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面向基础设施的美国2050远景规划 被引量:3
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作者 彼得拉·托多罗维奇 罗伯特·亚罗 +3 位作者 彭翀 刘合林 袁晓辉 韩青 《城市与区域规划研究》 CSSCI 2017年第1期18-38,共21页
文章从基础设施投资和建设的视角探讨了美国在未来几十年为应对新挑战而应采取的应对策略。首先通过历史回顾,肯定了基础设施相关规划和政策对国家发展的巨大带动作用;其次,对于今后的远景展望,提出在进行基础设施投资和相关政策制... 文章从基础设施投资和建设的视角探讨了美国在未来几十年为应对新挑战而应采取的应对策略。首先通过历史回顾,肯定了基础设施相关规划和政策对国家发展的巨大带动作用;其次,对于今后的远景展望,提出在进行基础设施投资和相关政策制定时,公平性是关键,应当综合考虑经济、生态和社会效益,而规划的实施需要各级政府、巨型城市区和私人部门多方共同努力;然后,从基础设施投资计划构成的三个方面(水、能源和交通运输)制定远景的原则和框架;最后,对远景规划的实施措施提出建议,这也正是“美国2050”团队未来的工作方向。 展开更多
关键词 基础设施投资 远景规划 美国 国家发展 社会效益 投资计划 交通运输 公平性
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Optimality of Group Testing with Differential Misclassification
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作者 LI Yiming ZHANG Hong LIU Aiyi 《应用概率统计》 CSCD 北大核心 2024年第4期644-662,共19页
Group testing is a method that can be used to estimate the prevalence of rare infectious diseases,which can effectively save time and reduce costs compared to the method of random sampling.However,previous literature ... Group testing is a method that can be used to estimate the prevalence of rare infectious diseases,which can effectively save time and reduce costs compared to the method of random sampling.However,previous literature only demonstrated the optimality of group testing strategy while estimating prevalence under some strong assumptions.This article weakens the assumption of misclassification rate in the previous literature,considers the misclassification rate of the infected samples as a differentiable function of the pool size,and explores some optimal properties of group testing for estimating prevalence in the presence of differential misclassification conforming to this assumption.This article theoretically demonstrates that the group testing strategy performs better than the sample by sample procedure in estimating disease prevalence when the total number of sample pools is given or the size of the test population is determined.Numerical simulation experiments were conducted to evaluate the performance of group tests in estimating prevalence in the presence of dilution effect. 展开更多
关键词 group testing sensitivity SPECIFICITY dilution effect differential misclassification PREVALENCE
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Solution of idle LBO problem for high FAR aero combustor
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作者 CHIN Jushan ZENG Qinghua 《推进技术》 EI CAS CSCD 北大核心 2024年第10期96-104,共9页
The paper sheds light on the idle lean blow off(LBO)problem for high fuel air ratio(FAR)com⁃bustor,which is impossible to be addressed with traditional aero combustor design.A significant improvement in aero combustor... The paper sheds light on the idle lean blow off(LBO)problem for high fuel air ratio(FAR)com⁃bustor,which is impossible to be addressed with traditional aero combustor design.A significant improvement in aero combustor design is required to resolve the idle LBO issue.The authors detailed a practical and efficient solu⁃tion,which not only solved the idle LBO issue but also defined the aero-thermal design for high-FAR combustor.The design will usher in a new era of aero combustor. 展开更多
关键词 Aero engine COMBUSTOR Idle lean blow off High fuel air ratio Concentric circle zoning combustion
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Attitudes Toward People Who Stutter in the Chinese Context: An Exploratory Study on the Impact of Knowledge Sources
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作者 Ran AN Judith D.OXLEY John A.TETNOWSKI 《Chinese Journal of Applied Linguistics》 2024年第4期591-611,687,共22页
The public’s attitudes can affect the experience of stuttering of people who stutter.This study investigated the attitudes held by the public about people who stutter in China.A web-based written survey with closed a... The public’s attitudes can affect the experience of stuttering of people who stutter.This study investigated the attitudes held by the public about people who stutter in China.A web-based written survey with closed and open-ended questions was implemented to develop a rich understanding.One hundred and two respondents in 26 provinces and 3 municipalities provided comments on people who stutter in their life aspects such as personality,speech,social life,work,life participation,education,dating and marriage,capability,and communication skills.The predominantly negative attitudes towards the overall domains were identified.Attitudes to people who stutter varied according to the different sources of knowledge.Familiarity with people who stutter might reduce stereotypes.However,knowledge from the media might aggravate stereotypes.Implications and future research orientation were also discussed. 展开更多
