The photoluminescence (PL) of nanocrystal present in porous silicon shifts from the near infrared to the ultraviolet depending on the size when the surface is passivated with Si-H bonds. After oxidation, the centre ...The photoluminescence (PL) of nanocrystal present in porous silicon shifts from the near infrared to the ultraviolet depending on the size when the surface is passivated with Si-H bonds. After oxidation, the centre wavelength of PL band is pinned in a region of 700-750 nm and its intensity increases obviously. Calculation shows that trap electronic states appear in the band gap of a smaller nanocrystal when Si = O bonds or Si-O-Si bonds are formed. The changes in PL intensity and wavelength can be explained by both quantum confinement and trap states in an oxidation layer of nanocrystal. In the theoretical model, the most important factor in the enhancement and the pinning effects of PL emission is the relative position between the level of the trap states and the level of the photoexcitation in the silicon nanocrystal.展开更多
In this work,grain boundary(GB)potential barrier(ΔφGB),dopant density(Pnet),and filled trap state density(PGB,trap)were manipulated at the nanoscale by exposing the fabricated perovskite films to various relative hu...In this work,grain boundary(GB)potential barrier(ΔφGB),dopant density(Pnet),and filled trap state density(PGB,trap)were manipulated at the nanoscale by exposing the fabricated perovskite films to various relative humidity(RH)environments.Spatial mapping of surface potential in the perovskite film revealed higher positive potential at GBs than inside the grains.The averageΔφGB,Pnet,and PGB,trap in the perovskite films decreased from 0%RH to 25%RH exposure,but increased when the RH increased to 35%RH and 45%RH.This clearly indicated that perovskite solar cells fabricated at 25%RH led to the lowest average GB potential,smallest dopant density,and least filled trap states density.This is consistent with the highest photovoltaic efficiency of 18.16%at 25%RH among the different relative humidities from 0%to 45%RH.展开更多
Suppressing the trap-state density and the energy loss via ternary strategy was demonstrated.Favorable vertical phase distribution with donors(acceptors)accumulated(depleted)at the interface of active layer and charge...Suppressing the trap-state density and the energy loss via ternary strategy was demonstrated.Favorable vertical phase distribution with donors(acceptors)accumulated(depleted)at the interface of active layer and charge extraction layer can be obtained by introducing appropriate amount of polymer acceptor N2200 into the systems of PBDB-T:IT-M and PBDB-TF:Y6.In addition,N2200 is gradiently distributed in the vertical direction in the ternary blend film.Various measurements were carried out to study the effects of N2200 on the binary systems.It was found that the optimized morphology especially in vertical direction can significantly decrease the trap state density of the binary blend films,which is beneficial for the charge transport and collection.All these features enable an obvious decrease in charge recombination in both PBDB-T:IT-M and PBDB-TF:Y6 based organic solar cells(OSCs),and power conversion efficiencies(PCEs)of 12.5%and 16.42%were obtained for the ternary OSCs,respectively.This work indicates that it is an effective method to suppress the trap state density and thus improve the device performance through ternary strategy.展开更多
This paper proposes an experimentally feasible scheme for implementing quantum dense coding of trapped-ion system in decoherence-free states. As the phase changes due to time evolution of components with different eig...This paper proposes an experimentally feasible scheme for implementing quantum dense coding of trapped-ion system in decoherence-free states. As the phase changes due to time evolution of components with different eigenenergies of quantum superposition are completely frozen, quantum dense coding based on this model would be perfect. The scheme is insensitive to heating of vibrational mode and Bell states can be exactly distinguished via detecting the ionic state.展开更多
Photoluminescence(PL) mechanism of carbon quantum dots(CQDs) remains controversial up to now even though a lot of approaches have been made. In order to do that, herein a PL color ladder from blue to near infrared of ...Photoluminescence(PL) mechanism of carbon quantum dots(CQDs) remains controversial up to now even though a lot of approaches have been made. In order to do that, herein a PL color ladder from blue to near infrared of CQDs with the absolute quantum yields higher than 70% were prepared via a one-pot hydrothermal synthesis route and separated by silica gel column.Time-correlated single photon counting measurements suggest that the electron transition takes in effect in the PL progress of the crystalline core-shell structured CQDs, and the PL properties could be coarsely adjusted by tuning the size of the crystalline carbon core owing to quantum confinement effects, and finely adjusted by changing the surface functional groups consisted shell owing to surface trap states,respectively. Both coarse and fine adjustments of PL, as optical and photoelectrical characterizations and density-functional theory(DFT) calculations have demonstrated, make it possible for top-level design and precise synthesis of new CQDs with specific optical properties.展开更多
