We study the above-threshold ionization(ATI)process of atoms exposed to fundamental and high-frequency lasers with arbitrary ellipticity by applying the frequency-domain theory.It is found that the angular-resolved AT...We study the above-threshold ionization(ATI)process of atoms exposed to fundamental and high-frequency lasers with arbitrary ellipticity by applying the frequency-domain theory.It is found that the angular-resolved ATI spectrum is sensitive to ellipticities of two lasers and emitted angles of the photoelectron.Particularly for the photon energy of the highfrequency laser more than atomic ionization potential,the width of plateau tends to a constant with increasing ellipticity of fundamental field,the dip structure disappears with increasing ellipticity of the high-frequency field.With the help of the quantum channel analysis,it is shown that the angular distribution depends mainly on the ellipticity of high-frequency field in the case that its frequency is high.Moreover,one can see that the maximal and minimal energies in quantum numerical results are in good agreement with the classical prediction.Our investigation may provide theoretical support for experimental research on polarization control of ionization in elliptically polarized two-color laser fields.展开更多
Electron dynamics during non-sequential double ionization(NSDI) is one of the most attractive areas of research in the field of laser–atom or laser–molecule interaction. Based on the classic two-dimensional model, w...Electron dynamics during non-sequential double ionization(NSDI) is one of the most attractive areas of research in the field of laser–atom or laser–molecule interaction. Based on the classic two-dimensional model, we study the process of NSDI of argon atoms driven by a few-cycle orthogonal two-color laser field composed of 800 nm and 400 nm laser pulses. By changing the relative phase of the two laser pulses, a localized enhancement of NSDI yield is observed at 0.5πand 1.5π, which could be attributed to a rapid and substantial increase in the number of electrons returning to the parent ion within extremely short time intervals at these specific phases. Through the analysis of the electron–electron momentum correlations within different time windows of NSDI events and the angular distributions of emitted electrons in different channels, we observe a more pronounced electron–electron correlation phenomenon in the recollision-induced ionization(RII) channel. This is attributed to the shorter delay time in the RII channel.展开更多
Using the semiclassical ensemble model,the dependence of relative amplitude for the recollision dynamics in nonsequential double ionization(NSDI)of neon atom driven by the orthogonally polarized two-color field(OTC)la...Using the semiclassical ensemble model,the dependence of relative amplitude for the recollision dynamics in nonsequential double ionization(NSDI)of neon atom driven by the orthogonally polarized two-color field(OTC)laser field is theoretically studied.And the dynamics in two typical collision pathways,recollision-impact-ionization(RII)and recollisionexcitation with subsequent ionization(RESI),is systematically explored.Our results reveal that the V-shaped structure in the correlated momentum distribution is mainly caused by the RII mechanism when the relative amplitude of the OTC laser field is zero,and the first ionized electrons will quickly skim through the nucleus and share few energy with the second electron.As the relative amplitude increases,the V-shaped structure gradually disappears and electrons are concentrated on the diagonal in the electron correlation spectrum,indicating that the energy sharing after electrons collision is symmetric for OTC laser fields with large relative amplitudes.Our studies show that changing the relative amplitude of the OTC laser field can efficiently control the electron–electron collisions and energy exchange efficiency in the NSDI process.展开更多
Ghanaian society and the world at large have shown a strong interest in the use of lampshades with evidence from hotels and residential dwellings. Table-top Lampshades direct the rays of light to make sight easier for...Ghanaian society and the world at large have shown a strong interest in the use of lampshades with evidence from hotels and residential dwellings. Table-top Lampshades direct the rays of light to make sight easier for reading whereas bedside lampshades provide romantic illumination and beautification in bedrooms. This art studio research sought to examine lampshades on Ghanaian market;their qualities, significance, shortcomings, etc. as the basis to design and produce inventive lampshades for private and public use. The study was conducted at an art studio condition using Practice-based research design method. Findings show that lampshades serve functional and aesthetic significance in public dwellings and the hospitality industry. Nonetheless, available lampshades on the Ghanaian market lack the multifunctional property as well as a local touch which arguably makes them misfit in Ghanaian context in terms of usage. The innovative results of the studio-produced lampshades revealed the possibility of creating symbolic and multifunctional lampshades which suit specific space and tradition. The study recommends the adoption of such innovative design approach in the creation of interior design and decoration artefacts for residential and public edifices.展开更多
The zebrafish embryos were widely employed in genetics,development and drug discovery studies as miniatured animal models.Sorting of two-color fluorescent embryos is often required in large-scale experiments but it is...The zebrafish embryos were widely employed in genetics,development and drug discovery studies as miniatured animal models.Sorting of two-color fluorescent embryos is often required in large-scale experiments but it is challenging to manually sort with high efficiency.Here,we reported a high-throughput sorting system for two-color fluorescent zebraflsh embryos.The embryos can be automatically loaded from a sample pool and sorted based on the average fluorescent intensity.The two-color fluorescent signals were split into two lines and detected by an area array camera.The system achieves the sorting of 100 embryos in less than 10 min with an accuracy of greater than 95%.展开更多