关键词 public’s attitudes people who stutter personality communication skills FAMILIARITY media
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Polar residual network model for assisting evaluation on rat myocardial infarction segment in myocardial contrast echocardiography
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作者 SHEN Wenqian GUO Yanhui +5 位作者 YU Bo CHEN Shuang LI Hairu WU Yan LI You DU Guoqing 《中国医学影像技术》 CSCD 北大核心 2024年第8期1130-1134,共5页
Objective To investigate the value of polar residual network(PResNet)model for assisting evaluation on rat myocardial infarction(MI)segment in myocardial contrast echocardiography(MCE).Methods Twenty-five male SD rats... Objective To investigate the value of polar residual network(PResNet)model for assisting evaluation on rat myocardial infarction(MI)segment in myocardial contrast echocardiography(MCE).Methods Twenty-five male SD rats were randomly divided into MI group(n=15)and sham operation group(n=10).MI models were established in MI group through ligation of the left anterior descending coronary artery using atraumatic suture,while no intervention was given to those in sham operation group after thoracotomy.MCE images of both basal and papillary muscle levels on the short axis section of left ventricles were acquired after 1 week,which were assessed independently by 2 junior and 2 senior ultrasound physicians.The evaluating efficacy of MI segment,the mean interpretation time and the consistency were compared whether under the assistance of PResNet model or not.Results No significant difference of efficacy of evaluation on MI segment was found for senior physicians with or without assistance of PResNet model(both P>0.05).Under the assistance of PResNet model,the efficacy of junior physicians for diagnosing MI segment was significantly improved compared with that without the assistance of PResNet model(both P<0.01),and was comparable to that of senior physicians.Under the assistance of PResNet model,the mean interpretation time of each physician was significantly shorter than that without assistance(all P<0.001),and the consistency between junior physicians and among junior and senior physicians were both moderate(Kappa=0.692,0.542),which became better under the assistance(Kappa=0.763,0.749).Conclusion PResNet could improve the efficacy of junior physicians for evaluation on rat MI segment in MCE images,shorten interpretation time with different aptitudes,also improve the consistency to some extent. 展开更多
关键词 myocardial infarction deep learning ULTRASONOGRAPHY animal experimentation
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Analysis of Smooth Cepstral Peak Prominence in Hypokinetic Dysarthria Associated With Parkinson’s Disease
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作者 Qiang LI Abigail WALLACE +4 位作者 Wesley DAVIS Beau ROTH Laura LANGHOFER Shalini NARAYANA Michael CANNITO 《Chinese Journal of Applied Linguistics》 2024年第4期657-669,688,共14页
Smoothed cepstral peak prominence(CPPs)is a measurement of the distance from the prominent cepstral peak to the linear regression line directly beneath it.Variations of CPPs data acquisition and analysis lead to the c... Smoothed cepstral peak prominence(CPPs)is a measurement of the distance from the prominent cepstral peak to the linear regression line directly beneath it.Variations of CPPs data acquisition and analysis lead to the complexity of the clinical cut-off values,and there are no agreeable values for a specific voice disorder,such as hypokinetic dysarthria associated with Parkinson’s disease(PD).This study examined the CPPs in people with hypokinetic dysarthria associated with PD compared with healthy participants.Results demonstrated significant differences in speech tasks of sustained vowel and connected speech,with CPPs of connected speech more sensitive to dysphonia and gender difference in PD participants.Males in PD participants presented higher CPPs for sustained vowels and lower CPPs for connected speech than females.It is implied that a consistent clinical application protocol is necessary,and multiple acoustic measures are needed to ensure the accuracy of clinical decisions. 展开更多
关键词 cepstral peak prominence hypokinetic dysarthria VOICE Parkinson’s disease motor speech disorders
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Is platinum-loaded titania the best material for dye-sensitized hydrogen evolution under visible light?
