Parity–time(PT) and quasi-anti-parity–time(quasi-APT) symmetric optical gyroscopes have been proposed recently which enhance Sagnac frequency splitting. However, the operation of gyroscopes at the exceptional point(...Parity–time(PT) and quasi-anti-parity–time(quasi-APT) symmetric optical gyroscopes have been proposed recently which enhance Sagnac frequency splitting. However, the operation of gyroscopes at the exceptional point(EP) is challenging due to strict fabrication requirements and experimental uncertainties. We propose a new quasi-APT-symmetric micro-optical gyroscope which can be operated at the EP by easily shifting the Kerr nonlinearity. A single resonator is used as the core sensitive component of the quasi-APT-symmetric optical gyroscope to reduce the size, overcome the strict structural requirements and detect small rotation rates. Moreover, the proposed scheme also has an easy readout method for the frequency splitting. As a result, the device achieves a frequency splitting 10~5 times higher than that of a classical resonant optical gyroscope with the Earth's rotation. This proposal paves the way for a new and valuable method for the engineering of micro-optical gyroscopes.展开更多
The study of nonlinear optical responses in the mid-infrared(mid-IR)regime is essential for advancing ultrafast mid-IR laser applications.However,nonlinear optical effects under mid-IR excitation are rarely reported d...The study of nonlinear optical responses in the mid-infrared(mid-IR)regime is essential for advancing ultrafast mid-IR laser applications.However,nonlinear optical effects under mid-IR excitation are rarely reported due to the lack of suitable nonlinear optical materials.The natural van derWaals heterostructure franckeite,known for its narrow bandgap and stability in air,shows great potential for developing mid-IR nonlinear optical devices.We have experimentally demonstrated that layered franckeite exhibits a broadband wavelength-dependent nonlinear optical response in the mid-IR spectral region.Franckeite nanosheets were prepared using a liquid-phase exfoliation method,and their nonlinear optical response was characterized in the spectral range of 3000 nm to 5000 nm.The franckeite nanosheets exhibit broadband wavelengthdependent third-order nonlinearities,with nonlinear absorption and refraction coefficients estimated to be about 10^(-7)cm/W and 10^(-11)cm^(2)/W,respectively.Additionally,a passively Q-switched fluoride fiber laser operating around a wavelength of 2800 nm was achieved,delivering nanosecond pulses with a signal-to-noise ratio of 43.6 dB,based on the nonlinear response of franckeite.These findings indicate that layered franckeite possesses broadband nonlinear optical characteristics in the mid-IR region,potentially enabling new possibilities for mid-IR photonic devices.展开更多
The ultrashort lasers working in pulse-burst mode reveal great machining performance in recent years. The number of pulses in bursts effects greatly on the removal rate and roughness. To generate a more equal amplitud...The ultrashort lasers working in pulse-burst mode reveal great machining performance in recent years. The number of pulses in bursts effects greatly on the removal rate and roughness. To generate a more equal amplitude of pulses in burst with linear polarization output and time gap adjustable, we propose a new method by the harmonic beam combining(HBC).The beam combining is commonly used in adding pulses into the output beam while maintaining the pulse waveform and beam quality. In the HBC, dichroic mirrors are used to combine laser pulses of fundamental wave(FW) into harmonic wave(HW), and nonlinear crystals are used to convert the FW into HW. Therefore, HBC can add arbitrarily more HW pulses to generate pulse-burst in linear polarization with simple structure. The amplitude of each pulse in bursts can be adjusted the same to increase the stability of the burst, the time gap of each pulse can be adjusted precisely by proper time delay. Because HBC adds pulses sequentially, the peak power density of the burst is the same as each pulse, pulses can be combined without concern of back-conversion which often occurs in high peak power density. In the demonstration, the extendibility of HBC was verified by combining two beams with a third beam. The combined efficiency rates were larger than 99%, and the beam quality of each beam was maintained at M^(2)≈1.4.展开更多
A Weyl node is characterized by its chirality and tilt.We develop a theory of how nth-order nonlinear optical conductivity behaves under transformations of anisotropic tensor and tilt, which clarifies how chirality-de...A Weyl node is characterized by its chirality and tilt.We develop a theory of how nth-order nonlinear optical conductivity behaves under transformations of anisotropic tensor and tilt, which clarifies how chirality-dependent and-independent parts of optical conductivity transform under the reversal of tilt and chirality.Built on this theory, we propose ferromagnetic Mn Bi2Te4as a magnetoelectrically regulated, terahertz optical device, by magnetoelectrically switching the chiralitydependent and-independent DC photocurrents.These results are useful for creating nonlinear optical devices based on the topological Weyl semimetals.展开更多
