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The Visual Analytics and Data Exploration Research Lab at Arizona State University
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作者 Ross Maciejewski Yuxin Ma Jonas Lukasczyk 《Visual Informatics》 EI 2021年第1期14-22,共9页
This article describes the research agenda for the Visual Analytics and Data Exploration Research(VADER)Lab at Arizona State University.Over the past decade,the VADER Lab has focused on creating novel algorithms,tools... This article describes the research agenda for the Visual Analytics and Data Exploration Research(VADER)Lab at Arizona State University.Over the past decade,the VADER Lab has focused on creating novel algorithms,tools and visualizations for spatiotemporal data.This article will highlight past success in spatiotemporal analysis,explainable AI,graph mining,and mathematical topology.While,at first,these topics seem largely disjoint,we will describe how the underpinnings of spatiotemporal analysis has informed the various research directions in the VADER Lab,and how this research agenda has served to form a network of strong international collaborations.Finally,we will outline a vision for the Lab’s future research. 展开更多
关键词 VISUALIZATION SPATIOTEMPORAL Explainable AI TOPOLOGY
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Feasibility of using pedometers in a state-based surveillance system:2014 Arizona Behavioral Risk Factor Surveillance System
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作者 Alberto Flórez-Pregonero Janet E.Fulton +1 位作者 Joan M.Dorn Barbara E.Ainsworth 《Journal of Sport and Health Science》 SCIE 2018年第1期34-41,共8页
Background: Despite their utility in accessing ambulatory movement, pedometers have not been used consistently to monitor physical activity in U.S. surveillance systems. This study was designed to determine the feasib... Background: Despite their utility in accessing ambulatory movement, pedometers have not been used consistently to monitor physical activity in U.S. surveillance systems. This study was designed to determine the feasibility of using pedometers to assess daily steps taken in a sub-sample of adults from Maricopa County who completed the 2014 Arizona Behavioral Risk Factor Surveillance System Survey.Methods: Respondents were sent an Omron HJ324 U pedometer, a logbook to record steps taken, and a walking questionnaire. The pedometer was worn for 7 days. Feasibility was assessed for acceptability(interest in study), demand(procedures followed correctly), implementation(time to complete study), and practicality(cost).Results: Acceptability was modest with 23.9%(830/3476) agreeing to participate. Among those participating(92.9%; 771/830), 50.1%(386/771)returned the logbook. Demand was modest with 39.3%(303/771) of logbooks returned with valid data. Implementation represented 5 months to recruit participants. The cost to obtain valid step-count data was USD61.60 per person. An average of 6363 ± 3049 steps/day were taken with most participants classified as sedentary(36.0%) or low active(35.6%).Conclusion: The feasibility of using pedometers in a state-based surveillance system is modest at best. Feasibility may potentially be improved with easy-to-use pedometers where data can be electronically downloaded. 展开更多
关键词 ASSESSMENT MEASUREMENT Physical activity Public health
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2024 Wheelchair Compendium of Physical Activities:An update of activity codes and energy expenditure values 被引量:4
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作者 Scott A.Conger Stephen D.Herrmann +3 位作者 Erik A.Willis Tom E.Nightingale Joseph R.Sherman Barbara E.Ainsworth 《Journal of Sport and Health Science》 SCIE CSCD 2024年第1期18-23,共6页
Purpose:This paper presents an update of the 2011 Wheelchair Compendium of Physical Activities designed for wheelchair users and is referred to as the 2024 Wheelchair Compendium.The Wheelchair Compendium aims to curat... Purpose:This paper presents an update of the 2011 Wheelchair Compendium of Physical Activities designed for wheelchair users and is referred to as the 2024 Wheelchair Compendium.The Wheelchair Compendium aims to curate existing knowledge of the energy expenditure for wheelchair physical activities(PAs).Methods:A systematic review of the published energy expenditure of PA for wheelchair users was completed between 2011 and May 2023.We added these data to the 2011 Wheelchair Compendium data that was compiled previously in a systematic review through 2011.Results:A total of 47 studies were included,and 124 different wheelchair PA reported energy expenditure values ranging from 0.8 metabolic equivalents for wheelchair users(filing papers,light effort)to 11.8 metabolic equivalents for wheelchair users(Nordic sit skiing).Conclusion:In introducing the updated 2024 Wheelchair Compendium,we hope to bridge the resource gap and challenge the prevailing narratives that inadvertently exclude wheelchair users from physical fitness and health PAs. 展开更多
关键词 DISABILITY EXERCISE MET Mobility
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General laws of funding for scientific citations:how citations change in funded and unfunded research between basic and applied sciences 被引量:1
