Spin-valley polarization and bandgap regulation are critical in the developing of quantum devices.Here,by employing the density functional theory,we investigate the effects of stacking form,thickness and magnetic mome...Spin-valley polarization and bandgap regulation are critical in the developing of quantum devices.Here,by employing the density functional theory,we investigate the effects of stacking form,thickness and magnetic moment in the electronic structures of WSe_(2)–MoS_(2)heterostructures.Calculations show that spin-valley polarization maintains in all situations.Increasing thickness of 2H-MoS_(2)not only tunes the bandgap but also changes the degeneracy of the conduction band minimums(CBM)at K/K_(1) points.Gradual increase of micro magnetic moment tunes the bandgap and raises the valence band maximums(VBM)atΓpoint.In addition,the regulation of band gap by the thickness of 2H-MoS_(2)and introduced magnetic moment depends on the stacking type.Results suggest that WSe_(2)–MoS_(2)heterostructure supports an ideal platform for valleytronics applications.Our methods also give new ways of optical absorption regulation in spin-valley devices.展开更多
Two-dimensional(2D)magnet/superconductor heterostructures can promote the design of artificial materials for exploring 2D physics and device applications by exotic proximity effects.However,plagued by the low Curie te...Two-dimensional(2D)magnet/superconductor heterostructures can promote the design of artificial materials for exploring 2D physics and device applications by exotic proximity effects.However,plagued by the low Curie temperature and instability in air,it is hard to realize practical applications for the reported layered magnetic materials at present.In this paper,we developed a space-confined chemical vapor deposition method to synthesize ultrathin air-stable ε-Fe_(2)O_(3) nanosheets with Curie temperature above 350 K.The ε-Fe_(2)O_(3)/NbSe_(2) heterojunction was constructed to study the magnetic proximity effect on the superconductivity of the NbSe_(2) multilayer.The electrical transport results show that the subtle proximity effect can modulate the interfacial spin–orbit interaction while undegrading the superconducting critical parameters.Our work paves the way to construct 2D heterojunctions with ultrathin nonlayered materials and layered van der Waals(vdW)materials for exploring new physical phenomena.展开更多
Moirésuperlattices in twisted two-dimensional materials have emerged as ideal platforms for engineering quantum phenomena,which are highly sensitive to twist angles,including both the global value and the spatial...Moirésuperlattices in twisted two-dimensional materials have emerged as ideal platforms for engineering quantum phenomena,which are highly sensitive to twist angles,including both the global value and the spatial inhomogeneity.However,only a few methods provide spatial-resolved information for characterizing local twist angle distribution.展开更多
The flexible materials exhibit more favorable properties than most rigid substrates in flexibility,weight saving,mechanical reliability,and excellent environmental toughness.Particularly,flexible graphene film with un...The flexible materials exhibit more favorable properties than most rigid substrates in flexibility,weight saving,mechanical reliability,and excellent environmental toughness.Particularly,flexible graphene film with unique mechanical properties was extensively explored in high frequency devices.Herein,we report the characteristics of structure and magnetic properties at high frequency of Co2FeAl thin film with different thicknesses grown on flexible graphene substrate at room temperature.The exciting finding for the columnar structure of Co2FeAl thin film lays the foundation for excellent high frequency property of Co2FeAl/flexible graphene structure.In-plane magnetic anisotropy field varying with increasing thickness of Co2FeAl thin film can be obtained by measurement of ferromagnetic resonance,which can be ascribed to the enhancement of crystallinity and the increase of grain size.Meanwhile,the resonance frequency which can be achieved by the measurement of vector network analyzer with the microstrip method increases with increasing thickness of Co2FeAl thin film.Moreover,in our case with graphene film,the resonance magnetic field is quite stable though folded for twenty cycles,which demonstrates that good flexibility of graphene film and the stability of high frequency magnetic property of Co2FeAl thin film grown on flexible graphene substrate.These results are promising for the design of microwave devices and wireless communication equipment.展开更多
