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马克思主义不是“科学”吗?——一个“证伪主义”的维度 被引量:6
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作者 赵磊 《当代经济研究》 CSSCI 北大核心 2011年第2期32-38,共7页
波普尔的"证伪主义",是学界指认马克思主义"非科学"的重要方法论依据。然而不论"证伪主义"是否被误读,要把马克思主义逐出"科学"殿堂,决非易事。其中的难度,并不在于"证伪者"所使用... 波普尔的"证伪主义",是学界指认马克思主义"非科学"的重要方法论依据。然而不论"证伪主义"是否被误读,要把马克思主义逐出"科学"殿堂,决非易事。其中的难度,并不在于"证伪者"所使用的方法不够"现代",也不在于"证伪主义"不够"科学",而是在于那些"证伪"马克思主义科学性的人,对基本逻辑和常识缺乏起码的尊重。企图利用"科学划界"的霸权,取消马克思主义被验证的起码资格,甚至把马克思主义打入"伪科学"行列的观点,未免太狭隘了;我们欢迎对马克思主义的合理批评和质疑,但也应当对意识形态偏见保持清醒认识。 展开更多
关键词 马克思主义 科学划界 证伪主义 波普尔 语言逻辑
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Effect of substrate temperature and oxygen plasma treatment on the properties of magnetron-sputtered CdS for solar cell applications
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作者 Runxuan Zang Haolin Wang +9 位作者 Xiaoqi Peng Ke Li Yuehao Gu Yizhe Dong Zhihao Yan Zhiyuan Cai Huihui Gao Shuwei Sheng Rongfeng Tang Tao Chen 《中国科学技术大学学报》 CAS CSCD 北大核心 2024年第6期22-33,I0010,共13页
Cadmium sulfide(CdS)is an n-type semiconductor with excellent electrical conductivity that is widely used as an electron transport material(ETM)in solar cells.At present,numerous methods for preparing CdS thin films h... Cadmium sulfide(CdS)is an n-type semiconductor with excellent electrical conductivity that is widely used as an electron transport material(ETM)in solar cells.At present,numerous methods for preparing CdS thin films have emerged,among which magnetron sputtering(MS)is one of the most commonly used vacuum techniques.For this type of technique,the substrate temperature is one of the key deposition parameters that affects the interfacial properties between the target film and substrate,determining the specific growth habits of the films.Herein,the effect of substrate temperature on the microstructure and electrical properties of magnetron-sputtered CdS(MS-CdS)films was studied and applied for the first time in hydrothermally deposited antimony selenosulfide(Sb_(2)(S,Se)_(3))solar cells.Adjusting the substrate temperature not only results in the design of the flat and dense film with enhanced crystallinity but also leads to the formation of an energy level arrangement with a Sb_(2)(S,Se)_(3)layer that is more favorable for electron transfer.In addition,we developed an oxygen plasma treatment for CdS,reducing the parasitic absorption of the device and resulting in an increase in the short-circuit current density of the solar cell.This study demonstrates the feasibility of MS-CdS in the fabrication of hydrothermal Sb_(2)(S,Se)_(3)solar cells and provides interface optimization strategies to improve device performance. 展开更多
关键词 magnetron sputtering CDS substrate heating plasma treatment Sb_(2)(S Se)_(3) thin film solar cell
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Engineering The Neck Hinge Reshapes The Processive Movement of Kinesin-3
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作者 LI Dong REN Jin-Qi +2 位作者 SONG Yin-Long LIANG Xin FENG Wei 《生物化学与生物物理进展》 SCIE CAS CSCD 北大核心 2024年第10期2730-2740,共11页
Objective In kinesin-3,the neck coil correlates with the following segments to form an extended neck that contains a characteristic hinge diverse from a proline in KIF13B to a long flexible linker in KIF1A.The functio... Objective In kinesin-3,the neck coil correlates with the following segments to form an extended neck that contains a characteristic hinge diverse from a proline in KIF13B to a long flexible linker in KIF1A.The function of this neck hinge for controlling processive movement,however,remains unclear.Methods We made a series of modifications to the neck hinges of KIF13B and KIF1A and tested their movement using a single-molecule motility assay.Results In KIF13B,the insertion of flexible residues before or after the proline differentially impacts the processivity or velocity,while the removal of this proline increases the both.In KIF1A,the deletion of entire flexible neck hinge merely enhances the processivity.The engineering of these hinge-truncated necks of kinesin-3 into kinesin-1 similarly boosts the processive movement of kinesin-1.Conclusion The neck hinge in kinesin-3 controls its processive movement and proper modifications tune the motor motility,which provides a novel strategy to reshape the processive movement of kinesin motors. 展开更多
关键词 intracellular transport molecular motor kinesin-3 neck hinge processive movement
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Charge-balanced codoping enables exceeding doping limit and ultralow thermal conductivity