Thin transparent oxide conducting films(TCOFs)of titanium and gallium substituted zinc oxide(TGZO)were fabricated via radio frequency(RF)magnetron sputtering technique.The effects of RF power on electrical,linear and ...Thin transparent oxide conducting films(TCOFs)of titanium and gallium substituted zinc oxide(TGZO)were fabricated via radio frequency(RF)magnetron sputtering technique.The effects of RF power on electrical,linear and nonlinear optical characteristics were investigated by Hall tester,Ultraviolet(UV)-visible spectrophotometer and optical characterization method.The results indicate that RF power significantly influences the electrical and optical properties of the deposited films.As RF power raises,the resistivity and Urbach energy fall initially and then rise,while the figure of merit,mean visible transmittance and optical bandgap show the reverse variation trend.At RF power of 190 W,the TGZO sample exhibits the highest electro-optical properties,with the maximum figure of merit(1.14×10^(4)Ω^(-1)∙cm^(-1)),mean visible transmittance(86.9%)and optical bandgap(3.50 eV),the minimum resistivity(6.26×10^(-4)Ω∙cm)and Urbach energy(174.23 meV).In addition,the optical constants of the deposited films were determined by the optical spectrum fitting method,and the RF power dependence of nonlinear optical properties was studied.It is observed that all the thin films exhibit normal dispersion characteristics in the visible region,and the nonlinear optical parameters are greatly affected by the RF power in the ultraviolet region.展开更多
Cyclo[18]carbon has received considerable attention thanks to its novel geometric configuration and special electronic structure.Superalkalis have low ionization energy.Doping a superalkali in cyclo[18]carbon is an ef...Cyclo[18]carbon has received considerable attention thanks to its novel geometric configuration and special electronic structure.Superalkalis have low ionization energy.Doping a superalkali in cyclo[18]carbon is an effective method to improve the optical properties of the system because considerable electron transfer occurs.In this paper,the geometry,bonding properties,electronic structure,absorption spectrum,and nonlinear optical(NLO)properties of superalkaline M_(3)O(M=Li,Na)-doped cyclo[18]carbon were studied by using density functional theory.M_(3)O and the C_(18) rings are not coplanar.The C_(18) ring still exhibits alternating long and short bonds.The charge transfer between M_(3)O and C_(18) forms stable[M_(3)O]+[C_(18)]-ionic complexes.C_(18)M_(3)O(M=Li,Na)shows striking optical nonlinearity,i.e.,their first-and second-order hyperpolarizability(βvec andγ||)increase considerably atλ=1907 nm and 1460 nm.展开更多
Optical dispersive nonlinearities in Er-doped optical fiber are discussed and measured at the third window wavelength 1.55 μm for optical communications firstly. The experimental method, which is developed by us, is ...Optical dispersive nonlinearities in Er-doped optical fiber are discussed and measured at the third window wavelength 1.55 μm for optical communications firstly. The experimental method, which is developed by us, is based on dynamic scanning for fixed-point-interference (DSFPI) of two fiber beams. The real part and complex value of the third-order susceptibility at the wavelength are also obtained from the measured Kerr coefficient and nonlinear-absorption coefficient reported elsewhere.展开更多
Four phenoxysilicon networks for nonlinear optical (NLO) applications were designed and prepared by an extended sol-gel process without additional H2O and catalyst. All poled polymer network films possess high second-...Four phenoxysilicon networks for nonlinear optical (NLO) applications were designed and prepared by an extended sol-gel process without additional H2O and catalyst. All poled polymer network films possess high second-order nonlinear optical coefficients (d(33)) Of 10(-7)similar to 10(-8) esu. The investigation of NLO temporal stability at room temperature and elevated temperature (120 degreesC) indicated that these films exhibit high d(33) stability because the orientation of the chromophores are locked in the phenoxysilicon organic/inorganic networks.展开更多
The influence of optical nonlinearity on combining efficiency in ultrashort pulse fiber laser coherent combining system is investigated theoretically and experimentally.In the theoretical work,a new theoretical algori...The influence of optical nonlinearity on combining efficiency in ultrashort pulse fiber laser coherent combining system is investigated theoretically and experimentally.In the theoretical work,a new theoretical algorithm is presented for the coherent combining efficiency,which can be used to quantify the spectral coherence decay induced by optical nonlinearity imbalance between the sub-beams.The spectral information of the sub-beam is obtained by numerically solving the nonlinear Schrödinger equation(NLSE)in this algorithm to ensure an accurate prediction.In the experimental work,the coherent combining of two all-fiber picosecond lasers is achieved,and the influence of imbalanced optical nonlinearity on the combining efficiency is studied,which agrees with the theoretical prediction.This paper reveals the physical mechanism for the influence of optical nonlinearity on the combining efficiency,which is valuable for the coherent combining of ultrashort pulse fiber laser beams.展开更多
