Climatic Features of Cloud Water Distribution and Cycle over China

Analyses of cloud water path （CWP） data over China available from the International Satellite Cloud Climatology Project （ISCCP） are performed for the period 1984-2004. Combined with GPCP precipitation data, cloud water cycle index （CWCI） is also calculated. The climatic distributions of CWP are found to be dependent on large-scale circulation, topographical features, water vapor transport and similar distribution features which are found in CWCI except in the Sichuan Basin. Influenced by the Asia monsoon, CWP over China exhibits very large seasonal variations in different regions. The seasonal cycles of CWCI in different regions are consistent and the largest CWCI occurs in July. The long-term trends of CWP and CWCI are investigated, too. Increasing trends of CWP are found during the period with the largest increase found in winter. The decreasing trends of CWCI dominate most regions of China. The differences in long-term trends between CWP and CWCI suggest that CWP only can influence the variation of CWCI to a certain extent and that other factors need to be involved in cloud water cycle researches. This phenomenon reveals the complexity of the hydrological cycle related to cloud water.

Sensitivity of the Grid-point Atmospheric Model of IAP LASG(GAMILI.I.0)Climate Simulations to Cloud Droplet Effective Radius and Liquid Water Path

This paper documents a study to examine the sensitivity to cloud droplet effective radius and liquid water path and the alleviation the energy imbalance at the top of the atmosphere and at the surface in the latest version of the Grid-point Atmospheric Model of the State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics （LASG）, Institute of Atmospheric Physics （IAP） （GAMIL1.1.0）. Considerable negative biases in all flux components, and thus an energy imbalance, are found in GAMIL1.1.0. In order to alleviate the energy imbalance, two modifications, namely an increase in cloud droplet effective radius and a decrease in cloud liquid water path, have been made to the cloud properties used in GAMIL. With the increased cloud droplet effective radius, the single scattering albedo of clouds is reduced, and thus the reflection of solar radiation into space by clouds is reduced and the net solar radiation flux at the top of the atmosphere is increased. With the reduced cloud optical depth, the net surface shortwave radiation flux is increased, causing a net warming over the land surface. This results in an increase in both sensible and latent heat fluxes over the land regions, which is largely balanced by the increased terrestrial radiation fluxes. Consequently, the energy balance at the top of atmosphere and at the surface is achieved with energy flux components consistent with available satellite observations.

Precipitation responses to radiative processes of water- and ice-clouds: an equilibrium cloud-resolving modeling study

云辐射过程对制约天气与气候很重要。本文通过分析二维云分辨模式敏感性试验模拟平衡态平均资料研究降水对水云及冰云辐射过程的响应。模式给定的垂直速度为零。存在冰云辐射过程时去除水云辐射过程,以及去除冰云辐射过程会加强大气长波辐射冷却和降低空气温度及饱和混合比。饱和混合比的减少导致水汽凝结增加及其相关的潜热释放的增加,从而增加降雨。去除水云辐射过程通过减少长波辐射冷却增加对流层上部局地大气变暖。而增强的变暖通过霰的融化增强而增加降水源与降水。

Parameterization for narrow band shortwave optical properties of water clouds

Based on the drop size distribution models built from the observational data of microphysical properties of water clouds, the relationships between the optical properties and microphysical characteristics of water clouds have been investigated, and some different parameterization schemes of cloud optical properties have been analyzed. It is found that with the parameterization scheme, in addition to the equivalent radius, also including the mean radius of cloud droplet size distribution, the role of small cloud drops might be able to be considered more properly and better accuracies of parameterization calculation of cloud optical properties can be obtained, compared with that of using only the equivalent radius as parameter.