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作者 Haruka Yamamoto Langqiu Xiao +5 位作者 Yugo Miseki Hiroto Ueki Megumi Okazaki Kazuhiro Sayama Thomas E.Mallouk Kazuhiko Maeda 《Chinese Journal of Catalysis》 SCIE CAS CSCD 2024年第8期124-132,共9页
A dye-sensitized photocatalyst combining Pt-loaded TiO_(2) and Ru(Ⅱ)tris-diimine sensitizer(RuP)was constructed and its activity for photochemical hydrogen evolution was compared with that of Pt-intercalated HCa_(2)N... A dye-sensitized photocatalyst combining Pt-loaded TiO_(2) and Ru(Ⅱ)tris-diimine sensitizer(RuP)was constructed and its activity for photochemical hydrogen evolution was compared with that of Pt-intercalated HCa_(2)Nb_(3)O_(10) nanosheets.When the sacrificial donor ethylenediaminetetraacetic acid(EDTA)disodium salt dihydrate was used,RuP/Pt/TiO_(2) showed higher activity than RuP/Pt/HCa_(2)Nb_(3)O_(10).In contrast,when NaI(a reversible electron donor)was used,RuP/Pt/TiO_(2) showed little activity due to back electron transfer to the electron acceptor(I_(3)-),which was gener-ated as the oxidation product of I-.By modification with anionic polymers(sodium poly(styrenesulfonate)or sodium polymethacrylate)that could inhibit the scavenging of conduction band electrons by I_(3)-,the H_(2) production activity from aqueous NaI was improved,but it did not exceed that of RuP/Pt/HCa_(2)Nb_(3)O_(10).Transient absorption measurements showed that the rate of semiconductor-to-dye back electron transfer was slower in the case of TiO_(2) than HCa_(2)Nb_(3)O_(10),but the electron transfer reaction to I3-was much faster.These results indicate that Pt/TiO_(2) is useful for reactions with sacrificial reductants(e.g.,EDTA),where the back electron transfer reaction to the more reducible product can be neglected.However,more careful design of the catalyst will be nec-essary when a reversible electron donor is employed. 展开更多
关键词 Artificial photosynthesis Solar fuel Water splitting Z-scheme
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Catalytically altering the redox pathway of sulfur in propylene carbonate electrolyte using dual-nitrogen/oxygen-containing carbon
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作者 Linghui Yu Heng Zhang +9 位作者 Luyuan Paul Wang Samuel Jun Hoong Ong Shibo Xi Bo Chen Rui Guo Ting Wang Yonghua Du Wei Chen Ovadia Lev Zhichuan J.Xu 《Chinese Journal of Catalysis》 SCIE CAS CSCD 2024年第8期224-233,共10页
Carbonate electrolytes are one of the most desirable electrolytes for high-energy lithium-sulfur batteries(LSBs)because of their successful implementation in commercial Li-ion batteries.The low-polysulfide-solubility ... Carbonate electrolytes are one of the most desirable electrolytes for high-energy lithium-sulfur batteries(LSBs)because of their successful implementation in commercial Li-ion batteries.The low-polysulfide-solubility feature of some carbonate solvents also makes them very promising for overcoming the shuttle effects of LSBs.However,regular sulfur electrodes experience undesired electrochemical mechanisms in carbonate electrolytes due to side reactions.In this study,we report a catalytic redox mechanism of sulfur in propylene carbonate(PC)electrolyte based on a compari-son study.The catalytic mechanism is characterized by the interactions between polysulfides and dual N/O functional groups on the host carbon,which largely prevents side reactions between polysulfides and the carbonate electrolyte.Such a mechanism coupled with the low-polysulfide-solubility feature leads to stable cycling of LSBs in PC electrolyte.Favorable dual N/O functional groups are identified via a density functional theory study.This work provides an alternative route for enabling LSBs in carbonate electrolytes. 展开更多
关键词 Energy storage Lithium-sulfur battery Catalytic redox reaction Porous carbon Carbonate electrolyte
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Warm forming behavior of high strength aluminum alloy AA7075 被引量:29
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作者 WANG Hui LUO Ying-bing +2 位作者 Peter FRIEDMAN CHEN Ming-he GAO Lin 《Transactions of Nonferrous Metals Society of China》 SCIE EI CAS CSCD 2012年第1期1-7,共7页
The formability of aluminum alloy AA7075 at elevated temperature was investigated through experiment. Stress-strain relationship at different temperatures and forming speeds were investigated through tensile testing. ... The formability of aluminum alloy AA7075 at elevated temperature was investigated through experiment. Stress-strain relationship at different temperatures and forming speeds were investigated through tensile testing. Deep drawing and stretch formability were also tested through limiting drawing ratio (LDR) and limiting dome height (LDH) tests. Finally, post forming mechanical property testing was conducted to investigate the effects of exposure to warm forming temperatures on the mechanical properties. Results show that deep drawing and stretch formability of AA7075 can be significantly improved when the blank is heated to 140-220 °C. At temperature over 260 °C, formability and post forming mechanical properties begin to decrease due to the effect of the heating and forming processes on the material's temper. 展开更多
