The vertical two-dimensional non-hydrostatic pressure models with multiple layers can make prediction more accurate than those obtained by the hydrostatic pres- sure assumption. However, they are time-consuming and un...The vertical two-dimensional non-hydrostatic pressure models with multiple layers can make prediction more accurate than those obtained by the hydrostatic pres- sure assumption. However, they are time-consuming and unstable, which makes them unsuitable for wider application. In this study, an efficient model with a single layer is developed. Decomposing the pressure into the hydrostatic and dynamic components and integrating the x-momentum equation from the bottom to the free surface can yield a horizontal momentum equation, in which the terms relevant to the dynamic pressure are discretized semi-implicitly. The convective terms in the vertical momentum equation are ignored, and the rest of the equation is approximated with the Keller-box scheme. The velocities expressed as the unknown dynamic pressure are substituted into the continuity equation, resulting in a tri-diagonal linear system solved by the Thomas algorithm. The validation of solitary and sinusoidal waves indicates that the present model can provide comparable results to the models with multiple layers but at much lower computation cost.展开更多
Two-dimensional transition metal dichalcogenides(TMDs)have intriguing physic properties and offer an exciting platform to explore many features that are important for future devices.In this work,we synthesized monolay...Two-dimensional transition metal dichalcogenides(TMDs)have intriguing physic properties and offer an exciting platform to explore many features that are important for future devices.In this work,we synthesized monolayer WS_(2)as an example to study the optical response with hydrostatic pressure.The Raman results show a continuous tuning of the lattice vibrations that is induced by hydrostatic pressure.We further demonstrate an efficient pressure-induced change of the band structure and carrier dynamics via transient absorption measurements.We found that two time constants can be attributed to the capture process of two kinds of defect states,with the pressure increasing from 0.55 GPa to 2.91 GPa,both of capture processes were accelerated,and there is an inflection point within the pressure range of 1.56 GPa to 1.89 GPa.Our findings provide valuable information for the design of future optoelectronic devices.展开更多
This paper presents the analytical solutions in Laplace domain for two-dimensional nonsteady flow of slightly compressible liquid in porous media with double porosity by using the methods of integral transforms and va...This paper presents the analytical solutions in Laplace domain for two-dimensional nonsteady flow of slightly compressible liquid in porous media with double porosity by using the methods of integral transforms and variables separation. The effects of the ratio of storativities to , interporosity flow parameter on the pressure behaviors for a vertically fractured well with infinite conductivity are investigated by using the method of numerical inversion. The new log-log diagnosis graph of the pressures is given and analysed.展开更多
Two-dimensional(2D)Ruddlesden-Popper(RP)halide perovskites with diverse structures and properties have drawn increasing attention due to their promising optoelectronic applications.Recently,a new all-inorganic Cs_(2)P...Two-dimensional(2D)Ruddlesden-Popper(RP)halide perovskites with diverse structures and properties have drawn increasing attention due to their promising optoelectronic applications.Recently,a new all-inorganic Cs_(2)Pb(SCN)_(2)Br_(2) has been reported that opens up new potential for the development of 2D RP perovskites.However,recent reports of unusual dual emissions and two-edge absorption in Cs_(2)Pb(SCN)_(2)Br_(2) have generated intense debate about its origin and remains controversial.Here,by combining continuous pressure tuning with in situ diagnostics,we have unambiguously revealed the underlying mechanisms that the 2D Cs_(2)Pb(SCN)_(2)Br_(2) exhibits an intrinsic blue emission at 2.66 eV and an absorption edge close to the emission peak.While the gradually formed CsPbBr_(3) is responsible for the green emission at 2.33 eV with the absorption shoulder at 2.41 eV.Furthermore,by fitting the temperature-dependent intensity of the intrinsic blue emission,we have determined the corrected value of exciton binding energy for 2D Cs_(2)Pb(SCN)_(2)Br_(2) to be 90 meV.Intriguingly,an emission enhancement of 2.5 times is achieved in Cs_(2)Pb(SCN)_(2)Br_(2) under a mild pressure within 0.8 GPa,caused by the pressuresuppressed exciton-phonon interaction.This work not only elucidates the origin of the dual emissions and two-edge absorption in Cs_(2)Pb(SCN)_(2)Br_(2),but it also provides a potential means to regulate and optimize the optoelectronic properties of 2D perovskites.展开更多
