We calculate the production of χ<sub>c</sub> and η<sub>c</sub> by the two-photon process in ultra-peripheral heavy ion collisions at Relativistic Heavy Ion Collider (RHIC) and Large Hadron Co...We calculate the production of χ<sub>c</sub> and η<sub>c</sub> by the two-photon process in ultra-peripheral heavy ion collisions at Relativistic Heavy Ion Collider (RHIC) and Large Hadron Collider (LHC) energies. The differential cross section of transverse momentum distribution and rapidity distribution for (H = χ<sub>c</sub> and η<sub>c</sub>), are estimated by using the equivalent photon flux in the impact parameter space. The numerical results indicate that the study of χ<sub>c</sub> and η<sub>c</sub> in ultra-peripheral heavy ion collisions are feasible at RHIC and LHC energies.展开更多
The title compound, trans 4 [p (N ethyl N (hydroxyethyl)amino) styryl] N methylpyridinium tetraphenylborate(abbreviated as ESMT, C 46 H 49 N 4OB) crystallizes in a space group P 1 with ...The title compound, trans 4 [p (N ethyl N (hydroxyethyl)amino) styryl] N methylpyridinium tetraphenylborate(abbreviated as ESMT, C 46 H 49 N 4OB) crystallizes in a space group P 1 with a =0 983 23(15) nm, b =1 410 73(16) nm, c =1 54 21(12) nm, α=95 252(13)°, β= 91 959(17)°, γ= 107 421(12)°, Z=2, F(000)=712, μ =0 1 mm -1 Mo Kα radiation, R =0 093 8. The result shows that the cation of the molecule almost lies in one plane, the hydroxyethyl group is perpendicular to the plane, the anion takes a slight distorted tetrahedral geometry. Also the thermal stability, two photon fluorescence, two photon pumped lasing property for the title compound were studied.展开更多
Two new bithiophene derivatives named as 5, 5-bis(p-N,N-dimethylaminostyryl)-2, 2 -bithiophene (BMSBT), and 5, 5-bis(p-N,N-diethylaminostyryl)-2, 2-bithiophene (BESBT) have been synthesized. Both compounds can emit s...Two new bithiophene derivatives named as 5, 5-bis(p-N,N-dimethylaminostyryl)-2, 2 -bithiophene (BMSBT), and 5, 5-bis(p-N,N-diethylaminostyryl)-2, 2-bithiophene (BESBT) have been synthesized. Both compounds can emit strong single-photon excited fluorescence (SPEF) and two-photon excited fluorescence (TPEF) with the emission peaks around ~560 nm and with the lifetime of ~1ns.展开更多
In this paper,the energy spectrum of the two-photon Jaynes-Cummings model(TPJCM) is calculated exactly in the non-rotating wave approximation(non-RWA),and we study the level-crossing problem by means of fidelity.A...In this paper,the energy spectrum of the two-photon Jaynes-Cummings model(TPJCM) is calculated exactly in the non-rotating wave approximation(non-RWA),and we study the level-crossing problem by means of fidelity.A narrow peak of the fidelity is observed at the level-crossing point,which does not appear at the avoided-crossing point.Therefore fidelity is perfectly suited for detecting the level-crossing point in the energy spectrum.展开更多
Arbitrary micro-scale three-dimensional(3D)structures fabrication is a dream to achieve many exciting goals that have been pursued for a long time.Among all these applications,the direct 3D printing to fabricate human...Arbitrary micro-scale three-dimensional(3D)structures fabrication is a dream to achieve many exciting goals that have been pursued for a long time.Among all these applications,the direct 3D printing to fabricate human organs and integrated photonic circuits are extraordinary attractive as they can promote the current technology to a new level.Among all the 3D printing methods available,two-photon polymerization(2PP)is very competitive as it is the unique method to achieve sub-micron resolution to make any desired tiny structures.For the conventional 2PP,the building block is the photoresist.However,the requirement for the building block is different for different purposes.It is very necessary to investigate and improve the photoresist properties according to different requirements.In this paper,we presented one hybrid method to modify the mechanical strength and light trapping efficiency of the photoresist,which transfers the photoresist into the micro-concretes.The micro-concrete structure can achieve±22%strength modification via a silica nano-particles doping.The structures doped with gold nano-particles show tunable plasmonic absorption.Dye doped hybrid structure shows great potential to fabricate 3D micro-chip laser.展开更多
