Turbulence in the nocturnal boundary layer(NBL)is still not well characterized,especially over complex underlying surfaces.Herein,gradient tower data and eddy covariance data collected by the Beijing 325-m tower were ...Turbulence in the nocturnal boundary layer(NBL)is still not well characterized,especially over complex underlying surfaces.Herein,gradient tower data and eddy covariance data collected by the Beijing 325-m tower were used to better understand the differentiating characteristics of turbulence regimes and vertical turbulence structure of urban the NBL.As for heights above the urban canopy layer(UCL),the relationship between turbulence velocity scale(VTKE)and wind speed(V)was consistent with the“HOckey-Stick”(HOST)theory proposed for a relatively flat area.Four regimes have been identified according to urban nocturnal stable boundary layer.Regime 1 occurs where local shear plays a leading role for weak turbulence under the constraint that the wind speed V<VT(threshold wind speed).Regime 2 is determined by the existence of strong turbulence that occurs when V>VT and is mainly driven by bulk shear.Regime 3 is identified by the existence of moderate turbulence when upside-down turbulence sporadic bursts occur in the presence of otherwise weak turbulence.Regime 4 is identified as buoyancy turbulence,when V>VT,and the turbulence regime is affected by a combination of local wind shear,bulk shear and buoyancy turbulence.The turbulence activities demonstrated a weak thermal stratification dependency in regime 1,for which within the UCL,the turbulence intensity was strongly affected by local wind shear when V<VT.This study further showed typical examples of different stable boundary layers and the variations between turbulence regimes by analyzing the evolution of wind vectors.Partly because of the influence of large-scale motions,the power spectral density of vertical velocity for upsidedown structure showed an increase at low frequencies.The upside-down structures were also characterized by the highest frequency of the stable stratifications in the higher layer.展开更多
In June 2013,a field experiment was conducted in Southeast Tibet in which the air temperature,moisture,and wind were measured by using a GPS sounding system.In the present study,based on these observations and ERA-Int...In June 2013,a field experiment was conducted in Southeast Tibet in which the air temperature,moisture,and wind were measured by using a GPS sounding system.In the present study,based on these observations and ERA-Interim reanalysis data,the vertical structures of these atmospheric properties and the possible influence of the South Asian summer monsoon(SASM) were investigated.On average,the temperature had a lapse rate of 6.8℃ km^(-1) below the tropopause of 18.0 km.A strong moisture inversion occurred at the near-surface,with a strength of 1.7 g kg^(-1)(100 m)^(-1) for specific humidity.During the observation period,the SASM experienced a south phase and a north phase in the middle and by the end of June,respectively.The monsoon's evolution led to large changes in convection and circulation over Southeast Tibet,which further affected the local thermal,moisture,and circulation conditions.The strong convection resulted in an elevated tropopause height over Southeast Tibet during the north phase of the SASM,and the large-scale warm and wet air masses delivered by the monsoon caused high local temperature and moisture conditions.展开更多
Vertical forest structure is closely linked to multiple ecosystem characteristics,such as biodiversity,habitat,and productivity.Mixing tree species in planted forests has the potential to create diverse vertical fores...Vertical forest structure is closely linked to multiple ecosystem characteristics,such as biodiversity,habitat,and productivity.Mixing tree species in planted forests has the potential to create diverse vertical forest structures due to the different physiological and morphological traits of the composing tree species.However,the relative importance of species richness,species identity and species interactions for the variation in vertical forest structure remains unclear,mainly because traditional forest inventories do not observe vertical stand structure in detail.Terrestrial laser scanning(TLS),however,allows to study vertical forest structure in an unprecedented way.Therefore,we used TLS single scan data from 126 plots across three experimental planted forests of a largescale tree diversity experiment in Belgium to study the drivers of vertical forest structure.These plots were 9–11years old young pure and mixed forests,characterized by four levels of tree species richness ranging from monocultures to four-species mixtures,across twenty composition levels.We generated vertical plant profiles from the TLS data and derived six stand structural variables.Linear mixed models were used to test the effect of species richness on structural variables.Employing a hierarchical diversity interaction modelling framework,we further assessed species identity effect and various species interaction effects on the six stand structural variables.Our results showed that species richness did not significantly influence most of the stand structure variables,except for canopy height and foliage height diversity.Species identity on the other hand exhibited a significant impact on vertical forest structure across all sites.Species interaction effects were observed to be site-dependent due to varying site conditions and species pools,and rapidly growing tree species tend to dominate these interactions.Overall,our results highlighted the importance of considering both species identity and interaction effects in choosing suitable species combinations for forest management practices aimed at enhancing vertical forest structure.展开更多
Knowledge of the vertical distribution of aerosols in the free troposphere is important for estimating their impact on climate. In this study, direct observations of the vertical distribution of aerosols in the free t...Knowledge of the vertical distribution of aerosols in the free troposphere is important for estimating their impact on climate. In this study, direct observations of the vertical distribution of aerosols in the free troposphere are made using surface Micro-Pulse Lidar (MPL) measurements. The MPL measurements were made at the Loess Plateau (35.95°N, 104.1°E), which is near the major dust source regions of the Taklimakan and Gobi deserts. The vertical distribution of the MPL backscattering suggested that nondust aerosols floated from ground level to an altitude of approximately 9 km around the source regions. Early morning hours are characterized by a shallow aerosol layer of a few hundred meters thick. As the day progresses, strong convective eddies transport the aero- sols vertically to more than 1500 m.展开更多
ABSTRACT The abilities of BCC-AGCM2.1 and BCC_AGCM2.2 to simulate the annual-mean cloud vertical structure (CVS) were evaluated through comparison with GCM-Oriented CALIPSO Cloud Product (CALIPSO-GOCCP) data. BCC...ABSTRACT The abilities of BCC-AGCM2.1 and BCC_AGCM2.2 to simulate the annual-mean cloud vertical structure (CVS) were evaluated through comparison with GCM-Oriented CALIPSO Cloud Product (CALIPSO-GOCCP) data. BCC-AGCM2.2 has a dynamical core and physical processes that are consistent with BCC-AGCM2.1, but has a higher horizontal resolution. Results showed that both BCC-AGCM versions underestimated the global-mean total cloud cover (TCC), middle cloud cover (MCC) and low cloud cover (LCC), and that BCC_AGCM2.2 underestimated the global-mean high cloud cover (HCC). The global-mean cloud cover shows a systematic decrease from BCCA-GCM2.1 to BCC_AGCM2.2, especially for HCC. Geographically, HCC is significantly overestimated in the tropics, particularly by BCC_AGCM2,1, while LCC is generally overestimated over extra-tropical lands, but significantly underestimated over most of the oceans, especially for subtropical marine stratocumulus clouds. The leading EOF modes of CVS were extracted. The BCC_AGCMs perform well in reproducing EOF1, but with a larger variance explained. The two models also capture the basic features of EOF3, except an obvious deficiency in eigen- vector peaks. EOF2 has the largest simulation biases in both position and strength of eigenvector peaks. Furthermore, we investigated the effects of CVS on relative shortwave and longwave cloud radiative forcing (RSCRF and RLCRF). Both BCC_AGCM versions successfully reproduce the sign of regression coefficients, except for RLCRF in PC1. However, the RSCRF relative contributions from PC1 and PC2 are overestimated, while the relative contribution from PC3 is underes timated in both BCC_AGCM versions. The RLCRF relative contribution is underestimated for PC2 and overestimated for PC3.展开更多
