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Forecast Error and Predictability for the Warm-sector and the Frontal Rainstorm in South China
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作者 孙璐 王秋萍 +4 位作者 陈思远 高彦青 张旭鹏 时洋 马旭林 《Journal of Tropical Meteorology》 SCIE 2023年第1期128-141,共14页
In south China, warm-sector rainstorms are significantly different from the traditional frontal rainstorms due to complex mechanism, which brings great challenges to their forecast. In this study, based on ensemble fo... In south China, warm-sector rainstorms are significantly different from the traditional frontal rainstorms due to complex mechanism, which brings great challenges to their forecast. In this study, based on ensemble forecasting, the high-resolution mesoscale numerical forecast model WRF was used to investigate the effect of initial errors on a warmsector rainstorm and a frontal rainstorm under the same circulation in south China, respectively. We analyzed the sensitivity of forecast errors to the initial errors and their evolution characteristics for the warm-sector and the frontal rainstorm. Additionally, the difference of the predictability was compared via adjusting the initial values of the GOOD member and the BAD member. Compared with the frontal rainstorm, the warm-sector rainstorm was more sensitive to initial error, which increased faster in the warm-sector. Furthermore, the magnitude of error in the warm-sector rainstorm was obviously larger than that of the frontal rainstorm, while the spatial scale of the error was smaller. Similarly, both types of the rainstorm were limited by practical predictability and inherent predictability, while the nonlinear increase characteristics occurred to be more distinct in the warm-sector rainstorm, resulting in the lower inherent predictability.The comparison between the warm-sector rainstorm and the frontal rainstorm revealed that the forecast field was closer to the real situation derived from more accurate initial errors, but only the increase rate in the frontal rainstorm was restrained evidently. 展开更多
关键词 warm-sector rainstorm frontal rainstorm error evolution PREDICTABILITY
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Construction Technology of Lightning Protection Devices in Building Electrical Installation Engineering
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作者 Xuhong Du 《Journal of Electronic Research and Application》 2024年第1期22-27,共6页
To better improve the electrical safety of buildings and fulfill the role of lightning protection and grounding,this article combines cases and discusses seven aspects of lightning protection devices’construction tec... To better improve the electrical safety of buildings and fulfill the role of lightning protection and grounding,this article combines cases and discusses seven aspects of lightning protection devices’construction technology.These aspects include the lightning protection classification of buildings,air terminals,down conductors,grounding devices,division of lightning protection zones,and lightning electromagnetic pulse shielding.Through the introduction of this article,readers can gain a comprehensive understanding of the application and value of lightning protection grounding construction technology in building electrical installation projects. 展开更多
关键词 Building electrical Installation engineering Lightning protection grounding
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Experimental study on the physico-mechanical properties of Tamusu mudstone — A potential host rock for high-level radioactive waste in Inner Mongolia of China 被引量:2
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作者 Chen Lu Hongdan Yu +1 位作者 Honghui Li Weizhong Chen 《Journal of Rock Mechanics and Geotechnical Engineering》 SCIE CSCD 2022年第6期1901-1909,共9页