Aligned carbon nanotube (CNRT) films exhibit excellent electron emission properties at very low fields. This has been attributed to the high aspect ratio of CNTs, I.e. Their emitting surface can have high local field ...Aligned carbon nanotube (CNRT) films exhibit excellent electron emission properties at very low fields. This has been attributed to the high aspect ratio of CNTs, I.e. Their emitting surface can have high local field due to geometrical enhancement. It is found that a new mechanism can be responsible for the enhancement of the local field on the emitting surface of CNTs. This results from the space charge in the vacuum gap, which is readily generated due to the high emission current density of CNTs. Details are given of both experimental and theoretical studies of this effect. The mechanism also accounts for the distinct nonlinearity in Fowler-Nordheim plots often observed with CNTs. The implication of the technical application of our findings is also included.展开更多
A way to determine some important etching parameters in the step fabrication for highTc step-edge Josephson junctions is described based on an analysis of the dynamics of the etching process.The optimum thickness of t...A way to determine some important etching parameters in the step fabrication for highTc step-edge Josephson junctions is described based on an analysis of the dynamics of the etching process.The optimum thickness of the etch mask is defined with negligible recession of the mask edge during the etch.Under this condition,the equilibrium angle of the steps etched on the SrTiO_(3)(STO)substrate with an Nb mask has been calculated to be about 76°.With optimized mask thickness,its sharp sidewall and straight edge,high-quality steps on STO substrates with step height from 200-300 nm and step angle above 70°are made.Josephson junctions and dc-SQUIDs with high reproducibility and less parameter scatter are obtained on the step substrates.展开更多
The Trapping force on Rayleigh particles in an optical tweezers system with an oil immersion objective is calculated by an electromagnetic model.The results indicate that the stability of particles trapped will be aff...The Trapping force on Rayleigh particles in an optical tweezers system with an oil immersion objective is calculated by an electromagnetic model.The results indicate that the stability of particles trapped will be affected by spherical aberration,which is caused by refractive difference between objective oil and water solution,when the specimen manipulated is suspended in a water solution.The trapping force and depth of potential well will decrease and the minimum of laser power for ensuring the stability of particles trapped will increase with the enhancing trapping depth.展开更多
We report temperature-dependent behavior of the zero bias tunneling conductance(ZBTC),derived from tun neling spectroscopies on as-grown Bi_(2)Sr_(2)CaCu_(2)O_(8+δ)(Bi2212)single crystals taken with evaporated Zn and...We report temperature-dependent behavior of the zero bias tunneling conductance(ZBTC),derived from tun neling spectroscopies on as-grown Bi_(2)Sr_(2)CaCu_(2)O_(8+δ)(Bi2212)single crystals taken with evaporated Zn and Pb planar junctions.At Tc the measured ZBTC shows a kink which gives an in situ measure of the superconducting transition temperature(T_(c)).Below T_(c),the T^(2)dependence of the ZBTC has been observed repeatedly as a new evidence of the d-wave symmetry in Bi2212.展开更多
Au approximate instantaneous eigenstate is presented for the many-spin system possessing the anisotropy exchange interaction in a strong magnetic field by the perturbation method.Based on the instantaneous eigenstate,...Au approximate instantaneous eigenstate is presented for the many-spin system possessing the anisotropy exchange interaction in a strong magnetic field by the perturbation method.Based on the instantaneous eigenstate,the Berry phase of this state is worked out.Furthermore,the effect of the anisotropy exchange interaction on the Berry phase of the state for the many-spin system is studied.展开更多
We have studied the magnetic reversal process of the magnetron sputtered Pt/Co multilayers by using magnetic force microscope with in situ bias magnetic fields.In thin films magnetic reversal is usually dominated eith...We have studied the magnetic reversal process of the magnetron sputtered Pt/Co multilayers by using magnetic force microscope with in situ bias magnetic fields.In thin films magnetic reversal is usually dominated either by domain nucleation or by domain wall motion.In our experiments,a series of magnetic images in situ captured in the same area indicates that the magnetic reversal in Pt/Co multilayers is dominated by domain nucleation,in stead of domain wall motion.In addition,the local demagnetized curve was obtained by using the bearing analysis of the domains in the series of magnetic images.展开更多
A procedure for fabricating novel TiO_(2) membrane materialwith sub-micrometre pores and large specific surface area from the template has been demonstrated. The morphology and structure of the membrane have been char...A procedure for fabricating novel TiO_(2) membrane materialwith sub-micrometre pores and large specific surface area from the template has been demonstrated. The morphology and structure of the membrane have been characterized by scanning electron microscopy. The results have indicated that the macroporous membraneconsists of uniform hollow spheres which are interconnected to each other by 'small windows'. Potential unique applications of this macroporous materialin the fields of catalysis, optics, sensors, etc, are suggested.展开更多