Efficient Ti-catalyzed reductive coupling methodology was first employed to synthesize the symmetrical bis-donor stilbene, trans-4, 4'-bis[diphenyl amino] stilbene (BDPAS). X-ray diffraction analyses reveal that t...Efficient Ti-catalyzed reductive coupling methodology was first employed to synthesize the symmetrical bis-donor stilbene, trans-4, 4'-bis[diphenyl amino] stilbene (BDPAS). X-ray diffraction analyses reveal that this new crystal belongs to the triclinic crystal system of centro-symmetric P-1 space group. The DBPAS solution, with the linear transmission at wavelength of greater than or equal to 450 nm, possesses large two-photon absorption cross section as high as 39.4x10(-48) cm(4).s/photon resulting in strong two-photon induced blue fluorescence of 460 nm, pumped by 740 nm laser irradiation.展开更多
An electron donor-π-bridge-electron acceptor(D-π-A) optical functional organic compound comprising a triphenylamine moiety as the electron donor and pyridine moiety as the electron acceptor was synthesized. The stru...An electron donor-π-bridge-electron acceptor(D-π-A) optical functional organic compound comprising a triphenylamine moiety as the electron donor and pyridine moiety as the electron acceptor was synthesized. The structure of the compound was solved by single-crystal X-ray diffraction analysis. It crystallizes in monoclinic, space group P21, with a = 9.753(5), b = 8.815(5), c = 25.554(5) ?, β = 96.315(5)°, V = 2184(2) ?~3, Z = 2, D_c = 1.136 g/m^3, F(000) = 792, Μr = 746.92, μ = 0.069 mm^(-1), the final R = 0.0658 and wR = 0.1730 for 6790 observed reflections with I > 2(I). Study of nonlinear optical properties shows that the compound exhibits excellent two-photon excited fluorescence with the two-photon absorption cross-section value of 116 GM. The structure-property relationship was researched in detail through X-ray crystallography and quantum chemical calculation. Result of living cell imaging experiment shows its potential in fluorescence microscopy bioimaging.展开更多
Completely solving the dissipative dynamics of nonlinear Jaynes-Cumming model is a very difficult task.In our recent work (Phys. Lett. A284 (2001) 156), we just obtained analytical results of the field dissipative dyn...Completely solving the dissipative dynamics of nonlinear Jaynes-Cumming model is a very difficult task.In our recent work (Phys. Lett. A284 (2001) 156), we just obtained analytical results of the field dissipative dynamicsof the nonlinear JCM. In the present paper, employing the perturbative expansion of master equation, we obtain thedensity operator of the system (field +atom). The coherence losses of the system and of the atom are investigated whentwo-photon process is involved. We also study the effect of different atomic initial states and the influence of the fieldamplitude on the atomic coherence loss.展开更多
Considering two atomic qubits initially in Bell states, we send one qubit into a vacuum cavity with two-photon resonance and leave the other one outside. Using quantum information entropy squeezing theory, the time ev...Considering two atomic qubits initially in Bell states, we send one qubit into a vacuum cavity with two-photon resonance and leave the other one outside. Using quantum information entropy squeezing theory, the time evolutions of the entropy squeezing factor of the atomic qubit inside the cavity are discussed for two cases, i.e., before and after rotation and measurement of the atomic qubit outside the cavity. It is shown that the atomic qubit inside the cavity has no entropy squeezing phenomenon and is always in a decoherent state before the operating atomic qubit outside the cavity. However,the periodical entropy squeezing phenomenon emerges and the optimal entropy squeezing state can be prepared for the atomic qubit inside the cavity by adjusting the rotation angle, choosing the interaction time between the atomic qubit and the cavity, controlling the probability amplitudes of subsystem states. Its physical essence is cutting the entanglement between the atomic qubit and its environment, causing the atomic qubit inside the cavity to change from the initial decoherent state into maximum coherent superposition state, which is a possible way of recovering the coherence of a single atomic qubit in the noise environment.展开更多
We theoretically study the system of a superconducting transmission line resonator coupled to two interacting super- conducting flux qubits. It is shown that under certain conditions the resonator mode can be tuned to...We theoretically study the system of a superconducting transmission line resonator coupled to two interacting super- conducting flux qubits. It is shown that under certain conditions the resonator mode can be tuned to two-photon resonance between the ground state and the highest excited state while the middle excited states are far-off resonance. Furthermore, we study the steady-state properties of the flux qubits and resonator, such as the photon statistics, the spectrum and squeezing of the resonator, and demonstrate that two-photon laser can be implemented with current experimental technology.展开更多