Tamusu mudstone, located in Bayin Gobi Basin in Inner Mongolia of China, has been selected as a potential host rock for high-level radioactive waste(HLW) disposal in China. A series of tests has been carried out, incl... Tamusu mudstone, located in Bayin Gobi Basin in Inner Mongolia of China, has been selected as a potential host rock for high-level radioactive waste(HLW) disposal in China. A series of tests has been carried out, including X-ray diffraction(XRD) tests, scanning electron microscopy(SEM) tests, disintegration tests, permeability tests and triaxial compression tests, to estimate the physico-mechanical properties of Tamusu mudstone in this work. The mineral composition of Tamusu mudstone was analyzed and it was considered as a stable rock due to its low disintegration rate, i.e. approximately 0.11%after several wet/dry cycles. Based on the results of permeability test, it was found that Tamusu mudstone has a low permeability, with the magnitude of about 10—20m^(2). The low permeability makes the mudstone well prevent nuclide migration and diffusion, and might be influenced by temperature.The triaxial tests show that Tamusu mudstone is a stiff mudstone with high compressive strength, which means that the excavation disturbed zone would be smaller compared to other types of mudstone due to construction and operation of HLW repositories. Finally, the properties of Tamusu mudstone were compared with those of Opalinus clay, Callovo-Oxfordian(COx) argillite, and Boom clay to further discuss the possibility of using Tamusu mudstone as a potential nuclear waste disposal medium. 展开更多
关键词 Tamusu mudstone Physico-mechanical properties High-level radioactive waste(HLW)repository Disintegration test Permeability test
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Assessing quinoline removal performances of an aerobic continuous moving bed biofilm reactor(MBBR) bioaugmented with Pseudomonas citronellolis LV1
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作者 Hu Chen Ying Wang +1 位作者 Puyu Wang Yongkang Lv 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2023年第5期132-140,共9页
This study evaluated the bioaugmentation potential of a quinoline-degrading strain Pseudomonas citronellolis LV1 inoculation into activated sludge for treating quinoline wastewater, and results indicated the inoculati... This study evaluated the bioaugmentation potential of a quinoline-degrading strain Pseudomonas citronellolis LV1 inoculation into activated sludge for treating quinoline wastewater, and results indicated the inoculation of LV1 in aerobic continuous MBBR could substantially improve the quinoline removal performance with an improved removal efficiency of 34% averagely when quinoline was used as the sole carbon and nitrogen source. Additionally, efficient removal of quinoline in enhanced MBBR occurred at the influent p H of 7.0–8.0, hydraulic retention time(HRT) of 24–28 h and influent quinoline concentration of 100–700 mg·L^(-1). High-throughput sequencing analysis indicated that bioaugmentation could increase microbial diversity and shape the microbial community structure. Although the inoculant LV1 did not remain its dominance in stage Ⅲ, bioaugmentation indeed induced the formation of effective microbial community, and the indigenous microbes including Flavobacterium, Pseudoxanthomonas,Pseudomonas, Vermamoeba, Dyadobacter and Sphingomonas might play the key role in quinoline removal.According to the PICRUSt, the enhanced genes encoding aromatic ring-cleavage enzyme, especially for Nheterocyclic ring-cleavage enzymes, could lead to the improved removal performance of quinoline in bioaugmentation stage. Moreover, the enhanced MBBR treated well actual coking wastewater, as indicated by high removal performance of quinoline, phenol and COD. 展开更多
关键词 Aerobic quinoline degradation Pseudomonas citronellolis LV1 BIOAUGMENTATION Microbial community Coking wastewater
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Instrument Automation Control System Faults and Maintenance
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作者 Jianwei Li 《Journal of Electronic Research and Application》 2024年第1期16-21,共6页
This article explores the topic of fault diagnosis and maintenance strategies for instrument automation control systems,analyzing them through specific cases.The aim of this research is to improve the stability and re... This article explores the topic of fault diagnosis and maintenance strategies for instrument automation control systems,analyzing them through specific cases.The aim of this research is to improve the stability and reliability of the system by conducting a thorough investigation of faults and maintenance in instrument automation control systems.By doing so,this research hopes to provide a strong guarantee for the smooth progress of industrial production. 展开更多
关键词 Instrument automation Control system failure Maintenance
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Experimental investigation on the radiation background inside body counters 被引量:2
