针对LASG/IAP发展的大气环流模式GAMIL(Grid-point Atmospheric Model of IAP LASG)的两个版本GAMIL2(G2)和GAMIL3(G3),评估了其对热带降水气候态以及对流垂直结构的模拟能力,在此基础上探究了新版本模式降水模拟改进的原因以及热带对...针对LASG/IAP发展的大气环流模式GAMIL(Grid-point Atmospheric Model of IAP LASG)的两个版本GAMIL2(G2)和GAMIL3(G3),评估了其对热带降水气候态以及对流垂直结构的模拟能力,在此基础上探究了新版本模式降水模拟改进的原因以及热带对流垂直结构与降水模拟偏差的关系。两个版本的GAMIL模式都较好地捕捉到了热带降水的主要特征,且G3的模拟结果整体优于G2。新版本的主要改进在于显著减小了热带西北太平洋正降水偏差。水汽收支诊断显示,模式降水偏差主要来源于蒸发项和水汽垂直平流动力项,而后者的偏差则来自于对流强度和对流垂直结构的共同作用。对流垂直结构偏差主要存在于赤道印度洋与赤道大西洋区域,表现为大气低层辐合分量偏小,对流卷出层高度偏高;在热带西北太平洋与赤道东太平洋区域,模式较好地还原了典型的“头重型”和“脚重型”对流垂直结构,但依然存在有整体性的对流偏深。湿静力能(MSE)收支显示,热带西北太平洋区域过量的净能量通量是模式垂直运动偏差的主要来源。而对流垂直结构偏深造成的总湿稳定度(Gross Moist Stability,简称GMS)偏大,在一定程度上抵消了模式中的净能量通量偏差,抑制了模拟的对流强度。诊断结果显示,G3中热带西北太平洋区域的降水改善主要源于对流强度正偏差的减小。G3中对流阈值和层云阈值的下调,使得对流发生频率增加,从而抑制了过大的对流强度。热带对流垂直结构与降水偏差有着紧密且多样的联系,在未来模式发展中应当予以重视。展开更多
The integration of electrochemical CO_(2)reduction(CO_(2)RR) and photoelectrochemical water oxidation offers a sustainable access to valuable chemicals and fuels. Here, we develop a rapidly annealed hematite photoanod...The integration of electrochemical CO_(2)reduction(CO_(2)RR) and photoelectrochemical water oxidation offers a sustainable access to valuable chemicals and fuels. Here, we develop a rapidly annealed hematite photoanode with a photocurrent density of 2.83 mA cm^(-2)at 1.7 VRHEto drive the full-reaction. We also present Cu-alloys electrocatalysis extended from CuInSnS4, which are superior in both activity and selectivity for CO_(2)RR. Specifically, the screened CuInSn achieves a CO_(2)to HCOOH Faradaic efficiency of 93% at a cell voltage of-2.0 V by assembling into artificial photosynthesis cell. The stability test of IT exhibits less than 3% degradation over 24 h. Furthermore, in-situ Raman spectroscopy reveals that both CO_(3)^(-2)and CO_(2)are involved in CO_(2)RR as reactants. The preferential affinity of C for H in the ^(*)HCO_(2)intermediate enables an improved HCOOH-selectivity, highlighting the role of multifunctional Cu in reducing the cell voltage and enhancing the photocurrent density.展开更多
Electrocatalytic splitting of water by means of renewable energy as the electricity supply is one of the most promising methods for storing green renewable energy as hydrogen. Although two-thirds of the earth’s surfa...Electrocatalytic splitting of water by means of renewable energy as the electricity supply is one of the most promising methods for storing green renewable energy as hydrogen. Although two-thirds of the earth’s surface is covered with water, there is inadequacy of freshwater in most parts of the world. Hence, splitting seawater instead of freshwater could be a truly sustainable alternative. However, direct seawater splitting faces challenges because of the complex composition of seawater. The composition, and hence, the local chemistry of seawater may vary depending on its origin, and in most cases, tracking of the side reactions and standardizing and customizing the catalytic process will be an extra challenge. The corrosion of catalysts and competitive side reactions due to the presence of various inorganic and organic pollutants create challenges for developing stable electro-catalysts. Hence, seawater splitting generally involves a two-step process, i.e., purification of seawater using reverse osmosis and then