Synthesis of multi-color laser pulses has been developed as a promising way to improve low conversion efficiency of high-order harmonic generation(HHG). Here we systematically study the effect of laser focus in a two-...Synthesis of multi-color laser pulses has been developed as a promising way to improve low conversion efficiency of high-order harmonic generation(HHG). Here we systematically study the effect of laser focus in a two-color waveform on generation of macroscopic HHG in soft x-rays. We find that the dependence of HHG yields on laser focus at low or high gas pressure is sensitive to the characteristics of single-atom harmonic response, in which “short”-or “long”-trajectory emissions can be selectively controlled by changing the waveform of two-color synthesized laser pulse. We uncover the phase-matching mechanism of HHG in the gas medium by examining the propagation of the two-color waveform and the evolution of time-frequency emissions of high-harmonic field. We further reveal that the nonlinear effects, such as geometric phase, atomic dispersion, and plasma defocusing, are responsible for modification of two-color waveform upon propagation. This work can be used to find better macroscopic conditions for generating soft x-ray HHG by employing two-color optimized waveforms.展开更多
The intrinsic chirp of high-order harmonic generation is an important factor limiting the production of ultrashort attosecond pulses.Based on numerically solving the time-dependent Schrodinger equation,the generation ...The intrinsic chirp of high-order harmonic generation is an important factor limiting the production of ultrashort attosecond pulses.Based on numerically solving the time-dependent Schrodinger equation,the generation process of highorder harmonic from the He atom under the action of orthogonal two-color combined pulse of fundamental frequency and higher intensity second harmonic fields is studied.In this paper,we propose to achieve quasi-chirp-free isolated attosecond pulses by superimposing a higher second-harmonic field on the orthogonal direction of the fundamental frequency field.It is found that the high-energy part of its harmonic emission exhibits small chirp characteristics,which can be used to synthesize isolated attosecond pulses.Through the analysis of the wave packets evolution and the classical motion trajectories of the electron,it is demonstrated that the quasi-chirp-free harmonic can be attributed to the simultaneous return of electrons ionized at different times to the parent particle.The influence of the relative phase of the two pulses on the harmonics is further analyzed,and it is observed that this phenomenon is sensitive to the relative phase,but it can still generate isolated attosecond pulses within a certain phase.展开更多
The flame propagation processes of MgH_(2)dust clouds with four different particle sizes were recorded by a high-speed camera.The dynamic flame temperature distributions of MgH_(2)dust clouds were reconstructed by the...The flame propagation processes of MgH_(2)dust clouds with four different particle sizes were recorded by a high-speed camera.The dynamic flame temperature distributions of MgH_(2)dust clouds were reconstructed by the two-color pyrometer technique,and the chemical composition of solid combustion residues were analyzed.The experimental results showed that the average flame propagation velocities of 23μm,40μm,60μm and 103μm MgH_(2)dust clouds in the stable propagation stage were 3.7 m/s,2.8 m/s,2.1 m/s and 0.9 m/s,respectively.The dust clouds with smaller particle sizes had faster flame propagation velocity and stronger oscillation intensity,and their flame temperature distributions were more even and the temperature gradients were smaller.The flame structures of MgH_(2)dust clouds were significantly affected by the particle sinking velocity,and the combustion processes were accompanied by micro-explosion of particles.The falling velocities of 23μm and 40μm MgH_(2)particles were 2.24 cm/s and 6.71 cm/s,respectively.While the falling velocities of 60μm and 103μm MgH_(2)particles were as high as 15.07 cm/s and 44.42 cm/s,respectively,leading to a more rapid downward development and irregular shape of the flame.Furthermore,the dehydrogenation reaction had a significant effect on the combustion performance of MgH_(2)dust.The combustion of H_(2)enhanced the ignition and combustion characteristics of MgH_(2)dust,resulting in a much higher explosion power than the pure Mg dust.The micro-structure characteristics and combustion residues composition analysis of MgH_(2)dust indicated that the combustion control mechanism of MgH_(2)dust flame was mainly the heterogeneous reaction,which was affected by the dehydrogenation reaction.展开更多
In the study,the two-color pyrometer technique was used to measure the transient temperature field of emulsion explosives with different contents of TiH_(2)powders.The experimental results showed that the introduction...In the study,the two-color pyrometer technique was used to measure the transient temperature field of emulsion explosives with different contents of TiH_(2)powders.The experimental results showed that the introduction of TiH_(2)powders could significantly increase the explosion temperature and fireball duration of emulsion explosive.When emulsion explosives were ignited,the average explosion temperature of pure emulsion explosive continuously decreased while emulsion explosives added with TiH_(2)powders increased at first and then decreased.When the content of TiH_(2)powders was 6 mass%,the explosion average temperature reached its maximum value of 3095 K,increasing by 43.7%as compared with that of pure emulsion explosive.In addition,the results of air blast experiment and explosion heat test showed that the variation trends of shock wave parameters,explosion heat and theoretical explosion temperature of emulsion explosives with different contents of TiH_(2)powders were basically consistent with that of explosion temperature measured by the two-color pyrometer technique.In conclusion,the two-color pyrometer technique would be conducive to the formula design of emulsion explosive by understanding the explosion temperature characteristics.展开更多