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作者 Mario Coccia Saeed Roshani 《Journal of Data and Information Science》 CSCD 2024年第4期71-89,共19页
Purpose:The goal of this study is to analyze the relationship between funded and unfunded papers and their citations in both basic and applied sciences.Design/methodology/approach:A power law model analyzes the relati... Purpose:The goal of this study is to analyze the relationship between funded and unfunded papers and their citations in both basic and applied sciences.Design/methodology/approach:A power law model analyzes the relationship between research funding and citations of papers using 831,337 documents recorded in the Web of Science database.Findings:The original results reveal general characteristics of the diffusion of science in research fields:a)Funded articles receive higher citations compared to unfunded papers in journals;b)Funded articles exhibit a super-linear growth in citations,surpassing the increase seen in unfunded articles.This finding reveals a higher diffusion of scientific knowledge in funded articles.Moreover,c)funded articles in both basic and applied sciences demonstrate a similar expected change in citations,equivalent to about 1.23%,when the number of funded papers increases by 1%in journals.This result suggests,for the first time,that funding effect of scientific research is an invariant driver,irrespective of the nature of the basic or applied sciences.Originality/value:This evidence suggests empirical laws of funding for scientific citations that explain the importance of robust funding mechanisms for achieving impactful research outcomes in science and society.These findings here also highlight that funding for scientific research is a critical driving force in supporting citations and the dissemination of scientific knowledge in recorded documents in both basic and applied sciences.Practical implications:This comprehensive result provides a holistic view of the relationship between funding and citation performance in science to guide policymakers and R&D managers with science policies by directing funding to research in promoting the scientific development and higher diffusion of results for the progress of human society. 展开更多
关键词 Research funding CITATIONS Scientific development Science diffusion Scientific laws Power law model Matthew effect Science policy Research policy Science of science Dynamics of science Evolution of science
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A brief history of the Compendium of Physical Activities 被引量:2
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作者 Barbara E.Ainsworth Stephen D.Herrmann +2 位作者 David R.Jacobs Jr. Melicia C.Whitt-Glover Catrine Tudor-Locke 《Journal of Sport and Health Science》 SCIE CSCD 2024年第1期3-5,共3页
The Compendium of Physical Activities(Compendium)was developed to address consistent assignment of physical activity(PA)intensity values used in PA epidemiology research of the association between PA and health outcom... The Compendium of Physical Activities(Compendium)was developed to address consistent assignment of physical activity(PA)intensity values used in PA epidemiology research of the association between PA and health outcomes.1The known protective effects of PA on incident health outcomes traces to the mid-1900s,with over 50 studies examining coronary heart disease(CHD)as the outcome of interest. 展开更多
关键词 EPIDEMIOLOGY ACTIVITIES protective
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2024 Adult Compendium of Physical Activities:A third update of the energy costs of human activities 被引量:10
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作者 Stephen D.Herrmann Erik A.Willis +10 位作者 Barbara E.Ainsworth Tiago V.Barreira Mary Hastert Chelsea L.Kracht John M.Schuna Jr. Zhenghui Cai Minghui Quan Catrine Tudor-Locke Melicia C.Whitt-Glover David R. Jacobs Jr. 《Journal of Sport and Health Science》 SCIE CSCD 2024年第1期6-12,共7页
Background:The Compendium of Physical Activities was published in 1993 to improve the comparability of energy expenditure values assigned to self-reported physical activity(PA)across studies.The original version was u... Background:The Compendium of Physical Activities was published in 1993 to improve the comparability of energy expenditure values assigned to self-reported physical activity(PA)across studies.The original version was updated in 2000,and again in 2011,and has been widely used to support PA research,practice,and public health guidelines.Methods:This 2024 update was tailored for adults 19-59 years of age by removing data from those≥60 years.Using a systematic review and supplementary searches,we identified new activities and their associated measured metabolic equivalent(MET)values(using indirect calorimetry)published since 2011.We replaced estimated METs with measured values when possible.Results:We screened 32,173 abstracts and 1507 full-text papers and extracted 2356 PA energy expenditure values from 701 papers.We added303 new PAs and adjusted 176 existing MET values and descriptions to reflect the addition of new data and removal of METs for older adults.We added a Major Heading(Video Games).The 2024 Adult Compendium includes 1114 PAs(912 with measured and 202 with estimated values)across 22 Major Headings.Conclusion:This comprehensive update and refinement led to the creation of The 2024 Adult Compendium,which has utility across research,public health,education,and healthcare domains,as well as in the development of consumer health technologies.The new website with the complete lists of PAs and supporting resources is available at https://pacompendium.com. 展开更多