This paper proposes a simple scheme to generate a four-atom entangled cluster state in cavity quantum electrodynamics. With the assistantce of a strong classical field the cavity is only virtually excited and no quant...This paper proposes a simple scheme to generate a four-atom entangled cluster state in cavity quantum electrodynamics. With the assistantce of a strong classical field the cavity is only virtually excited and no quantum information will be transferred from the atoms to the cavity during the preparation for a four-atom entangled cluster state, and thus the scheme is insensitive to the cavity field states and cavity decay. Assuming that deviation of laser intensity is 0.01 and that of simultaneity for the interaction is 0.01, it shows that the fidelity of the resulting four-atom entangled cluster state is about 0.9886. The scheme can also be used to generate a four-ion entangled cluster state in a hot trapped-ion system. Assuming that deviation of laser intensity is 0.01, it shows that the fidelity of the resulting four-ion entangled cluster state is about 0.9990. Experimental feasibility for achieving this scheme is also discussed.展开更多
We propose a scheme to generate entangled coherent states for the vibrational modes of N trapped ions.In the scheme the first ion is sequentially excited by two travelling wave laser fields tuned to the ion transition...We propose a scheme to generate entangled coherent states for the vibrational modes of N trapped ions.In the scheme the first ion is sequentially excited by two travelling wave laser fields tuned to the ion transition. The scheme works in the strong-excitation regime, which is of experimental importance in view of decoherence.展开更多
Several schemes have been proposed to prepare two-mode squeezed state and entanglement state betweenmotional states of a single trapped ion and light.Preparation of two-mode squeezed state is based on interaction ofa ...Several schemes have been proposed to prepare two-mode squeezed state and entanglement state betweenmotional states of a single trapped ion and light.Preparation of two-mode squeezed state is based on interaction ofa trapped ion located in light cavity with cavity field.Preparation of entanglement state is based on interaction of atrapped ion located in light cavity with cavity field and a traveling wave light field.展开更多
We propose a scheme for generating a four-particle cluster state in an ion-trap system.The scheme isinsensitive to the thermal motion of the ions,and needs less operations than previous ones.With such a setup,we alsod...We propose a scheme for generating a four-particle cluster state in an ion-trap system.The scheme isinsensitive to the thermal motion of the ions,and needs less operations than previous ones.With such a setup,we alsodemonstrate a procedure for perfectly teleporting an arbitrary two-particle state via a single multipartite entanglementchannel,a four-particle cluster state.展开更多
We propose a scheme for the preparation of one-dimensional and two-dimensional cluster states by using hot trapped ions. The scheme is based on the interaction between two ions and bichromatic radiation. The vibration...We propose a scheme for the preparation of one-dimensional and two-dimensional cluster states by using hot trapped ions. The scheme is based on the interaction between two ions and bichromatic radiation. The vibrational mode in our protocol is only virtually excited so that the system is insensitive to the thermal field. In addition, we only use two levels of ions as qubits and the successful probability may achieve 100%.展开更多
我们在离子陷井系统为一个任意的未知二水平的二离子的状态的确定、多控制的远距传物建议一个简单计划。在计划,当量隧道和需要的单一的转变可以分别地经由一个单个反响的相互作用被完成,特殊纠缠的 W 状态使用了。完成整个过程的要...我们在离子陷井系统为一个任意的未知二水平的二离子的状态的确定、多控制的远距传物建议一个简单计划。在计划,当量隧道和需要的单一的转变可以分别地经由一个单个反响的相互作用被完成,特殊纠缠的 W 状态使用了。完成整个过程的要求的时间不与代理人的数字增加。展开更多
We propose a fast scheme to generate the quantum-interference states of N trapped ions. In the scheme the ions are driven by a standing-wave laser beam whose carrier frequency is tuned such that the ion transition can...We propose a fast scheme to generate the quantum-interference states of N trapped ions. In the scheme the ions are driven by a standing-wave laser beam whose carrier frequency is tuned such that the ion transition can take place. We also propose a simple and fast scheme to produce the GHZ state of N hot trapped ions and this scheme is insensitive to the heating of vibrational motion, which is important from the viewpoint of decoherence.展开更多