subsequent fresh water splitting. However, this demands two separate chambers and larger space, and increases complexity of the reactor design. Recently, there have been efforts to directly split seawater without the reverse osmosis step. Herein, we represent the most recent innovative approaches to avoid the two-step process, and compare the potential application of membrane-assisted and membrane-less electrolyzers in direct seawater splitting(DSS). We particularly discuss the device engineering, and propose a novel electrolyzer design strategies for concentration gradient based membrane-less microfluidic electrolyzer.展开更多
本文应用WRF-Chem(Weather Research and Forecasting—Chemistry)模式研究中国东部地区气溶胶及其部分组分(硫酸盐、硝酸盐和黑碳气溶胶)在天气尺度下的辐射强迫和对地面气温的影响.5个无明显降水时间段(2006年8月23~25日、2008...本文应用WRF-Chem(Weather Research and Forecasting—Chemistry)模式研究中国东部地区气溶胶及其部分组分(硫酸盐、硝酸盐和黑碳气溶胶)在天气尺度下的辐射强迫和对地面气温的影响.5个无明显降水时间段(2006年8月23~25日、2008年11月10~12日、2008年12月16~18日、2009年1月15~17日和2009年4月27~29日)的模拟显示,气溶胶浓度呈现显著的白天低,夜间高的日变化特征,且北方区域(29.8°~42.6°N,110.2°~120.3°E)平均PM2.5近地面浓度(40~80μg m-3)高于南方区域(22.3°~29.9°N,109.7°~120.2°E,30~47 μg m-3).气溶胶对地面2m温度(地面气温)有明显的降温效果,在早上08:00(北京时,下同)和下午17:00左右最为显著,最高可降低约0.2~1 K,同时气溶胶的参与改善了模式对地面气温的模拟.本文还通过对2006年8月23~25日一次个例的模拟,定量分析了气溶胶及其部分组分(硫酸盐、硝酸盐和黑碳气溶胶)的总天气效应(直接效应+间接效应)、直接效应和间接效应分别对到达地面的短波辐射和地面气温的影响.北方区域平均气溶胶直接效应所造成的短波辐射强迫要高于南方区域,分别为-11.3 Wm^-2和-5.8Wm^-2,导致地面气温分别降低了0.074 K和0.039 K.南方区域平均气溶胶间接效应所产的短波辐射强迫高于北方区域,分别为-14.4 W m^-2和-12.4W m^-2,引起的地面气温的改变分别为-0.094K和-0.035K.对于气溶胶组分,硫酸盐气溶胶的直接效应和间接效应的作用相当,其总效应在北方和南方区域平均短波辐射强迫分别为-7.0 Wm^-2和-10.5 Wm^-2,对地面气温的影响为-0.062 K和-0.074 K,而硝酸盐气溶胶的作用略小.黑碳气溶胶使得北方和南方区域平均到达地表的太阳短波辐射分别减少了6.5 Wm^-2和5.8 W m^-2,而地表气温则分别增加了0.053 K和0.017 K,相比于间接效应,黑碳气溶胶的直接效应的影响更加显著.展开更多
利用WRF-Chem(Weather Research and Forecasting model coupled with Chemistry)模式研究2006年8月1日—9月1日中国区域硫酸盐和黑碳气溶胶对云特性的影响。模式验证利用了卫星和地面观测的气象要素、化学物质浓度、气溶胶光学特性和...利用WRF-Chem(Weather Research and Forecasting model coupled with Chemistry)模式研究2006年8月1日—9月1日中国区域硫酸盐和黑碳气溶胶对云特性的影响。模式验证利用了卫星和地面观测的气象要素、化学物质浓度、气溶胶光学特性和云微物理特性。模式性能评估表明该模式能较好地抓住气象要素(温度、降水、相对湿度和风速)的量级和空间分布特征。通过与地面观测和MODIS卫星数据对比发现,尽管模式模拟还存在偏差,但还是能较好模拟出气溶胶物种的地表浓度、气溶胶光学厚度(AOD)、云光学厚度(COD)、云量(CLDF)、云顶云滴有效半径(CER)和云水路径(LWP)。通过两个敏感性试验(分别增加二氧化硫和黑碳排放量至控制试验排放的3倍)与控制试验的对比发现硫酸盐比黑碳更易成为云凝结核,在中国东部云顶云滴数浓度和其它云特性参数对二氧化硫排放增加的响应均从北向南呈递增,这与地面湿度分布有关。云滴有效半径对硫酸盐气溶胶的响应符合气溶胶第一间接效应的定义,即硫酸盐气溶胶增多,云滴数浓度增加,云滴有效半径减少,但是对黑碳气溶胶的响应在各区域不尽相同。还发现黑碳对云量的影响远大于硫酸盐,主要原因是由于黑碳气溶胶直接辐射效应(对太阳光的吸收)导致的云的"燃烧"作用。展开更多
This paper investigates the variability of the break-up dates of the rivers in Northeast China from their icebound states for the period of 1957-2005 and explores some potential explanatory mechanisms. Results show th...This paper investigates the variability of the break-up dates of the rivers in Northeast China from their icebound states for the period of 1957-2005 and explores some potential explanatory mechanisms. Results show that the break-up of the two major rivers (the Heilongjiang River and Songhuajiang River) was about four days earlier, and their freeze-up was about 4-7 days delayed, during 1989 2005 as compared to 1971 1987. This interdecadal variation is evidently associated with the warming trend over the past 50 years. In addition, the break-up and freeze-up dates have large interannual variability, with a standard deviation of about 10-15 days. The break-up