Retrieval experiment was made for global total column ozone using the first year measurements of Total Ozone Unit (TOU) on board the second generation polar orbiting meteorological satellite of China, FY-3/A. The retr...Retrieval experiment was made for global total column ozone using the first year measurements of Total Ozone Unit (TOU) on board the second generation polar orbiting meteorological satellite of China, FY-3/A. The retrieval results were analyzed and validated by comparison with AURA/OMI, Meteop/GOME-2 global ozone products and ground-based ozone measurement data. The qualititative comparisons over the globe especially over Antarctica and the Tibetan Plateau show that the spatial and temporal distribution characteristics are consistent with OMI and GOME-2 products. The quantitative comparisons with ground-based measurements and AURA/OMI ozone product were made over 74 stations, the TOU total ozone retrieval has a 3% rms relative error compared with AURA/OMI ozone product and 4.2% rms relative error with ground-based measurements. The maximum difference between satellite retrieval and ground-based measurements was found in the Antarctica ozone hole. The TOU global ozone product is operational and distributed to all users.展开更多
An in-situ GC-ECD system was used to measure halocarbons at Shangdianzi (SDZ) GAW regional station. In this paper, we reported observational results of atmospheric CFC- 11 (CCI3F) mixing ratios from April 2007 to ...An in-situ GC-ECD system was used to measure halocarbons at Shangdianzi (SDZ) GAW regional station. In this paper, we reported observational results of atmospheric CFC- 11 (CCI3F) mixing ratios from April 2007 to March 2008. The CFC- 11 time series showed large variability. Approximately 62% observed values were filtered as non-background data. The median, 10% and 90% percentiles of CFC-11 background mixing ratios were 245.4 ppt (10-12 mol/mol), 244.6 ppt and 246.1 ppt, respectively; whereas those of non-background CFC- 11 mixing ratios were 254.7, 246.6 and 272.1 ppt, respectively. Significant differences in background and non-background CFC-11 mixing ratios were observed between summer and autumn, mainly because of the CFC-11 stored in loam being prone to atmospheric release in hot seasons. Comparison of tile SDZ data with the five AGAGE stations suggested agreement with mid-high latitude Northern Hemisphere stations MHD, THD and RPB. The SDZ data were higher than that of Southern Hemisphere stations CGO and SMO. Higher CFC-11 mixing ratios measured in different seasons were always associated with winds from the W-WSW-SW sector, indicating that the airflow coming from this wind sector has a positive contribution to CFC- 11 concentrations. The CFC-11 mixing ratios were higher in autumn and summer than in spring and winter, in which its mixing ratios were very close to the atmospheric background level. This was happened especially when airflow originated from the NNE-NE-ENE-E sector, indicating the air masses coming from these wind directions was relatively clean.展开更多
基金supported by the National High-Tech Research & Development Program of China (2008AA121703)the National Natural Science Foundation of China (40905056)+3 种基金the State Key Labora-tory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC-KF-2008-11)Beijing Urban Meteorology Research Fund (UMRF-200704)the 11th Five-Year Plan of National Science and Technology Key Project (2008BAC34B04-2)the National Basic Research Program of China (2005CB422200x and 2006CB403702)
文摘Retrieval experiment was made for global total column ozone using the first year measurements of Total Ozone Unit (TOU) on board the second generation polar orbiting meteorological satellite of China, FY-3/A. The retrieval results were analyzed and validated by comparison with AURA/OMI, Meteop/GOME-2 global ozone products and ground-based ozone measurement data. The qualititative comparisons over the globe especially over Antarctica and the Tibetan Plateau show that the spatial and temporal distribution characteristics are consistent with OMI and GOME-2 products. The quantitative comparisons with ground-based measurements and AURA/OMI ozone product were made over 74 stations, the TOU total ozone retrieval has a 3% rms relative error compared with AURA/OMI ozone product and 4.2% rms relative error with ground-based measurements. The maximum difference between satellite retrieval and ground-based measurements was found in the Antarctica ozone hole. The TOU global ozone product is operational and distributed to all users.
基金supported by Non-profit Research Project to Serve the Public Interest (Grant No. GYHY200806026)International S&T Cooperation Program of MOST (Grant No. 2007DFA20650)Research Fund for Returned Overseas Chinese Scholars of the State Education Ministry (Grant No. [2009]1108)
文摘An in-situ GC-ECD system was used to measure halocarbons at Shangdianzi (SDZ) GAW regional station. In this paper, we reported observational results of atmospheric CFC- 11 (CCI3F) mixing ratios from April 2007 to March 2008. The CFC- 11 time series showed large variability. Approximately 62% observed values were filtered as non-background data. The median, 10% and 90% percentiles of CFC-11 background mixing ratios were 245.4 ppt (10-12 mol/mol), 244.6 ppt and 246.1 ppt, respectively; whereas those of non-background CFC- 11 mixing ratios were 254.7, 246.6 and 272.1 ppt, respectively. Significant differences in background and non-background CFC-11 mixing ratios were observed between summer and autumn, mainly because of the CFC-11 stored in loam being prone to atmospheric release in hot seasons. Comparison of tile SDZ data with the five AGAGE stations suggested agreement with mid-high latitude Northern Hemisphere stations MHD, THD and RPB. The SDZ data were higher than that of Southern Hemisphere stations CGO and SMO. Higher CFC-11 mixing ratios measured in different seasons were always associated with winds from the W-WSW-SW sector, indicating that the airflow coming from this wind sector has a positive contribution to CFC- 11 concentrations. The CFC-11 mixing ratios were higher in autumn and summer than in spring and winter, in which its mixing ratios were very close to the atmospheric background level. This was happened especially when airflow originated from the NNE-NE-ENE-E sector, indicating the air masses coming from these wind directions was relatively clean.