This paper investigates the electronic relaxation of deep bulk trap and interface state in ZnO ceramics based on dielectric spectra measured in a wide range of temperature, frequency and bias, in addition to the stead...This paper investigates the electronic relaxation of deep bulk trap and interface state in ZnO ceramics based on dielectric spectra measured in a wide range of temperature, frequency and bias, in addition to the steady state response. It discusses the nature of net current flowing over the barrier affected by interface state, and then obtains temperature-dependent barrier height by approximate calculation from steady I-V (current-voltage) characteristics. Additional conductance and capacitance arising from deep bulk trap relaxation are calculated based on the displacement of the cross point between deep bulk trap and Fermi level under small AC signal. From the resonances due to deep bulk trap relaxation on dielectric spectra, the activation energies are obtained as 0.22 eV and 0.35 eV, which are consistent with the electronic levels of the main defect interstitial Zn and vacancy oxygen in the depletion layer. Under moderate bias, another resonance due to interface relaxation is shown on the dielectric spectra. The DC-like conductance is also observed in high temperature region on dielectric spectra, and the activation energy is much smaller than the barrier height in steady state condition, which is attributed to the displacement current coming from the shallow bulk trap relaxation or other factors.展开更多
A scheme is presented for teleportation of an unknown entangled ionic state between ions kept in two wellseparated traps,which is induced by means of two dispersive laser excitations.The scheme is insensitive to the t...A scheme is presented for teleportation of an unknown entangled ionic state between ions kept in two wellseparated traps,which is induced by means of two dispersive laser excitations.The scheme is insensitive to the thermalmotion and its successful probability can reach 1.展开更多
<正> This paper presents an alternative scheme to realize the storage of entangled states for multiple trappedions including W state,Bell states,and GHZ stares even with ions which exchange vibrational energy wi...<正> This paper presents an alternative scheme to realize the storage of entangled states for multiple trappedions including W state,Bell states,and GHZ stares even with ions which exchange vibrational energy with a heatingsurrounding.Our scheme requires that the ions be simultaneously excited by two laser beams with different frequencies.In this scheme the vibrational degrees of freedom are only regarded as intermediate states and the ions exchange energyvia the mediation of the vibration of the vibrational mode in coupling processes.The scheme is insensitive to both theinitial vibrational state and heating if the system remains in the Lamb-Dicke regime.Since the effective Rabi frequencyhas a small dependence on the vibrational quantum number the heating will have no direct effect on the internal stateevolution.展开更多
We propose a method for the generation of superpositions of two-mode coherent states for the center-of-mass and relative vibrational modes of two trapped ions. In the scheme the ions are driven by a single travelling-...We propose a method for the generation of superpositions of two-mode coherent states for the center-of-mass and relative vibrational modes of two trapped ions. In the scheme the ions are driven by a single travelling-wave laser field tuned to the carrier. Then a measurement of the internal states collapses the vibrational modes to the entangled coherent state.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant No 10764002)
文摘The photoluminescence (PL) of nanocrystal present in porous silicon shifts from the near infrared to the ultraviolet depending on the size when the surface is passivated with Si-H bonds. After oxidation, the centre wavelength of PL band is pinned in a region of 700-750 nm and its intensity increases obviously. Calculation shows that trap electronic states appear in the band gap of a smaller nanocrystal when Si = O bonds or Si-O-Si bonds are formed. The changes in PL intensity and wavelength can be explained by both quantum confinement and trap states in an oxidation layer of nanocrystal. In the theoretical model, the most important factor in the enhancement and the pinning effects of PL emission is the relative position between the level of the trap states and the level of the photoexcitation in the silicon nanocrystal.
