Polarization control of above-threshold ionization spectrum in elliptically polarized two-color laser fields

We study the above-threshold ionization(ATI)process of atoms exposed to fundamental and high-frequency lasers with arbitrary ellipticity by applying the frequency-domain theory.It is found that the angular-resolved ATI spectrum is sensitive to ellipticities of two lasers and emitted angles of the photoelectron.Particularly for the photon energy of the highfrequency laser more than atomic ionization potential,the width of plateau tends to a constant with increasing ellipticity of fundamental field,the dip structure disappears with increasing ellipticity of the high-frequency field.With the help of the quantum channel analysis,it is shown that the angular distribution depends mainly on the ellipticity of high-frequency field in the case that its frequency is high.Moreover,one can see that the maximal and minimal energies in quantum numerical results are in good agreement with the classical prediction.Our investigation may provide theoretical support for experimental research on polarization control of ionization in elliptically polarized two-color laser fields.

Turbulence-induced changes in degree of polarization,degree of coherence and spectrum of partially coherent electromagnetic beams

Based on a recently formulated unified theory of coherence and polarization, a method is described to study turbulence-induced changes in the polarization, the coherence and the spectrum of partially coherent electromagnetic beams on propagation. The electromagnetic Gaussian Schell-model beam is taken as a typical example of partially coherent electromagnetic beams, and the closed-form expressions for the degree of polarization, the degree of coherence and the spectrum of electromagnetic Gaussian Schell-model beams propagating through atmospheric turbulence are derived in the quadratic approximation of Rytov＇s phase structure function. Some interesting results are obtained, which are illustrated by numerical examples and are explained in physics.

Steering the energy sharing of electrons in nonsequential double ionization with orthogonally polarized two-color field

Using the semiclassical ensemble model,the dependence of relative amplitude for the recollision dynamics in nonsequential double ionization(NSDI)of neon atom driven by the orthogonally polarized two-color field(OTC)laser field is theoretically studied.And the dynamics in two typical collision pathways,recollision-impact-ionization(RII)and recollisionexcitation with subsequent ionization(RESI),is systematically explored.Our results reveal that the V-shaped structure in the correlated momentum distribution is mainly caused by the RII mechanism when the relative amplitude of the OTC laser field is zero,and the first ionized electrons will quickly skim through the nucleus and share few energy with the second electron.As the relative amplitude increases,the V-shaped structure gradually disappears and electrons are concentrated on the diagonal in the electron correlation spectrum,indicating that the energy sharing after electrons collision is symmetric for OTC laser fields with large relative amplitudes.Our studies show that changing the relative amplitude of the OTC laser field can efficiently control the electron–electron collisions and energy exchange efficiency in the NSDI process.

Generation of two-color polarization-adjustable radiation pulses for storage ring light source

To date, two-color pulses are widely used in pump–probe experiments. For a ring-based light source, the power of the spontaneous radiation fluctuates randomly in the longitudinal direction. It is difficult to produce twocolor double pulses by optical methods. In this paper, we introduce a method based on the echo-enabled harmonic generation scheme that generates two-color pulses in a storage ring light source. By adopting crossed undulators and a phase shifter, the polarization of the two-color pulses can be easily switched. A numerical simulation based on a diffraction-limited storage ring, the Hefei Advanced Light Source, suggests that the time delay and spectral separation of the two pulses can be adjusted linearly by changing the pulse duration and chirp parameters of the seed laser. A circular polarization degree above 80% could be achieved.

Effect of elliptical polarizations on nonsequential double ionization in two-color elliptically polarized laser fields

Using the classical ensemble model, we investigate the nonsequential double ionization（NSDI） of Ar and Mg in the two-color elliptically polarized laser pulse for different elliptical polarizations. Numerical results show that for Ar atoms the NSDI yield increases as the ellipticity increases, which is different from the case of Mg atoms. Moreover, the correlated behavior in the correlated electron momentum along the x direction and ion momentum distributions of Ar atoms are influenced by the ellipticity. By statistical analysis of different times, we can conclude that the ellipticity may be responsible for the NSDI processes. The correlated momenta distributions along the x direction at the recollision time are demonstrated and the results show that the travelling time and ellipticity can affect the emitted directions of both electrons.