Highly anisotropic thermal conductive materials are of significance in thermal management applications. However,accurate determination of ultrathin composite thermal properties is a daunting task due to the tiny therm...Highly anisotropic thermal conductive materials are of significance in thermal management applications. However,accurate determination of ultrathin composite thermal properties is a daunting task due to the tiny thermal conductance,severely hindering the further exploration of novel efficient thermal management materials, especially for size-confined environments. In this work, by utilizing a hybrid measuring method, we demonstrate an accurate determination of thermal properties for montmorillonite/reduced graphene oxide(MMT/r GO) composite film with a thickness range from 0.2 μm to2 μm. The in-plane thermal conductivity measurement is realized by one-dimensional(1D) steady-state heat conduction approach while the cross-plane one is achieved via a modified 3ω method. As-measured thermal conductivity results are cross-checked with different methods and known materials, revealing the high measurement accuracy. A high anisotropic ratio of 60.5, independent of composite thickness, is observed in our measurements, further ensuring the negligible measurement error. Notably, our work develops an effective approach to the determination of ultrathin composite thermal conductivity, which may promote the development of ultrathin composites for potential thermal-related applications.展开更多
Megabar pressures are of crucial importance for cutting-edge studies of condensed matter physics and geophysics.With the development of diamond anvil cell(DAC),laboratory studies of high pressure have entered the mega...Megabar pressures are of crucial importance for cutting-edge studies of condensed matter physics and geophysics.With the development of diamond anvil cell(DAC),laboratory studies of high pressure have entered the megabar era for decades.However,it is still challenging to implement in situ magnetic sensing under ultrahigh pressures.In this work,we demonstrate optically detected magnetic resonance and coherent quantum control of diamond nitrogen-vacancy(NV)center,a promising quantum sensor inside the DAC,up to 1.4 Mbar.The pressure dependence of optical and spin properties of NV centers in diamond are quantified,and the evolution of an external magnetic field has been successfully tracked at about 80 GPa.These results shed new light on our understanding of diamond NV centers and pave the way for quantum sensing under extreme conditions.展开更多
A highly flexible and continuous fibrous thermoelectric(TE)module with high-performance has been fabricated based on an ultra-long single-walled carbon nanotube fiber,which effectively avoids the drawbacks of traditio...A highly flexible and continuous fibrous thermoelectric(TE)module with high-performance has been fabricated based on an ultra-long single-walled carbon nanotube fiber,which effectively avoids the drawbacks of traditional inorganic TE based modules.The maximum output power density of a 1-cm long fibrous TE module with 8 p–n pairs can reach to 3436μW·cm^(-2),the power per unit weight to 2034μW·g^(-1),at a steady-state temperature difference of 50 K.The continuous fibrous TE module is used to detect temperature change of a single point,which exhibits a good responsiveness and excellent stability.Because of its adjustability in length,the flexible fibrous TE module can satisfy the transformation of the temperature difference between two distant heat sources into electrical energy.Based on the signal of the as-fabricated TE module,a multi-region recognizer has been designed and demonstrated.The highly flexible and continuous fibrous TE module with excellent performance shows a great potential in diversified applications of TE generation,temperature detection,and position identification.展开更多
Domain walls(DWs)in the charge-density-wave(CDW)Mott insulator 1T-TaS_(2)have unique localized states,which play an important role in exploring the electronic properties of the material.However,the electronic states i...Domain walls(DWs)in the charge-density-wave(CDW)Mott insulator 1T-TaS_(2)have unique localized states,which play an important role in exploring the electronic properties of the material.However,the electronic states in DWs in 1TTaS_(2)have not been clearly understood,mostly due to the complex structures,phases,and interlayer stacking orders in the DW areas.Here,we explored the electronic states of DWs in the large-area CDW phase and mosaic phase of 1T-TaS_(2)by scanning tunneling spectroscopy.Due to the different densities of DWs,the electronic states of DWs show distinct features in these phases.In the large area CDW phase,both the domain and the DWs(DW1,DW2,DW4)have zero conductance at the Fermi level;while in the mosaic phase,they can be metallic or insulating depending on their environments.In areas with a high density of DWs,some electronic states were observed both on the DWs and within the domains,indicating delocalized states over the whole region.Our work contributes to further understanding of the interplay between CDW and electron correlations in 1T-TaS_(2).展开更多