This paper introduces a joint nonlinearity and chromatic dispersion pre-compensation method for coherent optical orthogonal frequency-division multiplexing systems. The research results show that this method can reduc...This paper introduces a joint nonlinearity and chromatic dispersion pre-compensation method for coherent optical orthogonal frequency-division multiplexing systems. The research results show that this method can reduce the walk- off effect and can therefore equalize the nonlinear impairments effectively. Compared with the only other existing nonlinearity pre-compensation method, the joint nonlinearity and chromatic dispersion pre-compensation method is not only suitable for low-dispersion optical orthogonal frequency-division multiplexing system, but also effective for high- dispersion optical orthogonal frequency-division multiplexing transmission system with higher input power but without optical dispersion compensation. The suggested solution does not increase computation complexity compared with only nonlinearity pre-compensation method. For 40 Gbit/s coherent optical orthogonal frequency-division multiplexing 20 × 80 km standard single-mode fibre system, the suggested method can improve the nonlinear threshold (for Q 〉 10 dB) about 2.7, 1.2 and 1.0 dB, and the maximum Q factor about 1.2, 0.4 and 0.3 dB, for 2, 8 and 16 ps/(nm.km) dispersion coefficients.展开更多
Utilizing the linear-stability analysis, this paper analytically investigates and calculates the condition and gain spectra of cross-phase modulation instability in optical fibres in the ease of exponential saturable ...Utilizing the linear-stability analysis, this paper analytically investigates and calculates the condition and gain spectra of cross-phase modulation instability in optical fibres in the ease of exponential saturable nonlinearity and high-order dispersion. The results show that, the modulation instability characteristics here are similar to those of conventional saturable nonlinearity and Kerr nonlinearity. That is to say, when the fourth-order dispersion has the same sign as that of the second-order one, a new gain spectral region called the second one which is far away from the zero point may appear. The existence of the exponential saturable nonlinearity will make the spectral width as well as the peak gain of every spectral region increase with the input powers before decrease. Namely, for every spectral regime, this may lead to a unique value of peak gain and spectral width for two different input powers. In comparison with the case of conventional saturable nonlinearity, however, when the other parameters are the same, the variations of the spectral width and the peak gain with the input powers will be faster in case of exponential saturable nonlinearity.展开更多
Chalcogenide glasses (ChGs) are a promising candidate for applications in nonlinear photonic devices. In this paper, we review the research progress of the third-order optical nonlinearity (TONL) of ChGs from the ...Chalcogenide glasses (ChGs) are a promising candidate for applications in nonlinear photonic devices. In this paper, we review the research progress of the third-order optical nonlinearity (TONL) of ChGs from the following three aspects: chemical composition, excitation condition, and post processing. The deficiencies in previous studies and further research of the TONL property of ChGs are also discussed.展开更多
Optical absorptive nonlinearity in Er doped optical fiber has been discussed and measured at the window wavelength 1.55 μm for optical communications firstly. It is proposed that the mechanism of this absorptive...Optical absorptive nonlinearity in Er doped optical fiber has been discussed and measured at the window wavelength 1.55 μm for optical communications firstly. It is proposed that the mechanism of this absorptive nonlinearity is the induced absorption. The first order nonlinear absorptive coefficient and the imaginary part and the complex value of the third order susceptibility at that wavelength are obtained from the measured absorptive nonlinearity.展开更多
The third-order optical nonlinearity of two sandwich-type phthalocyaninato and porphyrinato europium com- plexes, including double- and triple-deckers (Eu[Pc(OC5H11)8]2, Eu2(Pc)(TPP)2, Pc=phthalocyanine, TPP=5,...The third-order optical nonlinearity of two sandwich-type phthalocyaninato and porphyrinato europium com- plexes, including double- and triple-deckers (Eu[Pc(OC5H11)8]2, Eu2(Pc)(TPP)2, Pc=phthalocyanine, TPP=5, 10, 15, 20- tetraphenylporphyrinate), was investigated by using the femtosecond time-resolved optical Kerr gate method at 830 nm wavelength. Their second-order hyperpolarizability is estimated to be 0.74× 10^-30esu and 3.0× 10^-3esu respectively. This exhibits an evident enhancement in comparison with 0.47×10^-30esu for one-decker Eu(Pc)(acac) (acac=acetylacetonate), which is also measured under the same conditions. The enhancement is attributed to the introduction of lanthanide metal to the large π-conjugated system, intermacrocycle interaction and two-photon resonance etc.展开更多
The optical wave breaking (OWB) characteristics in terms of the pulse shape, spectrum, and frequency chirp, in the normal dispersion regime of an optical fiber with both the third-order dispersion (TOD) and quinti...The optical wave breaking (OWB) characteristics in terms of the pulse shape, spectrum, and frequency chirp, in the normal dispersion regime of an optical fiber with both the third-order dispersion (TOD) and quintic nonlinearity (QN) are numerically calculated. The results show that the TOD causes the asymmetry of the temporal- and spectral-domain, and the chirp characteristics. The OWB generally appears near the pulse center and at the trailing edge of the pulse, instead of at the two edges of the pulse symmetrically in the case of no TOD. With the increase of distance, the relation of OWB to the TOD near the pulse center increases quickly, leading to the generation of ultra-short pulse trains, while the OWB resulting from the case of no TOD at the trailing edge of the pulse disappears gradually. In addition, the positive (negative) QN enhances (weakens) the chirp amount and the fine structures, thereby inducing the OWB phenomena to appear earlier (later). Thus, the TOD and the positive (negative) QN are beneficial (detrimental) to the OWB and the generation of ultra-short pulse trains.展开更多