为解决传统渐开线蜗杆斜齿轮副在开式传动或传动比过大时斜齿轮容易发生齿根断裂的情况,提出一种新型的基于不等模数不等压力角设计的渐开线蜗杆副,使斜齿轮的模数与压力角同时提高,大幅提高斜齿轮的齿根强度。通过对此种蜗杆副的传动...为解决传统渐开线蜗杆斜齿轮副在开式传动或传动比过大时斜齿轮容易发生齿根断裂的情况,提出一种新型的基于不等模数不等压力角设计的渐开线蜗杆副,使斜齿轮的模数与压力角同时提高,大幅提高斜齿轮的齿根强度。通过对此种蜗杆副的传动特性的分析,得到特殊的啮合角与中心距计算方式。另外,通过对同传动比、同蜗杆情况下基于不等模数设计的ZI蜗杆斜齿轮副和传统ZI蜗杆斜齿轮副的建模与有限元分析,得出在较大模数比情况下的斜齿轮齿根强度约为传统斜齿轮齿根强度的2.956倍,增大了渐开线蜗杆的应用范围。后续使用灰色预测,对比出误差平方和(Sum of Squared Errors,SSE)最小模型,予以验证预测的准确性,另外进行蜗杆施加不同转矩下的斜齿轮啮合齿受拉力处最大应力σ_(1max)的数据预测,为相应的工程分析与必要的校核设计给出了依据。展开更多
The development of pressure sensor arrays capable of distinguishing the shape and texture details of objects is of considerable interest in the emerging fields of smart robots,prostheses,human-machine interfaces,and a...The development of pressure sensor arrays capable of distinguishing the shape and texture details of objects is of considerable interest in the emerging fields of smart robots,prostheses,human-machine interfaces,and artificial intelligence(AI).Here we report an integrated pressure sensor array,by combining solution-processed two-dimensional(2D)MoS2 van der Waals(vdW)thin film transistor(TFT)active matrix and conductive micropyramidal pressure-sensitive rubber(PSR)electrodes made of polydimethylsiloxane/carbon nanotube composites,to achieve spatially revolved pressure mapping with excellent contrast and low power consumption.We demonstrate a 10×10 active matrix by using the 2D MoS2 vdW-TFTs with high on-off ratio>10^(6),minimal hysteresis,and excellent device-to-device uniformity.The combination of the vdW-TFT active matrix with the highly uniform micropyramidal PSR electrodes creates an integrated pressure sensing array for spatially resolved pressure mapping.This study demonstrates that the solution-processed 2D vdW-TFTs offer a solution for active-matrix control of pressure sensor arrays,and could be extended for other active-matrix arrays of electronic or optoelectronic devices.展开更多
Two-dimensional(2D)organic–inorganic halide perovskites present remarkable stability and diversity and are promising alternatives to their three-dimensional(3D)counterparts.The 2D halide perovskite[(HO)(CH_(2))_(2)NH...Two-dimensional(2D)organic–inorganic halide perovskites present remarkable stability and diversity and are promising alternatives to their three-dimensional(3D)counterparts.The 2D halide perovskite[(HO)(CH_(2))_(2)NH_(3)]_(2)PbI_(4)is regarded as a superior moisture-stabile“smooth”perovskite because of distinct hydrogen-bond networks that connect adjacent organic–inorganic layers.展开更多
Two-dimensional(2D)materials have attracted considerable research interest,leading to significant advances in energy applications in recent years,such as lithium batteries,catalysis,electronics,and thermoelectrics,owi...Two-dimensional(2D)materials have attracted considerable research interest,leading to significant advances in energy applications in recent years,such as lithium batteries,catalysis,electronics,and thermoelectrics,owing to their rich controllable properties and excellent performances.Recently,pressure has been successfully employed as an effective method for property modulation of 2D materials,through tuning electronic orbitals and bonding patterns.In this review,we summarize recent progresses in the pressure-driven property modulations and elucidate the underlying mechanism of the pressure modulation of 2D materials.Further,we identify the remaining challenges and opportunities in this new,vibrant area of research for energy conversion and utilization.Among the different property modulation strategies,the in situ application of high pressure is systematically identified as a promising knob for 2D materials.This review is expected to inspire further research on the fundamental understanding and practical applications of high-pressure modulation in 2D materials.展开更多
基金Project supported by the Specialized Research Fund for the Doctoral Program of Higher Education(No. 20110142110064)the Ministry of Water Resources’ Science and Technology Promotion Plan Program (No. TG1316)
文摘The vertical two-dimensional non-hydrostatic pressure models with multiple layers can make prediction more accurate than those obtained by the hydrostatic pres- sure assumption. However, they are time-consuming and unstable, which makes them unsuitable for wider application. In this study, an efficient model with a single layer is developed. Decomposing the pressure into the hydrostatic and dynamic components and integrating the x-momentum equation from the bottom to the free surface can yield a horizontal momentum equation, in which the terms relevant to the dynamic pressure are discretized semi-implicitly. The convective terms in the vertical momentum equation are ignored, and the rest of the equation is approximated with the Keller-box scheme. The velocities expressed as the unknown dynamic pressure are substituted into the continuity equation, resulting in a tri-diagonal linear system solved by the Thomas algorithm. The validation of solitary and sinusoidal waves indicates that the present model can provide comparable results to the models with multiple layers but at much lower computation cost.