The ability to control transport behaviors in nanostructure is crucial for usage as a fundamental research platform as well as a practical device.In this study,we report a gate-controlled crossover of electron transpo...The ability to control transport behaviors in nanostructure is crucial for usage as a fundamental research platform as well as a practical device.In this study,we report a gate-controlled crossover of electron transport behaviors using graphene nanoconstrictions as a platform.The observed transport properties span from Coulomb blockade-dominated single electron transmission to electron-wave interference-dominated quantum behavior.Such drastic modulation is achieved by utilizing a single back gate on a graphene nanoconstriction structure,where the size of nanostructure in the constriction and coupling strength of it to the electrodes can be tuned electrically.Our results indicate that electrostatic field by gate voltage upon the confined nanostructure defines both the size of the nanoconstriction as well as its interaction to electrodes.Increasing gate voltage raises Fermi level to cross the energy profile in the nanoconstriction,resulting in decreased energy barriers which affect the size of nanoconstriction and transmissivity of electrons.The gate-tunable nanoconstriction device can therefore become a potential platform to study quantum critical behaviors and enrich electronic and spintronic devices.展开更多
Two-dimensional honeycomb lattices show great potential in the realization of Dirac nodal line fermions(DNLFs).Here,we successfully synthesized a gold telluride(AuTe)monolayer by direct tellurizing an Au(111)substrate...Two-dimensional honeycomb lattices show great potential in the realization of Dirac nodal line fermions(DNLFs).Here,we successfully synthesized a gold telluride(AuTe)monolayer by direct tellurizing an Au(111)substrate.Low energy electron diffraction measurements reveal that it is(2×2)AuTe layer stacked onto(3×3)Au(111)substrate.Moreover,scanning tunneling microscopy images show that the AuTe layer has a honeycomb structure.Scanning transmission electron microscopy reveals that it is a single-atom layer.In addition,first-principles calculations demonstrate that the honeycomb AuTe monolayer exhibits Dirac nodal line features protected by mirror symmetry,which is validated by angle-resolved photoemission spectra.Our results establish that monolayer AuTe can be a good candidate to investigate 2D DNLFs and provides opportunities to realize high-speed low-dissipation devices.展开更多
We fabricated a new type of two-dimensional photonic crystal slab filter. The resonant cavities were directly put into the waveguide arms. The optical transmissions of the filters were measured and the results show th...We fabricated a new type of two-dimensional photonic crystal slab filter. The resonant cavities were directly put into the waveguide arms. The optical transmissions of the filters were measured and the results show that the optimized two-channel filters give good intensity distribution at the output ports of the waveguide. A minimum wavelength spacing of 5 nm of the filter outputs is realized by accurately controlling the size of the resonant cavities.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61975224 and 12104004)the University Synergy Innovation Program of Anhui Province(Grant No.GXXT-2020-050)+2 种基金the Fund of Anhui Provincial Natural Science Foundation(Grant No.2008085MF206)New magnetoelectric materials and devices,the Recruitment Program for Leading Talent Team of Anhui Province 2020,State Key Laboratory of Luminescence and Applications(Grant No.SKLA-2021-03)the Open Fund of Infrared and Low-Temperature Plasma Key Laboratory of Anhui Province(Grant No.IRKL2022KF03)。
文摘Spin-valley polarization and bandgap regulation are critical in the developing of quantum devices.Here,by employing the density functional theory,we investigate the effects of stacking form,thickness and magnetic moment in the electronic structures of WSe_(2)–MoS_(2)heterostructures.Calculations show that spin-valley polarization maintains in all situations.Increasing thickness of 2H-MoS_(2)not only tunes the bandgap but also changes the degeneracy of the conduction band minimums(CBM)at K/K_(1) points.Gradual increase of micro magnetic moment tunes the bandgap and raises the valence band maximums(VBM)atΓpoint.In addition,the regulation of band gap by the thickness of 2H-MoS_(2)and introduced magnetic moment depends on the stacking type.Results suggest that WSe_(2)–MoS_(2)heterostructure supports an ideal platform for valleytronics applications.Our methods also give new ways of optical absorption regulation in spin-valley devices.