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作者 Long Chen Chun Wang +3 位作者 Lin Wang Minghao Wang Yongchun Zhu Changzheng Wu 《中国科学技术大学学报》 CAS CSCD 北大核心 2024年第6期1-7,I0009,共8页
Materials with low thermal conductivity are applied extensively in energy management,and breaking the amorphous limits of thermal conductivity to solids has attracted widespread attention from scientists.Doping is a c... Materials with low thermal conductivity are applied extensively in energy management,and breaking the amorphous limits of thermal conductivity to solids has attracted widespread attention from scientists.Doping is a common strategy for achieving low thermal conductivity that can offer abundant scattering centers in which heavier dopants always result in lower phonon group velocities and lower thermal conductivities.However,the amount of equivalent heavyatom single dopant available is limited.Unfortunately,nonequivalent heavy dopants have finite solubility because of charge imbalance.Here,we propose a charge balance strategy for SnS by substituting Sn2+with Ag^(+)and heavy Bi^(3+),improving the doping limit of Ag from 2%to 3%.Ag and Bi codoping increases the point defect concentration and introduces abundant boundaries simultaneously,scattering the phonons at both the atomic scale and nanoscale.The thermal conductivity of Ag0.03Bi0.03Sn0.94S decreased to 0.535 W·m^(−1)·K^(−1)at room temperature and 0.388 W·m^(−1)·K^(−1)at 275°C,which is below the amorphous limit of 0.450 W·m^(−1)·K^(−1)for SnS.This strategy offers a simple way to enhance the doping limit and achieve ultralow thermal conductivity in solids below the amorphous limit without precise structural modification. 展开更多
关键词 charge-balanced codoping heavy atom point defect grain boundary ultralow thermal conductivity
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Boehmeria nivea var. strigosa (Urticaceae), a new variety from Southwest China
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作者 ZHAO Ying Richard I.MILNE +2 位作者 LI Zhipeng Amos KIPKOECH WU Zengyuan 《广西植物》 CAS CSCD 北大核心 2024年第9期1617-1624,I0001-I0006,共14页
Boehmeria nivea var.strigosa Zeng Y.Wu&Y.Zhao,a new variety of B.nivea(Urticaceae)from Southwest China,is here described based on evidence from morphology and molecular phylogeny.This new variety is mainly charact... Boehmeria nivea var.strigosa Zeng Y.Wu&Y.Zhao,a new variety of B.nivea(Urticaceae)from Southwest China,is here described based on evidence from morphology and molecular phylogeny.This new variety is mainly characterized by its green abaxial leaf blade,partly connate stipules,and densely patent strigose hairs on stems and potioles.The phylogenetic analysis based on rbc L,nrDNA and rbc L+nrDNA datasets,revealed that all individuals of B.nivea var.strigosa formed a monophyletic group.The conservation status of B.nivea var.strigosa is assessed as“Near Threatened”(NT)according to IUCN evaluation criteria.The discovery of this new variety is not only crucial for the taxonomy of ramie,but also provides reference for the exploration and utilization of ramie. 展开更多
关键词 Boehmeria nivea MORPHOLOGY molecular phylogeny new variety Southwest China YUNNAN
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On joint analysing XMM-NuSTAR spectra of active galactic nuclei
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作者 Jialai Kang Junxian Wang 《中国科学技术大学学报》 CAS CSCD 北大核心 2024年第7期19-33,18,I0002,共17页
A recently released XMM-Newton note revealed a significant calibration issue between nuclear spectroscopic telescope array(NuSTAR)and XMM-Newton European Photon Imaging Camera(EPIC)and provided an empirical correction... A recently released XMM-Newton note revealed a significant calibration issue between nuclear spectroscopic telescope array(NuSTAR)and XMM-Newton European Photon Imaging Camera(EPIC)and provided an empirical correction to the EPIC effective area.To quantify the bias caused by the calibration issue in the joint analysis of XMM-NuSTAR spectra and verify the effectiveness of the correction,in this work,we perform joint-fitting of the NuSTAR and EPIC-pn spectra for a large sample of 104 observation pairs of 44 X-ray bright active galactic nuclei(AGN).The spectra were extracted after requiring perfect simultaneity between the XMM-Newton and NuSTAR exposures(merging good time intervals(GTIs)from two missions)to avoid bias due to the rapid spectral variability of the AGN.Before the correction,the EPIC-pn spectra are systematically harder than the corresponding NuSTAR spectra by■subsequently yielding significantly underestimated cutoff energy E_(cut)and the strength of reflection component