关键词 aluminum alloy 7075 warm forming limiting drawing ratio (LDR) limiting dome height (LDH)
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One-step synthesis of Pt@ZIF-8 catalyst for the selective hydrogenation of 1,4-butynediol to 1,4-butenediol 被引量:16
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作者 Chuang Li Mingming Zhang +3 位作者 Xin Di Dongdong Yin Wenzhen Li Changhai Liang 《Chinese Journal of Catalysis》 SCIE EI CAS CSCD 北大核心 2016年第9期1555-1561,共7页
A catalyst consisting of platinum nanoparticles on a ZIF-8 support(Pt@ZIF-8) was synthesized in a straightforward one-step procedure,by adding a nanostructured platinum sol during the formation of ZIF-8 at room temp... A catalyst consisting of platinum nanoparticles on a ZIF-8 support(Pt@ZIF-8) was synthesized in a straightforward one-step procedure,by adding a nanostructured platinum sol during the formation of ZIF-8 at room temperature.Pt@ZIF-8 was highly porous and well crystallized.The Pt nanoparticles were well dispersed within the ZIF-8 support.In the hydrogenation of 1,4-butynediol,Pt@ZIF-8 exhibited high activity,excellent selectivity for 1,4-butenediol of greater than 94%,and reusability.The Pt@ZIF-8 catalyst did not require further additives.The favorable catalytic performance was attributed primarily to the modification of the ZIF-8 support by the platinum nanoparticles. 展开更多
关键词 Platinum sol ZIF-8 One-step synthesis 1 4-Butynediol Selective hydrogenation
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Pt alloy oxygen-reduction electrocatalysts: Synthesis, structure, and property 被引量:17
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作者 Xiao Xia Wang Joshua Sokolowski +1 位作者 Hui Liu Gang Wu 《Chinese Journal of Catalysis》 SCIE EI CAS CSCD 北大核心 2020年第5期739-755,共17页
Proton exchange membrane fuel cells(PEMFCs) are considered a promising power source for electric vehicles and stationary residential applications. However, current PEMFCs have several problems that require solutions, ... Proton exchange membrane fuel cells(PEMFCs) are considered a promising power source for electric vehicles and stationary residential applications. However, current PEMFCs have several problems that require solutions, including high cost, insufficient power density, and limited performance durability. A kinetically sluggish oxygen reduction reaction(ORR) is primarily responsible for these issues. The development of advanced Pt-based catalysts is crucial for solving these problems if the large-scale application of PEMFCs is to be realized. In this review, we summarize the recent progress in the development of Pt M alloy(M = Fe, Co, Ni, etc.) catalysts with an emphasis on ordered Pt M intermetallic catalysts, which exhibit significantly enhanced activity and stability. In addition to exploring the intrinsic catalytic performance in traditional aqueous electrolytes via engineering nanostructures, morphologies, and crystallinity of Pt M particles, we highlight recent efforts to study catalysts under real fuel cell environments by the membrane electrode assembly(MEA). 展开更多
关键词 Proton exchange membrane fuel cell Oxygen reduction reaction Low Pt catalyst Catalytic activity Stability
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L2 Syntactic Alignment in the Reading-Writing Integrated Continuation Task: Evidence From Chinese EFL Learners’ Description of Motion Events 被引量:7
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作者 Min WANG Qiao GAN Julie BOLAND 《Chinese Journal of Applied Linguistics》 2021年第3期292-313,430,共23页
This study investigated how the mode in which the reading-writing integrated continuation task was conducted modulates the effects of second language(L2) syntactic alignment, through the English motion event construct... This study investigated how the mode in which the reading-writing integrated continuation task was conducted modulates the effects of second language(L2) syntactic alignment, through the English motion event construction with manner verbs. Ninety Chinese students were assigned to either of the two experimental groups or a control group, and they all experienced a pretest, an alignment phase and a posttest. In the alignment phase, the two experimental groups completed a reading-writing integrated continuation task but in different modes. For the multi-turn mode,participants reconstructed a picture story by continuing the episodes extracted from the story with one episode presented and continued at a time;for the single-turn mode, the first half of the same picture story was presented as a chunk, and then participants read and continued it. Results show that L2 learners aligned with the target structure in completing the story, and the alignment effect was retained in the posttest conducted after a delay of two weeks. Moreover, syntactic alignment was modulated by task mode with the multi-turn group exhibiting stronger immediate and longterm alignment effects. We conclude that the continuation task is a fruitful context for L2 structural alignment, and the magnitude of alignment effect hinges on interactive intensity. 展开更多