The local density of photonic states (LDPS) of an infinite two-dimensional (2D) photonic crystal (PC) composed of rotated square-pillars in a 2D square lattice is calculated in terms of the plane-wave expansion ...The local density of photonic states (LDPS) of an infinite two-dimensional (2D) photonic crystal (PC) composed of rotated square-pillars in a 2D square lattice is calculated in terms of the plane-wave expansion method in a combination with the point group theory. The calculation results show that the LDPS strongly depends on the spatial positions. The variations of the LDPS as functions of the radial coordinate and frequency exhibit “mountain chain” structures with sharp peaks. The LDPS with large value spans a finite area and falls abruptly down to small value at the position corresponding to the interfaces between two different refractive index materials. The larger/lower LDPS occurs inward the lower/larger dielectric-constant medium. This feature can be well interpreted by the continuity of electricdisplacement vector at the interface. In the frequency range of the pseudo-PBG (photonic band gap), the LDPS keeps very low value over the whole Wiger-Seitz cell. It indicates that the spontaneous emission in 2D PCs cannot be prohibited completely, but it can be inhibited intensively when the resonate frequency falls into the pseudo-PBG.展开更多
<Abstract>A two-dimensional photonic crystal with a one-dimensional periodic dielectric background is proposed.The photonic band modulation effects due to the periodic background are investigated based on the pl...<Abstract>A two-dimensional photonic crystal with a one-dimensional periodic dielectric background is proposed.The photonic band modulation effects due to the periodic background are investigated based on the plane wave expansion method.We find that periodic modulation of the dielectric background greatly alters photonic band structures,especially for the E-polarization modes.The number,width and position of the photonie band gaps (PBGs) sensitively depend on the structure parameters (the layer thicknesses and dielectric constants) of the one-dimensional periodic background.展开更多
Two novel V-shaped symmetric chromophores: E-2,8-bis(4-vinyl-4-carbazol-9-yl)diben- zothiophene (abbreviated as SK-G1) and E-2,8-bis(4-vinyl-4-triphenylamino) dibenzothiophene (abbreviated as ST-G1) have been...Two novel V-shaped symmetric chromophores: E-2,8-bis(4-vinyl-4-carbazol-9-yl)diben- zothiophene (abbreviated as SK-G1) and E-2,8-bis(4-vinyl-4-triphenylamino) dibenzothiophene (abbreviated as ST-G1) have been synthesized and characterized. Their two photon absorption properties were measured by the open-aperture femtosecond Z-scan technique and the nanosecond nonlinear optical transmission (NLT), respectively, when pumped by Ti: sapphire laser at 750 nm and 800 nm.展开更多
文摘We calculate the production of χ<sub>c</sub> and η<sub>c</sub> by the two-photon process in ultra-peripheral heavy ion collisions at Relativistic Heavy Ion Collider (RHIC) and Large Hadron Collider (LHC) energies. The differential cross section of transverse momentum distribution and rapidity distribution for (H = χ<sub>c</sub> and η<sub>c</sub>), are estimated by using the equivalent photon flux in the impact parameter space. The numerical results indicate that the study of χ<sub>c</sub> and η<sub>c</sub> in ultra-peripheral heavy ion collisions are feasible at RHIC and LHC energies.
文摘The title compound, trans 4 [p (N ethyl N (hydroxyethyl)amino) styryl] N methylpyridinium tetraphenylborate(abbreviated as ESMT, C 46 H 49 N 4OB) crystallizes in a space group P 1 with a =0 983 23(15) nm, b =1 410 73(16) nm, c =1 54 21(12) nm, α=95 252(13)°, β= 91 959(17)°, γ= 107 421(12)°, Z=2, F(000)=712, μ =0 1 mm -1 Mo Kα radiation, R =0 093 8. The result shows that the cation of the molecule almost lies in one plane, the hydroxyethyl group is perpendicular to the plane, the anion takes a slight distorted tetrahedral geometry. Also the thermal stability, two photon fluorescence, two photon pumped lasing property for the title compound were studied.
基金This work is supported by the National Natural Science Foundation of China(No.20172034)grant for State Key Program of China.
文摘Two new bithiophene derivatives named as 5, 5-bis(p-N,N-dimethylaminostyryl)-2, 2 -bithiophene (BMSBT), and 5, 5-bis(p-N,N-diethylaminostyryl)-2, 2-bithiophene (BESBT) have been synthesized. Both compounds can emit strong single-photon excited fluorescence (SPEF) and two-photon excited fluorescence (TPEF) with the emission peaks around ~560 nm and with the lifetime of ~1ns.