Explicit visualization of different components of surface plasmon polaritons(SPPs) propagating at dielectric/metal interfaces is crucial in offering chances for the detailed design and control of the functionalities o...Explicit visualization of different components of surface plasmon polaritons(SPPs) propagating at dielectric/metal interfaces is crucial in offering chances for the detailed design and control of the functionalities of plasmonic nanodevices in the future. Here, we reported independent imaging of the vertical and horizontal components of SPPs launched from a rectangular trench in the gold film by a 400-nm laser-assisted near-infrared(NIR) femtosecond laser time-resolved photoemission electron microscopy(TR-PEEM). The experiments demonstrate that distinct imaging of different components of SPPs field can be easily achieved by introducing the 400-nm laser. It can circumvent the risk of sample damage and information loss of excited SPPs field that is generally confronted in the usual NIR laser TR-PEEM scheme. The underlying mechanism for realizing distinct imaging of different components of the SPPs field with two-color PEEM is revealed via measuring the double logarithmic dependence of photoemission yield with the 800-nm and 400-nm pulse powers of different polarizations. Moreover, it is found that the PEEM image quality of the vertical and horizontal components of the SPPs field is nearly independent of the 400-nm pulse polarization. These results pave a way for SPPs-based applications and offer a possible solution for drawing a space-time field of SPPs in three dimensions.展开更多
Using the frequency-domain theory, we investigate the above-threshold ionization(ATI) process of an atom in twocolor laser fields. When both photon energies of the two-color laser fields are much smaller than the at...Using the frequency-domain theory, we investigate the above-threshold ionization(ATI) process of an atom in twocolor laser fields. When both photon energies of the two-color laser fields are much smaller than the atomic ionization threshold, the ATI spectrum depends on the angle between the two lasers' polarization directions. While when the photon energy of one laser is comparable with or larger than the atomic ionization threshold, the ATI spectrum is independent of the angle, and only several dips appear at certain angles. By analyzing the contributions of different quantum channels, we find that, for the case that both frequencies of the two color lasers are low, the quantum interferences between the channels are strong, and hence the spectrum changes with the angle between the two lasers' polarization directions. While for the case that the frequency of one of the two color lasers is high, the contributions of the channels to the ATI spectrum decrease dramatically with increasing channel order, hence the interferences between the channels disappear, and the ATI spectrum has a step-like structure, which is independent of the angle between the two lasers' polarizations. These results can shed light on the study of the corresponding relation between classical and quantum mechanisms of the matter–laser interaction in high-frequency laser fields.展开更多
To date, two-color pulses are widely used in pump–probe experiments. For a ring-based light source, the power of the spontaneous radiation fluctuates randomly in the longitudinal direction. It is difficult to produce...To date, two-color pulses are widely used in pump–probe experiments. For a ring-based light source, the power of the spontaneous radiation fluctuates randomly in the longitudinal direction. It is difficult to produce twocolor double pulses by optical methods. In this paper, we introduce a method based on the echo-enabled harmonic generation scheme that generates two-color pulses in a storage ring light source. By adopting crossed undulators and a phase shifter, the polarization of the two-color pulses can be easily switched. A numerical simulation based on a diffraction-limited storage ring, the Hefei Advanced Light Source, suggests that the time delay and spectral separation of the two pulses can be adjusted linearly by changing the pulse duration and chirp parameters of the seed laser. A circular polarization degree above 80% could be achieved.展开更多
The coherent-mode representation theory is firstly used to analyze lensless two-color ghost imaging. A quite complicated expression about the point-spread function(PSF) needs to be given to analyze which wavelength ...The coherent-mode representation theory is firstly used to analyze lensless two-color ghost imaging. A quite complicated expression about the point-spread function(PSF) needs to be given to analyze which wavelength has a stronger affect on imaging quality when the usual integral representation theory is used to ghost imaging. Unlike this theory, the coherent-mode representation theory shows that imaging quality depends crucially on the distribution of the decomposition coefficients of the object imaged in a two-color ghost imaging. The analytical expression of the decomposition coefficients of the object is unconcerned with the wavelength of the light used in the reference arm, but has relevance with the wavelength in the object arm. In other words, imaging quality of two-color ghost imaging depends primarily on the wavelength of the light illuminating the object. Our simulation results also demonstrate this conclusion.展开更多
We theoretically study the high-order harmonic generation (HHG) in a two-color laser field using the Bohmian mechanics. Our results show that, for tile case of a weak second-color laser field, the simulation of the ...We theoretically study the high-order harmonic generation (HHG) in a two-color laser field using the Bohmian mechanics. Our results show that, for tile case of a weak second-color laser field, the simulation of the HHG with only one central Bohmian trajectory is in a good agreement with the ab initio time-dependent Schrodinger equation (TDSE) results. In contrast, with the increase of the amplitude of the second-color laser field, the HHG spectra from the single central Bohmian trajectory deviate from the TDSE results more and more significantly. By analyzing the Bohmian trajectories, we find that the significant deviation is due to the fact that the central Bohmian trajectory leaves the core quickly in the two-color laser field with the breaking of inversion symmetry. Interestingly, we find that another Bohmian trajectory with different initial position, which keeps oscillating around the core, could qualitatively well reproduce the TDSE results. Furthermore, we study the HHG spectrum in a two-color laser field with inversion symmetry and find that the HHG spectrum in TDSE can be still well simulated with the central Bohmian trajectory. These results indicate that, similar to the case of one color laser field, the HHG spectra in a two-color laser field can be also reproduced with a single Bohmian trajectory, although the initial position of the trajectory is dependent on the symmetry of the laser field. Our work thus demonstrates that Bohmian trajectory theory can be used as a promising tool in investigating the HHG process in a two-color laser field.展开更多