date is primarily determined by the January February-March mean surface air temperature over the Siberian-Northeast China region via changes in the melting rate, ice thickness, and snow cover over the ice cover. The interannual variability of the break-up date is also significantly connected with the Northern Annular Mode (NAM), with a correlation coefficient of 0.35-0.55 based on the data from four stations along the two rivers. This relationship is attributed to the fact that the NAM can modulate the East Asian winter monsoon circulation and Siberian-Northeast China surface air temperature in January February-March.展开更多
Projected changes in summer precipitation characteristics in China during the 21st century are assessed using the monthly precipitation outputs of the ensemble of three "best" models under the Special Report on Emis...Projected changes in summer precipitation characteristics in China during the 21st century are assessed using the monthly precipitation outputs of the ensemble of three "best" models under the Special Report on Emissions Scenarios (SRES) A1B, A2, and B1 scenarios. The excellent reproducibility of the models both in spatial and temporal patterns for the precipitation in China makes the projected summer precipitation change more believable for the future 100 years. All the three scenarios experiments indicate a consistent enhancement of summer precipitation in China in the 21st century. However, the projected summer precipitation in China demonstrates large variability between sub-regions. The projected increase in precipitation in South China is significant and persistent, as well as in North China. Meanwhile, in the early period of the 21st century, the region of Northeast China is projected to be much drier than the present. But, this situation changes and the precipitation intensifies later, with a precipitation anomaly increase of 12.4%0-20.4% at the end of the 21st century. The region of the Xinjiang Province probably undergoes a drying trend in the future 100 years, and is projected to decrease by 1.7%-3.6% at the end of the 21st century. There is no significant long-term change of the projected summer precipitation in the lower reaches of the Yangtze River valley. A high level of agreement of the ensemble of the regional precipitation change in some parts of China is found across scenarios but smaller changes are projected for the B1 scenario and slightly larger changes for the A2 scenario.展开更多
A unified chemistry-aerosol-climate model is applied in this work to compare climate responses to changing concentrations of long-lived greenhouse gases (GHGs, CO2, CH4, N2O), tropospheric O3, and aerosols during th...A unified chemistry-aerosol-climate model is applied in this work to compare climate responses to changing concentrations of long-lived greenhouse gases (GHGs, CO2, CH4, N2O), tropospheric O3, and aerosols during the years 1951-2000. Concentrations of sulfate, nitrate, primary organic carbon (POA), secondary organic carbon (SOA), black carbon (BC) aerosols, and tropospheric 03 for the years 1950 and 2000 are obtained a priori by coupled chemistry-aerosol-GCM simulations, and then monthly concentrations are interpolated linearly between 1951 and 2000. The annual concentrations of GHGs are taken