基金This work was supported by Shenzhen Science and Technology Innovation Commission(JCYJ20220530153004010).
文摘Two-dimensional transition metal dichalcogenides(TMDs)have intriguing physic properties and offer an exciting platform to explore many features that are important for future devices.In this work,we synthesized monolayer WS_(2)as an example to study the optical response with hydrostatic pressure.The Raman results show a continuous tuning of the lattice vibrations that is induced by hydrostatic pressure.We further demonstrate an efficient pressure-induced change of the band structure and carrier dynamics via transient absorption measurements.We found that two time constants can be attributed to the capture process of two kinds of defect states,with the pressure increasing from 0.55 GPa to 2.91 GPa,both of capture processes were accelerated,and there is an inflection point within the pressure range of 1.56 GPa to 1.89 GPa.Our findings provide valuable information for the design of future optoelectronic devices.
文摘This paper presents the analytical solutions in Laplace domain for two-dimensional nonsteady flow of slightly compressible liquid in porous media with double porosity by using the methods of integral transforms and variables separation. The effects of the ratio of storativities to , interporosity flow parameter on the pressure behaviors for a vertically fractured well with infinite conductivity are investigated by using the method of numerical inversion. The new log-log diagnosis graph of the pressures is given and analysed.
基金supported by the National Natural Science Foundation of China(NSFC)(grant nos.22275004,U1930401,and 52325309)the Shanghai Science and Technology Committee(grant no.22JC1410300)+2 种基金the Shanghai Key Laboratory of Novel Extreme Condition Materials(grant no.22dz2260800)supported by the NSFC(grant no.22275077).Q.H.is supported by the CAEP Research(grant no.CX20210048)the Tencent Xplorer Prize(grant no.XPLORER-2020-1013).
文摘Two-dimensional(2D)Ruddlesden-Popper(RP)halide perovskites with diverse structures and properties have drawn increasing attention due to their promising optoelectronic applications.Recently,a new all-inorganic Cs_(2)Pb(SCN)_(2)Br_(2) has been reported that opens up new potential for the development of 2D RP perovskites.However,recent reports of unusual dual emissions and two-edge absorption in Cs_(2)Pb(SCN)_(2)Br_(2) have generated intense debate about its origin and remains controversial.Here,by combining continuous pressure tuning with in situ diagnostics,we have unambiguously revealed the underlying mechanisms that the 2D Cs_(2)Pb(SCN)_(2)Br_(2) exhibits an intrinsic blue emission at 2.66 eV and an absorption edge close to the emission peak.While the gradually formed CsPbBr_(3) is responsible for the green emission at 2.33 eV with the absorption shoulder at 2.41 eV.Furthermore,by fitting the temperature-dependent intensity of the intrinsic blue emission,we have determined the corrected value of exciton binding energy for 2D Cs_(2)Pb(SCN)_(2)Br_(2) to be 90 meV.Intriguingly,an emission enhancement of 2.5 times is achieved in Cs_(2)Pb(SCN)_(2)Br_(2) under a mild pressure within 0.8 GPa,caused by the pressuresuppressed exciton-phonon interaction.This work not only elucidates the origin of the dual emissions and two-edge absorption in Cs_(2)Pb(SCN)_(2)Br_(2),but it also provides a potential means to regulate and optimize the optoelectronic properties of 2D perovskites.
