The intensity of third harmonic emission in air filamentation disturbed by copper fibers and alcohol droplets has been investigated experimentally. Enhancement of the third harmonic emission up to more than one order ...The intensity of third harmonic emission in air filamentation disturbed by copper fibers and alcohol droplets has been investigated experimentally. Enhancement of the third harmonic emission up to more than one order of magnitude has been observed. The physical mechanism of third harmonic enhancement is attributed to suppression of the destructive interference by comparison of the experimental results and it is closely related to the type, size, and relative position of the obstacles.展开更多
The characteristics of backward harmonic radiation due to electron oscillations driven by a linearly polarized fs laser pulse are analysed considering a single electron model. The spectral distributions of the electro...The characteristics of backward harmonic radiation due to electron oscillations driven by a linearly polarized fs laser pulse are analysed considering a single electron model. The spectral distributions of the electron＇s backward harmonic radiation are investigated in detail for different parameters of the driver laser pulse. Higher order harmonic radiations are possible for a sufficiently intense driving laser pulse. We have shown that for a realistic pulsed photon beam, the spectrum of the radiation is red shifted as well as broadened because of changes in the longitudinal velocity of the electrons during the laser pulse. These effects are more pronounced at higher laser intensities giving rise to higher order harmonics that eventually leads to a continuous spectrum. Numerical simulations have further shown that by increasing the laser pulse width the broadening of the high harmonic radiations can be controlled.展开更多
In this work we present experiments by focusing 42 femtosecond laser pulses in air using three differentfocal length lenses: f=100, 30 and 5 cm. For the longest focal length, only the filament, which is aweak plasma c...In this work we present experiments by focusing 42 femtosecond laser pulses in air using three differentfocal length lenses: f=100, 30 and 5 cm. For the longest focal length, only the filament, which is aweak plasma column,is observed. When the shorter focal length lens is used, a high density plasma isgenerated near the geometrical focus and coexists with a weak plasma channel of the filamemt. Under thetightest focusing condition, filamentation is prevented and only a strong plasma volume appears at tehgeometrical focus.展开更多
The filamentation characteristics of femtosecond laser pulses in ZK7 glass are in- vestigated experimentally as a function of initial negative chirps. It is found that the filament threshold power grows rapidly and th...The filamentation characteristics of femtosecond laser pulses in ZK7 glass are in- vestigated experimentally as a function of initial negative chirps. It is found that the filament threshold power grows rapidly and the filament length extends over a long distance with increasing initial temporal chirps. The measurement of supercon- tinuum reveals that the plasma generation process within filamentation becomes weaker as the initial negative chirp increases, leading to a self-guiding long light channel dominated by Kerr nonlinearity. The interference of transverse rings in multifilamentation of the chirped laser pulses is observed as well. Analyses and discussions give an interpretation of this chirp-induced ionization-free filamenta- tion. These results indicate that initial chirps will play a crucial role in the filament formation of ultrashort laser pulses in transparent media.展开更多
In double-pulse laser-induced breakdown spectroscopy(DP-LIBS), the collinear femtosecond double-pulse laser configuration is experimentally investigated with different initial sample temperatures using a Ti:sapphire l...In double-pulse laser-induced breakdown spectroscopy(DP-LIBS), the collinear femtosecond double-pulse laser configuration is experimentally investigated with different initial sample temperatures using a Ti:sapphire laser. The glass sample is ablated to produce the plasma spectroscopy. During the experiment, the detected spectral lines include two Na(I) lines(589.0 nm and 589.6 nm) and one Ca(I) line at the wavelength of 585.7 nm. The emission lines are measured at room temperature(22 ℃) and three higher initial sample temperatures(T_s?=?100 ℃, 200 ℃, and 250 ℃). The inter-pulse delay time ranges from-250 ps to 250 ps.The inter-pulse delay time and the sample temperature strongly influence the spectral intensity,and the spectral intensity can be significantly enhanced by increasing the sample temperature and selecting the optimized inter-pulse time. For the same inter-pulse time of 0 ps(single-pulse LIBS), the enhancement ratio is approximately 2.5 at T_s?=?200 ℃ compared with that obtained at T_s?=?22 ℃. For the same inter-pulse time of 150 ps, the enhancement ratio can be up to 4 at T_s?=?200 ℃ compared with that obtained at T_s?=?22 ℃. The combined enhancement effects of the different initial sample temperatures and the double-pulse configuration in femtosecond LIBS are much stronger than that of the different initial sample temperatures or the double-pulse configuration only.展开更多