Vertical differential structural deformation(VDSD),one of the most significant structural characteristics of strike-slip fault zones(SSFZs)in the Shunbei area,is crucial for understanding deformation in the SSFZ and i...Vertical differential structural deformation(VDSD),one of the most significant structural characteristics of strike-slip fault zones(SSFZs)in the Shunbei area,is crucial for understanding deformation in the SSFZ and its hydrocarbon accumulation significance.Based on drilling data and high-precision 3-D seismic data,we analyzed the geometric and kinematic characteristics of the SSFZs in the Shunbei area.Coupled with the stratification of the rock mechanism,the structural deformations of these SSFZs in different formations were differentiated and divided into four deformation layers.According to comprehensive structural interpretations and comparisons,three integrated 3-D structural models could describe the VDSD of these SSFZs.The time-space coupling of the material basis(rock mechanism stratification),changing dynamic conditions(e.g.,changing stress-strain states),and special deformation mechanism of the en echelon normal fault array uniformly controlled the formation of the VDSD in the SSFZs of the Shunbei area.The VDSD of the SSFZs in this area controlled the entire hydrocarbon accumulation process.Multi-stage structural superimposing deformation influenced the hydrocarbon migration,accumulation,distribution,preservation,and secondary adjustments.展开更多
This study investigates the vertical structure of variability in the cross-equatorial flows(CEFs)over the Maritime Continent and Indian Ocean in boreal summer,based on three reanalysis datasets:ERA-Interim,JRA-55 and ...This study investigates the vertical structure of variability in the cross-equatorial flows(CEFs)over the Maritime Continent and Indian Ocean in boreal summer,based on three reanalysis datasets:ERA-Interim,JRA-55 and NCEP-2.The results show a high consistency in the interannual variability among the reanalysis datasets,especially between ERAInterim and JRA-55,while great uncertainty exists in the decadal or long-term changes of CEFs.Further analyses on the interannual variability in CEFs indicate that there is a significant negative relationship between the upper-and lower-level CEFs over the Maritime Continent—that is,the northerlies at the upper level and southerlies at the lower level are both enhanced or weakened.This seesaw pattern is also significantly related to the CEFs over the Indian Ocean at the upper level and lower level(i.e.,the Somali jet).This close relationship between the upper-and lower-level CEFs and between the Maritime Continent and Indian Ocean is manifested as the leading mode of equatorial meridional winds in the vertical-zonal section over the Maritime Continent and Indian Ocean.Finally,it is found that ENSO is closely related to the vertical leading mode,and to all the CEFs at the upper and lower levels over the Maritime Continent and Indian Ocean.展开更多
Empirical Orthogonal Function (EOF) analysis is used in this study to generate main eigenvector fields of historical temperature for the China Seas (here referring to Chinese marine territories) and adjacent water...Empirical Orthogonal Function (EOF) analysis is used in this study to generate main eigenvector fields of historical temperature for the China Seas (here referring to Chinese marine territories) and adjacent waters from 1930 to 2002 (510 143 profiles). A good temperature profile is reconstructed based on several subsurface in situ temperature observations and the thermocline was estimated using the model. The results show that: 1) For the study area, the former four principal components can explain 95% of the overall variance, and the vertical distribution of temperature is most stable using the in situ temperature observations near the surface. 2) The model verifications based on the observed CTD data from the East China Sea (ECS), South China Sea (SCS) and the areas around Taiwan Island show that the reconstructed profiles have high correlation with the observed ones with the confidence level 〉95%, especially to describe the characteristics of the thermocline well. The average errors between the reconstructed and observed profiles in these three areas are 0.69℃, 0.52℃ and 1.18℃ respectively. It also shows the model RMS error is less than or close to the climatological error. The statistical model can be used to well estimate the temperature profile vertical structure. 3) Comparing the thermocline characteristics between the reconstructed and observed profiles, the results in the ECS show that the average absolute errors are 1.5m, 1.4 m and 0.17~C/m, and the average relative errors are 24.7%, 8.9% and 22.6% for the upper, lower thermocline boundaries and the gradient, respectively. Although the relative errors are obvious, the absolute error is small. In the SCS, the average absolute errors are 4.1 m, 27.7 m and 0.007℃/m, and the average relative errors are 16.1%, 16.8% and 9.5% for the upper, lower thermocline boundaries and the gradient, respectively. The average relative errors are all 〈20%. Although the average absolute error of the lower thermocline boundary is considerable, but contrast to the spatial scale of average depth of the lower thermocline boundary (165 m), the average relative error is small (16.8%). Therefore the model can be used to well estimate the thermocline.展开更多
The sensitive area of targeted observations for short-term(7 d)prediction of vertical thermal structure(VTS)in summer in the Yellow Sea was investigated.We applied the Conditional Nonlinear Optimal Perturbation(CNOP)m...The sensitive area of targeted observations for short-term(7 d)prediction of vertical thermal structure(VTS)in summer in the Yellow Sea was investigated.We applied the Conditional Nonlinear Optimal Perturbation(CNOP)method and an adjoint-free algorithm with the Regional Ocean Modeling System(ROMS).We used vertical integration of CNOP-type temperature errors to locate the sensitive areas,where reduction of initial errors is expected to yield the greatest improvement in VTS prediction for the selected verification area.The identified sensitive areas were northeast−southwest orientated northeast to the verification area,which were possibly related to the southwestward background currents.Then,we performed a series of sensitivity experiments to evaluate the effectiveness of the identified sensitive areas.Results show that initial errors in the identified sensitive areas had the greatest negative effect on VTS prediction in the verification area compared to errors in other areas(e.g.,the verification area and areas to its east and northeast).Moreover,removal of initial errors through deploying simulated observations in the identified sensitive areas led to more refined prediction than correction of initial conditions in the verification area itself.Our results suggest that implementation of targeted observation in the CNOP-based sensitive areas is an effective method to improve short-term prediction of VTS in summer in the Yellow Sea.展开更多