Using the classical ensemble model, we investigate the nonsequential double ionization(NSDI) of Ar and Mg in the two-color elliptically polarized laser pulse for different elliptical polarizations. Numerical results...Using the classical ensemble model, we investigate the nonsequential double ionization(NSDI) of Ar and Mg in the two-color elliptically polarized laser pulse for different elliptical polarizations. Numerical results show that for Ar atoms the NSDI yield increases as the ellipticity increases, which is different from the case of Mg atoms. Moreover, the correlated behavior in the correlated electron momentum along the x direction and ion momentum distributions of Ar atoms are influenced by the ellipticity. By statistical analysis of different times, we can conclude that the ellipticity may be responsible for the NSDI processes. The correlated momenta distributions along the x direction at the recollision time are demonstrated and the results show that the travelling time and ellipticity can affect the emitted directions of both electrons.展开更多
The generation of high-order harmonic and the attosecond pulse of the N2 molecule with an orthogonally polarized two-color laser field are investigated by the strong-field Lewenstein model.We show that the control of ...The generation of high-order harmonic and the attosecond pulse of the N2 molecule with an orthogonally polarized two-color laser field are investigated by the strong-field Lewenstein model.We show that the control of contributions to high-order harmonic generation(HHG) from different nuclei is realized by properly selecting the relative phase.When the relative phase is chosen to be φ= 0.4π,the contribution to HHG from one nucleus is much more than that from another.Interference between two nuclei can be suppressed greatly; a supercontinuum spectrum of HHG appears from 40 e V to125 e V.The underlying physical mechanism is well explained by the time–frequency analysis and the semi-classical threestep model with a finite initial transverse velocity.By superposing several orders of harmonics,an isolated attosecond pulse with a duration of 80 as can be generated.展开更多
The generation of high-order harmonics and the attosecond pulse of the N2 molecule in two-color circularly polarized laser fields are investigated by the strong-field Lewenstein model. We show that the plateau of spec...The generation of high-order harmonics and the attosecond pulse of the N2 molecule in two-color circularly polarized laser fields are investigated by the strong-field Lewenstein model. We show that the plateau of spectra is dramatically extended and a continuous harmonic spectrum with the bandwidth of 113 eV is obtained. When a static field is added to the x direction, the quantum path control is realized and a supercontinuum spectrum can be obtained, which is beneficial to obtain a shorter attosecond pulse. The underlying physical mechanism is well explained by the time-frequency analysis and the semi-classical three-step model with a finite initial transverse velocity. By superposing several orders of harmonics in the combination of two-color circularly polarized laser fields and a static field, an isolated attosecond pulse with a duration of 30 as can be generated.展开更多
Near-IR femtosecond lasers have been proposed to produce high-field terahertz radiation in the air via the laser-plasma interaction, but the physical mechanism still needs to be further explored. In this work, we theo...Near-IR femtosecond lasers have been proposed to produce high-field terahertz radiation in the air via the laser-plasma interaction, but the physical mechanism still needs to be further explored. In this work, we theoretically investigate the effect of the two-color laser wavelength on the terahertz generation in the air based on a transient photocurrent model.We show that the long wavelength laser excitation can greatly enhance the terahertz amplitude for a given total laser intensity. Furthermore, we utilize a local current model to illustrate the enhancement mechanism. Our analysis shows that the terahertz amplitude is determined by the superposition of contributions from individual ionization events, and for the long wavelength laser excitation, the electron production concentrates in a few ionization events and acquires the larger drift velocities, which results in the stronger terahertz radiation generation. These results will be very helpful for understanding the terahertz generation process and optimizing the terahertz output.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant Nos.12104285,12074240,12204135,12374260,12264013,12204136,92250303,and 12074418)the Guangdong Basicand Applied Basic Research Foundation (Grant No.2022A1515011742)+5 种基金the Special Scientific Research Program supported by the Shaanxi Education Department (Grant No.22JK0423)the Natural Science Basic Research Program of Shaanxi Province of China (Grant Nos.2023-JC-QN-0085 and 2023-JC-QN-0267)the Hainan Provincial Natural Science Foundation of China (Grant Nos.122CXTD504,123MS002,123QN179,123QN180,and 122QN217)the Sino-German Mobility Programme (Grant No.M-0031)the Xi’an Aeronautical Institute 2023 Innovation and Entrepreneurship Training Program for college students (Grant No.S202311736036)the Course Ideological and Political Education Program (Grant No.23ZLGC5030)。
文摘We study the above-threshold ionization(ATI)process of atoms exposed to fundamental and high-frequency lasers with arbitrary ellipticity by applying the frequency-domain theory.It is found that the angular-resolved ATI spectrum is sensitive to ellipticities of two lasers and emitted angles of the photoelectron.Particularly for the photon energy of the highfrequency laser more than atomic ionization potential,the width of plateau tends to a constant with increasing ellipticity of fundamental field,the dip structure disappears with increasing ellipticity of the high-frequency field.With the help of the quantum channel analysis,it is shown that the angular distribution depends mainly on the ellipticity of high-frequency field in the case that its frequency is high.Moreover,one can see that the maximal and minimal energies in quantum numerical results are in good agreement with the classical prediction.Our investigation may provide theoretical support for experimental research on polarization control of ionization in elliptically polarized two-color laser fields.