A harmonic dark pulse generation in an erbium-doped fiber laser is demonstrated based on a figure-of-eight configuration. It is found that the harmonic dark pulse can be shifted from the fundamental to the 5th order h...A harmonic dark pulse generation in an erbium-doped fiber laser is demonstrated based on a figure-of-eight configuration. It is found that the harmonic dark pulse can be shifted from the fundamental to the 5th order harmonic by increasing the pump power with an appropriate polarization controller orientation. The fundamental repetition rate of 2O kHz is obtained at the pump power of 29 m W. The highest pulse energy of 42.6 n3 is obtained at the fundamental repetition rate. The operating frequency of the dark pulse trains shifts to 2nd, 3rd, 4th and 5th harmonic as the pump powers are increased to 34mW, 50mW, 59mW and 137mW, respectively.展开更多
The generation of terahertz （THz） emission from air plasma induced by two-color femtosecond laser pulses is studied on the basis of a transient photocurrent model. While the gas is ionized by the two-color femtoseco...The generation of terahertz （THz） emission from air plasma induced by two-color femtosecond laser pulses is studied on the basis of a transient photocurrent model. While the gas is ionized by the two-color femtosecond laser-pulses com- posed of the fundamental and its second harmonic, a non-vanishing directional photoelectron current emerges, radiating a THz electromagnetic pulse. The gas ionization processes at three different laser-pulse energies are simulated, and the corresponding THz waveforms and spectra are plotted. The results demonstrate that, by keeping the laser-pulse width and the relative phase between two pulses invariant when the laser energy is at a moderate value, the emitted THz fields are significantly enhanced with a near-linear dependence on the optical energy.展开更多
The spatial distribution of the forward-propagating amplified spontaneous emission(ASE) of nitrogen molecular ions during femtosecond laser filamentation in air is studied via numerical simulations. The results sugges...The spatial distribution of the forward-propagating amplified spontaneous emission(ASE) of nitrogen molecular ions during femtosecond laser filamentation in air is studied via numerical simulations. The results suggest that the divergence angle and signal intensity are extremely sensitive to the external focal length. Concurrently, we show that the optical Kerr effect plays a significant role in concentrating the directivity of ASE signals, particularly in cases of loose focusing. Furthermore,the simulations demonstrate that ASE signals are enhanced for a tight focus, although the corresponding filament length is shorter. The main physical mechanism underlying this process is the competition between the plasma defocusing and optical Kerr effects. The result is important for filamentation-based light detection and ranging applied to remote sensing.展开更多
基金supported by the National Key Technology R&D Program of the Ministry of Science and Technology,China(Grant No.2012BAC23B00)the National Natural Science Foundation of China(Grants No.11404335)
文摘The intensity of third harmonic emission in air filamentation disturbed by copper fibers and alcohol droplets has been investigated experimentally. Enhancement of the third harmonic emission up to more than one order of magnitude has been observed. The physical mechanism of third harmonic enhancement is attributed to suppression of the destructive interference by comparison of the experimental results and it is closely related to the type, size, and relative position of the obstacles.
基金supported by the National High-Tech ICF Committee of China (No.10335020/A0506)National Natural Science Foundation of China (Nos.10474081 and 10576035)Shanghai Natural Science Foundation (No.05ZR14159)
文摘The characteristics of backward harmonic radiation due to electron oscillations driven by a linearly polarized fs laser pulse are analysed considering a single electron model. The spectral distributions of the electron＇s backward harmonic radiation are investigated in detail for different parameters of the driver laser pulse. Higher order harmonic radiations are possible for a sufficiently intense driving laser pulse. We have shown that for a realistic pulsed photon beam, the spectrum of the radiation is red shifted as well as broadened because of changes in the longitudinal velocity of the electrons during the laser pulse. These effects are more pronounced at higher laser intensities giving rise to higher order harmonics that eventually leads to a continuous spectrum. Numerical simulations have further shown that by increasing the laser pulse width the broadening of the high harmonic radiations can be controlled.
文摘In this work we present experiments by focusing 42 femtosecond laser pulses in air using three differentfocal length lenses: f=100, 30 and 5 cm. For the longest focal length, only the filament, which is aweak plasma column,is observed. When the shorter focal length lens is used, a high density plasma isgenerated near the geometrical focus and coexists with a weak plasma channel of the filamemt. Under thetightest focusing condition, filamentation is prevented and only a strong plasma volume appears at tehgeometrical focus.