关键词 ADULTS Energy expenditure EXERCISE MET Physical Activities
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Effect of corrosion behavior of cast and extruded ZK60 magnesium alloys processed via friction extrusion
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作者 A.Sharma V.Beura +7 位作者 D.Zhang J.Darsell S.Niverty V.Prabhakaran N.Overman D.R.Herling V.Joshi K.Solanki 《Journal of Magnesium and Alloys》 SCIE EI CAS CSCD 2024年第9期3553-3573,共21页
The increasing demand for high-strength,corrosion-resistant magnesium alloys in transportation has led to the development of new processing techniques.In this work,cast and extruded ZK60 magnesium alloys were processe... The increasing demand for high-strength,corrosion-resistant magnesium alloys in transportation has led to the development of new processing techniques.In this work,cast and extruded ZK60 magnesium alloys were processed using the innovative solid-phase process,Friction Extrusion(FE).The microstructure was analyzed using Scanning Electron Microscopy(SEM),and Energy Dispersive Spectroscopy(EDS),showing a marked reduction in grain size,uniform solute distribution(Zn and Zr),and second phases after FE processing.Moreover,optical micrographs and Electron Backscatter Diffraction(EBSD)were employed to further evaluate the alloy microstructure.The corro-sion resistance and electrochemical behavior were analyzed using potentiodynamic polarization,Scanning Electrochemical Cell Impedance Microscopy(SECCIM),and atomic emission spectroelectrochemistry analysis(AESEC).Time evolution surface imaging and post-corrosion microstructures were also analyzed to support the understanding of underlying corrosion mechanisms.Corrosion initiation and propagation in FE-processed samples followed grain boundary patterns,differing from cast and extruded ZK60 behaviors.Electrochemical measurements and in-situ time-dependent optical imaging demonstrated that FE processing enhanced corrosion potential,reduced corrosion current,and increased cathodic activity.Additionally,FE processing reduced the disparity in pitting potential between cast and extruded samples,resulting in intermediate pitting potentials.Higher Mg and lower Zn dissolution was observed in the lower anodic currents for FE-processed samples.During aggravated anodic current cycles,Mg dissolution equalized,but the Zn/Mg dissolution ratio increased for FE-processed extruded samples,suggesting less cathodic activation and better resistance to further pitting. 展开更多
关键词 Magnesium alloys Corrosion Atomic emission spectroelectrochemistry analysis Scanning electron microscopy
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Research funding and citations in papers of Nobel Laureates in Physics, Chemistry and Medicine, 2019-2020
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作者 Mario Coccia Saeed Roshani 《Journal of Data and Information Science》 CSCD 2024年第2期56-80,共25页
Purpose:The goal of this study is a comparative analysis of the relation between funding(a main driver for scientific research)and citations in papers of Nobel Laureates in physics,chemistry and medicine over 2019-202... Purpose:The goal of this study is a comparative analysis of the relation between funding(a main driver for scientific research)and citations in papers of Nobel Laureates in physics,chemistry and medicine over 2019-2020 and the same relation in these research fields as a whole.Design/methodology/approach:This study utilizes a power law model to explore the relationship between research funding and citations of related papers.The study here analyzes 3,539 recorded documents by Nobel Laureates in physics,chemistry and medicine and a broader dataset of 183,016 documents related to the fields of physics,medicine,and chemistry recorded in the Web of Science database.Findings:Results reveal that in chemistry and medicine,funded researches published in papers of Nobel Laureates have higher citations than unfunded studies published in articles;vice versa high citations of Nobel Laureates in physics are for unfunded studies published in papers.Instead,when overall data of publications and citations in physics,chemistry and medicine are analyzed,all papers based on funded researches show higher citations than unfunded ones.Originality/value:Results clarify the driving role of research funding for science diffusion that are systematized in general properties:a)articles concerning funded researches receive more citations than(un)funded studies published in papers of physics,chemistry and medicine sciences,generating a high Matthew effect(a higher growth of citations with the increase in the number of papers);b)research funding increases the citations of articles in fields oriented to applied research(e.g.,chemistry and medicine)more than fields oriented towards basic research(e.g.,physics).Practical implications:The results here explain some characteristics of scientific development and diffusion,highlighting the critical role of research funding in fostering citations and the expansion of scientific knowledge.This finding can support decision-making of policymakers and R&D managers to improve the effectiveness in allocating financial resources in science policies to generate a higher positive scientific and societal impact. 展开更多
