized waveguide resonance, the surface plasmon resonance and the coupling of the fiat-surface plasmon of the two layers.展开更多
We propose a design for efficient end-fire coupling of surface plasmon polaritons in a metal-insulator-metal(MIM) waveguide with an optical fiber as part of a simple photoplastic connector. The design was analyzed and...We propose a design for efficient end-fire coupling of surface plasmon polaritons in a metal-insulator-metal(MIM) waveguide with an optical fiber as part of a simple photoplastic connector. The design was analyzed and optimized using the three-dimensional finite-difference time-domain method. The calculated excitation efficiency coefficient of the waveguide is 83.7%(-0.77 dB) at a wavelength of 405 nm. This design enables simple connection of an optical fiber to a MIM waveguide and highly efficient local excitation of the waveguide.Moreover, the length of the metallic elements of the waveguide, and thus the dissipative losses, can be reduced.The proposed design may be useful in plasmonic-type waveguide applications such as near-field investigation of live cells and other objects with super-resolution.展开更多
Cavity optomechanics is applied to study the coupling behavior of interacting molecules in surface plasmon systems driven by two-color laser beams. Different from the traditional force–distance measurement, due to a ...Cavity optomechanics is applied to study the coupling behavior of interacting molecules in surface plasmon systems driven by two-color laser beams. Different from the traditional force–distance measurement, due to a resonant frequency shift or a peak splitting on the probe spectrum, we have proposed a convenient method to measure the van der Waals force strength and interaction energy via nonlinear spectroscopy. The minimum force value can reach approximately 10^(-15) N, which is 3 to 4 orders of magnitude smaller than the widely applied atomic force microscope(AFM). It is also shown that two adjacent molecules with similar chemical structures and nearly equal vibrational frequencies can be easily distinguished by the splitting of the transparency peak. Based on this coupled optomechanical system, we also conceptually design a tunable optical switch by van der Waals interaction. Our results will provide new approaches for understanding the complex and dynamic interactions inmolecule–plasmon systems.展开更多
Simultaneous acquisition of fluorescence property and refractive index using a single surface plasmon coupled emission(SPCE)measurement has been achieved,thus achieving synchronicity in real time.The SPCE sensor was e...Simultaneous acquisition of fluorescence property and refractive index using a single surface plasmon coupled emission(SPCE)measurement has been achieved,thus achieving synchronicity in real time.The SPCE sensor was employed for monitoring the adsorption of volatile organic compounds(VOCs)by dyeencapsulated metal-organic frameworks(Dye@MOFs).Refractive index can reveal surface molecular adsorption and the fluorescence with information on refractive index can provide a comprehensive analysis of the adsorption events of VOCs on the interface.Meantime,the signal intensity can be amplified by combining the responses caused by changes in refractive index and the fluorescence property in parallel.This all-in-one method opens up a route to monitoring multiple processes simultaneously occurring on the interface.展开更多
The obvious enhancement effect of magnetic nanoparticles(MNPs) introduced in Cr/Co/Cr/Au substrate on the pulsed magnetic field-modulated surface plasmon coupled emission(SPCE) was investigated,and the observed enhanc...The obvious enhancement effect of magnetic nanoparticles(MNPs) introduced in Cr/Co/Cr/Au substrate on the pulsed magnetic field-modulated surface plasmon coupled emission(SPCE) was investigated,and the observed enhancement factor was 4 comparing with the magnetic field modulated SPCE without MNPs.This is the new observation for the magnetic field modulated SPCE,and this method was designed as a biosensor,which to our knowledge,is the first application of magnetic field-modulated SPCE in biosensing and detection field.This strategy is a universal approach to increase the fluorescence signal and helps to build the new SPCE based stimulus-response system.展开更多
It is essential to develop a single mode operation and improve the performance of lasing in order to ensure practical applicability of microlasers and nanolasers. In this paper, two hexagonal microteeth with varied na...It is essential to develop a single mode operation and improve the performance of lasing in order to ensure practical applicability of microlasers and nanolasers. In this paper, two hexagonal microteeth with varied nanoscaled air-gaps of a ZnO microcomb are used to construct coupled whispering-gallery cavities. This is done to achieve a stable single mode lasing based on Vernier effect without requiring any complicated or sophisticated manipulation to achieve positioning with nanoscale precision. Optical gain and the corresponding ultraviolet lasing performance were improved greatly through coupling with localized surface plasmons of Pt nanoparticles. The ZnO/Pt hybrid microcavities achieved a seven-fold enhancement of intensity of single mode lasing with higher side- mode suppression ratio and lower threshold. The mechanism that led to this enhancement has been described in detail.展开更多