The propagation of spatial solitons is systematically investigated in nonlocal nonlinear media with an imprinted transverse periodic modulation of the refractive index. Based on the variational principle and the infin...The propagation of spatial solitons is systematically investigated in nonlocal nonlinear media with an imprinted transverse periodic modulation of the refractive index. Based on the variational principle and the infinitesimal approximation of Maclaurin series expansion, we obtain an analytical solution of such nonlocal spatial solitons and an interesting result that the critical power for such solitons propagation is smaller than that in uniform nonlocal self-focusing media. It is found that there exist thresholds in modulation period and lattice depth for such solitons. A stable spatial soliton propagation is maintained with proper adjustment of the modulation period and the lattice depth.展开更多
The transmittance technique with a phase object(T-PO),for measuring optical nonlinear coefficients is proposed with a top-hat beam.The sensitivity of the T-PO with a top-hat beam is a factor of 4 greater than that w...The transmittance technique with a phase object(T-PO),for measuring optical nonlinear coefficients is proposed with a top-hat beam.The sensitivity of the T-PO with a top-hat beam is a factor of 4 greater than that with a Gaussian beam.The validity of this method is verified by measuring the nonlinearity of a well-characterized liquid,CS 2 at 532-nm wavelength.The ease of use of this method has been proved by measuring a new compound 4-(N-methyl,N-hydroxyethyl)amino,4'-nitroazobenzene(ANAB) at 600-nm wavelength,indicating that this method can be extended to the measurement of optical nonlinearities in a wide-band spectrum.展开更多
In this paper, we present the results of numerical analysis of optical solitons in dual core couplers. We studied the optical couplers as an application for the non-linear Schrödinger equation in the case of ...In this paper, we present the results of numerical analysis of optical solitons in dual core couplers. We studied the optical couplers as an application for the non-linear Schrödinger equation in the case of Kerr law for non-linear and clarify the exact solution in this case. Then we have provided a numerical study of the effect of changing the constants in the form of the three types of solitons: bright soliton and dark solitons and singular soliton.展开更多
Ultrafine PbS particles with different sizes have been prepared in perfluorocarboxylated cation-exchanged films. The variation of PbS particle size was clarified by absorption spectra and TEM graphs. Time-resolved opt...Ultrafine PbS particles with different sizes have been prepared in perfluorocarboxylated cation-exchanged films. The variation of PbS particle size was clarified by absorption spectra and TEM graphs. Time-resolved optical Kerr effects were measured by femtosecond pump-probe techniques. Optical Kerr effect response time was estimated to be less than 165 fs. A third-order optical nonlinearity of χ(3)10-12 esu for PbS particles was obtained and it was found that it increases with the decrease of particle sizes, showing the influence of quantum confined effect on optical nonlinear behaviour of ultrafine particles.展开更多
We investigate the properties of fundamental,multi-peak,and multi-peaked twisted solitons in three types of finite waveguide lattices imprinted in photorefractive media with asymmetrical diffusion nonlinearity.Two opp...We investigate the properties of fundamental,multi-peak,and multi-peaked twisted solitons in three types of finite waveguide lattices imprinted in photorefractive media with asymmetrical diffusion nonlinearity.Two opposite soliton selfbending signals are considered for different families of solitons.Power thresholdless fundamental and multi-peaked solitons are stable in the low power region.The existence domain of two-peaked twisted solitons can be changed by the soliton self-bending signals.When solitons tend to self-bend toward the waveguide lattice,stable two-peaked twisted solitons can be found in a larger region in the middle of their existence region.Three-peaked twisted solitons are stable in the lower(upper)cutoff region for a shallow(deep)lattice depth.Our results provide an effective guidance for revealing the soliton characteristics supported by a finite waveguide lattice with diffusive nonlocal nonlinearity.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant Nos.62273115,62173105)the Fundamental Research Funds for the Central Universities (Grant No.3072022FSC0401)。
文摘Parity–time(PT) and quasi-anti-parity–time(quasi-APT) symmetric optical gyroscopes have been proposed recently which enhance Sagnac frequency splitting. However, the operation of gyroscopes at the exceptional point(EP) is challenging due to strict fabrication requirements and experimental uncertainties. We propose a new quasi-APT-symmetric micro-optical gyroscope which can be operated at the EP by easily shifting the Kerr nonlinearity. A single resonator is used as the core sensitive component of the quasi-APT-symmetric optical gyroscope to reduce the size, overcome the strict structural requirements and detect small rotation rates. Moreover, the proposed scheme also has an easy readout method for the frequency splitting. As a result, the device achieves a frequency splitting 10~5 times higher than that of a classical resonant optical gyroscope with the Earth's rotation. This proposal paves the way for a new and valuable method for the engineering of micro-optical gyroscopes.