基金The work is supported by the National Key Research and Development Program of China(Grant No.2022YFA1204104)the National Natural Science Foundation of China(Grant No.61888102)the Chinese Academy of Sciences(Grant Nos.ZDBS-SSW-WHC001 and XDB33030100).
文摘Two-dimensional(2D)magnet/superconductor heterostructures can promote the design of artificial materials for exploring 2D physics and device applications by exotic proximity effects.However,plagued by the low Curie temperature and instability in air,it is hard to realize practical applications for the reported layered magnetic materials at present.In this paper,we developed a space-confined chemical vapor deposition method to synthesize ultrathin air-stable ε-Fe_(2)O_(3) nanosheets with Curie temperature above 350 K.The ε-Fe_(2)O_(3)/NbSe_(2) heterojunction was constructed to study the magnetic proximity effect on the superconductivity of the NbSe_(2) multilayer.The electrical transport results show that the subtle proximity effect can modulate the interfacial spin–orbit interaction while undegrading the superconducting critical parameters.Our work paves the way to construct 2D heterojunctions with ultrathin nonlayered materials and layered van der Waals(vdW)materials for exploring new physical phenomena.
基金supported by the National Natural Science Foundation of China(Grant Nos.61888102 and 12374199)the National Key Research&Development Projects of China(Grant Nos.2022YFA1204100,2019YFA0308501,and 2021YFA1401300)+1 种基金the Chinese Academy of Sciences(Grant No.XDB33030100)the Innovation Program of Quantum Science and Technology(Grant No.2021ZD0302700)。
文摘Moirésuperlattices in twisted two-dimensional materials have emerged as ideal platforms for engineering quantum phenomena,which are highly sensitive to twist angles,including both the global value and the spatial inhomogeneity.However,only a few methods provide spatial-resolved information for characterizing local twist angle distribution.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.51901163 and 12104171)the Fundamental Research Funds for the Central Universities(Grant No.2021XXJS025).
文摘The flexible materials exhibit more favorable properties than most rigid substrates in flexibility,weight saving,mechanical reliability,and excellent environmental toughness.Particularly,flexible graphene film with unique mechanical properties was extensively explored in high frequency devices.Herein,we report the characteristics of structure and magnetic properties at high frequency of Co2FeAl thin film with different thicknesses grown on flexible graphene substrate at room temperature.The exciting finding for the columnar structure of Co2FeAl thin film lays the foundation for excellent high frequency property of Co2FeAl/flexible graphene structure.In-plane magnetic anisotropy field varying with increasing thickness of Co2FeAl thin film can be obtained by measurement of ferromagnetic resonance,which can be ascribed to the enhancement of crystallinity and the increase of grain size.Meanwhile,the resonance frequency which can be achieved by the measurement of vector network analyzer with the microstrip method increases with increasing thickness of Co2FeAl thin film.Moreover,in our case with graphene film,the resonance magnetic field is quite stable though folded for twenty cycles,which demonstrates that good flexibility of graphene film and the stability of high frequency magnetic property of Co2FeAl thin film grown on flexible graphene substrate.These results are promising for the design of microwave devices and wireless communication equipment.
基金Supported by the National Natural Science Foundation of China under Grant No.59525206the Education Ministry of China and the Higher Education Bureau,the Science and Technology Commission of Guangdong Province.