基金Project supported by the National Natural Science Foundation of China (Grant No. 1097602/A06)
文摘In this paper,the energy spectrum of the two-photon Jaynes-Cummings model(TPJCM) is calculated exactly in the non-rotating wave approximation(non-RWA),and we study the level-crossing problem by means of fidelity.A narrow peak of the fidelity is observed at the level-crossing point,which does not appear at the avoided-crossing point.Therefore fidelity is perfectly suited for detecting the level-crossing point in the energy spectrum.
基金The project supported by National Natural Science Foundation of China under Grant Nos. 10274093 and 10474118, the National Fundamental Research Program under Grant No. 2001CB309309, the Natural Science Foundatioa of Hunan Province of China, the Science Research Fund of Educational Department of Hunan Province of China, the Science Research Fund of Hunan Institute of Humanity and Science and Technology under Grant No. 2005A008, and the Foundation for Youth Core-Teachers of Hunan Province under Grant No. 2003165
基金financially supported by A*STAR, SERC 2014 Public Sector Research Funding (PSF) (Grant: SERC Project, 1421200080)973 Program of China (2013CBA01700)Chinese Nature Science Grant (61675207, U1609209)
文摘Arbitrary micro-scale three-dimensional(3D)structures fabrication is a dream to achieve many exciting goals that have been pursued for a long time.Among all these applications,the direct 3D printing to fabricate human organs and integrated photonic circuits are extraordinary attractive as they can promote the current technology to a new level.Among all the 3D printing methods available,two-photon polymerization(2PP)is very competitive as it is the unique method to achieve sub-micron resolution to make any desired tiny structures.For the conventional 2PP,the building block is the photoresist.However,the requirement for the building block is different for different purposes.It is very necessary to investigate and improve the photoresist properties according to different requirements.In this paper,we presented one hybrid method to modify the mechanical strength and light trapping efficiency of the photoresist,which transfers the photoresist into the micro-concretes.The micro-concrete structure can achieve±22%strength modification via a silica nano-particles doping.The structures doped with gold nano-particles show tunable plasmonic absorption.Dye doped hybrid structure shows great potential to fabricate 3D micro-chip laser.
文摘Efficient Ti-catalyzed reductive coupling methodology was first employed to synthesize the symmetrical bis-donor stilbene, trans-4, 4'-bis[diphenyl amino] stilbene (BDPAS). X-ray diffraction analyses reveal that this new crystal belongs to the triclinic crystal system of centro-symmetric P-1 space group. The DBPAS solution, with the linear transmission at wavelength of greater than or equal to 450 nm, possesses large two-photon absorption cross section as high as 39.4x10(-48) cm(4).s/photon resulting in strong two-photon induced blue fluorescence of 460 nm, pumped by 740 nm laser irradiation.
基金supported by the Major Project of Natural Science Research in Universities of Anhui Province(KJ2018ZD037,KJ2018A0333)Key Project of Youth Talents in Universities of Anhui Province(gxyqZD2017067)+5 种基金National Natural Science Foundation of China(21401024)Natural Science Foundation of Anhui Province(1508085MB21)National Students Research Training Program(201810371028)Research Innovation Team of Fuyang Normal University(kytd201710)Horizontal Cooperation Project of Fuyang Municipal Government and Fuyang Normal University(XDHX2016011,XDHX2016004)Anhui University Research Innovation Platform Team Project(201549)
文摘An electron donor-π-bridge-electron acceptor(D-π-A) optical functional organic compound comprising a triphenylamine moiety as the electron donor and pyridine moiety as the electron acceptor was synthesized. The structure of the compound was solved by single-crystal X-ray diffraction analysis. It crystallizes in monoclinic, space group P21, with a = 9.753(5), b = 8.815(5), c = 25.554(5) ?, β = 96.315(5)°, V = 2184(2) ?~3, Z = 2, D_c = 1.136 g/m^3, F(000) = 792, Μr = 746.92, μ = 0.069 mm^(-1), the final R = 0.0658 and wR = 0.1730 for 6790 observed reflections with I > 2(I). Study of nonlinear optical properties shows that the compound exhibits excellent two-photon excited fluorescence with the two-photon absorption cross-section value of 116 GM. The structure-property relationship was researched in detail through X-ray crystallography and quantum chemical calculation. Result of living cell imaging experiment shows its potential in fluorescence microscopy bioimaging.