基金supported by the National Natural Science Foundation of China(Grant No.61975055)the Natural Science Foundation of Hunan Province,China(Grant No.2023JJ30165)+1 种基金the Natural Science Foundation of Shandong Province,China(Grant No.ZR2022QF005)the Doctoral Fund of University of Heze(Grant No.XY22BS14).
文摘The study of nonlinear optical responses in the mid-infrared(mid-IR)regime is essential for advancing ultrafast mid-IR laser applications.However,nonlinear optical effects under mid-IR excitation are rarely reported due to the lack of suitable nonlinear optical materials.The natural van derWaals heterostructure franckeite,known for its narrow bandgap and stability in air,shows great potential for developing mid-IR nonlinear optical devices.We have experimentally demonstrated that layered franckeite exhibits a broadband wavelength-dependent nonlinear optical response in the mid-IR spectral region.Franckeite nanosheets were prepared using a liquid-phase exfoliation method,and their nonlinear optical response was characterized in the spectral range of 3000 nm to 5000 nm.The franckeite nanosheets exhibit broadband wavelengthdependent third-order nonlinearities,with nonlinear absorption and refraction coefficients estimated to be about 10^(-7)cm/W and 10^(-11)cm^(2)/W,respectively.Additionally,a passively Q-switched fluoride fiber laser operating around a wavelength of 2800 nm was achieved,delivering nanosecond pulses with a signal-to-noise ratio of 43.6 dB,based on the nonlinear response of franckeite.These findings indicate that layered franckeite possesses broadband nonlinear optical characteristics in the mid-IR region,potentially enabling new possibilities for mid-IR photonic devices.
基金Project supported by Youth Innovation Promotion Association of the Chinese Academy of Sciences (Grant No.2020029)。
文摘The ultrashort lasers working in pulse-burst mode reveal great machining performance in recent years. The number of pulses in bursts effects greatly on the removal rate and roughness. To generate a more equal amplitude of pulses in burst with linear polarization output and time gap adjustable, we propose a new method by the harmonic beam combining(HBC).The beam combining is commonly used in adding pulses into the output beam while maintaining the pulse waveform and beam quality. In the HBC, dichroic mirrors are used to combine laser pulses of fundamental wave(FW) into harmonic wave(HW), and nonlinear crystals are used to convert the FW into HW. Therefore, HBC can add arbitrarily more HW pulses to generate pulse-burst in linear polarization with simple structure. The amplitude of each pulse in bursts can be adjusted the same to increase the stability of the burst, the time gap of each pulse can be adjusted precisely by proper time delay. Because HBC adds pulses sequentially, the peak power density of the burst is the same as each pulse, pulses can be combined without concern of back-conversion which often occurs in high peak power density. In the demonstration, the extendibility of HBC was verified by combining two beams with a third beam. The combined efficiency rates were larger than 99%, and the beam quality of each beam was maintained at M^(2)≈1.4.
基金Project supported by the National Key R&D Program of China (Grant Nos.2018YFA, 0305601, and 2021YFA1400100)the National Natural Science Foundation of China (Grant Nos.12274003, 11725415, and 11934001)the Innovation Program for Quantum Science and Technology (Grant No.2021ZD0302600)。
文摘A Weyl node is characterized by its chirality and tilt.We develop a theory of how nth-order nonlinear optical conductivity behaves under transformations of anisotropic tensor and tilt, which clarifies how chirality-dependent and-independent parts of optical conductivity transform under the reversal of tilt and chirality.Built on this theory, we propose ferromagnetic Mn Bi2Te4as a magnetoelectrically regulated, terahertz optical device, by magnetoelectrically switching the chiralitydependent and-independent DC photocurrents.These results are useful for creating nonlinear optical devices based on the topological Weyl semimetals.
