We investigate the spectral redshift of high-order harmonics of the H_2~＋（D_2~＋） molecule by numerically solving the non-Born–Oppenheimer time-dependent Schr ¨odinger equation（TDSE）. The results show that ...We investigate the spectral redshift of high-order harmonics of the H_2~＋（D_2~＋） molecule by numerically solving the non-Born–Oppenheimer time-dependent Schr ¨odinger equation（TDSE）. The results show that the spectral redshift of highorder harmonics can be observed by adding a weak pulse in the falling part of the trapezoidal laser pulses. Comparing with the H_2~＋ molecule, the shift of high-order harmonic generation（HHG） spectrum for the D_2~＋ molecule is more obvious.We employ the spatial distribution in HHG and time-frequency analysis to illustrate the physical mechanism of the spectral redshift of high-order harmonics.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.61575077)the Graduate Innovation Fund of Jilin University(Grant No.2017107)
文摘We investigate the spectral redshift of high-order harmonics of the H_2~＋（D_2~＋） molecule by numerically solving the non-Born–Oppenheimer time-dependent Schr ¨odinger equation（TDSE）. The results show that the spectral redshift of highorder harmonics can be observed by adding a weak pulse in the falling part of the trapezoidal laser pulses. Comparing with the H_2~＋ molecule, the shift of high-order harmonic generation（HHG） spectrum for the D_2~＋ molecule is more obvious.We employ the spatial distribution in HHG and time-frequency analysis to illustrate the physical mechanism of the spectral redshift of high-order harmonics.