文摘Aligned carbon nanotube (CNRT) films exhibit excellent electron emission properties at very low fields. This has been attributed to the high aspect ratio of CNTs, I.e. Their emitting surface can have high local field due to geometrical enhancement. It is found that a new mechanism can be responsible for the enhancement of the local field on the emitting surface of CNTs. This results from the space charge in the vacuum gap, which is readily generated due to the high emission current density of CNTs. Details are given of both experimental and theoretical studies of this effect. The mechanism also accounts for the distinct nonlinearity in Fowler-Nordheim plots often observed with CNTs. The implication of the technical application of our findings is also included.
基金Supported by the National Key Basic Research Programme of China under Grant No 2002CB713805, and the National Natural Science Foundation of China under Grant Nos 10374112 and 10604065.
基金Supported by the National Center for R&D on Superconductivity and the Ministry of Science and Technology of China(NKBRSF-G19990646).
文摘A way to determine some important etching parameters in the step fabrication for highTc step-edge Josephson junctions is described based on an analysis of the dynamics of the etching process.The optimum thickness of the etch mask is defined with negligible recession of the mask edge during the etch.Under this condition,the equilibrium angle of the steps etched on the SrTiO_(3)(STO)substrate with an Nb mask has been calculated to be about 76°.With optimized mask thickness,its sharp sidewall and straight edge,high-quality steps on STO substrates with step height from 200-300 nm and step angle above 70°are made.Josephson junctions and dc-SQUIDs with high reproducibility and less parameter scatter are obtained on the step substrates.
基金Supported by the National Natural Science Foundation of China under Grant No.1989380.
文摘The Trapping force on Rayleigh particles in an optical tweezers system with an oil immersion objective is calculated by an electromagnetic model.The results indicate that the stability of particles trapped will be affected by spherical aberration,which is caused by refractive difference between objective oil and water solution,when the specimen manipulated is suspended in a water solution.The trapping force and depth of potential well will decrease and the minimum of laser power for ensuring the stability of particles trapped will increase with the enhancing trapping depth.
基金Supported by a grant for State Key Program for Basic Research of China,and the National Center for Research&Development on Superconductivity.
文摘We report temperature-dependent behavior of the zero bias tunneling conductance(ZBTC),derived from tun neling spectroscopies on as-grown Bi_(2)Sr_(2)CaCu_(2)O_(8+δ)(Bi2212)single crystals taken with evaporated Zn and Pb planar junctions.At Tc the measured ZBTC shows a kink which gives an in situ measure of the superconducting transition temperature(T_(c)).Below T_(c),the T^(2)dependence of the ZBTC has been observed repeatedly as a new evidence of the d-wave symmetry in Bi2212.
基金Supported by Hebei Natural Science Foundation under Grant No.196164.
文摘Au approximate instantaneous eigenstate is presented for the many-spin system possessing the anisotropy exchange interaction in a strong magnetic field by the perturbation method.Based on the instantaneous eigenstate,the Berry phase of this state is worked out.Furthermore,the effect of the anisotropy exchange interaction on the Berry phase of the state for the many-spin system is studied.
基金Supported by the National Natural Science Foundation of China under Grant No.10074081.
文摘We have studied the magnetic reversal process of the magnetron sputtered Pt/Co multilayers by using magnetic force microscope with in situ bias magnetic fields.In thin films magnetic reversal is usually dominated either by domain nucleation or by domain wall motion.In our experiments,a series of magnetic images in situ captured in the same area indicates that the magnetic reversal in Pt/Co multilayers is dominated by domain nucleation,in stead of domain wall motion.In addition,the local demagnetized curve was obtained by using the bearing analysis of the domains in the series of magnetic images.
基金Supported by the National Natural Science Foundation of China.
文摘A procedure for fabricating novel TiO_(2) membrane materialwith sub-micrometre pores and large specific surface area from the template has been demonstrated. The morphology and structure of the membrane have been characterized by scanning electron microscopy. The results have indicated that the macroporous membraneconsists of uniform hollow spheres which are interconnected to each other by 'small windows'. Potential unique applications of this macroporous materialin the fields of catalysis, optics, sensors, etc, are suggested.