文摘Thin transparent oxide conducting films(TCOFs)of titanium and gallium substituted zinc oxide(TGZO)were fabricated via radio frequency(RF)magnetron sputtering technique.The effects of RF power on electrical,linear and nonlinear optical characteristics were investigated by Hall tester,Ultraviolet(UV)-visible spectrophotometer and optical characterization method.The results indicate that RF power significantly influences the electrical and optical properties of the deposited films.As RF power raises,the resistivity and Urbach energy fall initially and then rise,while the figure of merit,mean visible transmittance and optical bandgap show the reverse variation trend.At RF power of 190 W,the TGZO sample exhibits the highest electro-optical properties,with the maximum figure of merit(1.14×10^(4)Ω^(-1)∙cm^(-1)),mean visible transmittance(86.9%)and optical bandgap(3.50 eV),the minimum resistivity(6.26×10^(-4)Ω∙cm)and Urbach energy(174.23 meV).In addition,the optical constants of the deposited films were determined by the optical spectrum fitting method,and the RF power dependence of nonlinear optical properties was studied.It is observed that all the thin films exhibit normal dispersion characteristics in the visible region,and the nonlinear optical parameters are greatly affected by the RF power in the ultraviolet region.
基金Project supported by the Natural Science Foundation of Anhui Province(Grant No.1908085MA12)the National Natural Science Foundation of China(Grant No.21703222)。
文摘Cyclo[18]carbon has received considerable attention thanks to its novel geometric configuration and special electronic structure.Superalkalis have low ionization energy.Doping a superalkali in cyclo[18]carbon is an effective method to improve the optical properties of the system because considerable electron transfer occurs.In this paper,the geometry,bonding properties,electronic structure,absorption spectrum,and nonlinear optical(NLO)properties of superalkaline M_(3)O(M=Li,Na)-doped cyclo[18]carbon were studied by using density functional theory.M_(3)O and the C_(18) rings are not coplanar.The C_(18) ring still exhibits alternating long and short bonds.The charge transfer between M_(3)O and C_(18) forms stable[M_(3)O]+[C_(18)]-ionic complexes.C_(18)M_(3)O(M=Li,Na)shows striking optical nonlinearity,i.e.,their first-and second-order hyperpolarizability(βvec andγ||)increase considerably atλ=1907 nm and 1460 nm.
文摘Optical dispersive nonlinearities in Er-doped optical fiber are discussed and measured at the third window wavelength 1.55 μm for optical communications firstly. The experimental method, which is developed by us, is based on dynamic scanning for fixed-point-interference (DSFPI) of two fiber beams. The real part and complex value of the third-order susceptibility at the wavelength are also obtained from the measured Kerr coefficient and nonlinear-absorption coefficient reported elsewhere.
文摘Four phenoxysilicon networks for nonlinear optical (NLO) applications were designed and prepared by an extended sol-gel process without additional H2O and catalyst. All poled polymer network films possess high second-order nonlinear optical coefficients (d(33)) Of 10(-7)similar to 10(-8) esu. The investigation of NLO temporal stability at room temperature and elevated temperature (120 degreesC) indicated that these films exhibit high d(33) stability because the orientation of the chromophores are locked in the phenoxysilicon organic/inorganic networks.
基金upported by the Key Program of Beijing Municipal Natural Science Foundation,China(Grant No.KZ201910005006)the National Natural Science Foundation of China(Grant No.62005004)+1 种基金Natural Science Foundation of Beijing Municipality,China(Grant No.4204091)National Science Foundation for Post-doctor Scientists of China(Grant No.212423)。
文摘The influence of optical nonlinearity on combining efficiency in ultrashort pulse fiber laser coherent combining system is investigated theoretically and experimentally.In the theoretical work,a new theoretical algorithm is presented for the coherent combining efficiency,which can be used to quantify the spectral coherence decay induced by optical nonlinearity imbalance between the sub-beams.The spectral information of the sub-beam is obtained by numerically solving the nonlinear Schrödinger equation(NLSE)in this algorithm to ensure an accurate prediction.In the experimental work,the coherent combining of two all-fiber picosecond lasers is achieved,and the influence of imbalanced optical nonlinearity on the combining efficiency is studied,which agrees with the theoretical prediction.This paper reveals the physical mechanism for the influence of optical nonlinearity on the combining efficiency,which is valuable for the coherent combining of ultrashort pulse fiber laser beams.