基金This work has been supported in part by NSF MRI(1428992)NASA EPSCoR(NNX15AM83A)+3 种基金U.S.-Egypt Science and Technology(S&T)Joint Fund,SDBoR R&D Program,and EDA University Center Program(ED18DEN3030025)This work is derived from the Subject Data supported in whole or part by NAS and USAID,and any opinions,findings,conclusions,or recommendations expressed in the paper are those of the authors alone,and do not necessarily reflect the views of USAID or NAS.We would like to thank Dr Brian Moore for assisting us with high performance computing facility at South Dakota State University.W.Y.acknowledges the support from International Cooperation Project of Anhui Province(1503062018)Visiting Research Scholar Project for Young/Middle Excellent Talents of Anhui Province(gxfxZD2016110)Preeminent Youth Foundation of Anhui Polytechnic University(2016JQ002).
文摘In this work,grain boundary(GB)potential barrier(ΔφGB),dopant density(Pnet),and filled trap state density(PGB,trap)were manipulated at the nanoscale by exposing the fabricated perovskite films to various relative humidity(RH)environments.Spatial mapping of surface potential in the perovskite film revealed higher positive potential at GBs than inside the grains.The averageΔφGB,Pnet,and PGB,trap in the perovskite films decreased from 0%RH to 25%RH exposure,but increased when the RH increased to 35%RH and 45%RH.This clearly indicated that perovskite solar cells fabricated at 25%RH led to the lowest average GB potential,smallest dopant density,and least filled trap states density.This is consistent with the highest photovoltaic efficiency of 18.16%at 25%RH among the different relative humidities from 0%to 45%RH.
基金supported by the National Natural Science Foundation of China(21835006,21704004)the Fundamental Research Funds for the Central Universities,China(FRF-TP-19-047A2)China Postdoctoral Science Foundation(2019M660799)。
文摘Suppressing the trap-state density and the energy loss via ternary strategy was demonstrated.Favorable vertical phase distribution with donors(acceptors)accumulated(depleted)at the interface of active layer and charge extraction layer can be obtained by introducing appropriate amount of polymer acceptor N2200 into the systems of PBDB-T:IT-M and PBDB-TF:Y6.In addition,N2200 is gradiently distributed in the vertical direction in the ternary blend film.Various measurements were carried out to study the effects of N2200 on the binary systems.It was found that the optimized morphology especially in vertical direction can significantly decrease the trap state density of the binary blend films,which is beneficial for the charge transport and collection.All these features enable an obvious decrease in charge recombination in both PBDB-T:IT-M and PBDB-TF:Y6 based organic solar cells(OSCs),and power conversion efficiencies(PCEs)of 12.5%and 16.42%were obtained for the ternary OSCs,respectively.This work indicates that it is an effective method to suppress the trap state density and thus improve the device performance through ternary strategy.
基金Project supported by the Important Program of Hunan Provincial Education Department (Grant No 06A038)Department of Education of Hunan Province (Grant No 06C080)Hunan Provincial Natural Science Foundation,China (Grant No 06JJ4003)
文摘This paper proposes an experimentally feasible scheme for implementing quantum dense coding of trapped-ion system in decoherence-free states. As the phase changes due to time evolution of components with different eigenenergies of quantum superposition are completely frozen, quantum dense coding based on this model would be perfect. The scheme is insensitive to heating of vibrational mode and Bell states can be exactly distinguished via detecting the ionic state.