Oil spill detection by a support vector machine based on polarization decomposition characteristics

Marine oil spills have caused major threats to marine environment over the past few years.The early detection of the oil spill is of great significance for the prevention and control of marine disasters.At present,remote sensing is one of the major approaches for monitoring the oil spill.Full polarization synthetic aperture radarc SAR data are employed to extract polarization decomposition parameters including entropy（H） and reflection entropy（A）.The characteristic spectrum of the entropy and reflection entropy combination has analyzed and the polarization characteristic spectrum of the oil spill has developed to support remote sensing of the oil spill.The findings show that the information extracted from（1-A）×（1-H） and（1-H）×A parameters is relatively evident effects.The results of extraction of the oil spill information based on H×A parameter are relatively not good.The combination of the two has something to do with H and A values.In general,when H〉0.7,A value is relatively small.Here,the extraction of the oil spill information using（1-A）×（1-H） and（1-H）×A parameters obtains evident effects.Whichever combined parameter is adopted,oil well data would cause certain false alarm to the extraction of the oil spill information.In particular the false alarm of the extracted oil spill information based on（1-A）×（1-H） is relatively high,while the false alarm based on（1-A）×H and（1-H）×A parameters is relatively small,but an image noise is relatively big.The oil spill detection employing polarization characteristic spectrum support vector machine can effectively identify the oil spill information with more accuracy than that of the detection method based on single polarization feature.

Near-field characteristics of highly non-paraxial subwavelength optical fields with hybrid states of polarization

The vectorial structure of an optical field with hybrid states of polarization （SOP） in the near-field is studied by using the angular spectrum method of an electromagnetic beam. Physical images of the longitudinal components of evanescent waves are illustrated and compared with those of the transverse components from the vectorial structure. Our results indicate that the relative weight integrated over the transverse plane of the evanescent wave depends strongly on the number of the polarization topological charges. The shapes of the intensity profiles of the longitudinal components are different from those of the transverse components, and it can be manipulated by changing the initial SoP of the field cross-section. The longitudinal component of evanescent wave dominates the near-field region. In addition, it also leads to three-dimensional shape variations of the optical field and the optical spin angular momentum flux density distributions.

Controlling the contributions to high-order harmonic generation from different nuclei of N_2 with an orthogonally polarized two-color laser field

The generation of high-order harmonic and the attosecond pulse of the N2 molecule with an orthogonally polarized two-color laser field are investigated by the strong-field Lewenstein model.We show that the control of contributions to high-order harmonic generation（HHG） from different nuclei is realized by properly selecting the relative phase.When the relative phase is chosen to be φ= 0.4π,the contribution to HHG from one nucleus is much more than that from another.Interference between two nuclei can be suppressed greatly; a supercontinuum spectrum of HHG appears from 40 e V to125 e V.The underlying physical mechanism is well explained by the time–frequency analysis and the semi-classical threestep model with a finite initial transverse velocity.By superposing several orders of harmonics,an isolated attosecond pulse with a duration of 80 as can be generated.

High-order harmonic generation of N2molecule in two-color circularly polarized laser fields

The generation of high-order harmonics and the attosecond pulse of the N2 molecule in two-color circularly polarized laser fields are investigated by the strong-field Lewenstein model. We show that the plateau of spectra is dramatically extended and a continuous harmonic spectrum with the bandwidth of 113 eV is obtained. When a static field is added to the x direction, the quantum path control is realized and a supercontinuum spectrum can be obtained, which is beneficial to obtain a shorter attosecond pulse. The underlying physical mechanism is well explained by the time-frequency analysis and the semi-classical three-step model with a finite initial transverse velocity. By superposing several orders of harmonics in the combination of two-color circularly polarized laser fields and a static field, an isolated attosecond pulse with a duration of 30 as can be generated.

Isolated attosecond pulse generation with few-cycle two-color counter-rotating circularly polarized laser pulses

Most of the schemes for generating isolated attosecond pulses（IAP） are sensitive to the carrier-envelope phase（CEP）of the driving lasers. We propose a scheme for generating IAP using two-color counter-rotating circularly polarized（TCCRCP） laser pulses. The results demonstrate that the dependence of the IAP generation on CEP stability is largely reduced in this scheme. IAP can be generated at most of CEPs. Therefore, the experiment requirements become lower.