In this paper, on the basis of the heat conduction equation without consideration of the advection and turbulence effects, one-dimensional model for describing surface sea temperature ( T1), bottom sea temperature ( T...In this paper, on the basis of the heat conduction equation without consideration of the advection and turbulence effects, one-dimensional model for describing surface sea temperature ( T1), bottom sea temperature ( Tt ) and the thickness of the upper homogeneous layer ( h ) is developed in terms of the dimensionless temperature θT and depth η and self-simulation function θT - f(η) of vertical temperature profile by means of historical temperature data.The results of trial prediction with our one-dimensional model on T, Th, h , the thickness and gradient of thermocline are satisfactory to some extent.展开更多
Three long-term fixed acoustic Doppler current profilers were first used for investigating the vertical structure of tidal currents in Xuliujing Section of Changjiang River Estuary.Moreover,three different periods(spr...Three long-term fixed acoustic Doppler current profilers were first used for investigating the vertical structure of tidal currents in Xuliujing Section of Changjiang River Estuary.Moreover,three different periods(spring,summer and fall)were also considered for investigating seasonal variations.The semi-diurnal tides were the most energetic,with along-channel speed of up to 80 cm/s for M_(2)constituent,which dominates at all stations with percent energy up to 65%–75%during seasons.The shape of tidal ellipses of the most energetic semi-diurnal constituent M_(2)showed obvious polarization of the flow paralleling to the riverbank,with the minor semi-axis being generally less than 20%of the major one.The maximum velocity of mean current is appeared in top layers at all the three stations,and the velocity decreased with the depth.The seasonal variations of direction are also observed,which is probably caused by complex local topography since the erosion and deposition in riverbed.Observed vertical variation of four parameters of M_(2)ellipses,agreed well with the optimally fit frictional solutions in top and middle layers.However,there was an obvious difference between frictional model and observed data in the lower water column.Discrepancies are probably on account of stratification,which strengthens in summer and fall due to the freshening influence of the Changjiang River Estuary outflow.展开更多
The algebraic solitary wave and its associated eigenvalue problem in a deep stratified fluid with a free surface and a shallow upper layer were studied. And its vertical structure was examined. An exact solution for t...The algebraic solitary wave and its associated eigenvalue problem in a deep stratified fluid with a free surface and a shallow upper layer were studied. And its vertical structure was examined. An exact solution for the derived 2D Benjamin-Ono equation was obtained, and physical explanation was given with the corresponding dispersion relation. As a special case, the vertical structure of the weakly nonlinear internal wave for the Holmboe density distribution was numerically investigated, and the propagating mechanism of the internal wave was studied by using the ray theory.展开更多
Cloud profiling radar(CPR) onboard Cloud Sat allows for deep penetration into dense clouds/precipitation. In this study, tropical cyclones(TCs) are classified into three stages as developing, mature, and decaying. The...Cloud profiling radar(CPR) onboard Cloud Sat allows for deep penetration into dense clouds/precipitation. In this study, tropical cyclones(TCs) are classified into three stages as developing, mature, and decaying. The circular TC area with the radius of 500 km is divided into five regions. The vertical structure characteristics of 94 Western Pacific TCs at different stages in different regions from June 2006 to February 2014 are statistically quantified using the Cloud Sat tropical cyclone overpass product(the CSTC Product). Contoured frequency by altitude diagrams(CFADs) of radar reflectivity show an arc-like feature and exhibit opposite distributions with a boundary at 5 km. Bright bands are found at this altitude, indicating melting layers. Deep convective(DC) clouds have the largest occurrence probability in the inner region, while Ci clouds occur more frequently in the outer region at 10-15 km. As clouds have the second largest vertical scale after DC clouds. Distributions of Ac, Cu, and Ns clouds at different stages have few distinctions.As the altitude increases, the ice effective radius and the distribution width parameter decrease while the particle number concentration increases. Moist static energy(MSE), cloud thickness(CT), liquid water path(LWP), ice water path(IWP), water vapor(WV), and rain rate(RR) all diminish along the radial direction and are significantly larger at the mature stage. The average value of MSE at the developing stage is larger than that at the decaying stage.展开更多
This vertically self‐pillared(VSP)structure extends the application range of traditional porous materials with facile mass/ion transport and enhanced reaction kinetics.Here,we prepare a single crystal metal‐organic ...This vertically self‐pillared(VSP)structure extends the application range of traditional porous materials with facile mass/ion transport and enhanced reaction kinetics.Here,we prepare a single crystal metal‐organic framework(MOF),employing the ZIF‐67 structure as a proof of concept,which is constructed by vertically self‐pillared nanosheets(VSP‐MOF).We further converted VSP‐MOF into VSP‐cobalt sulfide(VSP‐CoS2)through a sulfidation process.Catalysis plays an important role in almost all battery technologies;for metallic batteries,lithium anodes exhibit a high theoretical specific capacity,low density,and low redox potential.However,during the half‐cell reaction(Li++e=Li),uncontrolled dendritic Li penetrates the separator and solid electrolyte interphase layer.When employed as a composite scaffold for lithium metal deposition,there are many advantage to using this framework:1)the VSP‐CoS2 substrate provides a high specific surface area to dissipate the ion flux and mass transfer and acts as a pre‐catalyst,2)the catalytic Co center favors the charge transfer process and preferentially binds the Li+with the enhanced electrical fields,and 3)the VSP structure guides the metallic propagation along the nanosheet 2D orientation without the protrusive dendrites.All these features enable the VSP structure in metallic batteries with encouraging performances.展开更多
Based on L-band sounding data,threshold method of relative humidity was used to analyze vertical distribution characteristics of precipitation cloud system in Tianjin region.The results showed that main precipitation ...Based on L-band sounding data,threshold method of relative humidity was used to analyze vertical distribution characteristics of precipitation cloud system in Tianjin region.The results showed that main precipitation cloud system affecting Tianjin is cold and warm mixed cloud,followed by cold cloud,and precipitation of warm cloud is less.During May-November,precipitation of cold and warm mixed cloud is dominant,and it is dominant by precipitation of cold cloud from January to April.In four seasons,the precipitation frequency of double-layer cloud is the most,and precipitation of single-layer cloud mainly appears during March-November,and peak is in June.Peak of cloud system with three or more layers all appears in July and August.The cold cloud and warm cloud catalysts should be selected respectively for artificial precipitation enhancement in Tianjin.In winter,cold cloud catalyst operation is selected;in spring,summer and autumn,the cold cloud catalyst is spread in the cold cloud area,and the warm cloud catalyst is distributed in the warm cloud area according to the conditions of cloud layer.展开更多