关键词 Research funding CITATIONS Science diffusion Scientific change Science of Science Power-law distribution Basic research Applied research Matthew effect Nobel Laureates Nobel Prizes
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A systematic scoping review of study methodology for randomized controlled trials investigating probiotics in athletic and physically active populations
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作者 Alex E.Mohr David B.Pyne +2 位作者 Geovana Silva Fogaça Leite Deborah Akins Jamie Pugh 《Journal of Sport and Health Science》 SCIE CSCD 2024年第1期61-71,共11页
Background:The purported ergogenic and health effects of probiotics have been a topic of great intrigue among researchers,practitioners,and the lay public alike.There has also been an increased research focus within t... Background:The purported ergogenic and health effects of probiotics have been a topic of great intrigue among researchers,practitioners,and the lay public alike.There has also been an increased research focus within the realm of sports science and exercise medicine on the athletic gut microbiota.However,compared to other ergogenic aids and dietary supplements,probiotics present unique study challenges.The objectives of this systematic scoping review were to identify and characterize study methodologies of randomized controlled trials investigating supplementation with probiotics in athletes and physically active individuals.Methods:Four databases(MEDLINE,CINAHL,Cochrane CENTRAL,and Cochrane Database of Systematic Reviews)were searched for randomized controlled studies involving healthy athletes or physically active individuals.An intervention with probiotics and inclusion of a control and/or placebo group were essential.Only peer-reviewed articles in English were considered,and there were no date restrictions.Results were extracted and presented in tabular form to detail study protocols,characteristics,and outcomes.Bias in randomized controlled trials was determined with the RoB 2.0 tool.Results:A total of 45 studies were included in the review,with 35 using a parallel group design and 10 using a cross-over design.Approximately half the studies used a single probiotic and the other half a multi-strain preparation.The probiotic dose ranged from 2×10^(8)to 1×10^(11)colony forming units daily,and the length of intervention was between 7 and 150 days.Fewer than half the studies directly assessed gastrointestinal symptoms,gut permeability,or the gut microbiota.The sex ratio of participants was heavily weighted toward males,and only 3 studies exclusively investigated females.Low-level adverse events were reported in only 2 studies,although the methodology of reporting varied widely.The risk of bias was generally low,although details on randomization were lacking in some studies.Conclusion:There is a substantial body of research on the effects of prob iotic supplementation in healthy athletes and physically active individuals.Considerable heterogeneity in probiotic selection and dosage as well as outcome measures has made clinical and mechanistic interpretation challenging for both health care practitioners and researchers.Attention to issues of randomization of participants,treatments and interventions,selection of outcomes,demographics,and reporting of adverse events will facilitate more trustworthy interpretation of probiotic study results and inform evidence-based guidelines. 展开更多
关键词 EXERCISE Experimental methodology Gastrointestinal symptoms Gut microbiota Probiotic supplementation
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Promoting public health through the 2024 Compendium of Physical Activities:Strategies for adults,older adults,and wheelchair users
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作者 Stephen D.Herrmann Scott A.Conger +1 位作者 Erik A.Willis Barbara E.Ainsworth 《Journal of Sport and Health Science》 SCIE CAS CSCD 2024年第6期739-742,共4页
Physical activity(PA)is fundamentally linked to public health,^(1)providing benefits including chronic disease prevention and treatment,^(2)mental health,^(3)musculoskeletal health,^(4)and healthy aging,^(5)along with... Physical activity(PA)is fundamentally linked to public health,^(1)providing benefits including chronic disease prevention and treatment,^(2)mental health,^(3)musculoskeletal health,^(4)and healthy aging,^(5)along with socioeconomic advantages.^(6)These benefits highlight the importance of promoting PA for all populations.The recent publication of the Compendium of Physical Activities(Compendium)serves as a valuable resource,^(7)offering an updated and expanded guide for adults(ages 19-59)with tailored energy cost values for diverse populations. 展开更多
关键词 ACTIVITIES PREVENTION offering
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Global prevalence and gender inequalities in at least 60 min of self-reported moderate-to-vigorous physical activity 1 or more days per week:An analysis with 707,616 adolescents