R when performing joint-fitting.We confirm that the correction is highly effective and can commendably erase the discrepancy in best-fitΓ,E_(cut),and R.We thus urge the community to apply the correction when joint-fitting XMM-NuSTAR spectra,but note that the correction is limited to 3–12 keV and therefore not applicable when the soft X-ray band data are included.Besides,we show that as merging GTIs from two missions would cause severe loss of NuSTAR net exposure time,in many cases,joint-fitting yields no advantage compared with utilizing NuSTAR data alone.Finally,We present a technical note on filtering periods of high background flares for XMM-Newton EPIC-pn exposures in the small window(SW)mode. 展开更多
关键词 active galactic nuclei X-ray spectroscopy XMM-NEWTON NuSTAR cross-calibration issue
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Ecological environmental quality evaluation and driving factor analysis of the Lijiang River Basin,based on Google Earth Engine
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作者 WEI Xi YANG Dazhi +2 位作者 CAI Xiangwen SHAO Ya TANG Xiangling 《中国生态农业学报(中英文)》 CAS CSCD 北大核心 2024年第9期1592-1608,共17页
For regional ecological management,it is important to evaluate the quality of ecosystems and analyze the underlying causes of ecological changes.Using the Google Earth Engine(GEE)platform,the remote sensing ecological... For regional ecological management,it is important to evaluate the quality of ecosystems and analyze the underlying causes of ecological changes.Using the Google Earth Engine(GEE)platform,the remote sensing ecological index(RSEI)was calculated for the Lijiang River Basin in Guangxi Zhuang Autonomous Region for 1991,2001,2011,and 2021.Spatial autocorrelation analysis was employed to investigate spatiotemporal variations in the ecological environmental quality of the Lijiang River Basin.Furthermore,geographic detectors were used to quantitatively analyze influencing factors and their interaction effects on ecological environmental quality.The results verified that:1)From 1991 to 2021,the ecological environmental quality of the Lijiang River Basin demonstrated significant improvement.The area with good and excellent ecological environmental quality in proportion increased by 19.69%(3406.57 km^(2)),while the area with fair and poor ecological environmental quality in proportion decreased by 10.76%(1860.36 km^(2)).2)Spatially,the ecological environmental quality of the Lijiang River Basin exhibited a pattern of low quality in the central region and high quality in the periphery.Specifically,poor ecological environmental quality characterized the Guilin urban area,Pingle County,and Lingchuan County.3)From 1991 to 2021,a significant positive spatial correlation was observed in ecological environmental quality of the Lijiang River Basin.Areas with high-high agglomeration were predominantly forests and grasslands,indicating good ecological environmental quality,whereas areas with low-low agglomeration were dominated by cultivated land and construction land,indicating poor ecological environmental quality.4)Annual average precipitation and temperature exerted the most significant influence on the ecological environmental quality of the basin,and their interactions with other factors had the great influence.This study aimed to enhance understanding of the evolution of the ecological environment in the Lijiang River Basin of Guangxi Zhuang Autonomous Region and provide scientific guidance for decision-making and management related to ecology in the region. 展开更多
关键词 Ecological environmental quality Remote sensing ecological index Driving factor Google Earth Engine Lijiang River Basin
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Discovery of a geomorphological analog to Martian araneiforms in the Qaidam Basin, Tibetan Plateau
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作者 Shengxing Zhang Yiliang Li Wei Leng 《中国科学技术大学学报》 CAS CSCD 北大核心 2024年第5期1-9,I0006,共10页