Based on a synthetic geological study of drilling, well logging and core observations, two main genetic types of Chang 9sand body in Odors Basin were recognized, which included two effects, that is, delta environment ...Based on a synthetic geological study of drilling, well logging and core observations, two main genetic types of Chang 9sand body in Odors Basin were recognized, which included two effects, that is, delta environment and tractive current effects that lead to the development of mouth bar, distal bar, sheet sand and other sand bodies of subaerial and subaqueous distributary channel,natural levee, flood fan and delta front, and shore-shallow lake environment and lake flow transformation effects that result in the development of sandy beach bar, sheet sand and other sand bodies. Chang 9 sand body mainly developed five basic vertical structures, namely box shape, campaniform, infundibuliform, finger and dentoid. The vertical stacking patterns of multilayer sand body was complex, and the common shapes included box shape + box shape, campaniform + campaniform, campaniform + box shape, infundibuliform + infundibuliform, campaniform + infundibuliform, box shape + campaniform, box shape + infundibuliform,and finger + finger. Based on the analysis on major dominating factors of vertical structure of sand body, sedimentary environment,sedimentary facies and rise, fall and cycle of base level are identified as the major geological factors that control the vertical structure of single sand body as well as vertical stacking patterns and distribution of multistory sand bodies.展开更多
The tidal current is generally predominant in China's offshore areas. The vertical structure of the observedtidal current is quite complicated with the presence of seasonal thermocline. The observed tidal current ...The tidal current is generally predominant in China's offshore areas. The vertical structure of the observedtidal current is quite complicated with the presence of seasonal thermocline. The observed tidal current may be divided into two parts, an averaged barotropic tide current and a variation tide current. A method for studying the vertical structure of tidal current is developed from the constitution and distribution of energy, and the vertical structure of the observed tide current in the North Huanghai Sea is studied on the basis of the method. The result shows that the reason why the energy of the tidal current is concentrated on the neighbourhood of the thermocline mainly lies in the internal tides i under certain conditions, the fact that the direction of the internal tide current above the thermocline is opposite to the one below the thermocline will be able to cause the rotary directions of the observed tidal current above and below the thermocline to be in opposite. The interaction between the averaged barotropic and the variation tide current plays an important role in forming the vertical structure of the tidal current, and it is mainly the interaction that results in the inho-mogeneous distribution of the tide current energy in the entire water column ; the ratio between the total energies of the internal tide current above the thermocline and the variation tide current in the entire water column is greater than the ratio between the total energies of that below the thermocline and the variation's. In a strong internal tide area such as the neighbourhood of Station L4, at diurnal tide frequency, the above-mentioned corresponding ratios are about 38. 82% and 29. 88%, respectively, and the energy of the internal tide current is about 68. 70%of the energy of the variation tide current; at semidiurnal tide frequency, the above-mentioned corresponding ratios are about 26. 61 % and 19. 73% , respectively, and the total internal tide current energy is about 46. 36% of the total variation tide current energy.展开更多
This study evaluates the vertical profiles of aerosol and cloud optical properties in 40 dominated dust and smoke regions in Western-Northern Africa (WNA) and Central-Southern Africa (CSA), respectively, from the surf...This study evaluates the vertical profiles of aerosol and cloud optical properties in 40 dominated dust and smoke regions in Western-Northern Africa (WNA) and Central-Southern Africa (CSA), respectively, from the surface to 10km and from 2008 to 2011 based on LIVAS (LIdar climatology of Vertical Aerosol Structure for space-based lidar simulation studies). Aerosol extinction (AE), aerosol backscatter (AB), and aerosol depolarization (AD) generally increase from the surface to 1.2 km and decrease from 1.2 km to the upper layers in both WNA and CSA. AE and AB in CSA (maximum of 0.13 km<sup>-1</sup>, 0.14 km<sup>-1</sup>, 0.0021 km<sup>-1</sup>‧sr<sup>-1</sup>, 0.0033 km<sup>-1</sup>‧sr<sup>-1</sup>) are higher than in WNA (maximum of 0.07 km<sup>-1</sup>, 0.08 km<sup>-1</sup>, 0.0017 km<sup>-1</sup>‧sr<sup>-1</sup>, 0.0015 km<sup>-1</sup>‧sr<sup>-1</sup>) at 532 and 1064 nm respectively. AD in WNA (maximum of 0.25) is significantly higher than in CSA (maximum of 0.05). There is a smooth change with the height of cloud extinction and backscatter in WNA and CSA, while there is a remarkable increase of cloud depolarization with height, whereby it is high in CSA and low in WNA due to high and low fraction of cirrus respectively. Altocumulus has the highest extinction in NA (0.0139 km<sup>-1</sup>), CA (0.058 km<sup>-1</sup>), WA (0.013 km<sup>-1</sup>), while low overcast transparent (0.76 km<sup>-1</sup>) below 1 km in SA. The major findings of this study may contribute to the improvement of our understanding of aerosol-cloud interaction studies in dominated dust and smoke aerosol regions.展开更多
A n-type small molecule DC-IDT2E with 4,4,9,9-tetrakis(4-hexylphenyl)-indaceno[1,2-b:5,6-bt]dithiophene as a central building block, furan as rr-bridges, and 1,1 -dicyanomethylene-3-indanone as end acceptor groups,...A n-type small molecule DC-IDT2E with 4,4,9,9-tetrakis(4-hexylphenyl)-indaceno[1,2-b:5,6-bt]dithiophene as a central building block, furan as rr-bridges, and 1,1 -dicyanomethylene-3-indanone as end acceptor groups, was synthesized and used as an electron acceptor in solution-processed organic solar cells (OSCs). DC-IDT2F exhibited good thermal stability, broad and strong absorption in 500-850 rim, a narrow bandgap of 1.54 eV, LUMO of-3.88 eV, HOMO of-5.44 eV and an electron mobility of 6.5 × 10-4 cm2/(V.s). DC-IDT2F-based OSCs with conventional and inverted structures exhibited power conversion efficiencies of 2.26 and 3.08% respec- tively. The effect of vertical phase separation and morphology of the active layer on the device performance in the two structures was studied.展开更多
In this study,substantial satellitic remote sensing data and atmospheric observational data were used to study a snowfall caused by Bohai sea-effect snow cloud which occurred in Shandong Peninsula from 4 to 6,DEC 2008...In this study,substantial satellitic remote sensing data and atmospheric observational data were used to study a snowfall caused by Bohai sea-effect snow cloud which occurred in Shandong Peninsula from 4 to 6,DEC 2008.The study results show that the snow cloud emerged in the strong northwesterly cold flow in the middle-lower troposphere,the southwest of northeast cold vortex,and cyclonic bending on the surface pressure-field.Although the snowstorm cloud was shallow convective,its cold center was quite strong,the average snowfall rate was 0.41 mm/h during the exuberant period,and the snowfall rate was distributed in strip.The upwelling longwave fluxes on the cloud top were not only related to the temperature,but also related to the ice water content of the cloud,when we study the clouds effect on the radiation,we should consider the rainfall(snowfall)strength of the cloud.展开更多
基金supported by the National Natural Science Foundation of China (Grant No. 42105093 and 41975018)the China Postdoctoral Science Foundation (Grant No. 2020M670420)the Special Research Assistant Project。