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作者 Yu Wang Yuan-Yuan Liu +8 位作者 Bin Wu Xiang-Peng Meng Jian-Ping Cheng Ying Wang Li-Jiao Wang Yun-Shi Xiao Qin-Jian Cao Jian-Feng Zhang Fei Tuo 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2022年第2期66-78,共13页
In vivo measurement of radioactivity based on various body counters is arguably the leading measure used to determine the distribution and activity of radionuclides in human subjects,such as I-131 in the thyroid,Am-24... In vivo measurement of radioactivity based on various body counters is arguably the leading measure used to determine the distribution and activity of radionuclides in human subjects,such as I-131 in the thyroid,Am-241 in the lungs,and Pb-210 in the skull.Throughout the measurements,the radiation background is the key factor that determines the sensitivity of the counter.Therefore,to facilitate in vivo measurements,a well-designed shielding room is required to create a low-background environment.However,because the compositions of the radiation background are quite complicated,the respective contributions from each source remain obscure,which places a considerable burden on seeking an optimized design of shielding rooms that strikes the optimum balance between the construction cost and background suppression effect.In this study,we conducted a systematic experimental investigation on the radiation background outside and inside four representative body counters with assorted designs using a variety of radiation detectors,including high-purity germanium detectors,CdZnTe detector,radon emanometer,and gamma-ray dosimeter.By carefully controlling the experimental conditions and synergetic analysis of the measurement results,in conjunction with previous studies,we separated and determined the relative contributions induced by environmental radiation(4%),airborne radon and its daughters(2%),the normal radioactivity of human subjects arising from K-40(58%),cosmic rays(12%),and radioactivity in shielding materials and measuring instruments(24%).Furthermore,based on these results,we discuss practical guidelines to design a shielding room for body counters. 展开更多
关键词 Body counter Radiation background Shielding room In vivo measurement
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GRB 220408B:A Three-episode Burst from a Precessing Jet
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作者 Zijian Zhang Yi-Han Iris Yin +27 位作者 Chenyu Wang Xiangyu Ivy Wang Jun Yang Yan-Zhi Meng Zi-Ke Liu Guo-Yin Chen Xiaoping Fu Huaizhong Gao Sihao Li Yihui Liu Xiangyun Long Yong-Chang Ma Xiaofan Pan Yuanze Sun Wei Wu Zirui Yang Zhizhen Ye Xiaoyu Yu Shuheng Zhao Xutao Zheng Tao Zhou Qing-Wen Tang Qiurong Yan Rong Zhou Zhonghai Wang Hua Feng Ming Zeng Bin-Bin Zhang 《Research in Astronomy and Astrophysics》 SCIE CAS CSCD 2023年第11期214-224,共11页
Jet precession has previously been proposed to explain the apparently repeating features in the light curves of a few gamma-ray bursts(GRBs).In this paper,we further apply the precession model to a bright GRB 220408B ... Jet precession has previously been proposed to explain the apparently repeating features in the light curves of a few gamma-ray bursts(GRBs).In this paper,we further apply the precession model to a bright GRB 220408B by examining both its temporal and spectral consistency with the predictions of the model.As one of the recently confirmed GRBs observed by our GRID CubeSat mission,GRB 220408B is noteworthy as it exhibits three apparently similar emission episodes.Furthermore,the similarities are reinforced by their strong temporal correlations and similar features in terms of spectral evolution and spectral lags.Our analysis demonstrates that these features can be well explained by the modulated emission of a Fast-Rise-Exponential-Decay(FRED)shape light curve intrinsically produced by a precessing jet with a precession period of 18.4_(-0.2)~(+0.2)s,a nutation period of11.1_(-0.2)~(+0.2)s and viewed off-axis.This study provides a straightforward explanation for the complex yet similar multiepisode GRB light curves. 展开更多
关键词 gamma-rays:general (stars:)gamma-ray burst:individual(GRB 220408B) stars:jets
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Effect of E-44 Epoxy Resin and Pyrolysis Temperature on the Adhesion Strength of SiBCN Ceramic 被引量:3
