The combined effect of periodic water impoundment and seasonal natural flood events has created a 30 m high water-level fluctuation zone(WLFZ) around the Three Gorges Reservoir(TGR), China, forming a unique eco-landsc...The combined effect of periodic water impoundment and seasonal natural flood events has created a 30 m high water-level fluctuation zone(WLFZ) around the Three Gorges Reservoir(TGR), China, forming a unique eco-landscape. Siltation, eutrophication, enrichment of heavy metals, and methane emissions in the WLFZ have been widely associated with sediment and soil particles generated from the upstream catchment or upland slopes. However, little attention has been paid to the complexity of sediment particle-size distributions in the WLFZ. In the present study, core samples(from a 345 cm thick sediment core from the base of the WLFZ), slope transect surface samples(across/up a WLFZ slope), and along-river/longitudinal surface samples(from the reservoir reaches) were collected. Laser granulometry and a volume-based fractal model were used to reveal the characteristics of sediment particle-size distributions. Results indicate that the alternation of coarse and fine particles in the sedimentary core profile is represented as a fluctuation of low and high values of fractal dimension(D), ranging from 2.59 to 2.77. On the WLFZ slope transect, surface sediment particles coarsen with increasing elevation, sand content increases from 3.3% to 78.5%, and D decreases from 2.76 to 2.53. Longitudinally, surface sediments demonstrate a downstream-fining trend, and D increases gradually downstream. D is significantly positively correlated with the fine particle content. We conclude that D is a useful measure for evaluating sediment particle-size distribution.展开更多
Surface soil/sediment samples were collected from the Water-Level Fluctuation Zone(WLFZ), cultivated land and forest land at 50 different grid points from Shenjia watershed, the Three Gorges Reservoir area in August 2...Surface soil/sediment samples were collected from the Water-Level Fluctuation Zone(WLFZ), cultivated land and forest land at 50 different grid points from Shenjia watershed, the Three Gorges Reservoir area in August 2013. The spatial distribution, sources and ecological risk assessment for Arsenic(As), Cadmium(Cd),Chromium(Cr), Copper(Cu), Nickel(Ni), Lead(Pb)and Zinc(Zn) were analyzed in this study. The results showed all tested metals had similar distribution patterns except Ni and Cr, with areas of high concentrations distributed in the southwest(WLFZ and watershed outlet) of the study area. Ni and Cr,which were highly positively correlated and present in high concentrations, were primarily distributed in the south and middle zones of the study area. Lower concentration areas of all metals were uniformly distributed west of the high-elevation zones and forest land. Factor analysis(FA) and factor analysismultiple linear regression(FA-MLR) showed that the major sources of Cd were fertilizer and traffic sources,which together accounted for 87% of Cd. As, Zn and Cu levels were primarily supplied by industrial and domestic sources, accounting for 76% of As, 75% of Cu and 67% of Zn. Surface soils/sediments of the study watershed contaminated by Cd represent a high ecological risk, whereas other metals represent low ecological risks. The potential ecological risk index(PERI) analysis indicated that it had a low(widerange) ecological risk and a moderate(small-range)ecological risk primarily distributed in the outlet of the study watershed. Fertilizers and traffic are the primary sources of Cd pollution, which should be more closely controlled for the purposes of water quality and ecological conservation.展开更多
Ruxi River is a tributary of the Three Gorges Reservoir. This study examined the temporal and spatial dynamics in particle size characteristics and the associated nutrients and contaminants of the fluvial suspended an...Ruxi River is a tributary of the Three Gorges Reservoir. This study examined the temporal and spatial dynamics in particle size characteristics and the associated nutrients and contaminants of the fluvial suspended and deposited sediments along the Ruxi River. Temporal variations in the particle size distribution of the suspended sediment are controlled mainly by differences in sediment source during different seasons. Total organic carbon (TOC), total nitrogen (TN) and total phosphorous (TP) in the 〈 62 μm fraction of the