基金partly supported by the National Natural Science Foundation of China (Grant Nos. 12034008,12250003, and 11727810)the Program of Introducing Talents of Discipline to Universities 111 Project (B12024)。
文摘Electron dynamics during non-sequential double ionization(NSDI) is one of the most attractive areas of research in the field of laser–atom or laser–molecule interaction. Based on the classic two-dimensional model, we study the process of NSDI of argon atoms driven by a few-cycle orthogonal two-color laser field composed of 800 nm and 400 nm laser pulses. By changing the relative phase of the two laser pulses, a localized enhancement of NSDI yield is observed at 0.5πand 1.5π, which could be attributed to a rapid and substantial increase in the number of electrons returning to the parent ion within extremely short time intervals at these specific phases. Through the analysis of the electron–electron momentum correlations within different time windows of NSDI events and the angular distributions of emitted electrons in different channels, we observe a more pronounced electron–electron correlation phenomenon in the recollision-induced ionization(RII) channel. This is attributed to the shorter delay time in the RII channel.
基金Project supported by the National Natural Science Foundation of China (Grant Nos.12204132 and 12304376)Excellent Youth Science Foundation of Shandong Province (Overseas) (Grant No.2022HWYQ-073)+1 种基金the Fundamental Research Funds for the Central Universities (Grant No.HIT.OCEF.2022042)Natural Science Foundation of Shandong Province (Grant No.ZR2023QA075)。
文摘Using the semiclassical ensemble model,the dependence of relative amplitude for the recollision dynamics in nonsequential double ionization(NSDI)of neon atom driven by the orthogonally polarized two-color field(OTC)laser field is theoretically studied.And the dynamics in two typical collision pathways,recollision-impact-ionization(RII)and recollisionexcitation with subsequent ionization(RESI),is systematically explored.Our results reveal that the V-shaped structure in the correlated momentum distribution is mainly caused by the RII mechanism when the relative amplitude of the OTC laser field is zero,and the first ionized electrons will quickly skim through the nucleus and share few energy with the second electron.As the relative amplitude increases,the V-shaped structure gradually disappears and electrons are concentrated on the diagonal in the electron correlation spectrum,indicating that the energy sharing after electrons collision is symmetric for OTC laser fields with large relative amplitudes.Our studies show that changing the relative amplitude of the OTC laser field can efficiently control the electron–electron collisions and energy exchange efficiency in the NSDI process.
文摘Ghanaian society and the world at large have shown a strong interest in the use of lampshades with evidence from hotels and residential dwellings. Table-top Lampshades direct the rays of light to make sight easier for reading whereas bedside lampshades provide romantic illumination and beautification in bedrooms. This art studio research sought to examine lampshades on Ghanaian market;their qualities, significance, shortcomings, etc. as the basis to design and produce inventive lampshades for private and public use. The study was conducted at an art studio condition using Practice-based research design method. Findings show that lampshades serve functional and aesthetic significance in public dwellings and the hospitality industry. Nonetheless, available lampshades on the Ghanaian market lack the multifunctional property as well as a local touch which arguably makes them misfit in Ghanaian context in terms of usage. The innovative results of the studio-produced lampshades revealed the possibility of creating symbolic and multifunctional lampshades which suit specific space and tradition. The study recommends the adoption of such innovative design approach in the creation of interior design and decoration artefacts for residential and public edifices.
基金the National Natural Science Foundation of China(No.62205368)the Suzhou Basic Research Pilot Project(SJC2021013)the Key Research and Development Program of Jiangsu Province(BE2020664).
文摘The zebrafish embryos were widely employed in genetics,development and drug discovery studies as miniatured animal models.Sorting of two-color fluorescent embryos is often required in large-scale experiments but it is challenging to manually sort with high efficiency.Here,we reported a high-throughput sorting system for two-color fluorescent zebraflsh embryos.The embryos can be automatically loaded from a sample pool and sorted based on the average fluorescent intensity.The two-color fluorescent signals were split into two lines and detected by an area array camera.The system achieves the sorting of 100 embryos in less than 10 min with an accuracy of greater than 95%.