基金supported by the National High Technology Research and Development Program of China(Grant No.2009AA01A345)the National Basic Research Program of China(Grant No.2011CB302702)the National Natural Science Foundation of China(Grant No.60932004)
文摘This paper introduces a joint nonlinearity and chromatic dispersion pre-compensation method for coherent optical orthogonal frequency-division multiplexing systems. The research results show that this method can reduce the walk- off effect and can therefore equalize the nonlinear impairments effectively. Compared with the only other existing nonlinearity pre-compensation method, the joint nonlinearity and chromatic dispersion pre-compensation method is not only suitable for low-dispersion optical orthogonal frequency-division multiplexing system, but also effective for high- dispersion optical orthogonal frequency-division multiplexing transmission system with higher input power but without optical dispersion compensation. The suggested solution does not increase computation complexity compared with only nonlinearity pre-compensation method. For 40 Gbit/s coherent optical orthogonal frequency-division multiplexing 20 × 80 km standard single-mode fibre system, the suggested method can improve the nonlinear threshold (for Q 〉 10 dB) about 2.7, 1.2 and 1.0 dB, and the maximum Q factor about 1.2, 0.4 and 0.3 dB, for 2, 8 and 16 ps/(nm.km) dispersion coefficients.
基金Project supported by the Key Program of the Natural Science Foundation of Sichuan Provincial Education Department (Grant No. 2006A124)the Fundamental Application Research Project of the Department of Science & Technology of Sichuan Province (Grant No. 05JY029-084)
文摘Utilizing the linear-stability analysis, this paper analytically investigates and calculates the condition and gain spectra of cross-phase modulation instability in optical fibres in the ease of exponential saturable nonlinearity and high-order dispersion. The results show that, the modulation instability characteristics here are similar to those of conventional saturable nonlinearity and Kerr nonlinearity. That is to say, when the fourth-order dispersion has the same sign as that of the second-order one, a new gain spectral region called the second one which is far away from the zero point may appear. The existence of the exponential saturable nonlinearity will make the spectral width as well as the peak gain of every spectral region increase with the input powers before decrease. Namely, for every spectral regime, this may lead to a unique value of peak gain and spectral width for two different input powers. In comparison with the case of conventional saturable nonlinearity, however, when the other parameters are the same, the variations of the spectral width and the peak gain with the input powers will be faster in case of exponential saturable nonlinearity.
基金Project supported by the National Natural Science Foundation of China(Grant No.61675106)the National Key Research and Development Program of China(Grant No.2016YFB0303803)the K C Wong Magna Fund in Ningbo University
文摘Chalcogenide glasses (ChGs) are a promising candidate for applications in nonlinear photonic devices. In this paper, we review the research progress of the third-order optical nonlinearity (TONL) of ChGs from the following three aspects: chemical composition, excitation condition, and post processing. The deficiencies in previous studies and further research of the TONL property of ChGs are also discussed.
文摘Optical absorptive nonlinearity in Er doped optical fiber has been discussed and measured at the window wavelength 1.55 μm for optical communications firstly. It is proposed that the mechanism of this absorptive nonlinearity is the induced absorption. The first order nonlinear absorptive coefficient and the imaginary part and the complex value of the third order susceptibility at that wavelength are obtained from the measured absorptive nonlinearity.
基金Project supported by the National Key Research Program of China (Grant No TG1999075209) and the National Natural Science Foundation of China (Grant Nos 10434020, 90206003 and 60378012).
文摘The third-order optical nonlinearity of two sandwich-type phthalocyaninato and porphyrinato europium com- plexes, including double- and triple-deckers (Eu[Pc(OC5H11)8]2, Eu2(Pc)(TPP)2, Pc=phthalocyanine, TPP=5, 10, 15, 20- tetraphenylporphyrinate), was investigated by using the femtosecond time-resolved optical Kerr gate method at 830 nm wavelength. Their second-order hyperpolarizability is estimated to be 0.74× 10^-30esu and 3.0× 10^-3esu respectively. This exhibits an evident enhancement in comparison with 0.47×10^-30esu for one-decker Eu(Pc)(acac) (acac=acetylacetonate), which is also measured under the same conditions. The enhancement is attributed to the introduction of lanthanide metal to the large π-conjugated system, intermacrocycle interaction and two-photon resonance etc.