Araneiforms are spider-like ground patterns that are widespread in the southern polar regions of Mars.A gas erosion process driven by the seasonal sublimation of CO_(2) ice was proposed as an explanation for their for... Araneiforms are spider-like ground patterns that are widespread in the southern polar regions of Mars.A gas erosion process driven by the seasonal sublimation of CO_(2) ice was proposed as an explanation for their formation,which cannot occur on Earth due to the high climatic temperature.In this study,we propose an alternative mechanism that attrib-utes the araneiform formation to the erosion of upwelling salt water from the subsurface,relying on the identification of the first terrestrial analog found in a playa of the Qaidam Basin on the northern Tibetan Plateau.Morphological analysis indicates that the structures in the Qaidam Basin have fractal features comparable to araneiforms on Mars.A numerical model is developed to investigate the araneiform formation driven by the water-diffusion mechanism.The simulation res-ults indicate that the water-diffusion process,under varying ground conditions,may be responsible for the diverse aranei-form morphologies observed on both Earth and Mars.Our numerical simulations also demonstrate that the orientations of the saltwater diffusion networks are controlled by pre-existing polygonal cracks,which is consistent with observations of araneiforms on Mars and Earth.Our study thus suggests that a saltwater-related origin of the araneiform is possible and has significant implications for water searches on Mars. 展开更多
关键词 araneiform landform subsurface water Qaidam Basin Mars analog fractal simulations
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A review of the catalytic preparation of mesophase pitch
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作者 MA Zi-hui YANG Tao +7 位作者 SONG Yan CHEN Wen-sheng DUAN Chun-feng SONG Huai-he TIAN Xiao-dong GONG Xiang-jie LIU Zheng-yang LIU Zhan-jun 《新型炭材料(中英文)》 SCIE EI CAS CSCD 北大核心 2024年第4期583-610,共28页
Because of its high purity and excellent orientation, mesophase pitch is a superior precursor for high-performance car-bon materials. However, the preparation of top-notch mesophase pitch faces challenges. Catalytic p... Because of its high purity and excellent orientation, mesophase pitch is a superior precursor for high-performance car-bon materials. However, the preparation of top-notch mesophase pitch faces challenges. Catalytic polycondensation at low temperat-ures is more favorable for synthesizing mesophase pitch, because it circumvents the high-temperature free radical reaction of other thermal polycondensation approaches. The reaction is gentle and can be easily controlled. It has the potential to significantly im-prove the yield of mesophase pitch and easily introduce naphthenic characteristics into the molecules, catalytic polycondensation is therefore a preferred method of synthesizing highly spinnable mesophase pitch. This review provides a synopsis of the selective pre-treatment of the raw materials to prepare different mesophase pitches, and explains the reaction mechanism and associated research advances for different catalytic systems in recent years. Finally, how to manufacture high-quality mesophase pitch by using a cata-lyst-promoter system is summarized and proposed, which may provide a theoretical basis for the future design of high-quality pitch molecules. 展开更多
关键词 Mesophase pitch Catalytic polycondensation LEWIS-ACID Brønsted acid Catalyst-promoter system
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Effect of sintering temperature and holding time on structure and properties of Li_(1.5)Ga_(0.5)Ti_(1.5)(PO_4)_(3)electrolyte with fast ionic conductivity
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作者 Yin-yi LUO Hao-zhang LIANG +6 位作者 Ping ZHANG Lei HAN Qian ZHANG Li-dan LIU Zhi-wei LUO Tian-xiang NING An-xian LU 《Transactions of Nonferrous Metals Society of China》 SCIE EI CAS CSCD 2024年第9期2959-2971,共13页
Li1.5Ga0.5Ti1.5(PO4)3(LGTP)is recognized as a promising solid electrolyte material for lithium ions.In this work,LGTP solid electrolyte materials were prepared under different process conditions to explore the effects... Li1.5Ga0.5Ti1.5(PO4)3(LGTP)is recognized as a promising solid electrolyte material for lithium ions.In this work,LGTP solid electrolyte materials were prepared under different process conditions to explore the effects of sintering temperature and holding time on relative density,phase composition,microstructure,bulk conductivity,and total conductivity.In the impedance test under frequency of 1-10~6 Hz,the bulk conductivity of the samples increased with increasing sintering temperature,and the total conductivity first increased and then decreased.SEM results showed that the average grain size in the ceramics was controlled by the sintering temperature,which increased from(0.54±0.01)μm to(1.21±0.01)μm when the temperature changed from 750 to 950°C.The relative density of the ceramics increased and then decreased with increasing temperature as the porosity increased.The holding time had little effect on the grain size growth or sample density,but an extended holding time resulted in crack generation that served to reduce the conductivity of the solid electrolyte. 展开更多