from the IPCC Third Assessment Report. BC aerosol is internally mixed with other aerosols. Model results indicate that the sinmlated climate change over 1951-2000 is sensitive to anthropogenic changes in atmospheric components. The predicted year 2000 global mean surface air temperature can differ by 0.8℃ with different forcings. Relative to the climate simulation without changes in GHGs, O3, and aerosols, anthropogenic forcings of SO4^2-, BC, BC+SO4^2-, BC+SO4^2- +POA, BC+SO4^2- +POA+SOA+NO3^-, O3, and GHGs are predicted to change the surface air temperature averaged over 1971-2000 in eastern China, respectively, by -0.40℃, +0.62℃, +0.18℃, +0.15℃, -0.78℃, +0.43℃, and +0.85℃, and to change the precipitation, respectively, by -0.21, +0.07, -0.03, +0.02, -0.24, -0.08, and +0.10 mm d^-1. The authors conclude that all major aerosols are as important as GHGs in influencing climate change in eastern China, and tropospheric O3 also needs to be included in studies of regional climate change in China.展开更多
Recent observational study has shown that the southern center of the summer North Atlantic Oscillation (SNAO) was located farther eastward after the late 1970s compared to before. In this study, the cause for this p...Recent observational study has shown that the southern center of the summer North Atlantic Oscillation (SNAO) was located farther eastward after the late 1970s compared to before. In this study, the cause for this phenomenon is explored. The result shows that the eastward shift of the SNAO southern center after the late 1970s is related to the variability of the Mediterranean-Black Sea (MBS) SST. A warm MBS SST can heat and moisten its overlying atmosphere, consequently producing a negative sea level pressure (SLP) departure over the MBS region. Because the MBS SST is negatively correlated with the SNAO, the negative SLP departure can enhance the eastern part of the negative-phase of the SNAO southern center, consequently producing an eastward SNAO southern center shift. Similarly, a cold MBS SST produces an eastward positive-phase SNAO southern center shift. The reason for why the MBS SST has an impact on the SNAO after the late 1970s but why it is not the case beforehand is also discussed. It is found that this instable relationship is likely to be attributed to the change of the variability of the MBS SST on the decadal time-scale. In 1951 1975, the variability of the MBS SST is quite weak, but in 1978 2002, it becomes more active. The active SST can enhance the interaction between the sea and its overlying atmosphere, thus strengthening the connection between the MBS SST and the SNAO after the late 1970s. The above observational analysis results are further confirmed by sensitivity experiments.展开更多
文摘针对LASG/IAP发展的大气环流模式GAMIL(Grid-point Atmospheric Model of IAP LASG)的两个版本GAMIL2(G2)和GAMIL3(G3),评估了其对热带降水气候态以及对流垂直结构的模拟能力,在此基础上探究了新版本模式降水模拟改进的原因以及热带对流垂直结构与降水模拟偏差的关系。两个版本的GAMIL模式都较好地捕捉到了热带降水的主要特征,且G3的模拟结果整体优于G2。新版本的主要改进在于显著减小了热带西北太平洋正降水偏差。水汽收支诊断显示,模式降水偏差主要来源于蒸发项和水汽垂直平流动力项,而后者的偏差则来自于对流强度和对流垂直结构的共同作用。对流垂直结构偏差主要存在于赤道印度洋与赤道大西洋区域,表现为大气低层辐合分量偏小,对流卷出层高度偏高;在热带西北太平洋与赤道东太平洋区域,模式较好地还原了典型的“头重型”和“脚重型”对流垂直结构,但依然存在有整体性的对流偏深。湿静力能(MSE)收支显示,热带西北太平洋区域过量的净能量通量是模式垂直运动偏差的主要来源。而对流垂直结构偏深造成的总湿稳定度(Gross Moist Stability,简称GMS)偏大,在一定程度上抵消了模式中的净能量通量偏差,抑制了模拟的对流强度。诊断结果显示,G3中热带西北太平洋区域的降水改善主要源于对流强度正偏差的减小。G3中对流阈值和层云阈值的下调,使得对流发生频率增加,从而抑制了过大的对流强度。热带对流垂直结构与降水偏差有着紧密且多样的联系,在未来模式发展中应当予以重视。