关键词 reading-writing integrated continuation task syntactic alignment task mode interactive intensity motion event construction with manner verbs L2 learning
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Electrocatalytic H_(2)O_(2)generation for disinfection 被引量:5
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作者 Yachao Zeng Gang Wu 《Chinese Journal of Catalysis》 SCIE EI CAS CSCD 2021年第12期2149-2163,共15页
Epidemics are threatening public health and social development.Emerging as a green disinfectant,H_(2)O_(2)can prevent the breakout of epidemics in migration.Electrochemical H_(2)O_(2)production powered by renewable el... Epidemics are threatening public health and social development.Emerging as a green disinfectant,H_(2)O_(2)can prevent the breakout of epidemics in migration.Electrochemical H_(2)O_(2)production powered by renewable electricity provides a clean and decentralized solution for on-site disinfection.This review firstly discussed the efficacy of H_(2)O_(2)in disinfection.Then necessary fundamental principles are summarized to gain insight into electrochemical H_(2)O_(2)production.The focus is on exploring pathways to realize a highly efficient H_(2)O_(2)production.Progress in advanced electrocatalysts,typically single-atom catalysts for the two-electron oxygen reduction reaction(2e−ORR),are highlighted to provide high H_(2)O_(2)selectivity design strategies.Finally,a rational design of electrode and electrolytic cells is outlined to realize the on-site disinfection.Overall,this critical review contributes to exploiting the potentials and constraints of electrochemical H_(2)O_(2)generation in disinfection and pinpoints future research directions required for implementation. 展开更多
关键词 Hydrogen peroxide Oxygen reduction DISINFECTION ELECTROSYNTHESIS Single metal atom catalysts
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A facile sulfur-assisted method to synthesize porous alveolate Fe/g-C3N4 catalysts with ultra-small cluster and atomically dispersed Fe sites 被引量:6
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作者 Sufeng An Guanghui Zhang +9 位作者 Jiaqiang Liu Keyan Li Gang Wan Yan Liang Donghui Ji Jeffrey T.Miller Chunshan Song Wei Liu Zhongmin Liu Xinwen Guo 《Chinese Journal of Catalysis》 SCIE EI CAS CSCD 北大核心 2020年第8期1198-1207,共10页
Heterogeneous catalysts with ultra-small clusters and atomically dispersed(USCAD)active sites have gained increasing attention in recent years.However,developing USCAD catalysts with high-density metal sites anchored ... Heterogeneous catalysts with ultra-small clusters and atomically dispersed(USCAD)active sites have gained increasing attention in recent years.However,developing USCAD catalysts with high-density metal sites anchored in porous nanomaterials is still challenging.Here,through the template-free S-assisted pyrolysis of low-cost Fe-salts with melamine(MA),porous alveolate Fe/g-C3N4 catalysts with high-density(Fe loading up to 17.7 wt%)and increased USCAD Fe sites were synthesized.The presence of a certain amount of S species in the Fe-salts/MA system plays an important role in the formation of USCAD S-Fe-salt/CN catalysts;the S species act as a"sacrificial carrier"to increase the dispersion of Fe species through Fe-S coordination and generate porous alveolate structure by escaping in the form of SO2 during pyrolysis.The S-Fe-salt/CN catalysts exhibit greatly promoted activity and reusability for degrading various organic pollutants in advanced oxidation processes compared to the corresponding Fe-salt/CN catalysts,due to the promoted accessibility of USCAD Fe sites by the porous alveolate structure.This S-assisted method exhibits good feasibility in a large variety of S species(thiourea,S powder,and NH4SCN)and Fe salts,providing a new avenue for the low-cost and large-scale synthesis of high-density USCAD metal/g-C3N4 catalysts. 展开更多
关键词 Sulfur-assisted synthesis Porous alveolate structure Ultra-small cluster and atomically dispersed active sites Fe/g-C3N4 Advanced oxidation processes
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From Xu to the Development of L2 Interactional Competence: A Conversation Analytic Case Study 被引量:7
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作者 Mei YANG Xiaofei LU 《Chinese Journal of Applied Linguistics》 2021年第3期273-291,430,共20页