suspended sediment exhibit considerably higher concentrations in spring, indicating high probability of algal blooms in the backwater areas. Downstream trends in the nutrient contents of 〈 62 pm deposited sediments imply the greatest potential for eutrophication in the backwater ends, where highest nutrient concentrations were detected. Assessment of metal contamination shows that the sediments deposited in the water-level fluctuation zone were moderately to strongly contaminated by Cadmium (Cd), with a considerably high potential ecological risk. The findings reported have emphasized the impacts of reservoir impoundment on aquatic and/or terrestrial environment in this region. More information on physical, chemical and biological processes of sediment and sediment-associated materials are needed for developing ecologically sound policies management. environmentally and of water and sediment展开更多
The water-level fluctuation zone(WLFZ) has been considered as a hotspot for mercury(Hg) methylation. Flooding-tolerant herbs are gradually acclimated to this water-land ecotone, tending to form substantial root system...The water-level fluctuation zone(WLFZ) has been considered as a hotspot for mercury(Hg) methylation. Flooding-tolerant herbs are gradually acclimated to this water-land ecotone, tending to form substantial root systems for improving erosion resistance. Accompanying rhizosphere microzone plays crucial but unclear roles in methylmercury(Me Hg) formation in the WLFZ. Thus, we conducted this study in the WLFZ of the Three Gorges Reservoir, to explore effects of the rhizosphere of a dominant flooding-tolerant herb(bermudagrass) on Me Hg production. The elevated Hg and Me Hg in rhizosphere soils suggest that the rhizosphere environment provides favorable conditions for Hg accumulation and methylation. The increased bioavailable Hg and microbial activity in the rhizosphere probably serve as important factors driving Me Hg formation in the presence of bermudagrass. Simultaneously, the rhizosphere environments changed the richness, diversity, and distribution of hgc A-containing microorganisms. Here, a typical ironreducing bacterium( Geobacteraceae) has been screened, however, the majority of hgc A genes detected in rhizosphere, near-, and non-rhizosphere soils of the WLFZ were unclassified. Collectively, these results provide new insights into the elevated Me Hg production as related to microbial processes in the rhizosphere of perennial herbs in the WLFZ, with general implications for Hg cycling in other ecosystems with water-level fluctuations.展开更多
基金funded by the National Natural Science Foundation of China (Grant nos. 41771320, 41771321, and 41571278)the Opening Project of Chongqing Key Laboratory of Earth Surface Processes and Environmental Remote Sensing in the Three Gorges Reservoir Area (Grant no. DBGC201801)the Sichuan Science and Technology Program (Grant no. 2018SZ0132)
文摘The combined effect of periodic water impoundment and seasonal natural flood events has created a 30 m high water-level fluctuation zone(WLFZ) around the Three Gorges Reservoir(TGR), China, forming a unique eco-landscape. Siltation, eutrophication, enrichment of heavy metals, and methane emissions in the WLFZ have been widely associated with sediment and soil particles generated from the upstream catchment or upland slopes. However, little attention has been paid to the complexity of sediment particle-size distributions in the WLFZ. In the present study, core samples(from a 345 cm thick sediment core from the base of the WLFZ), slope transect surface samples(across/up a WLFZ slope), and along-river/longitudinal surface samples(from the reservoir reaches) were collected. Laser granulometry and a volume-based fractal model were used to reveal the characteristics of sediment particle-size distributions. Results indicate that the alternation of coarse and fine particles in the sedimentary core profile is represented as a fluctuation of low and high values of fractal dimension(D), ranging from 2.59 to 2.77. On the WLFZ slope transect, surface sediment particles coarsen with increasing elevation, sand content increases from 3.3% to 78.5%, and D decreases from 2.76 to 2.53. Longitudinally, surface sediments demonstrate a downstream-fining trend, and D increases gradually downstream. D is significantly positively correlated with the fine particle content. We conclude that D is a useful measure for evaluating sediment particle-size distribution.