基金financially supported by the National Key R&D Program of China (2018YFE0208500)the National Natural Science Foundation of China (Grants No. 22072022)funded by King Abdullah University of Science and Technology (KAUST) through the baseline funding (BAS/1/1413-01-01)。
文摘The integration of electrochemical CO_(2)reduction(CO_(2)RR) and photoelectrochemical water oxidation offers a sustainable access to valuable chemicals and fuels. Here, we develop a rapidly annealed hematite photoanode with a photocurrent density of 2.83 mA cm^(-2)at 1.7 VRHEto drive the full-reaction. We also present Cu-alloys electrocatalysis extended from CuInSnS4, which are superior in both activity and selectivity for CO_(2)RR. Specifically, the screened CuInSn achieves a CO_(2)to HCOOH Faradaic efficiency of 93% at a cell voltage of-2.0 V by assembling into artificial photosynthesis cell. The stability test of IT exhibits less than 3% degradation over 24 h. Furthermore, in-situ Raman spectroscopy reveals that both CO_(3)^(-2)and CO_(2)are involved in CO_(2)RR as reactants. The preferential affinity of C for H in the ^(*)HCO_(2)intermediate enables an improved HCOOH-selectivity, highlighting the role of multifunctional Cu in reducing the cell voltage and enhancing the photocurrent density.
基金King Abdullah University of Science and Technology for funding through the funding grant (BAS/1/1413-01-01)the Engineering and Physical Sciences Research Council (EPSRC,EP/V027433/1)+1 种基金the Royal Society (RGSR1211080IESR2212115)。
文摘Electrocatalytic splitting of water by means of renewable energy as the electricity supply is one of the most promising methods for storing green renewable energy as hydrogen. Although two-thirds of the earth’s surface is covered with water, there is inadequacy of freshwater in most parts of the world. Hence, splitting seawater instead of freshwater could be a truly sustainable alternative. However, direct seawater splitting faces challenges because of the complex composition of seawater. The composition, and hence, the local chemistry of seawater may vary depending on its origin, and in most cases, tracking of the side reactions and standardizing and customizing the catalytic process will be an extra challenge. The corrosion of catalysts and competitive side reactions due to the presence of various inorganic and organic pollutants create challenges for developing stable electro-catalysts. Hence, seawater splitting generally involves a two-step process, i.e., purification of seawater using reverse osmosis and then subsequent fresh water splitting. However, this demands two separate chambers and larger space, and increases complexity of the reactor design. Recently, there have been efforts to directly split seawater without the reverse osmosis step. Herein, we represent the most recent innovative approaches to avoid the two-step process, and compare the potential application of membrane-assisted and membrane-less electrolyzers in direct seawater splitting(DSS). We particularly discuss the device engineering, and propose a novel electrolyzer design strategies for concentration gradient based membrane-less microfluidic electrolyzer.