基金supported by the National Natural Science Foundation of China(21535006)
文摘Photoluminescence(PL) mechanism of carbon quantum dots(CQDs) remains controversial up to now even though a lot of approaches have been made. In order to do that, herein a PL color ladder from blue to near infrared of CQDs with the absolute quantum yields higher than 70% were prepared via a one-pot hydrothermal synthesis route and separated by silica gel column.Time-correlated single photon counting measurements suggest that the electron transition takes in effect in the PL progress of the crystalline core-shell structured CQDs, and the PL properties could be coarsely adjusted by tuning the size of the crystalline carbon core owing to quantum confinement effects, and finely adjusted by changing the surface functional groups consisted shell owing to surface trap states,respectively. Both coarse and fine adjustments of PL, as optical and photoelectrical characterizations and density-functional theory(DFT) calculations have demonstrated, make it possible for top-level design and precise synthesis of new CQDs with specific optical properties.
基金The project supported by the Scientific Research Fund of the Education Department of Hunan Province under Grant No.06C354the Natural Science Foundation of Hunan Province under Grant No.06JJ5015
基金Project supported by the Postdoctal Foundation of Central South University of Chinathe Important Program of Hunan Provincial Education Department of China (Grant No. 06A038)+1 种基金Department of Education of Hunan Province of China (Grant No. 06C080)Hunan Provincial Natural Science Foundation,China (Grant No. 07JJ3013)
文摘This paper proposes a simple scheme to generate a four-atom entangled cluster state in cavity quantum electrodynamics. With the assistantce of a strong classical field the cavity is only virtually excited and no quantum information will be transferred from the atoms to the cavity during the preparation for a four-atom entangled cluster state, and thus the scheme is insensitive to the cavity field states and cavity decay. Assuming that deviation of laser intensity is 0.01 and that of simultaneity for the interaction is 0.01, it shows that the fidelity of the resulting four-atom entangled cluster state is about 0.9886. The scheme can also be used to generate a four-ion entangled cluster state in a hot trapped-ion system. Assuming that deviation of laser intensity is 0.01, it shows that the fidelity of the resulting four-ion entangled cluster state is about 0.9990. Experimental feasibility for achieving this scheme is also discussed.
文摘We propose a scheme to generate entangled coherent states for the vibrational modes of N trapped ions.In the scheme the first ion is sequentially excited by two travelling wave laser fields tuned to the ion transition. The scheme works in the strong-excitation regime, which is of experimental importance in view of decoherence.
基金Supported by the Natural Science Foundation of Anhui Province of China under Grant No.090412060 Natural Science Foundation of the Education Committee of Anhui Province of China under Grant No.KJ2008A029
文摘Several schemes have been proposed to prepare two-mode squeezed state and entanglement state betweenmotional states of a single trapped ion and light.Preparation of two-mode squeezed state is based on interaction ofa trapped ion located in light cavity with cavity field.Preparation of entanglement state is based on interaction of atrapped ion located in light cavity with cavity field and a traveling wave light field.
基金Supported by the National Natural Science Foundation of China under Grant No.10674018the National Fundamental Research Program of China under Grant No.2004CB719903
文摘We propose a scheme for generating a four-particle cluster state in an ion-trap system.The scheme isinsensitive to the thermal motion of the ions,and needs less operations than previous ones.With such a setup,we alsodemonstrate a procedure for perfectly teleporting an arbitrary two-particle state via a single multipartite entanglementchannel,a four-particle cluster state.
基金Project supported by the National Natural Science Foundation of China (Grant No 10574022), and the Funds of the Natural . Science of Fujian Province, China (Grant No Z0512006).
文摘We propose a scheme for the preparation of one-dimensional and two-dimensional cluster states by using hot trapped ions. The scheme is based on the interaction between two ions and bichromatic radiation. The vibrational mode in our protocol is only virtually excited so that the system is insensitive to the thermal field. In addition, we only use two levels of ions as qubits and the successful probability may achieve 100%.
基金Supported by National Natural Science Foundation of China under Grant Nos.60878059 and 10947147the Funds of Educational Committee of Fujian Province under Grant Nos.JA09014 and JB08066the Funds from Fujian Normal University under Grant No.2008100220
文摘我们在离子陷井系统为一个任意的未知二水平的二离子的状态的确定、多控制的远距传物建议一个简单计划。在计划,当量隧道和需要的单一的转变可以分别地经由一个单个反响的相互作用被完成,特殊纠缠的 W 状态使用了。完成整个过程的要求的时间不与代理人的数字增加。
基金Project supported by the National Natural Science Foundation of China (Grant No 10374025) and the Hunan Provincial Natural Science Foundation of China (Grant No 06JJ4003).