文摘Turbulence in the nocturnal boundary layer(NBL)is still not well characterized,especially over complex underlying surfaces.Herein,gradient tower data and eddy covariance data collected by the Beijing 325-m tower were used to better understand the differentiating characteristics of turbulence regimes and vertical turbulence structure of urban the NBL.As for heights above the urban canopy layer(UCL),the relationship between turbulence velocity scale(VTKE)and wind speed(V)was consistent with the“HOckey-Stick”(HOST)theory proposed for a relatively flat area.Four regimes have been identified according to urban nocturnal stable boundary layer.Regime 1 occurs where local shear plays a leading role for weak turbulence under the constraint that the wind speed V<VT(threshold wind speed).Regime 2 is determined by the existence of strong turbulence that occurs when V>VT and is mainly driven by bulk shear.Regime 3 is identified by the existence of moderate turbulence when upside-down turbulence sporadic bursts occur in the presence of otherwise weak turbulence.Regime 4 is identified as buoyancy turbulence,when V>VT,and the turbulence regime is affected by a combination of local wind shear,bulk shear and buoyancy turbulence.The turbulence activities demonstrated a weak thermal stratification dependency in regime 1,for which within the UCL,the turbulence intensity was strongly affected by local wind shear when V<VT.This study further showed typical examples of different stable boundary layers and the variations between turbulence regimes by analyzing the evolution of wind vectors.Partly because of the influence of large-scale motions,the power spectral density of vertical velocity for upsidedown structure showed an increase at low frequencies.The upside-down structures were also characterized by the highest frequency of the stable stratifications in the higher layer.
基金Supported by the China Meteorological Administration Special Public Welfare Research Fund(GYHY201206041)Project of Comprehensive Evaluation of Polar Areas on Global and Regional Climate Changes(CHINARE2016-04-04)Polar Environment Comprehensive Investigation and Assessment(CHINARE2016-02-03)
文摘In June 2013,a field experiment was conducted in Southeast Tibet in which the air temperature,moisture,and wind were measured by using a GPS sounding system.In the present study,based on these observations and ERA-Interim reanalysis data,the vertical structures of these atmospheric properties and the possible influence of the South Asian summer monsoon(SASM) were investigated.On average,the temperature had a lapse rate of 6.8℃ km^(-1) below the tropopause of 18.0 km.A strong moisture inversion occurred at the near-surface,with a strength of 1.7 g kg^(-1)(100 m)^(-1) for specific humidity.During the observation period,the SASM experienced a south phase and a north phase in the middle and by the end of June,respectively.The monsoon's evolution led to large changes in convection and circulation over Southeast Tibet,which further affected the local thermal,moisture,and circulation conditions.The strong convection resulted in an elevated tropopause height over Southeast Tibet during the north phase of the SASM,and the large-scale warm and wet air masses delivered by the monsoon caused high local temperature and moisture conditions.
基金Mengxi Wang holds a doctoral scholarship from the China scholarship council(CSC:202003270025)。
文摘Vertical forest structure is closely linked to multiple ecosystem characteristics,such as biodiversity,habitat,and productivity.Mixing tree species in planted forests has the potential to create diverse vertical forest structures due to the different physiological and morphological traits of the composing tree species.However,the relative importance of species richness,species identity and species interactions for the variation in vertical forest structure remains unclear,mainly because traditional forest inventories do not observe vertical stand structure in detail.Terrestrial laser scanning(TLS),however,allows to study vertical forest structure in an unprecedented way.Therefore,we used TLS single scan data from 126 plots across three experimental planted forests of a largescale tree diversity experiment in Belgium to study the drivers of vertical forest structure.These plots were 9–11years old young pure and mixed forests,characterized by four levels of tree species richness ranging from monocultures to four-species mixtures,across twenty composition levels.We generated vertical plant profiles from the TLS data and derived six stand structural variables.Linear mixed models were used to test the effect of species richness on structural variables.Employing a hierarchical diversity interaction modelling framework,we further assessed species identity effect and various species interaction effects on the six stand structural variables.Our results showed that species richness did not significantly influence most of the stand structure variables,except for canopy height and foliage height diversity.Species identity on the other hand exhibited a significant impact on vertical forest structure across all sites.Species interaction effects were observed to be site-dependent due to varying site conditions and species pools,and rapidly growing tree species tend to dominate these interactions.Overall,our results highlighted the importance of considering both species identity and interaction effects in choosing suitable species combinations for forest management practices aimed at enhancing vertical forest structure.
基金supported by the National Natural Science Foundation of China under Grant Nos. 40628005 and 40633017
文摘Knowledge of the vertical distribution of aerosols in the free troposphere is important for estimating their impact on climate. In this study, direct observations of the vertical distribution of aerosols in the free troposphere are made using surface Micro-Pulse Lidar (MPL) measurements. The MPL measurements were made at the Loess Plateau (35.95°N, 104.1°E), which is near the major dust source regions of the Taklimakan and Gobi deserts. The vertical distribution of the MPL backscattering suggested that nondust aerosols floated from ground level to an altitude of approximately 9 km around the source regions. Early morning hours are characterized by a shallow aerosol layer of a few hundred meters thick. As the day progresses, strong convective eddies transport the aero- sols vertically to more than 1500 m.
基金jointly supported by the National Natural Science Foundation of China (Grant Nos.41275077 and 41105054)the National Basic Research Program of China (973 Program:2010CB951902)+1 种基金the China Meteorological Administration (Grant Nos.GYHY201106022 and GYHY201306048)the Sun Yat-sen University "985 Project", Phase 3
文摘ABSTRACT The abilities of BCC-AGCM2.1 and BCC_AGCM2.2 to simulate the annual-mean cloud vertical structure (CVS) were evaluated through comparison with GCM-Oriented CALIPSO Cloud Product (CALIPSO-GOCCP) data. BCC-AGCM2.2 has a dynamical core and physical processes that are consistent with BCC-AGCM2.1, but has a higher horizontal resolution. Results showed that both BCC-AGCM versions underestimated the global-mean total cloud cover (TCC), middle cloud cover (MCC) and low cloud cover (LCC), and that BCC_AGCM2.2 underestimated the global-mean high cloud cover (HCC). The global-mean cloud cover shows a systematic decrease from BCCA-GCM2.1 to BCC_AGCM2.2, especially for HCC. Geographically, HCC is significantly overestimated in the tropics, particularly by BCC_AGCM2,1, while LCC is generally overestimated over extra-tropical lands, but significantly underestimated over most of the oceans, especially for subtropical marine stratocumulus clouds. The leading EOF modes of CVS were extracted. The BCC_AGCMs perform well in reproducing EOF1, but with a larger variance explained. The two models also capture the basic features of EOF3, except an obvious deficiency in eigen- vector peaks. EOF2 has the largest simulation biases in both position and strength of eigenvector peaks. Furthermore, we investigated the effects of CVS on relative shortwave and longwave cloud radiative forcing (RSCRF and RLCRF). Both BCC_AGCM versions successfully reproduce the sign of regression coefficients, except for RLCRF in PC1. However, the RSCRF relative contributions from PC1 and PC2 are overestimated, while the relative contribution from PC3 is underes timated in both BCC_AGCM versions. The RLCRF relative contribution is underestimated for PC2 and overestimated for PC3.