基金The project supported by National Natural Science Foundation of China under Grant No.10305002
文摘Completely solving the dissipative dynamics of nonlinear Jaynes-Cumming model is a very difficult task.In our recent work (Phys. Lett. A284 (2001) 156), we just obtained analytical results of the field dissipative dynamicsof the nonlinear JCM. In the present paper, employing the perturbative expansion of master equation, we obtain thedensity operator of the system (field +atom). The coherence losses of the system and of the atom are investigated whentwo-photon process is involved. We also study the effect of different atomic initial states and the influence of the fieldamplitude on the atomic coherence loss.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11374096 and 11405052)
文摘Considering two atomic qubits initially in Bell states, we send one qubit into a vacuum cavity with two-photon resonance and leave the other one outside. Using quantum information entropy squeezing theory, the time evolutions of the entropy squeezing factor of the atomic qubit inside the cavity are discussed for two cases, i.e., before and after rotation and measurement of the atomic qubit outside the cavity. It is shown that the atomic qubit inside the cavity has no entropy squeezing phenomenon and is always in a decoherent state before the operating atomic qubit outside the cavity. However,the periodical entropy squeezing phenomenon emerges and the optimal entropy squeezing state can be prepared for the atomic qubit inside the cavity by adjusting the rotation angle, choosing the interaction time between the atomic qubit and the cavity, controlling the probability amplitudes of subsystem states. Its physical essence is cutting the entanglement between the atomic qubit and its environment, causing the atomic qubit inside the cavity to change from the initial decoherent state into maximum coherent superposition state, which is a possible way of recovering the coherence of a single atomic qubit in the noise environment.
基金Project supported by the National Fundamental Research Program of China(Grant No.2011cba00200)the National Natural Science Foundation of China(Grant No.11274295)the Doctor Foundation of Education Ministry of China(Grant No.20113402110059)
文摘We theoretically study the system of a superconducting transmission line resonator coupled to two interacting super- conducting flux qubits. It is shown that under certain conditions the resonator mode can be tuned to two-photon resonance between the ground state and the highest excited state while the middle excited states are far-off resonance. Furthermore, we study the steady-state properties of the flux qubits and resonator, such as the photon statistics, the spectrum and squeezing of the resonator, and demonstrate that two-photon laser can be implemented with current experimental technology.
基金Project supported by National Key Basic Research Special Fund of China and by Natural Science Foundation of Beijing, China.
文摘The local density of photonic states (LDPS) of an infinite two-dimensional (2D) photonic crystal (PC) composed of rotated square-pillars in a 2D square lattice is calculated in terms of the plane-wave expansion method in a combination with the point group theory. The calculation results show that the LDPS strongly depends on the spatial positions. The variations of the LDPS as functions of the radial coordinate and frequency exhibit “mountain chain” structures with sharp peaks. The LDPS with large value spans a finite area and falls abruptly down to small value at the position corresponding to the interfaces between two different refractive index materials. The larger/lower LDPS occurs inward the lower/larger dielectric-constant medium. This feature can be well interpreted by the continuity of electricdisplacement vector at the interface. In the frequency range of the pseudo-PBG (photonic band gap), the LDPS keeps very low value over the whole Wiger-Seitz cell. It indicates that the spontaneous emission in 2D PCs cannot be prohibited completely, but it can be inhibited intensively when the resonate frequency falls into the pseudo-PBG.
基金supported by the State Key Basic Research Program of China under Grant No.2006CB921607China-Australia Special Fund for Science and Technology
文摘<Abstract>A two-dimensional photonic crystal with a one-dimensional periodic dielectric background is proposed.The photonic band modulation effects due to the periodic background are investigated based on the plane wave expansion method.We find that periodic modulation of the dielectric background greatly alters photonic band structures,especially for the E-polarization modes.The number,width and position of the photonie band gaps (PBGs) sensitively depend on the structure parameters (the layer thicknesses and dielectric constants) of the one-dimensional periodic background.
基金the National Natural Science Foundation of China(No.50273024)the Foundation for the Author of National Excellent Doctoral Dissertation of PR China(FANEDD,No 200333)+1 种基金Natural Foundation of Jiangsu Province(No.BK2003031)the Foundation of Jiangsu Province Education Committee(No.03KJB 150115)for financial support.
文摘Two novel V-shaped symmetric chromophores: E-2,8-bis(4-vinyl-4-carbazol-9-yl)diben- zothiophene (abbreviated as SK-G1) and E-2,8-bis(4-vinyl-4-triphenylamino) dibenzothiophene (abbreviated as ST-G1) have been synthesized and characterized. Their two photon absorption properties were measured by the open-aperture femtosecond Z-scan technique and the nanosecond nonlinear optical transmission (NLT), respectively, when pumped by Ti: sapphire laser at 750 nm and 800 nm.