文摘利用WRF-Chem(Weather Research and Forecasting model coupled with Chemistry)模式研究2006年8月1日—9月1日中国区域硫酸盐和黑碳气溶胶对云特性的影响。模式验证利用了卫星和地面观测的气象要素、化学物质浓度、气溶胶光学特性和云微物理特性。模式性能评估表明该模式能较好地抓住气象要素(温度、降水、相对湿度和风速)的量级和空间分布特征。通过与地面观测和MODIS卫星数据对比发现,尽管模式模拟还存在偏差,但还是能较好模拟出气溶胶物种的地表浓度、气溶胶光学厚度(AOD)、云光学厚度(COD)、云量(CLDF)、云顶云滴有效半径(CER)和云水路径(LWP)。通过两个敏感性试验(分别增加二氧化硫和黑碳排放量至控制试验排放的3倍)与控制试验的对比发现硫酸盐比黑碳更易成为云凝结核,在中国东部云顶云滴数浓度和其它云特性参数对二氧化硫排放增加的响应均从北向南呈递增,这与地面湿度分布有关。云滴有效半径对硫酸盐气溶胶的响应符合气溶胶第一间接效应的定义,即硫酸盐气溶胶增多,云滴数浓度增加,云滴有效半径减少,但是对黑碳气溶胶的响应在各区域不尽相同。还发现黑碳对云量的影响远大于硫酸盐,主要原因是由于黑碳气溶胶直接辐射效应(对太阳光的吸收)导致的云的"燃烧"作用。
基金supported by Na-tional Basic Research Program of China (973 Program) under Grant No. 2009CB421406the Chinese Academy of Sciences under Grant KZCX2-YW-Q1-02the Na-tional Natural Science Foundation of China under Grant No. 40631005
文摘This paper investigates the variability of the break-up dates of the rivers in Northeast China from their icebound states for the period of 1957-2005 and explores some potential explanatory mechanisms. Results show that the break-up of the two major rivers (the Heilongjiang River and Songhuajiang River) was about four days earlier, and their freeze-up was about 4-7 days delayed, during 1989 2005 as compared to 1971 1987. This interdecadal variation is evidently associated with the warming trend over the past 50 years. In addition, the break-up and freeze-up dates have large interannual variability, with a standard deviation of about 10-15 days. The break-up date is primarily determined by the January February-March mean surface air temperature over the Siberian-Northeast China region via changes in the melting rate, ice thickness, and snow cover over the ice cover. The interannual variability of the break-up date is also significantly connected with the Northern Annular Mode (NAM), with a correlation coefficient of 0.35-0.55 based on the data from four stations along the two rivers. This relationship is attributed to the fact that the NAM can modulate the East Asian winter monsoon circulation and Siberian-Northeast China surface air temperature in January February-March.
基金supported by the National Basic Research Program of China (Grant No2009CB421406)the Chinese Academy of Sciences under Grant KZCX2-YW-Q1-02+1 种基金National Key Technologies R & D Program Project (Grant No 2007BAC03A01)the National Natural Science Foundation of China (GrantNo 40631005)
文摘Projected changes in summer precipitation characteristics in China during the 21st century are assessed using the monthly precipitation outputs of the ensemble of three "best" models under the Special Report on Emissions Scenarios (SRES) A1B, A2, and B1 scenarios. The excellent reproducibility of the models both in spatial and temporal patterns for the precipitation in China makes the projected summer precipitation change more believable for the future 100 years. All the three scenarios experiments indicate a consistent enhancement of summer precipitation in China in the 21st century. However, the projected summer precipitation in China demonstrates large variability between sub-regions. The projected increase in precipitation in South China is significant and persistent, as well as in North China. Meanwhile, in the early period of the 21st century, the region of Northeast China is projected to be much drier than the present. But, this situation changes and the precipitation intensifies later, with a precipitation anomaly increase of 12.4%0-20.4% at the end of the 21st century. The region of the Xinjiang Province probably undergoes a drying trend in the future 100 years, and is projected to decrease by 1.7%-3.6% at the end of the 21st century. There is no significant long-term change of the projected summer precipitation in the lower reaches of the Yangtze River valley. A high level of agreement of the ensemble of the regional precipitation change in some parts of China is found across scenarios but smaller changes are projected for the B1 scenario and slightly larger changes for the A2 scenario.