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作者 马志波 常森 +9 位作者 SONG Xuemei LI Min WANG Kunjun LI Yongguo XU Xinming ZHANG Qiqi WANG Lei YU Rong LUAN Xin’gang CHENG Laifei 《Journal of Wuhan University of Technology(Materials Science)》 SCIE EI CAS 2020年第1期81-86,共6页
An adhesive of the SiBCN ceramic was synthesized through the polymer derived ceramics(PDC)route.Meanwhile with higher adhesion strength and simpler process condition,the polyborosilazane(PSNB)was modified by E-44 epox... An adhesive of the SiBCN ceramic was synthesized through the polymer derived ceramics(PDC)route.Meanwhile with higher adhesion strength and simpler process condition,the polyborosilazane(PSNB)was modified by E-44 epoxy resin.The E-44 epoxy resin was used to promote the oxidation process of SiBCN,in other words,to produce more amount of SiO2-B2O3 glasses.The phase composition,elemental analysis,chemical bonds and microstructure were investigated by using X-ray diffraction(XRD),X-ray photoelectron spectroscopy(XPS),and scanning electron microscope(SEM)measurements.The E-44 modified adhesives were cured at 120℃in air for 2 h,and were pyrolyzed at 1200,1400,and 1500℃for 2 h in air,respectively.The highest adhesion strength of the modified adhesive was up to 5.33,12.23,and 12.50 MPa after being heat treated at 1200,1400,and 1500℃,respectively.Finally,we proposed an adhesion model and revealed the adhesion mechanism of SiBCN ceramic. 展开更多
关键词 SiBCN CERAMIC PDC route E-44 EPOXY resin PYROLYSIS temperature SiO2-B2O3 GLASSES
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Reliability analysis of the gasification process of nuclear fuel manufacturing facilities based on the GO methodology 被引量:1
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作者 Yan Wang Zhi-Jie Gu +2 位作者 Bing Lian Jie Yang Yang-Jun Zhao 《Nuclear Science and Techniques》 SCIE CAS CSCD 2019年第10期85-94,共10页
Uranium hexafluoride(UF6)leakage accidents represent one of the most serious classes of accidents in the gasification process in nuclear fuel manufacturing facilities.Common UF6 leakage accidents include various fault... Uranium hexafluoride(UF6)leakage accidents represent one of the most serious classes of accidents in the gasification process in nuclear fuel manufacturing facilities.Common UF6 leakage accidents include various fault conditions,such as pipeline and valve breakages or ruptures and pipeline blockages.By establishing goal-oriented(GO)operators that can represent multi-fault states,this study estimates the probabilities of various fault states corresponding to UF6 leakage accidents in the gasification process using the GO methodology and analyzes the system reliability.This article expands the scope of the GO methodology and provides technical support for reliability analysis using the GO methodology in multi-fault systems. 展开更多
关键词 GO METHODOLOGY OPERATOR Multi-fault state Reliability analysis UF6 LEAKAGE
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Safety study on HIC containing waste resin with respect to hydrogen release 被引量:1
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作者 Shuai-Wei Zhao Mei-Lan Jia +6 位作者 Xing-Qian Jiao Meng-Qi Qiu Hong-Hui Li Yu-Chen Liu Liang Mao Wei Liu Dong Liang 《Nuclear Science and Techniques》 SCIE CAS CSCD 2019年第4期35-43,共9页
To explore the behavior of radiolytically produced hydrogen release from the waste resin stored in a high integrated container(HIC), and the mechanism of hydrogen diffusion in a near-surface disposal facility, both ex... To explore the behavior of radiolytically produced hydrogen release from the waste resin stored in a high integrated container(HIC), and the mechanism of hydrogen diffusion in a near-surface disposal facility, both experimental studies and numerical simulations were performed through an accelerated irradiation test and simulated disposal, respectively. Results indicated that,100 years after disposal, the highest hydrogen concentration appeared in the cell where the HICs were placed. The volume fraction for different scenarios postulated in the numerical simulation was 2.64% for Scenario 1, 2.28% for Scenario 2, and 3.965% for Scenario 3, all of which are lower than the hydrogen explosion limit of 4.1%. The results indicated that the simulated HIC disposal scheme is safe. 展开更多
关键词 RADIOACTIVE WASTE RESIN High integrated container REPOSITORY RADIOLYSIS Hydrogen release
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Degradation of Spent Radioactive Ion Exchange Resins and Its Mechanisms by Fenton Process 被引量:1