We present both theoretical and experimental investigation on significantly enhanced transmission through (Ag/Au) double-layered metallic aperture arrays with sub-skin-depth Ag film due to the coupling role of a sur...We present both theoretical and experimental investigation on significantly enhanced transmission through (Ag/Au) double-layered metallic aperture arrays with sub-skin-depth Ag film due to the coupling role of a surface plasmon polariton at the Ag/Au interface by evanescent waves. The results indicate that the enhanced transmittance is highly dependent on the Ag film thickness. When the Ag film thickness increases, the peak transmit- tance firstly increases and then decreases. Moreover, other metal material properties are also discussed. The highest peak transmittance is obtained when the Ag film thickness is 4 nm. The finite-difference time-domain simulations agree well with the experimental results. This finding provides an effective way to control the enhanced transmis- sion for double-layered metallic aperture arrays, which has potential applications in designing a high-performance plasmonic thermal emitter.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.60708014)the Science Foundation for Postdoctorate of China(Grant No.2004035083)+2 种基金the Natural Science Foundation of Hunan Province of China(Grant No.06JJ2034)the Excellent Doctorate Dissertation Foundation of Central South University(Grant No.2008yb039)the Hunan Provincial Innovation Foundation for Postgraduate(Grant No.CX2009B029)
文摘Based on the finite difference time domain method, we investigated theoretically the optical properties and the plasmonic interactions between a gold film perforated with periodic sub-wavelength holes and a thin gold film. We showed that the plasmon resonant energies and intensities depend strongly on the thicknesses of the two films and the lattice constant. Based on the distributions of normal electric field component Ez, tangential electric field component Ey and total energy, we showed that the optical transmission is due to the collaboration of the localized waveguide resonance, the surface plasmon resonance and the coupling of the fiat-surface plasmon of the two layers.
基金National Natural Science Foundation of China(NSFC)(61571399)“The Belt and Road”International Cooperation of Zhejiang Province,China(2015C04005)
文摘We propose a design for efficient end-fire coupling of surface plasmon polaritons in a metal-insulator-metal(MIM) waveguide with an optical fiber as part of a simple photoplastic connector. The design was analyzed and optimized using the three-dimensional finite-difference time-domain method. The calculated excitation efficiency coefficient of the waveguide is 83.7%(-0.77 dB) at a wavelength of 405 nm. This design enables simple connection of an optical fiber to a MIM waveguide and highly efficient local excitation of the waveguide.Moreover, the length of the metallic elements of the waveguide, and thus the dissipative losses, can be reduced.The proposed design may be useful in plasmonic-type waveguide applications such as near-field investigation of live cells and other objects with super-resolution.
基金National Natural Science Foundation of China(NSFC)(11274230,11574206)Basic Research Program of the Committee of Science and Technology of Shanghai(14JC1491700)
文摘Cavity optomechanics is applied to study the coupling behavior of interacting molecules in surface plasmon systems driven by two-color laser beams. Different from the traditional force–distance measurement, due to a resonant frequency shift or a peak splitting on the probe spectrum, we have proposed a convenient method to measure the van der Waals force strength and interaction energy via nonlinear spectroscopy. The minimum force value can reach approximately 10^(-15) N, which is 3 to 4 orders of magnitude smaller than the widely applied atomic force microscope(AFM). It is also shown that two adjacent molecules with similar chemical structures and nearly equal vibrational frequencies can be easily distinguished by the splitting of the transparency peak. Based on this coupled optomechanical system, we also conceptually design a tunable optical switch by van der Waals interaction. Our results will provide new approaches for understanding the complex and dynamic interactions inmolecule–plasmon systems.