基金Project supported by the National Basic Research Program of China (Grant No. 2016YFA0200800)the Strategic Priority Research Program of Chinese Academy of Sciences (Grant Nos. XDB30000000 and XDB07030100)+2 种基金the Sinopec Innovation Scheme (A-527)the National Key Research and Development Program of China (Grant No. 2021YFA0715700)the National Science Fund for Distinguished Young Scholars, China (Grant No. 52125302)。
文摘Highly anisotropic thermal conductive materials are of significance in thermal management applications. However,accurate determination of ultrathin composite thermal properties is a daunting task due to the tiny thermal conductance,severely hindering the further exploration of novel efficient thermal management materials, especially for size-confined environments. In this work, by utilizing a hybrid measuring method, we demonstrate an accurate determination of thermal properties for montmorillonite/reduced graphene oxide(MMT/r GO) composite film with a thickness range from 0.2 μm to2 μm. The in-plane thermal conductivity measurement is realized by one-dimensional(1D) steady-state heat conduction approach while the cross-plane one is achieved via a modified 3ω method. As-measured thermal conductivity results are cross-checked with different methods and known materials, revealing the high measurement accuracy. A high anisotropic ratio of 60.5, independent of composite thickness, is observed in our measurements, further ensuring the negligible measurement error. Notably, our work develops an effective approach to the determination of ultrathin composite thermal conductivity, which may promote the development of ultrathin composites for potential thermal-related applications.
基金supported by the Beijing Natural Science Foundation(Grant No.Z200009)Chinese Academy of Sciences(Grant Nos.YJKYYQ20190082,XDB28000000,XDB33000000,XDB25000000,and QYZDBSSW-SLH013)+2 种基金the National Natural Science Foundation of China(Grant Nos.11974020,12022509,12074422,11934018,and T2121001)the National Key Research and Development Program of China(Grant Nos.2019YFA0308100,2021YFA1400300,and 2018YFA0305700)the Youth Innovation Promotion Association of Chinese Academy of Sciences(Grant No.202003)。
文摘Megabar pressures are of crucial importance for cutting-edge studies of condensed matter physics and geophysics.With the development of diamond anvil cell(DAC),laboratory studies of high pressure have entered the megabar era for decades.However,it is still challenging to implement in situ magnetic sensing under ultrahigh pressures.In this work,we demonstrate optically detected magnetic resonance and coherent quantum control of diamond nitrogen-vacancy(NV)center,a promising quantum sensor inside the DAC,up to 1.4 Mbar.The pressure dependence of optical and spin properties of NV centers in diamond are quantified,and the evolution of an external magnetic field has been successfully tracked at about 80 GPa.These results shed new light on our understanding of diamond NV centers and pave the way for quantum sensing under extreme conditions.
基金the National Key Research and Development Program of China(Grant No.2018YFA0208402)the National Natural Science Foundation of China(Grant Nos.11634014,51172271,and 51372269)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDA09040202)。
文摘A highly flexible and continuous fibrous thermoelectric(TE)module with high-performance has been fabricated based on an ultra-long single-walled carbon nanotube fiber,which effectively avoids the drawbacks of traditional inorganic TE based modules.The maximum output power density of a 1-cm long fibrous TE module with 8 p–n pairs can reach to 3436μW·cm^(-2),the power per unit weight to 2034μW·g^(-1),at a steady-state temperature difference of 50 K.The continuous fibrous TE module is used to detect temperature change of a single point,which exhibits a good responsiveness and excellent stability.Because of its adjustability in length,the flexible fibrous TE module can satisfy the transformation of the temperature difference between two distant heat sources into electrical energy.Based on the signal of the as-fabricated TE module,a multi-region recognizer has been designed and demonstrated.The highly flexible and continuous fibrous TE module with excellent performance shows a great potential in diversified applications of TE generation,temperature detection,and position identification.
基金Project supported by the National Key Research and Development Project of China(Grant No.2019YFA0308500)the National Natural Science Foundation of China(Grant No.61888102)the Chinese Academy of Sciences(Grant Nos.XDB30000000 and YSBR-003).