An assessment of Arctic cloud water paths in atmospheric reanalyses

The role of Arctic clouds in the recent rapid Arctic warming has attracted much attention.However,Arctic cloud water paths(CWPs)from reanalysis datasets have not been well evaluated.This study evaluated the CWPs as well as LWPs(cloud liquid water paths)and IWPs(cloud ice water paths)from five reanalysis datasets(MERRA-2,MERRA,ERA-Interim,JRA-55,and ERA5)against the COSP(Cloud Feedback Model Intercomparison Project Observations Simulator Package)output for MODIS from the MERRA-2 CSP(COSP satellite simulator)collection(defined as M2Modis in short).Averaged over 1980-2015 and over the Arctic region(north of 60°N),the mean CWPs of these five datasets range from 49.5 g/m^(2)(MERRA)to 82.7 g/m^(2)(ERA-Interim),much smaller than that from M2Modis(140.0 g/m^(2)).However,the spatial distributions of CWPs,show similar patterns among these reanalyses,with relatively small values over Greenland and large values over the North Atlantic.Consistent with M2Modis,these reanalyses show larger LWPs than IWPs,except for ERA-Interim.However,MERRA-2 and MERRA underestimate the ratio of IWPs to CWPs over the entire Arctic,while ERA-Interim and JRA-55 overestimate this ratio.ERA5 shows the best performance in terms of the ratio of IWPs to CWPs.All datasets exhibit larger CWPs and LWPs in summer than in winter.For M2Modis,IWPs hold seasonal variation similar with LWPs over the land but opposite over the ocean.Following the Arctic warming,the trends in LWPs and IWPs during 1980~2015 show that LWPs increase and IWPs decrease across all datasets,although not statistically significant.Correlation analysis suggests that all datasets have similar interannual variability.The study further found that the inclusion of re-evaporation processes increases the humidity in the atmosphere over the land and that a more realistic liquid/ice phase can be obtained by independently treating the liquid and ice water contents.

EnKF Assimilation of Satellite-retrieved Cloud Water Path to Improve Tropical Cyclone Rainfall Forecast

Tropical cyclone(TC) rainfall forecast has remained a challenge. To create initial conditions with high quality for simulation, the present study implemented a data assimilation scheme based on the EnKF method to ingest the satellite-retrieved cloud water path(C_(w)) and tested it in WRF. The scheme uses the vertical integration of forecasted cloud water content to transform control variables to the observation space, and creates the correlations between C_(w) and control variables in the flow-dependent background error covariance based on all the ensemble members, so that the observed cloud information can affect the background temperature and humidity. For two typhoons in 2018(Yagi and Rumiba), assimilating C_(w) significantly increases the simulated rainfalls and TC intensities. In terms of the average equitable threat score of daily moderate to heavy rainfall(5-120 mm), the improvements are over 130%, and the dry biases are cut by about 30%. Such improvements are traced down to the fact that C_(w) assimilation increases the moisture content, especially that further away from the TC center, which provides more precipitable water for the rainfall,strengthens the TC and broadens the TC size via latent heat release and internal wind field adjustment.

Effects of Doubled Carbon Dioxide on Rainfall Responses to Radiative Processes of Water Clouds

The effects of doubled carbon dioxide on rainfall responses to radiative processes of water clouds are investigated in this study.Two groups of two-dimensional cloud-resolving model sensitivity experiments with regard to pre-summer heavy rainfall around the summer solstice and tropical rainfall around the winter solstice are conducted and their five-day averages over the model domain are analyzed.In the presence of radiative effects of ice clouds,doubled carbon dioxide changes pre-summer rainfall from the decrease associated with the enhanced atmospheric cooling to the increase associated with the enhanced infrared cooling as a result of the exclusion of radiative effects of water clouds.Doubled carbon dioxide leads to the reduction in tropical rainfall,caused by the removal of radiative effects of water clouds through the suppressed infrared cooling.In the absence of radiative effects of ice clouds,doubled carbon dioxide changes pre-summer rainfall from the increase associated with the strengthened atmospheric warming to the decrease associated with the weakened release of latent heat caused by the elimination of radiative effects of water clouds.The exclusion of radiative effects of water clouds increases tropical rainfall through the strengthened infrared cooling,which is insensitive to the change in carbon dioxide.

Analysis of the Relationship between the Cloud Water Path and Precipitation Intensity of Mature Typhoons in the Northwest Pacific Ocean

The relationship between precipitation intensity and cloud water in typhoon systems remains unclear.This study combined time-and space-synchronized precipitation and spectral data obtained by the Precipitation Radar(PR)as well as the Visible and Infrared Scanner(VIRS)onboard the TRMM satellite,to overcome the limitations of precipitation properties and cloud parameters not being synchronized in previous studies.A merged dataset of near-surface rain rate(RR)and corresponding cloud water path(CWP)was established and used to analyze the potential correlation between cloud microphysical properties and precipitation,to deepen our understanding of the evolution of cloud to rain.In addition,25 collocated satellite overpasses of mature typhoon cases in the Northwest Pacific Ocean from 1998 to 2012 were obtained,and the relationships between the CWP and RR of 144515 pixels were analyzed in detail.The results show that the CWP and RR of mature typhoon systems with different precipitation types,precipitation cloud phases,and vertical depths of precipitation can be fitted by a notable sigmoid function,which may be useful for estimating CWP and parameterizing precipitation in models.Furthermore,the relationship was applied and tested with an independent sample to show that RR is a significant indicator of CWP.