基金Financial support from the National Natural Science Foundation of China (Nos. 21874110, 21804098, 21974117 and 22274137)the Science and Technology Program of Fujian Province (No. 2022Y4008)
文摘Simultaneous acquisition of fluorescence property and refractive index using a single surface plasmon coupled emission(SPCE)measurement has been achieved,thus achieving synchronicity in real time.The SPCE sensor was employed for monitoring the adsorption of volatile organic compounds(VOCs)by dyeencapsulated metal-organic frameworks(Dye@MOFs).Refractive index can reveal surface molecular adsorption and the fluorescence with information on refractive index can provide a comprehensive analysis of the adsorption events of VOCs on the interface.Meantime,the signal intensity can be amplified by combining the responses caused by changes in refractive index and the fluorescence property in parallel.This all-in-one method opens up a route to monitoring multiple processes simultaneously occurring on the interface.
基金Financial support from the National Natural Science Foundation of China(Nos.21874110,21375111,21505109,21521004 and 21804098)the Fund of the Ministry of Education of China(No. IRT17R66)Scientific and Technological Innovation Programs of Higher Education Institutions in Shanxi(No.201802104)
文摘The obvious enhancement effect of magnetic nanoparticles(MNPs) introduced in Cr/Co/Cr/Au substrate on the pulsed magnetic field-modulated surface plasmon coupled emission(SPCE) was investigated,and the observed enhancement factor was 4 comparing with the magnetic field modulated SPCE without MNPs.This is the new observation for the magnetic field modulated SPCE,and this method was designed as a biosensor,which to our knowledge,is the first application of magnetic field-modulated SPCE in biosensing and detection field.This strategy is a universal approach to increase the fluorescence signal and helps to build the new SPCE based stimulus-response system.
基金Acknowledgements The authors sincerely appreciate the help of Shufeng Wang and Yu Li at Peking University and Andong Xia at Institute of Chemistry Chinese Academy of Sciences for their technical support on time-resolved PL. This work was supported by the National Basic Research Program (No. 2013CB932903), National Natural Science Foundation (Nos. 61275054, 61475035, and 11404289), Jiangsu Province Science and Technology Support Program (No. BE2016177) and Natural Science Foundation of Zhejiang Province (No. LY17A040011).
文摘It is essential to develop a single mode operation and improve the performance of lasing in order to ensure practical applicability of microlasers and nanolasers. In this paper, two hexagonal microteeth with varied nanoscaled air-gaps of a ZnO microcomb are used to construct coupled whispering-gallery cavities. This is done to achieve a stable single mode lasing based on Vernier effect without requiring any complicated or sophisticated manipulation to achieve positioning with nanoscale precision. Optical gain and the corresponding ultraviolet lasing performance were improved greatly through coupling with localized surface plasmons of Pt nanoparticles. The ZnO/Pt hybrid microcavities achieved a seven-fold enhancement of intensity of single mode lasing with higher side- mode suppression ratio and lower threshold. The mechanism that led to this enhancement has been described in detail.
文摘We present both theoretical and experimental investigation on significantly enhanced transmission through (Ag/Au) double-layered metallic aperture arrays with sub-skin-depth Ag film due to the coupling role of a surface plasmon polariton at the Ag/Au interface by evanescent waves. The results indicate that the enhanced transmittance is highly dependent on the Ag film thickness. When the Ag film thickness increases, the peak transmit- tance firstly increases and then decreases. Moreover, other metal material properties are also discussed. The highest peak transmittance is obtained when the Ag film thickness is 4 nm. The finite-difference time-domain simulations agree well with the experimental results. This finding provides an effective way to control the enhanced transmis- sion for double-layered metallic aperture arrays, which has potential applications in designing a high-performance plasmonic thermal emitter.