文摘为解决传统渐开线蜗杆斜齿轮副在开式传动或传动比过大时斜齿轮容易发生齿根断裂的情况,提出一种新型的基于不等模数不等压力角设计的渐开线蜗杆副,使斜齿轮的模数与压力角同时提高,大幅提高斜齿轮的齿根强度。通过对此种蜗杆副的传动特性的分析,得到特殊的啮合角与中心距计算方式。另外,通过对同传动比、同蜗杆情况下基于不等模数设计的ZI蜗杆斜齿轮副和传统ZI蜗杆斜齿轮副的建模与有限元分析,得出在较大模数比情况下的斜齿轮齿根强度约为传统斜齿轮齿根强度的2.956倍,增大了渐开线蜗杆的应用范围。后续使用灰色预测,对比出误差平方和(Sum of Squared Errors,SSE)最小模型,予以验证预测的准确性,另外进行蜗杆施加不同转矩下的斜齿轮啮合齿受拉力处最大应力σ_(1max)的数据预测,为相应的工程分析与必要的校核设计给出了依据。
基金Y.H.acknowledges the financial support from the Office of Naval Research through award N00014-18-1-2491.X.F.D.acknowledged the support from the US Department of Energy,Office of Basic Energy Sciences,Division of Materials Science and Engineering through award DE-SC0018828(material preparation).
文摘The development of pressure sensor arrays capable of distinguishing the shape and texture details of objects is of considerable interest in the emerging fields of smart robots,prostheses,human-machine interfaces,and artificial intelligence(AI).Here we report an integrated pressure sensor array,by combining solution-processed two-dimensional(2D)MoS2 van der Waals(vdW)thin film transistor(TFT)active matrix and conductive micropyramidal pressure-sensitive rubber(PSR)electrodes made of polydimethylsiloxane/carbon nanotube composites,to achieve spatially revolved pressure mapping with excellent contrast and low power consumption.We demonstrate a 10×10 active matrix by using the 2D MoS2 vdW-TFTs with high on-off ratio>10^(6),minimal hysteresis,and excellent device-to-device uniformity.The combination of the vdW-TFT active matrix with the highly uniform micropyramidal PSR electrodes creates an integrated pressure sensing array for spatially resolved pressure mapping.This study demonstrates that the solution-processed 2D vdW-TFTs offer a solution for active-matrix control of pressure sensor arrays,and could be extended for other active-matrix arrays of electronic or optoelectronic devices.
基金supported by the National Science Foundation of China(NSFC)(nos.21725304 and 11774120)the Chang Jiang Scholars Program of China(no.T2016051).Angle-dispersive XRD measurement was performed on the BL15U1 at the Shanghai Synchrotron Radiation Facility(SSRF).
文摘Two-dimensional(2D)organic–inorganic halide perovskites present remarkable stability and diversity and are promising alternatives to their three-dimensional(3D)counterparts.The 2D halide perovskite[(HO)(CH_(2))_(2)NH_(3)]_(2)PbI_(4)is regarded as a superior moisture-stabile“smooth”perovskite because of distinct hydrogen-bond networks that connect adjacent organic–inorganic layers.
基金The authors acknowledge the micro-fabrication center of National Laboratory of Solid State Microstructures(NLSSM)for technique supportProf.Jia Zhu acknowledges the support from the XPLORER PRIZE+3 种基金This work is jointly supported by the National Key Research and Development Program of China(No.2021YFA140070)the National Natural Science Foundation of China(Nos.61735008,51925204,12022403)Excellent Research Program of Nanjing University(ZYJH005)Carbon Peaking and Carbon Neutrality Science and Technology Innovation Fund of Jiangsu Province(BK20220035).
文摘Two-dimensional(2D)materials have attracted considerable research interest,leading to significant advances in energy applications in recent years,such as lithium batteries,catalysis,electronics,and thermoelectrics,owing to their rich controllable properties and excellent performances.Recently,pressure has been successfully employed as an effective method for property modulation of 2D materials,through tuning electronic orbitals and bonding patterns.In this review,we summarize recent progresses in the pressure-driven property modulations and elucidate the underlying mechanism of the pressure modulation of 2D materials.Further,we identify the remaining challenges and opportunities in this new,vibrant area of research for energy conversion and utilization.Among the different property modulation strategies,the in situ application of high pressure is systematically identified as a promising knob for 2D materials.This review is expected to inspire further research on the fundamental understanding and practical applications of high-pressure modulation in 2D materials.