关键词 sintering temperature holding time CONDUCTIVITY cracks solid-state electrolyte
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3D seismic forward modeling from the multiphysical inversion at the Ketzin CO_(2) storage site
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作者 Yi-kang Zheng Chong Wang +2 位作者 Hao-hong Liang Yi-bo Wang Rong-shu Zeng 《Applied Geophysics》 SCIE CSCD 2024年第3期593-605,620,共14页
From June 2008 to August 2013,approximately 67 kt of CO_(2) was injected into a deep saline formation at the Ketzin pilot CO_(2) storage site.During injection,3D seismic surveys have been performed to monitor the migr... From June 2008 to August 2013,approximately 67 kt of CO_(2) was injected into a deep saline formation at the Ketzin pilot CO_(2) storage site.During injection,3D seismic surveys have been performed to monitor the migration of sequestered CO_(2).Seismic monitoring results are limited by the acquisition and signal-to-noise ratio of the acquired data.The multiphysical reservoir simulation provides information regarding the CO_(2) fluid behavior,and the approximated model should be calibrated with the monitoring results.In this work,property models are delivered from the multiphysical model during 3D repeated seismic surveys.The simulated seismic data based on the models are compared with the real data,and the results validate the effectiveness of the multiphysical inversion method.Time-lapse analysis shows the trend of CO_(2) migration during and after injection. 展开更多
关键词 Seismic forward modeling reservoir simulation CO_(2)storage time-lapse analysis
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Optical-neural Stimulation in Non-human Primates:Modulating Brain Function and Behavior
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作者 CHEN Yi-Bing WANG Huan YANG Yan 《生物化学与生物物理进展》 SCIE CAS CSCD 北大核心 2024年第10期2379-2391,共13页
Optical-neural stimulation,which encompasses cutting-edge techniques such as optogenetics and infrared neurostimulation,employs distinct mechanisms to modulate brain function and behavior.These advanced neuromodulatio... Optical-neural stimulation,which encompasses cutting-edge techniques such as optogenetics and infrared neurostimulation,employs distinct mechanisms to modulate brain function and behavior.These advanced neuromodulation techniques offer accurate manipulation of targeted areas,even selectively modulating specific neurons,in the brain.This makes it possible to investigate the cause-and-effect connections between neural activity and behavior,allowing for a better comprehension of the intricate brain dynamics towards complex environments.Non-human primates serve as an essential animal model for investigating these complex functions in brain research,bridging the gap between the basic research and clinical applications.One of the earliest optical studies utilizing optogenetic neuromodulation in monkeys was conducted in 2009.Since then,the optical-neural stimulations have been effectively applied in non-human primates.This review summarises recent research that employed optogenetics or infrared neurostimulation techniques to regulate brain function and behavior in non-human primates.The current state of optical-neural stimulations discussed here demonstrates their efficacy in advancing the understanding of brain systems.Nevertheless,there are still challenges that need to be addressed before they can fully achieve their potential. 展开更多
关键词 optical-neural stimulation OPTOGENETICS infrared neurostimulation non-human primates
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Nickel catalysts with asymmetric steric hindrance for ethylene polymerization
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作者 Wanlu Tian Fuzhou Wang Chen Zou 《中国科学技术大学学报》 CAS CSCD 北大核心 2024年第6期48-52,59,I0010,I0011,共8页
α-Diimide catalysts have attracted widespread attention due to their unique chain walking characteristics.A series ofα-diimide nickel/palladium catalysts with different electronic effects and steric hindrances were ... α-Diimide catalysts have attracted widespread attention due to their unique chain walking characteristics.A series ofα-diimide nickel/palladium catalysts with different electronic effects and steric hindrances were designed and synthesized for olefin polymerization.In this work,we synthesized a series of asymmetricα-diimide nickel complexes with different steric hindrances and used them for ethylene polymerization.These nickel catalysts have high ethylene polymerization activity,up to 6.51×10^(6)g·mol^(−1)·h^(−1),and the prepared polyethylene has a moderate melting point and high molecular weight(up to 38.2×10^(4)g·mol^(−1)),with a branching density distribution between 7 and 94 branches per 1000 carbons.More importantly,the polyethylene prepared by these catalysts exhibits excellent tensile properties,with strain and stress reaching 800%and 30 MPa,respectively. 展开更多