基金Project supported by the National Natural Science Foundation of China (Grant Nos.91950102,12274230,and 11834004)the Funding of Nanjing University of Science and Technology (Grant No.TSXK2022D005)。
文摘Synthesis of multi-color laser pulses has been developed as a promising way to improve low conversion efficiency of high-order harmonic generation(HHG). Here we systematically study the effect of laser focus in a two-color waveform on generation of macroscopic HHG in soft x-rays. We find that the dependence of HHG yields on laser focus at low or high gas pressure is sensitive to the characteristics of single-atom harmonic response, in which “short”-or “long”-trajectory emissions can be selectively controlled by changing the waveform of two-color synthesized laser pulse. We uncover the phase-matching mechanism of HHG in the gas medium by examining the propagation of the two-color waveform and the evolution of time-frequency emissions of high-harmonic field. We further reveal that the nonlinear effects, such as geometric phase, atomic dispersion, and plasma defocusing, are responsible for modification of two-color waveform upon propagation. This work can be used to find better macroscopic conditions for generating soft x-ray HHG by employing two-color optimized waveforms.
基金Project supported by the National Key Research and Development Program of China(Grant No.2019YFA0307700)the National Natural Science Foundation of China(Grant Nos.12074145,11627807,and 11975012)+2 种基金the Research Foundation for Basic Research of Jilin Province,China(Grant No.20220101003JC)the Fundamental Research Funds for the Central Universities of China(Grant No.30916011207)the Outstanding Youth Project of Taizhou University(Grant No.2019JQ002)。
文摘The intrinsic chirp of high-order harmonic generation is an important factor limiting the production of ultrashort attosecond pulses.Based on numerically solving the time-dependent Schrodinger equation,the generation process of highorder harmonic from the He atom under the action of orthogonal two-color combined pulse of fundamental frequency and higher intensity second harmonic fields is studied.In this paper,we propose to achieve quasi-chirp-free isolated attosecond pulses by superimposing a higher second-harmonic field on the orthogonal direction of the fundamental frequency field.It is found that the high-energy part of its harmonic emission exhibits small chirp characteristics,which can be used to synthesize isolated attosecond pulses.Through the analysis of the wave packets evolution and the classical motion trajectories of the electron,it is demonstrated that the quasi-chirp-free harmonic can be attributed to the simultaneous return of electrons ionized at different times to the parent particle.The influence of the relative phase of the two pulses on the harmonics is further analyzed,and it is observed that this phenomenon is sensitive to the relative phase,but it can still generate isolated attosecond pulses within a certain phase.
基金supported by the National Natural Science Foundation of China(Grant Nos.12272001,11972046)the Outstanding Youth Project of Natural Science Foundation of Anhui Province(Grant No.2108085Y02)the Major Project of Anhui University Natural Science Foundation(Grant No.KJ2020ZD30)。
文摘The flame propagation processes of MgH_(2)dust clouds with four different particle sizes were recorded by a high-speed camera.The dynamic flame temperature distributions of MgH_(2)dust clouds were reconstructed by the two-color pyrometer technique,and the chemical composition of solid combustion residues were analyzed.The experimental results showed that the average flame propagation velocities of 23μm,40μm,60μm and 103μm MgH_(2)dust clouds in the stable propagation stage were 3.7 m/s,2.8 m/s,2.1 m/s and 0.9 m/s,respectively.The dust clouds with smaller particle sizes had faster flame propagation velocity and stronger oscillation intensity,and their flame temperature distributions were more even and the temperature gradients were smaller.The flame structures of MgH_(2)dust clouds were significantly affected by the particle sinking velocity,and the combustion processes were accompanied by micro-explosion of particles.The falling velocities of 23μm and 40μm MgH_(2)particles were 2.24 cm/s and 6.71 cm/s,respectively.While the falling velocities of 60μm and 103μm MgH_(2)particles were as high as 15.07 cm/s and 44.42 cm/s,respectively,leading to a more rapid downward development and irregular shape of the flame.Furthermore,the dehydrogenation reaction had a significant effect on the combustion performance of MgH_(2)dust.The combustion of H_(2)enhanced the ignition and combustion characteristics of MgH_(2)dust,resulting in a much higher explosion power than the pure Mg dust.The micro-structure characteristics and combustion residues composition analysis of MgH_(2)dust indicated that the combustion control mechanism of MgH_(2)dust flame was mainly the heterogeneous reaction,which was affected by the dehydrogenation reaction.