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作者 Raphael H.O.Araujo AndrúO.Werneck +13 位作者 Clarice L.Martins Luciana L.Barboza Rafael M.Tassitano Nicolas Aguilar-Farias Gilmar M.Jesus Robinson Ramírez-Véelez Riki Tesler Adewale L.Oyeyemi Ellen C.M.Silva Robert G.Weaver Mark S.Tremblay Javier Brazo-Sayavera Grégore I.Mielke Danilo R.P.Silva 《Journal of Sport and Health Science》 SCIE CAS CSCD 2024年第5期709-716,共8页
Background:Guidelines recommend that adolescents should accumulate an average of 60 min per day of moderate-to-vigorous physical activity(MVPA).However,using only this cut-off could hide important information.For inst... Background:Guidelines recommend that adolescents should accumulate an average of 60 min per day of moderate-to-vigorous physical activity(MVPA).However,using only this cut-off could hide important information.For instance,from a population-level point of view,increasing physical activity for those with no or low physical activity could provide more health benefits than increasing physical activity for those with intermediate levels.Also,including a more sensitive cut-point of≥1 days per week could be an additional strategy for identifying those with low access/opportunities for physical activity practice.Thus,the current study aims to estimate the prevalence of≥60 min of MVPA≥1 days per week among adolescents globally,and to describe any relevant gender inequalities.Methods:We used representative datasets from 146 countries/territories collected between 2003 and 2019.MVPA was self-reported.Participants were grouped into younger(≤14 years old)and older(>14 years old)adolescents.Crude Poisson regression models were used to identify the relative differences in≥60 min of MVPA≥1 days per week between boys and girls,and random-effects meta-analysis models were used to identify the pooled estimates.Analyses were stratified by country and region.Results:Approximately 80%of both younger and older adolescents reported≥60 min of MVPA≥1 days per week.This prevalence was≥94%in Europe and Central Asia and North America,while the estimates for the other regions were<77%.The prevalence of≥60 min of MVPA≥1 days per week was higher among boys than girls,with the largest differences occurring among the oldest adolescents(Prevalence ratio_(≤14y)=1.04(95%confidence interval(95%CI)):1.03-1.04)vs.Prevalence ratio_(>14y)=1.09(95%CI:1.08-1.10)).Conclusion:Approximately 8 out of 10 adolescents reported accumulating≥60 min of MVPA≥1 days per week,with notable differences between regions.Gender differences were observed in several countries,especially among the oldest adolescents.Priorities for physical activity promotion among adolescents should include increasing access/opportunities for physical activity among those who do not achieve≥60 min of MVPA≥1 days per week and reducing gender inequalities. 展开更多
关键词 Global School-based Student Health Survey Health Behaviour Among School-aged Children survey Inequality Surveillance Youth
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Measured and Predicted Aging Properties of Arizona Asphalt Binders
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作者 Krishna Prapooma Biligiril George Bert Way 《Journal of Civil Engineering and Architecture》 2011年第4期297-313,共17页
The Arizona Department of Transportation (ADOT) in the USA conducted a series of asphalt aging related research and special studies between the 1970s and 1990s. The studies covered over 157 test sections representin... The Arizona Department of Transportation (ADOT) in the USA conducted a series of asphalt aging related research and special studies between the 1970s and 1990s. The studies covered over 157 test sections representing both neat (virgin) asphalt and crumb rubber modified (asphalt-rubber) binders. The data comprised of a wide range of penetration, viscosity, and Performance Grade (PG) parameters, at original and aged conditions. In the late 1990s, asphalt PG complex shear modulus (G*), and phase angle (5) data were collected. The main purpose of this paper was to use the assembled database of the field core-aged asphalt test data and compare the test results to the American Association of State Highway and Transportation Officials approved Mechanistic-Empirical Pavement Design Guide (MEPDG) predictive modeled asphalt properties such as penetration and viscosity, G*, and 5. Furthermore, G* and laboratory measurements on neat and asphalt-rubber binders extracted from the field cores of the pavement sections aged ten or more years were compared to the pressure aging vessel PG G* and ~. values. It was observed that the MEPDG predicted asphalt binder properties were rational for originally (tank) sampled binders, but fairly correlated for the aged binders. Additionally, penetration and viscosity aging indices representing over 20 years of field aged sections were established for a wide variety of asphalt binder grades. Overall, the relationships for aging indices were meaningful and rational. Results of this research indicated the degree of difficulty in predicting asphalt binder properties for pavements with ten or more years of field aging. The findings from this research study are envisioned to be of substantial value in future asphalt binder aging studies. 展开更多
关键词 AGING neat asphalt asphalt-rubber binder shear modulus phase angle PENETRATION VISCOSITY performance-grade