关键词 Α-DIIMINE nickel complex POLYETHYLENE POLYMERIZATION asymmetric steric hindrance
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Variations of phyllosphere microorganisms in asymptomatic and tobacco brown spot leaves before and after spraying 12% difenoconazole + fluxapyroxad SC
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作者 LI Tong WANG Hancheng +6 位作者 YE Guo WANG Qing NGANGUEM NZALLE Yranney Brice WANG Feng CAI Liuti FENG Ruichao ZHANG Songbai 《农药学学报》 CAS CSCD 北大核心 2024年第5期932-948,共17页
12%difenoconazole+fluxapyroxad SC(commercial name:Jiangong)was first released by BASF in China in 2016.It has been registered to control many diseases,including pear scab,apple Alternaria leaf spot,tomato early blight... 12%difenoconazole+fluxapyroxad SC(commercial name:Jiangong)was first released by BASF in China in 2016.It has been registered to control many diseases,including pear scab,apple Alternaria leaf spot,tomato early blight,cucumber powdery mildew,etc.This study evaluated the bioactivity of Jiangong against Alternaria alternata and explored variations of phyllosphere microorganisms in both asymptomatic and tobacco brown spot leaves at different persistence periods(0,5,10,and 15 days post-fungicide application)using high-throughput sequencing technology.The results indicated that Jiangong effectively inhibited mycelial growth(average EC_(50) value of 0.51μg/mL),conidia germination(average EC_(50) value of 3.47μg/mL),and the carbon metabolism of A.alternata.Both asymptomatic and symptomatic leaves presented complex microbial communities.Higher fungal diversity was noted in asymptomatic leaves,while higher bacterial diversity was found in symptomatic leaves.After application,the diversity and abundance of microbial community structures in both types of leaves changed over time.Fungal microbiome communities showed greater sensitivity than bacterial groups,with the microbiome communities of asymptomatic leaves being more affected than those of symptomatic leaves.Fungal community diversity decreased for both symptomatic and asymptomatic leaves after 5 days of application,while the diversity of fungal community in symptomatic leaves showed an upward trend after 10 days of application.Meanwhile,bacterial community diversity increased in both symptomatic and asymptomatic leaves after 5 days of application but then declined in asymptomatic leaves after 15 days.The abundance of the dominant function group of phyllosphere bacteria(metabolism,genetic information processing,environmental information processing)was not affected by the application of Jiangong.However,the abundance of the dominant function group of phyllosphere fungi(animal pathogen-endophyte-wood saprotroph,endophyte-plant pathogen,plant pathogen-undefined saprotroph)was significantly affected by the application of Jiangong,and high variation was found in symptomatic leaves than that of asymptomatic leaves.The application of Jiangong-induced alterations in the community structure of the tobacco phyllosphere microbiome provides a basis for future tobacco brown spot control strategies based on phyllospheric microecology. 展开更多
关键词 tobacco brown spot DIFENOCONAZOLE fluxapyroxad microorganism communities diversity high-throughput sequencing
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Osteology of Turfanodon bogdaensis (Dicynodontia)
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作者 SHI Yu-Tai LIU Jun 《古脊椎动物学报(中英文)》 CSCD 北大核心 2024年第3期186-200,共15页
Within the dicynodont genus Turfanodon,there are two recognized species,T.bogdaensis and T.jiufengensis.Both species are known by relatively complete cranial materials,but the mandibles and most postcranial bones have... Within the dicynodont genus Turfanodon,there are two recognized species,T.bogdaensis and T.jiufengensis.Both species are known by relatively complete cranial materials,but the mandibles and most postcranial bones have been described only for T.jiufengensis.This paper reports new dicynodont specimens from Turpan,Xinjiang,referring them to T.bogdaensis.They can clearly be differentiated from T.jiufengensis by the flatter lateral surface of the snout region,a prominent swelling on the lateral dentary shelf,and the rounded femoral head.The diagnosis of Turfanodon is revised.The combination of a flat circumorbital rim,posterior portion of anterior pterygoid rami with converging ventral ridges,and a possible autapomorphy,a deep notch on scapula forming procoracoid foramen,are confirmed.It also differentiated from all dicynodonts other than Myosaurus,Kembawacela and Lystrosaurus by having accessory ridges lateral to the median palatal ridge. 展开更多