基金Financial support for this study was jointly provided by the National Natural Science Foundation of China(Grant No.41430750)National Key Basic Research Program of China(Grant Nos.2015CB452704,2016YFC0402301)the Chinese Academy of Sciences(Grant Nos.KFJ-EW-STS-008,KFJSW-STS-175)
文摘Surface soil/sediment samples were collected from the Water-Level Fluctuation Zone(WLFZ), cultivated land and forest land at 50 different grid points from Shenjia watershed, the Three Gorges Reservoir area in August 2013. The spatial distribution, sources and ecological risk assessment for Arsenic(As), Cadmium(Cd),Chromium(Cr), Copper(Cu), Nickel(Ni), Lead(Pb)and Zinc(Zn) were analyzed in this study. The results showed all tested metals had similar distribution patterns except Ni and Cr, with areas of high concentrations distributed in the southwest(WLFZ and watershed outlet) of the study area. Ni and Cr,which were highly positively correlated and present in high concentrations, were primarily distributed in the south and middle zones of the study area. Lower concentration areas of all metals were uniformly distributed west of the high-elevation zones and forest land. Factor analysis(FA) and factor analysismultiple linear regression(FA-MLR) showed that the major sources of Cd were fertilizer and traffic sources,which together accounted for 87% of Cd. As, Zn and Cu levels were primarily supplied by industrial and domestic sources, accounting for 76% of As, 75% of Cu and 67% of Zn. Surface soils/sediments of the study watershed contaminated by Cd represent a high ecological risk, whereas other metals represent low ecological risks. The potential ecological risk index(PERI) analysis indicated that it had a low(widerange) ecological risk and a moderate(small-range)ecological risk primarily distributed in the outlet of the study watershed. Fertilizers and traffic are the primary sources of Cd pollution, which should be more closely controlled for the purposes of water quality and ecological conservation.
基金financially supported by the National Natural Science Foundation of China (41430750, 41301293)the National Key R&D Program of China (2017YFD0800505, 2016YFC0402301)
文摘Ruxi River is a tributary of the Three Gorges Reservoir. This study examined the temporal and spatial dynamics in particle size characteristics and the associated nutrients and contaminants of the fluvial suspended and deposited sediments along the Ruxi River. Temporal variations in the particle size distribution of the suspended sediment are controlled mainly by differences in sediment source during different seasons. Total organic carbon (TOC), total nitrogen (TN) and total phosphorous (TP) in the 〈 62 μm fraction of the suspended sediment exhibit considerably higher concentrations in spring, indicating high probability of algal blooms in the backwater areas. Downstream trends in the nutrient contents of 〈 62 pm deposited sediments imply the greatest potential for eutrophication in the backwater ends, where highest nutrient concentrations were detected. Assessment of metal contamination shows that the sediments deposited in the water-level fluctuation zone were moderately to strongly contaminated by Cadmium (Cd), with a considerably high potential ecological risk. The findings reported have emphasized the impacts of reservoir impoundment on aquatic and/or terrestrial environment in this region. More information on physical, chemical and biological processes of sediment and sediment-associated materials are needed for developing ecologically sound policies management. environmentally and of water and sediment
基金the funding support from the National Natural Science Foundation of China (No. 41877384 )the Fundamental Research Funds for the Central Universities (No. XDJK2017B035 )Chongqing Graduate Scientific Research Innovation Project (No. CYS21112 ) for its support。
文摘The water-level fluctuation zone(WLFZ) has been considered as a hotspot for mercury(Hg) methylation. Flooding-tolerant herbs are gradually acclimated to this water-land ecotone, tending to form substantial root systems for improving erosion resistance. Accompanying rhizosphere microzone plays crucial but unclear roles in methylmercury(Me Hg) formation in the WLFZ. Thus, we conducted this study in the WLFZ of the Three Gorges Reservoir, to explore effects of the rhizosphere of a dominant flooding-tolerant herb(bermudagrass) on Me Hg production. The elevated Hg and Me Hg in rhizosphere soils suggest that the rhizosphere environment provides favorable conditions for Hg accumulation and methylation. The increased bioavailable Hg and microbial activity in the rhizosphere probably serve as important factors driving Me Hg formation in the presence of bermudagrass. Simultaneously, the rhizosphere environments changed the richness, diversity, and distribution of hgc A-containing microorganisms. Here, a typical ironreducing bacterium( Geobacteraceae) has been screened, however, the majority of hgc A genes detected in rhizosphere, near-, and non-rhizosphere soils of the WLFZ were unclassified. Collectively, these results provide new insights into the elevated Me Hg production as related to microbial processes in the rhizosphere of perennial herbs in the WLFZ, with general implications for Hg cycling in other ecosystems with water-level fluctuations.