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Statins and Metformin Use Is Associated with Lower PSA Levels in Prostate Cancer Patients Presenting for Radiation Therapy
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作者 Xiaonan Liu Jing Li +5 位作者 Steven E. Schild Michael H. Schild William Wong Sujay Vora Michael G. Herman Mirek Fatyga 《Journal of Cancer Therapy》 2017年第2期73-85,共13页
Background: A possible association between the level of prostate specific antigen (PSA) and the use of some commonly prescribed medications has been reported in recent studies. Most of these studies were carried out i... Background: A possible association between the level of prostate specific antigen (PSA) and the use of some commonly prescribed medications has been reported in recent studies. Most of these studies were carried out in general populations of men who were screened for prostate cancer using the PSA test. We reported on the association between the initial PSA level and the use of statins, metformin and alpha-blockers in patients who were diagnosed with prostate cancer and presented for radiation therapy. Methods: Three hundred and eighty one patients treated between the years of 2000-2005 and 2009-2012 were included in this retrospective study. The information about statin, metformin and alpha-blockers use was recorded immediately prior to treatment. Differences in PSA levels prior to treatment by medication status were estimated using univariate and multivariate linear regression on log PSA values. Results: Compared with men who were not on these medications, the PSA level at presentation was 20% lower for statin users (p = 0.002) and 33% lower for metformin users (p = 0.004). We did not observe statistically significant associations between the use of statins or metformin and cancer stage, National Comprehensive Cancer Network (NCCN) risk score, or therapy outcome. A statistically significant association between the NCCN risk score and the use of alpha-blockers was observed (p = 0.002). Conclusions: We found that statins and metformin were associated with lower PSA levels in prostate cancer patients to an extent that could influence management decisions. We found no statistically significant associations between the use of these medications and treatment outcomes. 展开更多
关键词 PSA STATINS METFORMIN PROSTATE Cancer
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Trade-offs between ion-conducting and mechanical properties: The case of polyacrylate electrolytes 被引量:2
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作者 Guoli Lu Yaojian Zhang +7 位作者 Jianjun Zhang Xiaofan Du Zhaolin Lv Junzhe Du Zhiming Zhao Yue Tang Jingwen Zhao Guanglei Cui 《Carbon Energy》 SCIE CSCD 2023年第2期24-60,共37页
Polymer electrolytes(PEs)have been long recognized as the key materials to enable energy-dense batteries and render flexible energy devices practically viable,owing to their chemical and mechanical reliability.However... Polymer electrolytes(PEs)have been long recognized as the key materials to enable energy-dense batteries and render flexible energy devices practically viable,owing to their chemical and mechanical reliability.However,much of their promise is yet to be realized.The roomtemperature ion conductivity of existing PEs still falls short of the implementation criterion of 10^(-4) S cm^(-1) on the promise of acceptable mechanical properties,thereby precluding their practical application.The twin but inversely related duties of polymers,that is,functioning as both an ion-conducting medium and a structural backbone,underlie this issue but are less elucidated systematically.The polyacrylate(PA)family is among promising polymer matrices on account of ester polarity,electrode compatibility,chemical tunability,and mechanical durability.The extensive applicability of PA in plasticized gels,dry solids,and emerging composites makes PA-based PEs representative to illustrate the trade-off between ion conduction and mechanical strength.We herein seek to outline the stated long-standing conflict exemplified by PA-based PEs,focusing on crucial strategies toward balancing and reconciling the two mutually exclusive properties,with the intention of offering designing guidelines for next-generation PEs. 展开更多
关键词 ionic conductivity lithium batteries mechanical properties POLYACRYLATE polymer electrolytes trade-offs
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Nucleation and growth control for iron-and phosphorus-rich phases from a modified steelmaking waste slag 被引量:1
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作者 Juncheng Li Guoxuan Li +7 位作者 Feng Qiu Rong Wang Jinshan Liang Yi Zhong Dong Guan Jingwei Li Seetharaman Sridhar Zushu Li 《International Journal of Minerals,Metallurgy and Materials》 SCIE EI CAS CSCD 2023年第2期378-387,共10页