Dialogues are fundamentally driven by xu(C. Wang, 2016, 2017), a Chinese word meaning continuation that captures the process in which interlocutors participate in interaction through the actions of(utterance) completi... Dialogues are fundamentally driven by xu(C. Wang, 2016, 2017), a Chinese word meaning continuation that captures the process in which interlocutors participate in interaction through the actions of(utterance) completion,(content) extension, and(topic) creation(CEC). This article reports a conversation analytic case study designed to investigate how the continuation strategies of CEC are used in real-time communication to achieve mutual understanding, and thus to construct intersubjectivity(Verhagen, 2005) and promote the development of second language(L2)interactional competence. Our data consisted of audio and video recordings of a 25-minute conversation between two L2 English speakers, one expert and one novice, and a stimulated recall interview with them. Results revealed that the expert employed CEC at the early stage of interaction to maintain successful communication, and the novice gradually aligned with the expert and used CEC to achieve mutual understanding, construct intersubjectivity, and create opportunities for interaction and learning at the late stage, displaying her development of L2 interactional competence. Our findings have useful implications for theoretical and methodological development of the xu-argument studies as well as for xu-based L2 pedagogy. 展开更多
关键词 the xu-argument INTERSUBJECTIVITY interactional competence continuation strategies conversation analysis
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Determining number of sites on ceria stabilizing single atoms via metal nanoparticle redispersion 被引量:4
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作者 Aisulu Aitbekova Cody JWrasman +2 位作者 Andrew RRiscoe Larissa YKunz Matteo Cargnello 《Chinese Journal of Catalysis》 SCIE EI CAS CSCD 北大核心 2020年第6期998-1005,共8页
Single atom catalysts have recently attracted interest due to their maximization of the utilization of expensive noble metals as well as their unique catalytic properties. Based on its surface atomic properties, CeO2 ... Single atom catalysts have recently attracted interest due to their maximization of the utilization of expensive noble metals as well as their unique catalytic properties. Based on its surface atomic properties, CeO2 is one of the most common supports for stabilizing single metal atoms. Many single atom catalysts are limited in their metal contents by the formation of metal nanoparticles once the catalyst support capacity for single atoms has been exceeded. Currently, there are no direct measurements to determine the capacity of a support to stabilize single atoms. In this work we develop a nanoparticle-based technique that allows for quantification of that capacity by redispersing Ru nanoparticles into single atoms and taking advantage of the different catalytic properties of Ru single atoms and nanoparticles in the CO2 hydrogenation reaction. This method avoids complications in metal loading caused by counterions in incipient wetness impregnation and can eventually be applied to a variety of different metals. Results using this technique follow trends in oxygen vacancy concentration and surface oxygen content and show promise as a new method for quantifying support single atom stabilization capacity. 展开更多
关键词 CERIA Single-atom catalyst Oxygen vacancies CO2 hydrogenation REDISPERSION
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Co-MOF as an electron donor for promoting visible-light photoactivities of g-C3N4 nanosheets for CO2 reduction 被引量:13
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作者 Qiuyu Chen Sijia Li +4 位作者 Hongyi Xu Guofeng Wang Yang Qu Peifen Zhu Dingsheng Wang 《Chinese Journal of Catalysis》 SCIE EI CAS CSCD 北大核心 2020年第3期514-523,共10页
A possible mechanism for boosting the visible-light photoactivities of graphitic carbon nitride(g-C3N4)nanosheets for CO2 reduction via coupling with the electron donor Co-metal-organic framework(MOF)is proposed in th... A possible mechanism for boosting the visible-light photoactivities of graphitic carbon nitride(g-C3N4)nanosheets for CO2 reduction via coupling with the electron donor Co-metal-organic framework(MOF)is proposed in this study.Specifically,Co-MOF as an electron donor is capable of transferring the photogenerated electrons in the lowest unoccupied molecular orbital(LUMO)to the conduction band of g-C3N4 to facilitate charge separation.As expected,the prepared Co-MOF/g-C3N4 nanocomposites display excellent visible-light-driven photocatalytic CO2 reduction activities.The CO production rate of 6.75μmol g–1 h–1 and CH4 evolution rate of 5.47μmol g–1 h–1 are obtained,which are approximately 2 times those obtained with the original g-C3N4 under the same conditions.Based on a series of analyses,it is shown that the introduction of Co-MOF not only broadens the range of visible-light absorption but also enhances the charge separation,which improves the photocatalytic activity of g-C3N4 to a higher level.In particular,the hydroxyl radical(·OH)experiment was operated under 590 nm(single-wavelength)irradiation,which further proved that the photogenerated electrons in the LUMO of Co-MOF can successfully migrate to g-C3N4.This work may provide an important strategy for the design of highly efficient g-C3N4-based photocatalysts for CO2 reduction. 展开更多