基金supported by the National Natural Science Foundation of China(Grant Nos90711004 and 40825016)the Chinese Academy of Sciences(Grant Nos:KZCX2-YW-Q1-02,KZCX2-YW-Q11-03)
文摘A unified chemistry-aerosol-climate model is applied in this work to compare climate responses to changing concentrations of long-lived greenhouse gases (GHGs, CO2, CH4, N2O), tropospheric O3, and aerosols during the years 1951-2000. Concentrations of sulfate, nitrate, primary organic carbon (POA), secondary organic carbon (SOA), black carbon (BC) aerosols, and tropospheric 03 for the years 1950 and 2000 are obtained a priori by coupled chemistry-aerosol-GCM simulations, and then monthly concentrations are interpolated linearly between 1951 and 2000. The annual concentrations of GHGs are taken from the IPCC Third Assessment Report. BC aerosol is internally mixed with other aerosols. Model results indicate that the sinmlated climate change over 1951-2000 is sensitive to anthropogenic changes in atmospheric components. The predicted year 2000 global mean surface air temperature can differ by 0.8℃ with different forcings. Relative to the climate simulation without changes in GHGs, O3, and aerosols, anthropogenic forcings of SO4^2-, BC, BC+SO4^2-, BC+SO4^2- +POA, BC+SO4^2- +POA+SOA+NO3^-, O3, and GHGs are predicted to change the surface air temperature averaged over 1971-2000 in eastern China, respectively, by -0.40℃, +0.62℃, +0.18℃, +0.15℃, -0.78℃, +0.43℃, and +0.85℃, and to change the precipitation, respectively, by -0.21, +0.07, -0.03, +0.02, -0.24, -0.08, and +0.10 mm d^-1. The authors conclude that all major aerosols are as important as GHGs in influencing climate change in eastern China, and tropospheric O3 also needs to be included in studies of regional climate change in China.
基金supported by National Basic Research Program of China(Grant No2009CB421406)the Chinese Academy of Sciences(Grant NosKZCX2-YW-Q1-02 and KZCX2-YW-BR-14)the National Natural Science Foundation of China(Grant Nos40631005 and 90711004)
文摘Recent observational study has shown that the southern center of the summer North Atlantic Oscillation (SNAO) was located farther eastward after the late 1970s compared to before. In this study, the cause for this phenomenon is explored. The result shows that the eastward shift of the SNAO southern center after the late 1970s is related to the variability of the Mediterranean-Black Sea (MBS) SST. A warm MBS SST can heat and moisten its overlying atmosphere, consequently producing a negative sea level pressure (SLP) departure over the MBS region. Because the MBS SST is negatively correlated with the SNAO, the negative SLP departure can enhance the eastern part of the negative-phase of the SNAO southern center, consequently producing an eastward SNAO southern center shift. Similarly, a cold MBS SST produces an eastward positive-phase SNAO southern center shift. The reason for why the MBS SST has an impact on the SNAO after the late 1970s but why it is not the case beforehand is also discussed. It is found that this instable relationship is likely to be attributed to the change of the variability of the MBS SST on the decadal time-scale. In 1951 1975, the variability of the MBS SST is quite weak, but in 1978 2002, it becomes more active. The active SST can enhance the interaction between the sea and its overlying atmosphere, thus strengthening the connection between the MBS SST and the SNAO after the late 1970s. The above observational analysis results are further confirmed by sensitivity experiments.