基金financially supported by the China Petroleum&Chemical Corporation(SINOPEC)(Grant No.P18047-2)the National Natural Science Foundation of China(Grant No.U19B6003-01)the National Key Research and Development Program of China(Grant No.2017YFC0601405)。
文摘Vertical differential structural deformation(VDSD),one of the most significant structural characteristics of strike-slip fault zones(SSFZs)in the Shunbei area,is crucial for understanding deformation in the SSFZ and its hydrocarbon accumulation significance.Based on drilling data and high-precision 3-D seismic data,we analyzed the geometric and kinematic characteristics of the SSFZs in the Shunbei area.Coupled with the stratification of the rock mechanism,the structural deformations of these SSFZs in different formations were differentiated and divided into four deformation layers.According to comprehensive structural interpretations and comparisons,three integrated 3-D structural models could describe the VDSD of these SSFZs.The time-space coupling of the material basis(rock mechanism stratification),changing dynamic conditions(e.g.,changing stress-strain states),and special deformation mechanism of the en echelon normal fault array uniformly controlled the formation of the VDSD in the SSFZs of the Shunbei area.The VDSD of the SSFZs in this area controlled the entire hydrocarbon accumulation process.Multi-stage structural superimposing deformation influenced the hydrocarbon migration,accumulation,distribution,preservation,and secondary adjustments.
基金supported by the National Natural Science Foundation of China (Grant No. 41721004)
文摘This study investigates the vertical structure of variability in the cross-equatorial flows(CEFs)over the Maritime Continent and Indian Ocean in boreal summer,based on three reanalysis datasets:ERA-Interim,JRA-55 and NCEP-2.The results show a high consistency in the interannual variability among the reanalysis datasets,especially between ERAInterim and JRA-55,while great uncertainty exists in the decadal or long-term changes of CEFs.Further analyses on the interannual variability in CEFs indicate that there is a significant negative relationship between the upper-and lower-level CEFs over the Maritime Continent—that is,the northerlies at the upper level and southerlies at the lower level are both enhanced or weakened.This seesaw pattern is also significantly related to the CEFs over the Indian Ocean at the upper level and lower level(i.e.,the Somali jet).This close relationship between the upper-and lower-level CEFs and between the Maritime Continent and Indian Ocean is manifested as the leading mode of equatorial meridional winds in the vertical-zonal section over the Maritime Continent and Indian Ocean.Finally,it is found that ENSO is closely related to the vertical leading mode,and to all the CEFs at the upper and lower levels over the Maritime Continent and Indian Ocean.
基金Supported by the Knowledge Innovation Program of Chinese Academy of Sciences (No.KZCX-3W-222 KZCX2-YW-Q11-02)+1 种基金National Basic Research Program of China (No.2007CB411802 2006CB403601)
文摘Empirical Orthogonal Function (EOF) analysis is used in this study to generate main eigenvector fields of historical temperature for the China Seas (here referring to Chinese marine territories) and adjacent waters from 1930 to 2002 (510 143 profiles). A good temperature profile is reconstructed based on several subsurface in situ temperature observations and the thermocline was estimated using the model. The results show that: 1) For the study area, the former four principal components can explain 95% of the overall variance, and the vertical distribution of temperature is most stable using the in situ temperature observations near the surface. 2) The model verifications based on the observed CTD data from the East China Sea (ECS), South China Sea (SCS) and the areas around Taiwan Island show that the reconstructed profiles have high correlation with the observed ones with the confidence level 〉95%, especially to describe the characteristics of the thermocline well. The average errors between the reconstructed and observed profiles in these three areas are 0.69℃, 0.52℃ and 1.18℃ respectively. It also shows the model RMS error is less than or close to the climatological error. The statistical model can be used to well estimate the temperature profile vertical structure. 3) Comparing the thermocline characteristics between the reconstructed and observed profiles, the results in the ECS show that the average absolute errors are 1.5m, 1.4 m and 0.17~C/m, and the average relative errors are 24.7%, 8.9% and 22.6% for the upper, lower thermocline boundaries and the gradient, respectively. Although the relative errors are obvious, the absolute error is small. In the SCS, the average absolute errors are 4.1 m, 27.7 m and 0.007℃/m, and the average relative errors are 16.1%, 16.8% and 9.5% for the upper, lower thermocline boundaries and the gradient, respectively. The average relative errors are all 〈20%. Although the average absolute error of the lower thermocline boundary is considerable, but contrast to the spatial scale of average depth of the lower thermocline boundary (165 m), the average relative error is small (16.8%). Therefore the model can be used to well estimate the thermocline.
基金The National Natural Science Foundation of China under contract Nos 41705081 and 41906005the Innovation Special Zone Project under contract No.18-H863-05-ZT-001-012-06the Open Project Fund of the Laboratory for Regional Oceanography and Numerical Modeling,Pilot National Laboratory for Marine Science and Technology(Qingdao)under contract No.2019A05.
文摘The sensitive area of targeted observations for short-term(7 d)prediction of vertical thermal structure(VTS)in summer in the Yellow Sea was investigated.We applied the Conditional Nonlinear Optimal Perturbation(CNOP)method and an adjoint-free algorithm with the Regional Ocean Modeling System(ROMS).We used vertical integration of CNOP-type temperature errors to locate the sensitive areas,where reduction of initial errors is expected to yield the greatest improvement in VTS prediction for the selected verification area.The identified sensitive areas were northeast−southwest orientated northeast to the verification area,which were possibly related to the southwestward background currents.Then,we performed a series of sensitivity experiments to evaluate the effectiveness of the identified sensitive areas.Results show that initial errors in the identified sensitive areas had the greatest negative effect on VTS prediction in the verification area compared to errors in other areas(e.g.,the verification area and areas to its east and northeast).Moreover,removal of initial errors through deploying simulated observations in the identified sensitive areas led to more refined prediction than correction of initial conditions in the verification area itself.Our results suggest that implementation of targeted observation in the CNOP-based sensitive areas is an effective method to improve short-term prediction of VTS in summer in the Yellow Sea.