文摘We propose a fast scheme to generate the quantum-interference states of N trapped ions. In the scheme the ions are driven by a standing-wave laser beam whose carrier frequency is tuned such that the ion transition can take place. We also propose a simple and fast scheme to produce the GHZ state of N hot trapped ions and this scheme is insensitive to the heating of vibrational motion, which is important from the viewpoint of decoherence.
基金supported by the National Outstanding Young Investigator Grant of China (Grant No. 50625721)the National Natural Science Foundation of China (Grant No. 50972118)
文摘This paper investigates the electronic relaxation of deep bulk trap and interface state in ZnO ceramics based on dielectric spectra measured in a wide range of temperature, frequency and bias, in addition to the steady state response. It discusses the nature of net current flowing over the barrier affected by interface state, and then obtains temperature-dependent barrier height by approximate calculation from steady I-V (current-voltage) characteristics. Additional conductance and capacitance arising from deep bulk trap relaxation are calculated based on the displacement of the cross point between deep bulk trap and Fermi level under small AC signal. From the resonances due to deep bulk trap relaxation on dielectric spectra, the activation energies are obtained as 0.22 eV and 0.35 eV, which are consistent with the electronic levels of the main defect interstitial Zn and vacancy oxygen in the depletion layer. Under moderate bias, another resonance due to interface relaxation is shown on the dielectric spectra. The DC-like conductance is also observed in high temperature region on dielectric spectra, and the activation energy is much smaller than the barrier height in steady state condition, which is attributed to the displacement current coming from the shallow bulk trap relaxation or other factors.
基金The project partially supported by the National Fundamental Research Program of China under Grant No. 2005CB724508 and National Natural Science Foundation of China under Grant Nos. 60478029, 10575040, and 90503010 Acknowledgments The authors thank Prof. Ying Wu for many enlighten- ing discussions.
基金the Science Foundation of Educational Committee of Fujian Province under Grant No.JB06037
文摘A scheme is presented for teleportation of an unknown entangled ionic state between ions kept in two wellseparated traps,which is induced by means of two dispersive laser excitations.The scheme is insensitive to the thermalmotion and its successful probability can reach 1.
基金The project supported by the Natural Science Foundation of Education Bureau of Jiangsu Province of China under Grant No. 05KJB140008. The author is grateful to Prof. Z.D. Wang, Dr. S.L. Zhu, and Prof. Z.C. Dong for critical reading of the manuscript and useful suggestions.
基金The project supported by the State Key Basic Research Development Program of China under Grant No. 20010B309310 and National Natural Science Foundation of China under Grant Nos, 60478029, 90103026, and 10125419,Acknowledgment We would like to thank Prof. Wu Ying for many enlightening discussions.
文摘<正> This paper presents an alternative scheme to realize the storage of entangled states for multiple trappedions including W state,Bell states,and GHZ stares even with ions which exchange vibrational energy with a heatingsurrounding.Our scheme requires that the ions be simultaneously excited by two laser beams with different frequencies.In this scheme the vibrational degrees of freedom are only regarded as intermediate states and the ions exchange energyvia the mediation of the vibration of the vibrational mode in coupling processes.The scheme is insensitive to both theinitial vibrational state and heating if the system remains in the Lamb-Dicke regime.Since the effective Rabi frequencyhas a small dependence on the vibrational quantum number the heating will have no direct effect on the internal stateevolution.
基金教育部霍英东教育基金,the National Natural Science Foundation of China under,Funds from Fuzhou University
文摘We propose a method for the generation of superpositions of two-mode coherent states for the center-of-mass and relative vibrational modes of two trapped ions. In the scheme the ions are driven by a single travelling-wave laser field tuned to the carrier. Then a measurement of the internal states collapses the vibrational modes to the entangled coherent state.