Periodic Behavior of Cavitation Cloud Shedding in Submerged Water Jets Issuing from a Sheathed Pipe Nozzle

The behavior of cavitation cloud shedding in submerged water jets issuing from a sheathed pipe nozzle is investigated experimentally by high-speed camera visualization observation. Experiments are carried out under different cavitation numbers decreased to 0.01 with increase of the injection pressure, and the frequency spectrum of cavitation cloud shedding is evaluated by statistical analysis of a sequence of high-speed camera images. Experiments demonstrate that cavitation clouds appear when the cavitation number σ decreases to the level of 0.5-0.7 and developed cavitation clouds shed downstream periodically at multiple frequencies. The low frequency components of cavitation cloud shedding is basically dependent upon the pressure pulsation of plunger pump, which is often employed in various industry application of water jets. However, the high frequency components are closely related to the shedding of vortexes and the collapsing of cavitation clouds, which are dependent on the flow structure of submerged jets and the property of cavitation clouds consisted of numerous bubbles.

Effects of water and ice clouds on cloud microphysical budget:An equilibrium modeling study

The effects of water and ice clouds on the cloud microphysical budget associated with rainfall are investigated through the analysis of grid-scale data from a series of two-dimensional cloud-resolving model equilibrium sensitivity simulations. The model is imposed without large-scale vertical velocity. In the control experiment, the contribution from rainfall （cM） associated with net evaporation and hydrometeor loss/convergence is about 29% of that from the rainfall （Cm） associated with net condensation and hydrometeor gain/divergence and about 39% of that from the rainfall （CM） associated with net condensation and hydrometeor loss/convergence. The exclusion of ice clouds enhances rainfall contribution of CM, whereas it reduces rainfall contributions of Cm and cM. The removal of radiative effects of water clouds increases rainfall contribution of CM, barely changes rainfall contribution of Cm and reduces the rainfall contribution of cM in the presence of the radiative effects of ice clouds. Elimination of the radiative effects of water clouds reduces the rainfall contributions of CM and Cm, whereas it increases the rainfall contribution of cM in the absence of the radiative effects of ice clouds.

Temporal and spatial distribution characteristics of water resources in Guangdong Province based on a cloud model

With a focus on the difficulty of quantitatively describing the degree of nonuniformity of temporal and spatial distributions of water resources, quantitative research was carried out on the temporal and spatial distribution characteristics of water resources in Guangdong Province from 1956 to 2000 based on a cloud model. The spatial variation of the temporal distribution characteristics and the temporal variation of the spatial distribution characteristics were both analyzed. In addition, the relationships between the numerical characteristics of the cloud model of temporal and spatial distributions of water resources and precipitation were also studied. The results show that, using a cloud model, it is possible to intuitively describe the temporal and spatial distribution characteristics of water resources in cloud images. Water resources in Guangdong Province and their temporal and spatial distribution characteristics are differentiated by their geographic locations. Downstream and coastal areas have a larger amount of water resources with greater uniformity and stronger stability in terms of temporal distribution. Regions with more precipitation possess larger amounts of water resources, and years with more precipitation show greater nonuniformity in the spatial distribution of water resources. The correlation between the nonuniformity of the temporal distribution and local precipitation is small, and no correlation is found between the stability of the nonuniformity of the temporal and spatial distributions of water resources and precipitation. The amount of water resources in Guangdong Province shows an increasing trend from 1956 to 2000, the nonuniformity of the spatial distribution of water resources declines, and the stability of the nonuniformity of the spatial distribution of water resources is enhanced.

A Thin Cloud Removal Method from Remote Sensing Image for Water Body Identification

In this paper,a thin cloud removal method was put forward based on the linear relationships between the thin cloud reflectance in the channels from 0.4 μm to 1.0 μm and 1.38 μm.Channels of 0.66 μm,0.86 μm and 1.38 μm were chosen to extract the water body information under the thin cloud.Two study cases were selected to validate the thin cloud removal method.One case was applied with the Earth Observation System Moderate Resolution Imaging Spectroradiometer(EOS/MODIS) data,and the other with the Medium Resolution Spectral Imager(MERSI) and Visible and Infrared Radiometer(VIRR) data from Fengyun-3A(FY-3A).The test results showed that thin cloud removal method did not change the reflectivity of the ground surface under the clear sky.To the area contaminated by the thin cloud,the reflectance decreased to be closer to the reference reflectance under the clear sky after the thin cloud removal.The spatial distribution of the water body area could not be extracted before the thin cloud removal,while water information could be easily identified by using proper near infrared channel threshold after removing the thin cloud.The thin cloud removal method could improve the image quality and water body extraction precision effectively.