关键词 Turpan Xinjiang Lopingian Permian Guodikeng Formation Dicynodontia Turfanodon osteology postcranial skeleton
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Machine learning molecular dynamics simulations of liquid methanol
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作者 Jie Qian Junfan Xia Bin Jiang 《中国科学技术大学学报》 CAS CSCD 北大核心 2024年第6期12-21,I0009,I0010,共12页
As the simplest hydrogen-bonded alcohol,liquid methanol has attracted intensive experimental and theoretical interest.However,theoretical investigations on this system have primarily relied on empirical intermolecular... As the simplest hydrogen-bonded alcohol,liquid methanol has attracted intensive experimental and theoretical interest.However,theoretical investigations on this system have primarily relied on empirical intermolecular force fields or ab initio molecular dynamics with semilocal density functionals.Inspired by recent studies on bulk water using increasingly accurate machine learning force fields,we report a new machine learning force field for liquid methanol with a hybrid functional revPBE0 plus dispersion correction.Molecular dynamics simulations on this machine learning force field are orders of magnitude faster than ab initio molecular dynamics simulations,yielding the radial distribution functions,selfdiffusion coefficients,and hydrogen bond network properties with very small statistical errors.The resulting structural and dynamical properties are compared well with the experimental data,demonstrating the superior accuracy of this machine learning force field.This work represents a successful step toward a first-principles description of this benchmark system and showcases the general applicability of the machine learning force field in studying liquid systems. 展开更多
关键词 liquid methanol molecular dynamics machine learning hydrogen bond force field
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Regulating crystal phase of TiO_(2) to enhance catalytic activity of Ni/TiO_(2) for solar-driven dry reforming of methane
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作者 HE Zhanjun GONG Kun +3 位作者 DAI Yuanyuan NIU Qiang LIN Tiejun ZHONG Liangshu 《燃料化学学报(中英文)》 EI CAS CSCD 北大核心 2024年第9期1203-1213,共11页
Ni/TiO_(2) catalyst is widely employed for photo-driven DRM reaction while the influence of crystal structure of TiO_(2) remains unclear.In this work,the rutile/anatase ratio in supports was successfully controlled by... Ni/TiO_(2) catalyst is widely employed for photo-driven DRM reaction while the influence of crystal structure of TiO_(2) remains unclear.In this work,the rutile/anatase ratio in supports was successfully controlled by varying the calcination temperature of anatase-TiO_(2).Structural characterizations revealed that a distinct TiO_(x) coating on the Ni nanoparticles(NPs)was evident for Ni/TiO_(2)-700 catalyst due to strong metal-support interaction.It is observed that the TiOx overlayer gradually disappeared as the ratio of rutile/anatase increased,thereby enhancing the exposure of Ni active sites.The exposed Ni sites enhanced visible light absorption and boosted the dissociation capability of CH4,which led to the much elevated catalytic activity for Ni/TiO_(2)-950 in which rutile dominated.Therefore,the catalytic activity of solar-driven DRM reaction was significantly influenced by the rutile/anatase ratio.Ni/TiO_(2)-950,characterized by a predominant rutile phase,exhibited the highest DRM reactivity,with remarkable H_(2) and CO production rates reaching as high as 87.4 and 220.2 mmol/(g·h),respectively.These rates were approximately 257 and 130 times higher,respectively,compared to those obtained on Ni/TiO_(2)-700 with anatase.This study suggests that the optimization of crystal structure of TiO_(2) support can effectively enhance the performance of photothermal DRM reaction. 展开更多
关键词 dry reforming of methane photothermal catalysis crystal phase TiO_(2) metal-support interaction
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综合类自然科学期刊组稿的定位和思路 被引量:6
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作者 黎贞崇 黄日波 +3 位作者 陆海生 尹闯 李智娟 陆雁 《广西师范学院学报(自然科学版)》 2014年第2期103-106,共4页