Recovering the iron(Fe)and phosphorus(P)contained in steelmaking slags not only reduces the environmental burden caused by the accumulated slag,but also is the way to develop a circular economy and achieve sustainable... Recovering the iron(Fe)and phosphorus(P)contained in steelmaking slags not only reduces the environmental burden caused by the accumulated slag,but also is the way to develop a circular economy and achieve sustainable development in the steel industry.We had pre-viously found the possibility of recovering Fe and P resources,i.e.,magnetite(Fe_(3)O_(4)) and calcium phosphate(Ca_(10)P_(6)O_(25)),contained in steel-making slags by adjusting oxygen partial pressure and adding modifier B_(2)O_(3).As a fundamental study for efficiently recovering Fe and P from steelmaking slag,in this study,the crystallization behavior of the CaO-SiO_(2)-FeO-P_(2)O_(5)-B_(2)O_(3) melt has been observed in situ,using a confocal scanning laser microscope(CLSM).The kinetics of nucleation and growth of Fe-and P-rich phases have been calculated using a classical crys-tallization kinetic theory.During cooling,a Fe_(3)O_(4) phase with faceted morphology was observed as the 1st precipitated phase in the isothermal interval of 1300-1150℃,while Ca_(10)P_(6)O_(25),with rod-shaped morphology,was found to be the 2nd phase to precipitate in the interval of 1150-1000℃.The crystallization abilities of Fe_(3)O_(4) and Ca_(10)P_(6)O_(25) phases in the CaO-SiO_(2)-FeO-P_(2)O_(5)-B_(2)O_(3) melt were quantified with the in-dex of(T_(U)−T_(I))/T_(I)(where T_(I) represents the peak temperature of the nucleation rate and TU stands for that of growth rate),and the crystalliza-tion ability of Fe_(3)O_(4) was found to be larger than that of Ca_(10)P_(6)O_(25) phase.The range of crystallization temperature for Fe_(3)O_(4) and Ca_(10)P_(6)O_(25) phases was optimized subsequently.The Fe_(3)O_(4) and Ca_(10)P_(6)O_(25) phases are the potential sources for ferrous feedstock and phosphate fertilizer,respectively. 展开更多
关键词 steelmaking slag MAGNETITE calcium phosphate NUCLEATION GROWTH KINETICS
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Switching CO_(2) Electroreduction Selectivity Between C_(1) and C_(2) Hydrocarbons on Cu Gas-Diffusion Electrodes 被引量:1
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作者 Jianfang Zhang Zhengyuan Li +6 位作者 Rui Cai Tianyu Zhang Shize Yang Lu Ma Yan Wang Yucheng Wu Jingjie Wu 《Energy & Environmental Materials》 SCIE EI CAS CSCD 2023年第2期17-25,共9页
Regulating the selectivity toward a target hydrocarbon product is still the focus of CO_(2)electroreduction.Here,we discover that the original surface Cu species in Cu gas-diffusion electrodes plays a more important r... Regulating the selectivity toward a target hydrocarbon product is still the focus of CO_(2)electroreduction.Here,we discover that the original surface Cu species in Cu gas-diffusion electrodes plays a more important role than the surface roughness,local pH,and facet in governing the selectivity toward C_(1)or C_(2)hydrocarbons.The selectivity toward C_(2)H_(4) progressively increases,while CH_(4) decreases steadily upon lowering the Cu oxidation species fraction.At a relatively low electrodeposition voltage of 1.5 V,the Cu gas-diffusion electrode with the highest Cu^(δ+)/Cu^(0)ratio favors the pathways of∗CO hydrogenation to form CH_(4) with maximum Faradaic efficiency of 65.4%and partial current density of 228 mA cm^(−2)at−0.83 V vs RHE.At 2.0 V,the Cu gas-diffusion electrode with the lowest Cu^(δ+)/Cu^(0)ratio prefers C-C coupling to form C_(2)+products with Faradaic efficiency topping 80.1%at−0.75 V vs RHE,where the Faradaic efficiency of C_(2)H_(4) accounts for 46.4%and the partial current density of C_(2)H_(4) achieves 279 mA cm^(−2).This work demonstrates that the selectivity from CH_(4) to C_(2)H_(4) is switchable by tuning surface Cu species composition of Cu gas-diffusion electrodes. 展开更多
关键词 C_(2)H_(4) CH_(4) CO_(2)electroreduction ELECTRODEPOSITION switchable selectivity
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Public health research on physical activity and COVID-19:Progress and updated priorities 被引量:1
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作者 James F.Sallis Deepti Adlakha +1 位作者 Adewale Oyeyemi Deborah Salvo 《Journal of Sport and Health Science》 SCIE CAS CSCD 2023年第5期553-556,F0003,共5页
1.Introduction Before coronavirus disease 2019 (COVID-19) became a global health emergency in early 2020,there was substantial evidence of physical activity’s (PA’s) multiple benefits with direct relevance to reduci... 1.Introduction Before coronavirus disease 2019 (COVID-19) became a global health emergency in early 2020,there was substantial evidence of physical activity’s (PA’s) multiple benefits with direct relevance to reducing the harms of the pandemic:improved immune functioning and reduced inflammation to lessen severity of infections,enhanced efficacy of vaccines. 展开更多
关键词 INFLAMMATION SEVERITY vaccines
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Activation of Transition Metal(Fe,Co and Ni)-Oxide Nanoclusters by Nitrogen Defects in Carbon Nanotube for Selective CO_(2) Reduction Reaction 被引量:1
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作者 Yi Cheng Jinfan Chen +7 位作者 Chujie Yang Huiping Wang Bernt Johannessen Lars Thomsen Martin Saunders Jianping Xiao Shize Yang San Ping Jiang 《Energy & Environmental Materials》 SCIE EI CAS CSCD 2023年第1期253-263,共11页
