The wavelength dependence of electron localization of H2^＋ and its isotopomers in the ultraviolet pump-probe scheme is investigated by numerically solving the time-dependent Schrodinger equation. By combining with a ...The wavelength dependence of electron localization of H2^＋ and its isotopomers in the ultraviolet pump-probe scheme is investigated by numerically solving the time-dependent Schrodinger equation. By combining with a semiclassical method,an effective analytical formula expressed in the adiabatic representation is established to describe the localization probability with several zero crossings. A stable zone with respect to the laser intensity and carrier envelope phase is found at a relatively long probe wavelength. Finally, the critical probe wavelengths to reach at the stable zone are derived by using the three-dimensional model. Slower nuclear motion of heavier isotopomers leads to a longer critical wavelength.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11404153,11135002,11475076,and 11405077)the Fundamental Research Funds for the Central Universities of China(Grants Nos.lzujbky-2016-29,lzujbky-2016-31,and lzujbky-2016-209)
文摘The wavelength dependence of electron localization of H2^＋ and its isotopomers in the ultraviolet pump-probe scheme is investigated by numerically solving the time-dependent Schrodinger equation. By combining with a semiclassical method,an effective analytical formula expressed in the adiabatic representation is established to describe the localization probability with several zero crossings. A stable zone with respect to the laser intensity and carrier envelope phase is found at a relatively long probe wavelength. Finally, the critical probe wavelengths to reach at the stable zone are derived by using the three-dimensional model. Slower nuclear motion of heavier isotopomers leads to a longer critical wavelength.