基金supported by the Postdoctoral Fund of China(Grant No.2011M501402)the National Natural Science Foundation of China(Grant No.61275039)+2 种基金the 973 Program of China(Grant No.2012CB315702)the Key Project of the Chinese Ministry of Education,China(Grant No.210186)the Major Project of the Natural Science Foundation supported by the Educational Department of Sichuan Province,China(Grant Nos.13ZA0081 and 12ZB019)
文摘The optical wave breaking (OWB) characteristics in terms of the pulse shape, spectrum, and frequency chirp, in the normal dispersion regime of an optical fiber with both the third-order dispersion (TOD) and quintic nonlinearity (QN) are numerically calculated. The results show that the TOD causes the asymmetry of the temporal- and spectral-domain, and the chirp characteristics. The OWB generally appears near the pulse center and at the trailing edge of the pulse, instead of at the two edges of the pulse symmetrically in the case of no TOD. With the increase of distance, the relation of OWB to the TOD near the pulse center increases quickly, leading to the generation of ultra-short pulse trains, while the OWB resulting from the case of no TOD at the trailing edge of the pulse disappears gradually. In addition, the positive (negative) QN enhances (weakens) the chirp amount and the fine structures, thereby inducing the OWB phenomena to appear earlier (later). Thus, the TOD and the positive (negative) QN are beneficial (detrimental) to the OWB and the generation of ultra-short pulse trains.
基金supported in part by the National Natural Science Foundation of China (Grant Nos 60677030 and 60808002)the Specialized Research Fund for the Doctoral Program of Higher Education, China (Grant No 20060280007)+2 种基金the Science and Technology Commission of Shanghai Municipality, China (Grant No 06ZR14034)Ming Shen is also supported by the Australian Endeavor Research Fellowship scholarshipappreciates the hospitality of the Laser Physics Center during his stay in Canberra
文摘The propagation of spatial solitons is systematically investigated in nonlocal nonlinear media with an imprinted transverse periodic modulation of the refractive index. Based on the variational principle and the infinitesimal approximation of Maclaurin series expansion, we obtain an analytical solution of such nonlocal spatial solitons and an interesting result that the critical power for such solitons propagation is smaller than that in uniform nonlocal self-focusing media. It is found that there exist thresholds in modulation period and lattice depth for such solitons. A stable spatial soliton propagation is maintained with proper adjustment of the modulation period and the lattice depth.
文摘The transmittance technique with a phase object(T-PO),for measuring optical nonlinear coefficients is proposed with a top-hat beam.The sensitivity of the T-PO with a top-hat beam is a factor of 4 greater than that with a Gaussian beam.The validity of this method is verified by measuring the nonlinearity of a well-characterized liquid,CS 2 at 532-nm wavelength.The ease of use of this method has been proved by measuring a new compound 4-(N-methyl,N-hydroxyethyl)amino,4'-nitroazobenzene(ANAB) at 600-nm wavelength,indicating that this method can be extended to the measurement of optical nonlinearities in a wide-band spectrum.
文摘In this paper, we present the results of numerical analysis of optical solitons in dual core couplers. We studied the optical couplers as an application for the non-linear Schrödinger equation in the case of Kerr law for non-linear and clarify the exact solution in this case. Then we have provided a numerical study of the effect of changing the constants in the form of the three types of solitons: bright soliton and dark solitons and singular soliton.
基金the High Technology Research and Development Programme of China and Academia Sinica.
文摘Ultrafine PbS particles with different sizes have been prepared in perfluorocarboxylated cation-exchanged films. The variation of PbS particle size was clarified by absorption spectra and TEM graphs. Time-resolved optical Kerr effects were measured by femtosecond pump-probe techniques. Optical Kerr effect response time was estimated to be less than 165 fs. A third-order optical nonlinearity of χ(3)10-12 esu for PbS particles was obtained and it was found that it increases with the decrease of particle sizes, showing the influence of quantum confined effect on optical nonlinear behaviour of ultrafine particles.
基金Project supported by the National Natural Science Foundation of China(Grant No.11704339)the Applied Basic Research Program of Shanxi Province,China(Grant No.201901D211466)+1 种基金the Natural Science Basic Research Plan in Shaanxi Province of China(Grant No.2019JM-307)the Scientific and Technological Innovation Programs of Higher Education Institutions in Shanxi(STIP),China(Grant Nos.2019L0896 and 2019L0905)。
文摘We investigate the properties of fundamental,multi-peak,and multi-peaked twisted solitons in three types of finite waveguide lattices imprinted in photorefractive media with asymmetrical diffusion nonlinearity.Two opposite soliton selfbending signals are considered for different families of solitons.Power thresholdless fundamental and multi-peaked solitons are stable in the low power region.The existence domain of two-peaked twisted solitons can be changed by the soliton self-bending signals.When solitons tend to self-bend toward the waveguide lattice,stable two-peaked twisted solitons can be found in a larger region in the middle of their existence region.Three-peaked twisted solitons are stable in the lower(upper)cutoff region for a shallow(deep)lattice depth.Our results provide an effective guidance for revealing the soliton characteristics supported by a finite waveguide lattice with diffusive nonlocal nonlinearity.