关键词 Co-MOF g-C3N4 nanosheets Charge separation Visible-light photoactivity Photocatalytic CO2 conversion
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Anomaly detection of earthquake precursor data using long short-term memory networks 被引量:7
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作者 Cai Yin Mei-Ling Shyu +2 位作者 Tu Yue-Xuan Teng Yun-Tian Hu Xing-Xing 《Applied Geophysics》 SCIE CSCD 2019年第3期257-266,394,共11页
Earthquake precursor data have been used as an important basis for earthquake prediction.In this study,a recurrent neural network(RNN)architecture with long short-term memory(LSTM)units is utilized to develop a predic... Earthquake precursor data have been used as an important basis for earthquake prediction.In this study,a recurrent neural network(RNN)architecture with long short-term memory(LSTM)units is utilized to develop a predictive model for normal data.Furthermore,the prediction errors from the predictive models are used to indicate normal or abnormal behavior.An additional advantage of using the LSTM networks is that the earthquake precursor data can be directly fed into the network without any elaborate preprocessing as required by other approaches.Furthermore,no prior information on abnormal data is needed by these networks as they are trained only using normal data.Experiments using three groups of real data were conducted to compare the anomaly detection results of the proposed method with those of manual recognition.The comparison results indicated that the proposed LSTM network achieves promising results and is viable for detecting anomalies in earthquake precursor data. 展开更多
关键词 Earthquake precursor data deep learning LSTM-RNN prediction model anomaly detect io n
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Social Security Development in China and Its Support to Economic Transition 被引量:7
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作者 Zheng Bingwen Zhang Xiaoli 《China Economist》 2019年第4期96-121,共26页
In 70 years since the founding of the People’s Republic of China,China has successfully transitioned from a closed economy to an open economy with the watershed year of reform and opening up in 1978 and modernized it... In 70 years since the founding of the People’s Republic of China,China has successfully transitioned from a closed economy to an open economy with the watershed year of reform and opening up in 1978 and modernized its social security system accordingly.This paper divides the transition of China’s social security system into seven stages before and after 1978.The traditional social security system was predicated on the dominant public ownership,a highly centralized economy,and“full employment.”It was congruous with the ownership structure,income distribution,and labor systems under the closed economy.The modern social security system is developed to meet the needs of an open economy and promotes economic development by giving play to consumption and investment,facilitating labor flow,and boosting productivity.The modern social security system requires further supply-side structural reforms to promote the high-quality development of the open economy. 展开更多
关键词 closed economy open economy social security system production factor labor market
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Atomic layer deposition: Catalytic preparation and modification technique for the next generation 被引量:5
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作者 Hongbo Zhang Christopher L. Marshall 《Chinese Journal of Catalysis》 SCIE EI CAS CSCD 北大核心 2019年第9期1311-1323,共13页
Atomic layer deposition(ALD)attracts great attention nowadays due to its ability for designing and modifying catalytic systems at the molecular level.There are several reported review papers published recently discuss... Atomic layer deposition(ALD)attracts great attention nowadays due to its ability for designing and modifying catalytic systems at the molecular level.There are several reported review papers published recently discussing this technique in catalysis.However,the mechanism on how the deposited materials improve the catalyst stability and tune the reaction selectivity is still unclear.Herein,catalytic systems created via ALD on stepwise preparation and/or modification under self-limiting reaction conditions are summarized.The effects of deposited materials in terms of electronic/geometry modification over the catalytic nanoparticles(NPs)are discussed.These effects explain the mechanism of the catalytic stability improvement and the selectivity modification.The unique properties of ALD for designing new catalytic systems are further investigated for building up photocatalytic reaction nanobowls,tandem catalyst and bi-active-component metallic catalytic systems. 展开更多
关键词 Atomic layer deposition Catalyst modification Catalyst preparation Redox properties Terrace site Step site
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