基金supported by the National Natural Science Foundation of China(No.11972046)Outstanding Youth Project of Natural Science Foundation of Anhui Province(No.2108085Y02)+1 种基金Major Project of Anhui University Natural Science Foundation(No.KJ2020ZD30)Anhui University of Science and Technology Postgraduate Innovation Fund(No.2020CX2066)。
文摘In the study,the two-color pyrometer technique was used to measure the transient temperature field of emulsion explosives with different contents of TiH_(2)powders.The experimental results showed that the introduction of TiH_(2)powders could significantly increase the explosion temperature and fireball duration of emulsion explosive.When emulsion explosives were ignited,the average explosion temperature of pure emulsion explosive continuously decreased while emulsion explosives added with TiH_(2)powders increased at first and then decreased.When the content of TiH_(2)powders was 6 mass%,the explosion average temperature reached its maximum value of 3095 K,increasing by 43.7%as compared with that of pure emulsion explosive.In addition,the results of air blast experiment and explosion heat test showed that the variation trends of shock wave parameters,explosion heat and theoretical explosion temperature of emulsion explosives with different contents of TiH_(2)powders were basically consistent with that of explosion temperature measured by the two-color pyrometer technique.In conclusion,the two-color pyrometer technique would be conducive to the formula design of emulsion explosive by understanding the explosion temperature characteristics.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 62005022, 12004052, and 62175018)the Fund from Jilin Provincial Key Laboratory of Ultrafast and Extreme Ultraviolet Optics (Grant No. YDZJ202102CXJD028)+2 种基金Department of Science and Technology of the Jilin Province, China (Grant Nos. 20200201268JC and 20200401052GX)the “111” Project of China (Grant No. D17017)the Fund from the Ministry of Education Key Laboratory for Cross-Scale Micro and Nano Manufacturing, Changchun University of Science and Technology。
文摘Explicit visualization of different components of surface plasmon polaritons(SPPs) propagating at dielectric/metal interfaces is crucial in offering chances for the detailed design and control of the functionalities of plasmonic nanodevices in the future. Here, we reported independent imaging of the vertical and horizontal components of SPPs launched from a rectangular trench in the gold film by a 400-nm laser-assisted near-infrared(NIR) femtosecond laser time-resolved photoemission electron microscopy(TR-PEEM). The experiments demonstrate that distinct imaging of different components of SPPs field can be easily achieved by introducing the 400-nm laser. It can circumvent the risk of sample damage and information loss of excited SPPs field that is generally confronted in the usual NIR laser TR-PEEM scheme. The underlying mechanism for realizing distinct imaging of different components of the SPPs field with two-color PEEM is revealed via measuring the double logarithmic dependence of photoemission yield with the 800-nm and 400-nm pulse powers of different polarizations. Moreover, it is found that the PEEM image quality of the vertical and horizontal components of the SPPs field is nearly independent of the 400-nm pulse polarization. These results pave a way for SPPs-based applications and offer a possible solution for drawing a space-time field of SPPs in three dimensions.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11474348 and 61275128)
文摘Using the frequency-domain theory, we investigate the above-threshold ionization(ATI) process of an atom in twocolor laser fields. When both photon energies of the two-color laser fields are much smaller than the atomic ionization threshold, the ATI spectrum depends on the angle between the two lasers' polarization directions. While when the photon energy of one laser is comparable with or larger than the atomic ionization threshold, the ATI spectrum is independent of the angle, and only several dips appear at certain angles. By analyzing the contributions of different quantum channels, we find that, for the case that both frequencies of the two color lasers are low, the quantum interferences between the channels are strong, and hence the spectrum changes with the angle between the two lasers' polarization directions. While for the case that the frequency of one of the two color lasers is high, the contributions of the channels to the ATI spectrum decrease dramatically with increasing channel order, hence the interferences between the channels disappear, and the ATI spectrum has a step-like structure, which is independent of the angle between the two lasers' polarizations. These results can shed light on the study of the corresponding relation between classical and quantum mechanisms of the matter–laser interaction in high-frequency laser fields.
基金supported by the National Natural Science Foundation of China(Nos.11475202,11405187)Youth Innovation Association of Chinese Academy of Sciences,and Bureau of Frontier Sciences and Education,Chinese Academy of Sciences(No.QYZDJ-SSWSLH001)National Key R&D Program of China(No.2016YFA0401900)
文摘To date, two-color pulses are widely used in pump–probe experiments. For a ring-based light source, the power of the spontaneous radiation fluctuates randomly in the longitudinal direction. It is difficult to produce twocolor double pulses by optical methods. In this paper, we introduce a method based on the echo-enabled harmonic generation scheme that generates two-color pulses in a storage ring light source. By adopting crossed undulators and a phase shifter, the polarization of the two-color pulses can be easily switched. A numerical simulation based on a diffraction-limited storage ring, the Hefei Advanced Light Source, suggests that the time delay and spectral separation of the two pulses can be adjusted linearly by changing the pulse duration and chirp parameters of the seed laser. A circular polarization degree above 80% could be achieved.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61771067,61631014,61471051,and 61401036)the Youth Research and Innovation Program of Beijing University of Posts and Telecommunications,China(Grant Nos.2015RC12 and 2017RC10)