A Comparative Study of Cloud Liquid Water Content from Radiosonde Data at a Tropical Location

In this paper, some features of cloud liquid water content with respect to rain and water vapor are presented. Cloud liquid water density profile is obtained from radiosonde observation with Salonen's model and Karsten's model at Kolkata, a tropical location in the Indian region. Cloud liquid water contents (LWC) are obtained from these profiles which show a prominent seasonal variation. The monsoon months exhibit much higher values of LWC than in other months. However Salonen's model yields higher LWC values than that obtained with Karsten's model. The variation of daily total rainfall with LWC shows a positive relationship indicating the role of LWC in controlling the rainfall. Also the variation pattern of LWC with integrated water vapor (IWV) content of the atmosphere indicates that a threshold value of water vapor is required for cloud to form and once cloud is formed LWC increases with IWV.

基于Sentinel-1/2改进极化指数和纹理特征的土壤含盐量反演模型

目前Sentinel-1/2协同反演植被土壤含盐量的研究大多是基于Sentinel-2光谱信息和Sentinel-1后向散射系数,没有考虑Sentinel-2光谱信息容易受土壤亮度等信息影响,Sentinel-1后向散射系数容易受土壤粗糙度和水分影响。为进一步提高Sentinel-1/2协同反演植被土壤含盐量的精度,用水云模型对雷达卫星后向散射系数进行校正,消除植被影响;然后协同Sentinel-2纹理特征,基于VIP、OOB、PCA 3种变量筛选和RF、ELM、Cubist 3种机器学习回归模型构建植被土壤含盐量反演模型。研究结果表明:经过水云模型去除植被影响后的雷达后向散射系数及其极化组合指数与土壤含盐量的相关性有一定程度的提高。不同变量选择方法与不同机器学习方法耦合模型在反演土壤含盐量中,OOB变量筛选方法与RF、ELM和Cubist 3种机器学习方法的耦合模型精度最佳,建模集和验证集的R2都在0.750以上,且验证集的RMSE和MAE均最小;其中OOB-Cubist耦合模型精度最高,且R_(v)^(2)/R_(c)^(2)为0.955,具有良好的鲁棒性。研究可为机器学习协同物理模型、光学卫星协同雷达卫星在土壤含盐量反演中的进一步应用提供思路。

Cloud-point extraction and preconcentration of bisphenol A from water samples

A novel cloud-point extraction (CPE) was successfully used in preconcentration of biphenol A (BPA) from aqueous solutions. Majority of BPA is extracted into the surfactant-rich phase. The parameters affecting the CPE such as concentration of surfactant and electrolyte, equilibration temperature and time and pH of sample solution were investigated. The samples were analyzed by high-performance liquid chromatography with ultraviolet detection. Under the optimized conditions, preconcentration of 10 mL sample gives a preconcentration factor of 11. The limit of detection (LOD) and limit of quantification (LOQ) are 0.1 μg/L and 0.33 μg/L, respectively. The linear range of the proposed method is 0.2-20 μg/L with correlation coefficients greater than 0.998 7 and the spiking recoveries are 97.96%-100.42%. The interference factor was tested and the extraction mechanism was also investigated. Thus, the developed CPE has proven to be an efficient, green, rapid and inexpensive approach for extraction and preconcentration of BPA from water samples.

基于三维点云计算的CO_(2)-水-岩反应程度量化表征方法

CO_(2)地质封存是减少大气中CO_(2)排放,降低温室效应的重要途径,CO_(2)注入含水地层中时,CO_(2)-水-岩反应可能引起岩石矿物的侵蚀,对CO_(2)地质封存安全性产生显著影响。在室内实验中,通过表征岩石表面的形貌特征可以有效地评估CO_(2)-水-岩反应程度,为CO_(2)地质封存的安全性评估提供科学依据。通过三维点云计算可以精确量化地表征CO_(2)-水-岩反应程度,这种方法首先运用三维激光扫描技术,构建岩石表面的三维模型,确定CO_(2)-水处理前岩石表面三维模型的基准面,并基于处理前的均方根粗糙度确定处理后岩石表面三维模型的基准面。基于三维模型点云信息,提出了两种不同的体积计算新方法,并通过对规则模型体积的计算比较了两种计算方法的准确性与适用性,可根据实际情况选择两种计算方法量化表征CO_(2)-水处理前后岩石表面的侵蚀体积。最后,以陕西省咸阳市某煤矿煤样为例,开展了CO_(2)-水-岩反应模拟试验,验证了计算的可行性。试验结果表明:该文提出的侵蚀体积计算方法可有效地量化表征CO_(2)-水-岩反应程度,CO_(2)-水处理后岩石表面不同区域的侵蚀差异性明显,岩石表面的侵蚀体积与均方根粗糙度之间存在显著的正比关系,随着均方根粗糙度的增大,侵蚀体积也相应上升。