文摘In this paper, on the basis of the heat conduction equation without consideration of the advection and turbulence effects, one-dimensional model for describing surface sea temperature ( T1), bottom sea temperature ( Tt ) and the thickness of the upper homogeneous layer ( h ) is developed in terms of the dimensionless temperature θT and depth η and self-simulation function θT - f(η) of vertical temperature profile by means of historical temperature data.The results of trial prediction with our one-dimensional model on T, Th, h , the thickness and gradient of thermocline are satisfactory to some extent.
基金The National Natural Science Foundation of China under contract Nos 41806114 and 42266006the Jiangxi Provincial Natural Science Foundation under contract Nos 20202ACBL214019,20181BAB216031 and 20212BBE53031+2 种基金the Technological Innovation and Application Development in Chongqing under contract No.CSTB2022TIAD-GPX0016the Incentive and Guidance Project of Scientific Research Performance for Scientific Research Institutes in Chongqing under contract No.cstc2021jxjl120017the Open Fund of the Key Laboratory of Marine Environmental Survey Technology and Application of Ministry of Natural Resources under contract Nos MESTA-2020-A002 and MESTA-2021-B001.
文摘Three long-term fixed acoustic Doppler current profilers were first used for investigating the vertical structure of tidal currents in Xuliujing Section of Changjiang River Estuary.Moreover,three different periods(spring,summer and fall)were also considered for investigating seasonal variations.The semi-diurnal tides were the most energetic,with along-channel speed of up to 80 cm/s for M_(2)constituent,which dominates at all stations with percent energy up to 65%–75%during seasons.The shape of tidal ellipses of the most energetic semi-diurnal constituent M_(2)showed obvious polarization of the flow paralleling to the riverbank,with the minor semi-axis being generally less than 20%of the major one.The maximum velocity of mean current is appeared in top layers at all the three stations,and the velocity decreased with the depth.The seasonal variations of direction are also observed,which is probably caused by complex local topography since the erosion and deposition in riverbed.Observed vertical variation of four parameters of M_(2)ellipses,agreed well with the optimally fit frictional solutions in top and middle layers.However,there was an obvious difference between frictional model and observed data in the lower water column.Discrepancies are probably on account of stratification,which strengthens in summer and fall due to the freshening influence of the Changjiang River Estuary outflow.
文摘The algebraic solitary wave and its associated eigenvalue problem in a deep stratified fluid with a free surface and a shallow upper layer were studied. And its vertical structure was examined. An exact solution for the derived 2D Benjamin-Ono equation was obtained, and physical explanation was given with the corresponding dispersion relation. As a special case, the vertical structure of the weakly nonlinear internal wave for the Holmboe density distribution was numerically investigated, and the propagating mechanism of the internal wave was studied by using the ray theory.
基金National Natural Science Foundation of China(41076118)Young Scientists Fund of National Natural Science Foundation of China Grant(41005018)
文摘Cloud profiling radar(CPR) onboard Cloud Sat allows for deep penetration into dense clouds/precipitation. In this study, tropical cyclones(TCs) are classified into three stages as developing, mature, and decaying. The circular TC area with the radius of 500 km is divided into five regions. The vertical structure characteristics of 94 Western Pacific TCs at different stages in different regions from June 2006 to February 2014 are statistically quantified using the Cloud Sat tropical cyclone overpass product(the CSTC Product). Contoured frequency by altitude diagrams(CFADs) of radar reflectivity show an arc-like feature and exhibit opposite distributions with a boundary at 5 km. Bright bands are found at this altitude, indicating melting layers. Deep convective(DC) clouds have the largest occurrence probability in the inner region, while Ci clouds occur more frequently in the outer region at 10-15 km. As clouds have the second largest vertical scale after DC clouds. Distributions of Ac, Cu, and Ns clouds at different stages have few distinctions.As the altitude increases, the ice effective radius and the distribution width parameter decrease while the particle number concentration increases. Moist static energy(MSE), cloud thickness(CT), liquid water path(LWP), ice water path(IWP), water vapor(WV), and rain rate(RR) all diminish along the radial direction and are significantly larger at the mature stage. The average value of MSE at the developing stage is larger than that at the decaying stage.
文摘This vertically self‐pillared(VSP)structure extends the application range of traditional porous materials with facile mass/ion transport and enhanced reaction kinetics.Here,we prepare a single crystal metal‐organic framework(MOF),employing the ZIF‐67 structure as a proof of concept,which is constructed by vertically self‐pillared nanosheets(VSP‐MOF).We further converted VSP‐MOF into VSP‐cobalt sulfide(VSP‐CoS2)through a sulfidation process.Catalysis plays an important role in almost all battery technologies;for metallic batteries,lithium anodes exhibit a high theoretical specific capacity,low density,and low redox potential.However,during the half‐cell reaction(Li++e=Li),uncontrolled dendritic Li penetrates the separator and solid electrolyte interphase layer.When employed as a composite scaffold for lithium metal deposition,there are many advantage to using this framework:1)the VSP‐CoS2 substrate provides a high specific surface area to dissipate the ion flux and mass transfer and acts as a pre‐catalyst,2)the catalytic Co center favors the charge transfer process and preferentially binds the Li+with the enhanced electrical fields,and 3)the VSP structure guides the metallic propagation along the nanosheet 2D orientation without the protrusive dendrites.All these features enable the VSP structure in metallic batteries with encouraging performances.
基金Supported by Open Research Fund Project of Key Laboratory of Meteorology and Ecological Environment of Hebei Province(Z202001Z,Z201602Z)Science and Technology Collaborative Innovation Fund Project in Bohai Rim Region(QYXM202004)Key Projects of Tianjin Meteorological Bureau(201801zdxm01)。
文摘Based on L-band sounding data,threshold method of relative humidity was used to analyze vertical distribution characteristics of precipitation cloud system in Tianjin region.The results showed that main precipitation cloud system affecting Tianjin is cold and warm mixed cloud,followed by cold cloud,and precipitation of warm cloud is less.During May-November,precipitation of cold and warm mixed cloud is dominant,and it is dominant by precipitation of cold cloud from January to April.In four seasons,the precipitation frequency of double-layer cloud is the most,and precipitation of single-layer cloud mainly appears during March-November,and peak is in June.Peak of cloud system with three or more layers all appears in July and August.The cold cloud and warm cloud catalysts should be selected respectively for artificial precipitation enhancement in Tianjin.In winter,cold cloud catalyst operation is selected;in spring,summer and autumn,the cold cloud catalyst is spread in the cold cloud area,and the warm cloud catalyst is distributed in the warm cloud area according to the conditions of cloud layer.