文摘The coherent-mode representation theory is firstly used to analyze lensless two-color ghost imaging. A quite complicated expression about the point-spread function(PSF) needs to be given to analyze which wavelength has a stronger affect on imaging quality when the usual integral representation theory is used to ghost imaging. Unlike this theory, the coherent-mode representation theory shows that imaging quality depends crucially on the distribution of the decomposition coefficients of the object imaged in a two-color ghost imaging. The analytical expression of the decomposition coefficients of the object is unconcerned with the wavelength of the light used in the reference arm, but has relevance with the wavelength in the object arm. In other words, imaging quality of two-color ghost imaging depends primarily on the wavelength of the light illuminating the object. Our simulation results also demonstrate this conclusion.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11334009,11474321,and 11527807)
文摘We theoretically study the high-order harmonic generation (HHG) in a two-color laser field using the Bohmian mechanics. Our results show that, for tile case of a weak second-color laser field, the simulation of the HHG with only one central Bohmian trajectory is in a good agreement with the ab initio time-dependent Schrodinger equation (TDSE) results. In contrast, with the increase of the amplitude of the second-color laser field, the HHG spectra from the single central Bohmian trajectory deviate from the TDSE results more and more significantly. By analyzing the Bohmian trajectories, we find that the significant deviation is due to the fact that the central Bohmian trajectory leaves the core quickly in the two-color laser field with the breaking of inversion symmetry. Interestingly, we find that another Bohmian trajectory with different initial position, which keeps oscillating around the core, could qualitatively well reproduce the TDSE results. Furthermore, we study the HHG spectrum in a two-color laser field with inversion symmetry and find that the HHG spectrum in TDSE can be still well simulated with the central Bohmian trajectory. These results indicate that, similar to the case of one color laser field, the HHG spectra in a two-color laser field can be also reproduced with a single Bohmian trajectory, although the initial position of the trajectory is dependent on the symmetry of the laser field. Our work thus demonstrates that Bohmian trajectory theory can be used as a promising tool in investigating the HHG process in a two-color laser field.
基金Project supported by the National Natural Science Foundation of China(Grant No.61575077)the Natural Science Foundation of Jilin Province,China(Grant No.20180101225JC)
文摘Using the classical ensemble model, we investigate the nonsequential double ionization(NSDI) of Ar and Mg in the two-color elliptically polarized laser pulse for different elliptical polarizations. Numerical results show that for Ar atoms the NSDI yield increases as the ellipticity increases, which is different from the case of Mg atoms. Moreover, the correlated behavior in the correlated electron momentum along the x direction and ion momentum distributions of Ar atoms are influenced by the ellipticity. By statistical analysis of different times, we can conclude that the ellipticity may be responsible for the NSDI processes. The correlated momenta distributions along the x direction at the recollision time are demonstrated and the results show that the travelling time and ellipticity can affect the emitted directions of both electrons.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11271158,61575077,and 11574117)
文摘The generation of high-order harmonic and the attosecond pulse of the N2 molecule with an orthogonally polarized two-color laser field are investigated by the strong-field Lewenstein model.We show that the control of contributions to high-order harmonic generation(HHG) from different nuclei is realized by properly selecting the relative phase.When the relative phase is chosen to be φ= 0.4π,the contribution to HHG from one nucleus is much more than that from another.Interference between two nuclei can be suppressed greatly; a supercontinuum spectrum of HHG appears from 40 e V to125 e V.The underlying physical mechanism is well explained by the time–frequency analysis and the semi-classical threestep model with a finite initial transverse velocity.By superposing several orders of harmonics,an isolated attosecond pulse with a duration of 80 as can be generated.
基金supported by the National Natural Science Foundation of China(Grant Nos.61575077,11271158,and 11574117)
文摘The generation of high-order harmonics and the attosecond pulse of the N2 molecule in two-color circularly polarized laser fields are investigated by the strong-field Lewenstein model. We show that the plateau of spectra is dramatically extended and a continuous harmonic spectrum with the bandwidth of 113 eV is obtained. When a static field is added to the x direction, the quantum path control is realized and a supercontinuum spectrum can be obtained, which is beneficial to obtain a shorter attosecond pulse. The underlying physical mechanism is well explained by the time-frequency analysis and the semi-classical three-step model with a finite initial transverse velocity. By superposing several orders of harmonics in the combination of two-color circularly polarized laser fields and a static field, an isolated attosecond pulse with a duration of 30 as can be generated.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.51132004,11604205,and 11474096)Science and Technology Commission of Shanghai Municipality,China(Grant No.14JC1401500)+1 种基金Shanghai Municipal Education Commission,China(Grant No.ZZGCD15066)Foundation of Fujian Educational Committee,China(Grant No.JAT160412)
文摘Near-IR femtosecond lasers have been proposed to produce high-field terahertz radiation in the air via the laser-plasma interaction, but the physical mechanism still needs to be further explored. In this work, we theoretically investigate the effect of the two-color laser wavelength on the terahertz generation in the air based on a transient photocurrent model.We show that the long wavelength laser excitation can greatly enhance the terahertz amplitude for a given total laser intensity. Furthermore, we utilize a local current model to illustrate the enhancement mechanism. Our analysis shows that the terahertz amplitude is determined by the superposition of contributions from individual ionization events, and for the long wavelength laser excitation, the electron production concentrates in a few ionization events and acquires the larger drift velocities, which results in the stronger terahertz radiation generation. These results will be very helpful for understanding the terahertz generation process and optimizing the terahertz output.