基金the National Natural Science Foundation of China (Grant No. 60637020)
文摘The filamentation characteristics of femtosecond laser pulses in ZK7 glass are in- vestigated experimentally as a function of initial negative chirps. It is found that the filament threshold power grows rapidly and the filament length extends over a long distance with increasing initial temporal chirps. The measurement of supercon- tinuum reveals that the plasma generation process within filamentation becomes weaker as the initial negative chirp increases, leading to a self-guiding long light channel dominated by Kerr nonlinearity. The interference of transverse rings in multifilamentation of the chirped laser pulses is observed as well. Analyses and discussions give an interpretation of this chirp-induced ionization-free filamenta- tion. These results indicate that initial chirps will play a crucial role in the filament formation of ultrashort laser pulses in transparent media.
基金support by National Natural Science Foundation of China (Grant Nos. 11674128, 11504129, and 11674124)Jilin Province Scientific and Technological Development Program, China (Grant No. 20170101063JC)Fundamental Research Project of Chinese State Key Laboratory of Laser Interaction with Matter (Grant No. SKLLIM1605)
文摘In double-pulse laser-induced breakdown spectroscopy(DP-LIBS), the collinear femtosecond double-pulse laser configuration is experimentally investigated with different initial sample temperatures using a Ti:sapphire laser. The glass sample is ablated to produce the plasma spectroscopy. During the experiment, the detected spectral lines include two Na(I) lines(589.0 nm and 589.6 nm) and one Ca(I) line at the wavelength of 585.7 nm. The emission lines are measured at room temperature(22 ℃) and three higher initial sample temperatures(T_s?=?100 ℃, 200 ℃, and 250 ℃). The inter-pulse delay time ranges from-250 ps to 250 ps.The inter-pulse delay time and the sample temperature strongly influence the spectral intensity,and the spectral intensity can be significantly enhanced by increasing the sample temperature and selecting the optimized inter-pulse time. For the same inter-pulse time of 0 ps(single-pulse LIBS), the enhancement ratio is approximately 2.5 at T_s?=?200 ℃ compared with that obtained at T_s?=?22 ℃. For the same inter-pulse time of 150 ps, the enhancement ratio can be up to 4 at T_s?=?200 ℃ compared with that obtained at T_s?=?22 ℃. The combined enhancement effects of the different initial sample temperatures and the double-pulse configuration in femtosecond LIBS are much stronger than that of the different initial sample temperatures or the double-pulse configuration only.
文摘A harmonic dark pulse generation in an erbium-doped fiber laser is demonstrated based on a figure-of-eight configuration. It is found that the harmonic dark pulse can be shifted from the fundamental to the 5th order harmonic by increasing the pump power with an appropriate polarization controller orientation. The fundamental repetition rate of 2O kHz is obtained at the pump power of 29 m W. The highest pulse energy of 42.6 n3 is obtained at the fundamental repetition rate. The operating frequency of the dark pulse trains shifts to 2nd, 3rd, 4th and 5th harmonic as the pump powers are increased to 34mW, 50mW, 59mW and 137mW, respectively.
基金Project supported by the National Natural Science Foundation of China (Grant No.61177095)the Natural Science Foundation of Hubei Province,China(Grant No.2012FFA074)+1 种基金the Ph.D.Programs Foundation of Ministry of Education of China (Grant No.20100142110042)the Fundamental Research Funds for the Central Universities (Grant Nos.2012QN094 and 2012QN097)
文摘The generation of terahertz （THz） emission from air plasma induced by two-color femtosecond laser pulses is studied on the basis of a transient photocurrent model. While the gas is ionized by the two-color femtosecond laser-pulses com- posed of the fundamental and its second harmonic, a non-vanishing directional photoelectron current emerges, radiating a THz electromagnetic pulse. The gas ionization processes at three different laser-pulse energies are simulated, and the corresponding THz waveforms and spectra are plotted. The results demonstrate that, by keeping the laser-pulse width and the relative phase between two pulses invariant when the laser energy is at a moderate value, the emitted THz fields are significantly enhanced with a near-linear dependence on the optical energy.
基金supported by the National Key R&D Program of China (No.2018YFB0504400)。
文摘The spatial distribution of the forward-propagating amplified spontaneous emission(ASE) of nitrogen molecular ions during femtosecond laser filamentation in air is studied via numerical simulations. The results suggest that the divergence angle and signal intensity are extremely sensitive to the external focal length. Concurrently, we show that the optical Kerr effect plays a significant role in concentrating the directivity of ASE signals, particularly in cases of loose focusing. Furthermore,the simulations demonstrate that ASE signals are enhanced for a tight focus, although the corresponding filament length is shorter. The main physical mechanism underlying this process is the competition between the plasma defocusing and optical Kerr effects. The result is important for filamentation-based light detection and ranging applied to remote sensing.