针对综合类自然科学期刊面临的办刊困境,深入分析了综合类自然科学期刊组稿劣势和优势,指出了综合类自然科学期刊组稿的定位,提出了综合类自然科学期刊的组稿思路,认为综合类自然科学期刊应该立足学科和资源特色,以学术带头人为栏目主编... 针对综合类自然科学期刊面临的办刊困境,深入分析了综合类自然科学期刊组稿劣势和优势,指出了综合类自然科学期刊组稿的定位,提出了综合类自然科学期刊的组稿思路,认为综合类自然科学期刊应该立足学科和资源特色,以学术带头人为栏目主编,根据资源特色、学科带头人专业方向、产业科技需要、新兴学科和交叉学科方向设置栏目,办出特色,创出品牌。 展开更多
关键词 自然科学期刊 综合类 组稿 定位 思路
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Freestanding oxide membranes:synthesis,tunable physical properties,and functional devices
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作者 Ao Wang Jinfeng Zhang Lingfei Wang 《中国科学技术大学学报》 CAS CSCD 北大核心 2024年第7期2-17,1,I0002,共18页
The study of oxide heteroepitaxy has been hindered by the issues of misfit strain and substrate clamping,which impede both the optimization of performance and the acquisition of a fundamental understanding of oxide sy... The study of oxide heteroepitaxy has been hindered by the issues of misfit strain and substrate clamping,which impede both the optimization of performance and the acquisition of a fundamental understanding of oxide systems.Recently,however,the development of freestanding oxide membranes has provided a plausible solution to these substrate limitations.Single-crystalline functional oxide films can be released from their substrates without incurring significant damage and can subsequently be transferred to any substrate of choice.This paper discusses recent advancements in the fabrication,adjustable physical properties,and various applications of freestanding oxide perovskite films.First,we present the primary strategies employed for the synthesis and transfer of these freestanding perovskite thin films.Second,we explore the main functionalities observed in freestanding perovskite oxide thin films,with special attention to the tunable functionalities and physical properties of these freestanding perovskite membranes under varying strain states.Next,we encapsulate three representative devices based on freestanding oxide films.Overall,this review highlights the potential of freestanding oxide films for the study of novel functionalities and flexible electronics. 展开更多
关键词 freestanding oxide membranes transition metal oxides thin films electronic devices
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Genetic Evidence for Causal Association Between Hypertension and Chronic Pain:A Bidirectional Two-Sample Mendelian Randomization Study
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作者 Shuai-Lei Wang Wei-Yun Chen +1 位作者 Zi-Jia Liu Yu-Guang Huang 《Chinese Medical Sciences Journal》 CAS CSCD 2024年第3期155-162,共8页
Objective The extent to which the association between hypertension and chronic pain in observational studies is either causally linked or influenced by other shared risk factors has not been substantially addressed.In... Objective The extent to which the association between hypertension and chronic pain in observational studies is either causally linked or influenced by other shared risk factors has not been substantially addressed.In the present study,Mendelian randomization(MR)was employed to examine the potential causal relationship between hypertension and risk of chronic pain.Methods The study data were derived from the pooled dataset of the genome-wide association study(GWAS),enabling the evaluation of the causal effects of hypertension on various types of chronic pain including chronic headache as well as chest,abdominal,joint,back,limb,and multisite chronic pain.We performed a bidirectional two-sample MR analysis using random effect inverse variance weighting(IVW),MR-Egger,weighted median,and weighted mode,quantified by odds ratio(OR).Results Genetically predicted essential hypertension was associated with an increased risk of chronic headache(OR=1.007,95%CI:1.003-1.011,P=0.002)and limb pain(OR=1.219,95%CI:1.033-1.439,P=0.019).No potential causal associations were identified between chronic pain and essential hypertension in the reverse direction MR(P>0.05).In addition,there was no potential causal association between secondary hypertension and chronic pain(P>0.05).Conclusion This study provided genetic evidence that a unidirectional causal relationship exists between essential hypertension and the increased risks of chronic headache and limb pain,and no causal relationship was found between secondary hypertension and chronic pain.These findings offer theoretical underpinnings for future research on managing hypertension and chronic pain. 展开更多
关键词 HYPERTENSION chronic pain Mendelian randomization health chronic headache genetic evidence limb pain
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