The electrochemical carbon dioxide reduction reaction(CO_(2)RR),which can produce value-added chemical feedstocks,is a proton-coupled-electron process with sluggish kinetics.Thus,highly efficient,cheap catalysts are u... The electrochemical carbon dioxide reduction reaction(CO_(2)RR),which can produce value-added chemical feedstocks,is a proton-coupled-electron process with sluggish kinetics.Thus,highly efficient,cheap catalysts are urgently required.Transition metal oxides such as CoO_(x),FeO_(x),and NiO_(x)are low-cost,low toxicity,and abundant materials for a wide range of electrochemical reactions,but are almost inert for CO_(2)RR.Here,we report for the first time that nitrogen doped carbon nanotubes(N-CNT)have a surprising activation effect on the activity and selectivity of transition metal-oxide(MO_(x)where M=Fe,Ni,and Co)nanoclusters for CO_(2)RR.MO_(x)supported on N-CNT,MO_(x)/N-CNT,achieves a CO yield of 2.6–2.8 mmol cm−2 min−1 at an overpotential of−0.55 V,which is two orders of magnitude higher than MO_(x)supported on acid treated CNTs(MO_(x)/O-CNT)and four times higher than pristine N-CNT.The faraday efficiency for electrochemical CO_(2)-to-CO conversion is as high as 90.3%at overpotential of 0.44 V.Both in-situ XAS measurements and DFT calculations disclose that MO_(x)nanoclusters can be hydrated in CO_(2)saturated KHCO_(3),and the N defects of N-CNT effectively stabilize these metal hydroxyl species under carbon dioxide reduction reaction conditions,which can split the water molecules and provide local protons to inhibit the poisoning of active sites under carbon dioxide reduction reaction conditions. 展开更多
关键词 activation effect electrochemical CO_(2)reduction reaction N defect proton-coupled electron transfer process transition metal oxide nanocluster
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One-step ethylene separation from ternary C_(2) hydrocarbon mixture with a robust zirconium metal-organic framework
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作者 Yuan Liu Hanting Xiong +5 位作者 Jingwen Chen Shixia Chen Zhenyu Zhou Zheling Zeng Shuguang Deng Jun Wang 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2023年第7期9-15,共7页
One-step separation of high-purity ethylene(C_(2)H_(4))from C_(2) hydrocarbon mixture is critical but challenging because of the very similar molecular sizes and physical properties of C_(2)H_(4),ethane(C_(2)H_(6)),an... One-step separation of high-purity ethylene(C_(2)H_(4))from C_(2) hydrocarbon mixture is critical but challenging because of the very similar molecular sizes and physical properties of C_(2)H_(4),ethane(C_(2)H_(6)),and acetylene(C_(2)H_(2)).Herein,we report a robust zirconium metal-organic framework(MOF)Zr-TCA(H3TCA=4,4',4"-tricarboxytriphenylamine)with suitable pore size(0.6 nm×0.7 nm)and pore environment for direct C_(2)H_(4) purification from C_(2)H_(4)/C_(2)H_(2)/C_(2)H_(6) gas-mixture.Computational studies indicate that the abundant oxygen atoms and non-polar phenyl rings created favorable pore environments for the preferential binding of C_(2)H_(2) and C_(2)H_(6) over C_(2)H_(4).As a result,Zr-TCA exhibits not only high C_(2)H_(6)(2.28 mmol·g^(-1))and C_(2)H_(2)(2.78 mmol·g^(-1))adsorption capacity but also excellent C_(2)H_(6)/C_(2)H_(4)(2.72)and C_(2)H_(2)/C_(2)H_(4)(5.64)selectivity,surpassing most of one-step C_(2)H_(4) purification MOF materials.Dynamic breakthrough experiments confirm that Zr-TCA can produce high-purity C_(2)H_(4)(>99.9%)from a ternary gas mixture(1/9/90 C_(2)H_(2)/C_(2)H_(6)/C_(2)H_(4))in a single step with a high C_(2)H_(4) productivity of 5.61 L·kg^(-1). 展开更多
关键词 Zirconium metal-organic framework Adsorption Separation One-step ethylene purification
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Novel multi‐domain attention for abstractive summarisation
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作者 Chunxia Qu Ling Lu +2 位作者 Aijuan Wang Wu Yang Yinong Chen 《CAAI Transactions on Intelligence Technology》 SCIE EI 2023年第3期796-806,共11页
The existing abstractive text summarisation models only consider the word sequence correlations between the source document and the reference summary,and the summary generated by models lacks the cover of the subject ... The existing abstractive text summarisation models only consider the word sequence correlations between the source document and the reference summary,and the summary generated by models lacks the cover of the subject of source document due to models'small perspective.In order to make up these disadvantages,a multi‐domain attention pointer(MDA‐Pointer)abstractive summarisation model is proposed in this work.First,the model uses bidirectional long short‐term memory to encode,respectively,the word and sentence sequence of source document for obtaining the semantic representations at word and sentence level.Furthermore,the multi‐domain attention mechanism between the semantic representations and the summary word is established,and the proposed model can generate summary words under the proposed attention mechanism based on the words and sen-tences.Then,the words are extracted from the vocabulary or the original word sequences through the pointer network to form the summary,and the coverage mechanism is introduced,respectively,into word and sentence level to reduce the redundancy of sum-mary content.Finally,experiment validation is conducted on CNN/Daily Mail dataset.ROUGE evaluation indexes of the model without and with the coverage mechanism are improved respectively,and the results verify the validation of model proposed by this paper. 展开更多
关键词 abstractive summarisation attention mechanism Bi‐LSTM coverage mechanism pointer network
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