东亚地区云微物理量分布特征的CloudSat卫星观测研究

本文利用2007～2010年整四年最新可利用的CloudSat卫星资料,对东亚地区（15°～60°N,70°～150°E）云的微物理量包括冰/液态水含量、冰/液态水路径、云滴数浓度和有效半径等的分布特征和季节变化进行了分析.本文将整个东亚地区划分为北方、南方、西北、青藏高原地区和东部海域五个子区域进行研究,结果显示：东亚地区冰水路径值的范围基本在700 g m-2以下,高值区分布在北纬40度以南区域,在南方地区夏季的平均值最大,为394.3 g m-2,而在西北地区冬季的平均值最小,为78.5 g m-2;而液态水路径的范围基本在600 g m-2以下,冬季在东部海域的值最大,达到300.8 g m-2,夏季最大值为281.5 g m-2,分布在南方地区上空.冰水含量的最高值为170 mg m-3,发生在8km附近,南方地区夏季的值达到最大,青藏高原地区的季节差异最大;而液态水含量在东亚地区的范围小于360 mg m-3,垂直廓线从10km向下基本呈现逐渐增大的趋势,峰值位于1～2 km高度上.冰云云滴数浓度在东亚地区的范围在150 L-1以下,水云云滴数浓度的值小于80 cm-3,垂直廓线的峰值均在夏季最大.冰云有效半径在东亚地区的最大值为90 μm,发生在5km左右;水云有效半径在东亚地区的值分布在10km以下,最大值为10～12 μm,基本位于1～2 km高度上.从概率分布函数来看,东亚地区冰/水云云滴数浓度的分布呈现明显的双峰型,其他量基本为单峰型.本文的结果可以为全球和区域气候模式在东亚地区对以上云微物理量的模拟提供一定的观测参考依据.

青藏高原东侧九龙夏季非降水云的观测特征

青藏高原东侧九龙地区是西南涡多发区,利用该地区新型探测设备开展云探测,有助于增强对西南涡多发区云特征的认识。利用2018—2019年6—8月九龙站地基微波辐射计资料,分析了该地区夏季非降水云的出现率、液态水路径及过冷水路径的观测特征。结果表明:九龙夏季非降水云出现率月均值在67%~82%之间,以低云和中云为主,高云较少;低云出现率表现为白天低、夜间高,而中云和高云则相反;云出现率的垂直分布表现为单峰形态,在约2km高度存在云出现率峰值8.1%;受大气热力层结日变化影响,云出现率的单峰垂直分布呈现日夜差异。另外,九龙夏季非降水云的液态水路径均值为0.433kg·m^(-2),其中低云、中云、高云的液态水路径均值分别为0.665、0.240、0.102kg·m^(-2);低云的液态水路径日变化特征与其出现率相似,而中云和高云的液态水路径日变化特征不明显。此外,九龙夏季非降水云中冷云的过冷水路径均值为0.154kg·m^(-2),其中低云、中云、高云的过冷水路径均值分别为0.065、0.166、0.102kg·m^(-2);总体上过冷水路径在液态水路径中的占比约为34.3%~38.8%,过冷水路径占比随云的高度而增大,这使得中云和高云的过冷水路径日变化与其液态水路径相似。与同纬度华中地区相比,九龙夏季非降水云具有明显不同的特征,这与两地之间的大气水汽特征差异密切相关。

基于CloudSat卫星资料分析青藏高原东部夏季云的垂直结构

本文利用CloudSat卫星资料,对青藏高原东部2006-2010年6-8月云垂直结构的空间分布进行分析,结果表明：（1）夏季青藏高原东部云发展可达到平流层,且高原东部云在5km以下以水云存在,5-10km以液相和固相共存的混态存在,在垂直高度10km以上以冰云存在。由于CloudSat卫星资料云相的反演问题,可能会造成水云和混态云的发展上限偏低,冰云的发展下限抬升。（2）研究区整层水汽输送和云水平均路径空间分布存在一定的差异性,云水含量纬向分布表现为在26.5°-30.5°N附近存在一个明显的峰值区,经向分布表现为95°E以西云水含量低于以东。（3）研究区以单云层为主,尤其在青藏高原主体。单云层平均云层厚度4182 m,云顶高度、云厚限于水汽的输送,表现为由南向北波动下降。多层云发生频率在27°N以北明显减少,说明强烈的对流运动更容易激发多层云的产生。