文摘Domain walls(DWs)in the charge-density-wave(CDW)Mott insulator 1T-TaS_(2)have unique localized states,which play an important role in exploring the electronic properties of the material.However,the electronic states in DWs in 1TTaS_(2)have not been clearly understood,mostly due to the complex structures,phases,and interlayer stacking orders in the DW areas.Here,we explored the electronic states of DWs in the large-area CDW phase and mosaic phase of 1T-TaS_(2)by scanning tunneling spectroscopy.Due to the different densities of DWs,the electronic states of DWs show distinct features in these phases.In the large area CDW phase,both the domain and the DWs(DW1,DW2,DW4)have zero conductance at the Fermi level;while in the mosaic phase,they can be metallic or insulating depending on their environments.In areas with a high density of DWs,some electronic states were observed both on the DWs and within the domains,indicating delocalized states over the whole region.Our work contributes to further understanding of the interplay between CDW and electron correlations in 1T-TaS_(2).
基金Project supported by the National Basic Research Program of China(Grant No.2016YFA0200800)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant Nos.XDB30000000 and XDB07030100)the Sinopec Innovation Scheme(Grant No.A-527).
文摘The ability to control transport behaviors in nanostructure is crucial for usage as a fundamental research platform as well as a practical device.In this study,we report a gate-controlled crossover of electron transport behaviors using graphene nanoconstrictions as a platform.The observed transport properties span from Coulomb blockade-dominated single electron transmission to electron-wave interference-dominated quantum behavior.Such drastic modulation is achieved by utilizing a single back gate on a graphene nanoconstriction structure,where the size of nanostructure in the constriction and coupling strength of it to the electrodes can be tuned electrically.Our results indicate that electrostatic field by gate voltage upon the confined nanostructure defines both the size of the nanoconstriction as well as its interaction to electrodes.Increasing gate voltage raises Fermi level to cross the energy profile in the nanoconstriction,resulting in decreased energy barriers which affect the size of nanoconstriction and transmissivity of electrons.The gate-tunable nanoconstriction device can therefore become a potential platform to study quantum critical behaviors and enrich electronic and spintronic devices.
基金Project supported by the National Key R&D Program of China (Grant No.2018YFA0305800)the National Natural Science Foundation of China (Grant Nos.61925111,61888102,and 52102193)+2 种基金the Strategic Priority Research Program of Chinese Academy of Sciences (Grant Nos.XDB28000000 and XDB30000000)CAS Project for Young Scientists in Basic Research (Grant No.YSBR-003)the Fundamental Research Funds for the Central Universities。
文摘Two-dimensional honeycomb lattices show great potential in the realization of Dirac nodal line fermions(DNLFs).Here,we successfully synthesized a gold telluride(AuTe)monolayer by direct tellurizing an Au(111)substrate.Low energy electron diffraction measurements reveal that it is(2×2)AuTe layer stacked onto(3×3)Au(111)substrate.Moreover,scanning tunneling microscopy images show that the AuTe layer has a honeycomb structure.Scanning transmission electron microscopy reveals that it is a single-atom layer.In addition,first-principles calculations demonstrate that the honeycomb AuTe monolayer exhibits Dirac nodal line features protected by mirror symmetry,which is validated by angle-resolved photoemission spectra.Our results establish that monolayer AuTe can be a good candidate to investigate 2D DNLFs and provides opportunities to realize high-speed low-dissipation devices.
基金Supported by the National Natural Science Foundation of China under Grant Nos 10390160 and 39890390. This work was performed at the Research Centre for Superconductor Photonics, 0saka University, Japan. We acknowledge Masato Suzuki for his technical assistance.
基金Project supported by the National Key Basic Research and Development Programme of China (Grant No 2001CB6104), the National Center for Nanoscience and Technology, China (Grant No 2003CB7169) and the National Natural Science Foundation of China (Grant No 10474036).
文摘We fabricated a new type of two-dimensional photonic crystal slab filter. The resonant cavities were directly put into the waveguide arms. The optical transmissions of the filters were measured and the results show that the optimized two-channel filters give good intensity distribution at the output ports of the waveguide. A minimum wavelength spacing of 5 nm of the filter outputs is realized by accurately controlling the size of the resonant cavities.