Effects of Hydrogen-bonding Interaction and Polarity on Emission Spectrum of Naphthalene-Triethylamine in Mixed Solvent

The effects of the protic and aprotic polar solvents on the emission spectrum of the naphthalene-triethyl-amine system in THF were studied under conditions of steady-state illumination. The fluorescence spectrum of the naphthalene-triethylamine system consists of two emission bands, the fluorescence band of naphthalene(band A, 329 nm) and the emission band of the exciplex(band B, 468 nm). The intensities of both the emission bands decrease with increasing the solvent polarity. The intensity of band B also decreases due to the hydrogen-bonding interaction between triethylamine and protic solvent, while that of band A increases. It is thus suggested that the quenching of naphthalene fluorescence by triethylamine in THF occurs through the charge transfer and electron transfer reactions. The spectral changes upon the increase of solvent polarity can be explained by the dependences of the equilibrium constant between exciplex and ion-pair and the rate constant for the electron transfer reaction from triethylamine to the excited naphthalene on the relative permittivity of solvent. It is shown that the formation of intermolecular hydrogen-bonding between triethylamine and protic solvent suppresses the quenching reaction by the decrease in free amine. Acetonitrile has only a polar effect and trichloroacetic acid only a hydrogen-bonding(or protonation) effect, while alcohols have both the effects. The effects of alcohols could be separated into the effects of solvent polarity and intermolecular hydrogen-bonding interaction quantitatively.

Spectral decomposition at a complex laser polarization configuration

We study the role of laser polarization in the diamagnetic spectrum for the transition from the ground state to the highly excited Rydberg states through a single photon absorption. For simplicity, one usually polarizes the irradiation laser to the selected main quantum axis, which is along the applied external electric or magnetic field. The transition selection rule is simply expressed as Am = O, which corresponds to the π transition. When the polarization is circularly polarized around the main axis, the σ＋ or σ- transition occurs, corresponding to the selection rule of △m = 1 or △m = - 1, respectively. A slightly more complex case is that the laser is linearly polarized perpendicular to the main axis. The numerical calculation shows that we can decompose the transition into the sum of σ＋ and σ- transitions, it is noted as the σ transition. For the more complex case in which the laser is linearly polarized with an arbitrary angle with respect to the main axis, we have to decompose the polarization into one along the main axis and the other one perpendicular to the main axis. They correspond to π and σ transitions, respectively. We demonstrate that these transitions in the diamagnetic spectrum and the above spectral decomposition well explain the experimentally observed spectra.

Relative phase effect of nonsequential double ionization in Ar by two-color elliptically polarized laser field

We investigated the nonsequential double ionization(NSDI)in Ar by two-color elliptically polarized laser field with a three-dimensional(3D)classical ensemble method.We study the relative phase effect of NSDI and distinguish two particular recollision channels in NSDI,which are recollision–impact ionization(RII)and recollision-induced excitation with subsequent ionization(RESI),according to the delay-time between the recollision and the final double ionization.The numerical results indicate that the ion momentum distribution is changed and the triangle structure is more obvious with the decrease of the relative phase.We also demonstrate that the RESI process always dominates in the whole double ionization process and the ratio of RESI and RII channels can be influenced by the relative phase.

Exploration of High-Harmonic Generation from the CS2 Molecule by the Lewenstein Method in Two-Color Circularly Polarized Laser Field

The high harmonic generation (HHG) from the CS2 molecule in intense laser fields is investigated using the extended Lewenstein method. The initial state is the highest-occupied molecular orbital of the CS2 molecule, which can be well described by Gaussian wave packet using GAMESS-UK package. Compared with the case of the elliptical laser, the HHG can be extended in two-color circularly polarized laser field. The time-frequency analysis and classical electron trajectory as well as the ionization yield curve are also presented to further explain the underlying mechanism. After adding a static electric field on the z-direction, the single quantum path control is realized and the supercontinuum spectra are obtained. Moreover, an isolated 110 as pulse can be obtained by superposing the harmonics from 130th to 180th order.

Analytical Dielectric Spectrum Formula Based on Representative Frequencies

According to experimental data available for the complex refractive index of particular dielectrics, a dielectric spectrum formula is proposed by the least square fitting technique combined with selected natural frequencies. From the dielectric spectrum formula, the spectra of optical and dielectric constants can be obtained in the whole frequency region. Three dielectrics, water, ethanol, and toluene, are taken as examples. In the region where the ex- perimental data are available, the spectra of the optical constants calculated by the formula are in good agreement with the real refractive spectrum obtained by Kramers-Kronig （K-K） transform and the experimental imaginary refractive spectrum. In the region where no ex- perimental data are available, the extrapolation of our formula can make predictions. The merits of the present treatment are that we are able to get the uniform spectrum formula, without splitting into different frequency sections, and the analytical form of the dielectric spectra will be useful in the theoretical description of solvation dynamics.