基金Project(2011D-5006-0105)supported by the Technology Innovation Foundation of CNPC,ChinaProject(SZD0414)supported by the Key Discipline of Mineral Prospecting and Exploration of Sichuan Province,China
文摘Based on a synthetic geological study of drilling, well logging and core observations, two main genetic types of Chang 9sand body in Odors Basin were recognized, which included two effects, that is, delta environment and tractive current effects that lead to the development of mouth bar, distal bar, sheet sand and other sand bodies of subaerial and subaqueous distributary channel,natural levee, flood fan and delta front, and shore-shallow lake environment and lake flow transformation effects that result in the development of sandy beach bar, sheet sand and other sand bodies. Chang 9 sand body mainly developed five basic vertical structures, namely box shape, campaniform, infundibuliform, finger and dentoid. The vertical stacking patterns of multilayer sand body was complex, and the common shapes included box shape + box shape, campaniform + campaniform, campaniform + box shape, infundibuliform + infundibuliform, campaniform + infundibuliform, box shape + campaniform, box shape + infundibuliform,and finger + finger. Based on the analysis on major dominating factors of vertical structure of sand body, sedimentary environment,sedimentary facies and rise, fall and cycle of base level are identified as the major geological factors that control the vertical structure of single sand body as well as vertical stacking patterns and distribution of multistory sand bodies.
基金The project supported by National Natural science Foundation of China
文摘The tidal current is generally predominant in China's offshore areas. The vertical structure of the observedtidal current is quite complicated with the presence of seasonal thermocline. The observed tidal current may be divided into two parts, an averaged barotropic tide current and a variation tide current. A method for studying the vertical structure of tidal current is developed from the constitution and distribution of energy, and the vertical structure of the observed tide current in the North Huanghai Sea is studied on the basis of the method. The result shows that the reason why the energy of the tidal current is concentrated on the neighbourhood of the thermocline mainly lies in the internal tides i under certain conditions, the fact that the direction of the internal tide current above the thermocline is opposite to the one below the thermocline will be able to cause the rotary directions of the observed tidal current above and below the thermocline to be in opposite. The interaction between the averaged barotropic and the variation tide current plays an important role in forming the vertical structure of the tidal current, and it is mainly the interaction that results in the inho-mogeneous distribution of the tide current energy in the entire water column ; the ratio between the total energies of the internal tide current above the thermocline and the variation tide current in the entire water column is greater than the ratio between the total energies of that below the thermocline and the variation's. In a strong internal tide area such as the neighbourhood of Station L4, at diurnal tide frequency, the above-mentioned corresponding ratios are about 38. 82% and 29. 88%, respectively, and the energy of the internal tide current is about 68. 70%of the energy of the variation tide current; at semidiurnal tide frequency, the above-mentioned corresponding ratios are about 26. 61 % and 19. 73% , respectively, and the total internal tide current energy is about 46. 36% of the total variation tide current energy.
文摘This study evaluates the vertical profiles of aerosol and cloud optical properties in 40 dominated dust and smoke regions in Western-Northern Africa (WNA) and Central-Southern Africa (CSA), respectively, from the surface to 10km and from 2008 to 2011 based on LIVAS (LIdar climatology of Vertical Aerosol Structure for space-based lidar simulation studies). Aerosol extinction (AE), aerosol backscatter (AB), and aerosol depolarization (AD) generally increase from the surface to 1.2 km and decrease from 1.2 km to the upper layers in both WNA and CSA. AE and AB in CSA (maximum of 0.13 km<sup>-1</sup>, 0.14 km<sup>-1</sup>, 0.0021 km<sup>-1</sup>‧sr<sup>-1</sup>, 0.0033 km<sup>-1</sup>‧sr<sup>-1</sup>) are higher than in WNA (maximum of 0.07 km<sup>-1</sup>, 0.08 km<sup>-1</sup>, 0.0017 km<sup>-1</sup>‧sr<sup>-1</sup>, 0.0015 km<sup>-1</sup>‧sr<sup>-1</sup>) at 532 and 1064 nm respectively. AD in WNA (maximum of 0.25) is significantly higher than in CSA (maximum of 0.05). There is a smooth change with the height of cloud extinction and backscatter in WNA and CSA, while there is a remarkable increase of cloud depolarization with height, whereby it is high in CSA and low in WNA due to high and low fraction of cirrus respectively. Altocumulus has the highest extinction in NA (0.0139 km<sup>-1</sup>), CA (0.058 km<sup>-1</sup>), WA (0.013 km<sup>-1</sup>), while low overcast transparent (0.76 km<sup>-1</sup>) below 1 km in SA. The major findings of this study may contribute to the improvement of our understanding of aerosol-cloud interaction studies in dominated dust and smoke aerosol regions.
基金supported by the National Natural Science Foundation of China(91433114,51261130582,21025418)the 973 Program(2011CB808401)the Chinese Academy of Sciences
文摘A n-type small molecule DC-IDT2E with 4,4,9,9-tetrakis(4-hexylphenyl)-indaceno[1,2-b:5,6-bt]dithiophene as a central building block, furan as rr-bridges, and 1,1 -dicyanomethylene-3-indanone as end acceptor groups, was synthesized and used as an electron acceptor in solution-processed organic solar cells (OSCs). DC-IDT2F exhibited good thermal stability, broad and strong absorption in 500-850 rim, a narrow bandgap of 1.54 eV, LUMO of-3.88 eV, HOMO of-5.44 eV and an electron mobility of 6.5 × 10-4 cm2/(V.s). DC-IDT2F-based OSCs with conventional and inverted structures exhibited power conversion efficiencies of 2.26 and 3.08% respec- tively. The effect of vertical phase separation and morphology of the active layer on the device performance in the two structures was studied.
文摘In this study,substantial satellitic remote sensing data and atmospheric observational data were used to study a snowfall caused by Bohai sea-effect snow cloud which occurred in Shandong Peninsula from 4 to 6,DEC 2008.The study results show that the snow cloud emerged in the strong northwesterly cold flow in the middle-lower troposphere,the southwest of northeast cold vortex,and cyclonic bending on the surface pressure-field.Although the snowstorm cloud was shallow convective,its cold center was quite strong,the average snowfall rate was 0.41 mm/h during the exuberant period,and the snowfall rate was distributed in strip.The upwelling longwave fluxes on the cloud top were not only related to the temperature,but also related to the ice water content of the cloud,when we study the clouds effect on the radiation,we should consider the rainfall(snowfall)strength of the cloud.