Signal processing method of a novel polarized array radar seeker

This paper proposes a novel polarized radar seeker based on the polarized antenna array. A fully polarized signal processing method for the proposed radar seeker is studied under the environments with electromagnetic interferences. A dual polarized antenna array is employed to transmit and receive the radar signals. The instantaneous polarization signal processing technique is used to detect and recognize the targets. The direction of arrival （DOA） of the target is measured through the spatial spectrum with high resolution for the polarized array radar seeker system. The fully polarized signal model of the polarized array radar seeker is formulated and a specific signal processing algorithm is expounded. The theoretical research and numerical simulation results demonstrate that the proposed radar seeker has good performances in target detection and electronic warfare. The research results can provide an effective technical approach to develop and research the new generation radar seeker.

Electron acceleration by tightly focused radially polarized few-cycle laser pulses

Within the framework of plane-wave angular spectrum analysis of the electromagnetic field structure, a solution valid for tightly focused radially polarized few-cycle laser pulses propagating in vacuum is presented. The resulting field distribution is significantly different from that based on the paraxial approximation for pulses with either small or large beam diameters. We compare the electron accelerations obtained with the two solutions and find that the energy gain obtained with our new solution is usually much larger than that with the paraxial approximation solution.

Asymmetrical spiral spectra and orbital angular momentum density of non-uniformly polarized vortex beams in uniaxial crystals

To explore the effect of non-uniform polarization on orbital angular momentum(OAM) in anisotropic medium, in this work investigated are the evolution of the spiral spectra and OAM densities of non-uniformly polarized vortex(NUPV)beams in uniaxial crystals propagating orthogonal to the optical axis, and also the case of uniformly polarized vortex(UPV)beams with left-handed elliptical polarization. In the input plane, the NUPV beams present their spiral spectra of m-mode concentrated at m = l ± 1 modes rather than m = l mode, and reveal the relation among topological charge l, mode of spiral spectra m and the power weight value Rmexpressed by l=∑^(∞)_(m)=-∞Rm. is still satisfied for UPV beams in uniaxially anisotropic crystals, whereas for NUPV beams their relations are no longer valid owing to non-uniform polarization. Furthermore, the analysis indicates that the asymmetrical distribution of power weight of spiral spectra and the non-zero value in the sum of longitudinal OAM densities originate from the initial non-uniform polarization and anisotropy in uniaxial crystals rather than topological charges. In addition, the relation between spiral spectrum and longitudinal OAM density is numerically discussed. This work may provide an avenue for OAM-based communications,optical metrology, and imaging by varying the initial non-uniform polarization.

Effect of PMD-induced Pulse Broadening on Sensitivity and Frequency Spectrum

The PMD-induced pulse broadening may cause the degradation ofreceiver sensitivity and has negative effects on the power spectrumof received signals. The expression s of PMO-induced pulse broadeningeffects on receiver sensitivity are derived based on the concept ofman square pulse width. The effects of PMD on the spectrum ofreceived power are analyzed in detail. Finally, the scheme isdiscussed with which the poser of a certain frequency component isextracted as a feedback control signal in a PMD compensation system.

Effect of Solvent Polarity on Excited-State Double Proton Transfer Process of 1,5-Dihydroxyanthraquinone

The excited-state double proton transfer(ESDPT)properties of 1,5-dihydroxyanthraquinone(1,5-DHAQ)in various solvents were investigated using femtosecond transient absorption spectroscopy and the DFT/TDDFT method.The steady-state fluorescence spectra in toluene,tetrahydrofuran(THF)and acetonitrile(ACN)solvents presented that the solvent polarity has an effect on the position of the ESDPT fluorescence emission peak for the 1,5-DHAQ system.Transient absorption spectra show that the increasing polarity of the solvent accelerates the rate of excited state dynamics.Calculated potential energy curves analysis further verified the experimental results.The ESDPT barrier decreases gradually with the increase of solvent polarity from toluene,THF to ACN solvent.It is convinced that the increase of solvent polarity can promote the occurrence of the ESDPT dynamic processes for the 1,5-DHAQ system.This work clarifies the mechanism of the influence of solvent polarity on the ESDPT process of 1,5-DHAQ,which provides novel ideas for design and synthesis of new hydroxyanthraquinone derivatives.