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作者 Wendong Feng Jian Li +1 位作者 Hongxiang An Yunhai Wang 《Journal of Renewable Materials》 SCIE EI 2020年第10期1283-1293,共11页
Spent IERs are released during the operation and decommissioning of nuclear facilities.The safe and efficient treatment of spent IERs is an emergent problem in nuclear industry.IRN77 is a typical ion exchange resin wi... Spent IERs are released during the operation and decommissioning of nuclear facilities.The safe and efficient treatment of spent IERs is an emergent problem in nuclear industry.IRN77 is a typical ion exchange resin widely used in many nuclear power plants.Fenton process can degrade organic resins and reduce the radioactive residues volume and the disposal cost significantly.In this work,the IRN77 resin was selected as a model ion exchange resin and its treatment via Fenton process was investigated.The influencing factors for resin degradation,including catalyst dosage,reaction time,initial pH,temperature and oxidant dosage were investigated and optimized via the single-factor experimental method.Under the reaction temperature of 100℃ and reaction time of 120 min at initial pH of 2,more than 97%COD was removed with 1.66 g H_(2)O_(2) and 32 mg FeSO_(4)·7H_(2)O added to per gram of wet resin.The catalyst dosage and H_(2)O_(2) dosage can decrease 78%and 50%respectively compared to previous results.SEM,FT-IR and ion chromatograph were employed to characterize the resin beads,soluble organics and intermediates during the degradation reaction.Based on the characterization results,the resin degradation pathway was discussed in detail and it is proposed to three stages including beads dissociation,styrene and divinylbenzene decomposition and carboxylic acids mineralization.During the IERs degradation,formic acid,acetic acid,propionic acid and oxalic acid were quantitatively monitored as main intermediates,and oxalic acid accounted for over 90%of COD in the final residue solution.Fenton process is suggested as a promising resin degradation method. 展开更多
关键词 FENTON RESIN DEGRADATION mechanism
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Estimation of the radionuclide distribution in sediment in coast area
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作者 SHEN Zhen-yao YANG Zhi-feng +3 位作者 LI Wei-juan NI Shi-wei YAO Lang-gen CAI Yuan 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2001年第4期398-400,共3页
The study of the radionuclide distribution in sediment is a very important aspect in environmental impact of the low level radioactive liquid waste (LLW) from coastal nuclear facilities or nuclear power plant. Even no... The study of the radionuclide distribution in sediment is a very important aspect in environmental impact of the low level radioactive liquid waste (LLW) from coastal nuclear facilities or nuclear power plant. Even now we do not know much about it. In this paper, a simple and useful method is put forward and it is used to estimate the nuclide distribution in sediment. The result showed that the LLW from nuclear facility or nuclear power plant will do a little harm to the sediment nearby. But the harm is not very serious. Much works have to be done before full understanding of the situation. 展开更多
关键词 RADIONUCLIDE COAST area DEPOSIT CHARACTERISTIC SEDIMENT
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Simulation study of the dose and energy responses of FNTD personal neutron dosimetry
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作者 Yi-Hang Wang Qiang Li +2 位作者 Li Chen Yong-Gang Yuan Tai-Ping Peng 《Nuclear Science and Techniques》 SCIE CAS CSCD 2019年第2期29-38,共10页
The objective of this work was to use the Geant4 toolkit to perform simulation studies on the personal dose response of fluorescent nuclear track detectors(FNTDs).The entire structure of the FNTD response can be desig... The objective of this work was to use the Geant4 toolkit to perform simulation studies on the personal dose response of fluorescent nuclear track detectors(FNTDs).The entire structure of the FNTD response can be designed,and the detector's energy and dose responses can be optimized in a broad energy range(0.01 eV-20 MeV). In general, the detectors used ~6LiF and CH_2 converters that have high energy and high dose response at neutron energies lower than 10 eV and greater than 1 MeV, respectively. The method of least squares was used to optimize the dose response of H*(10) and the energy response corresponding to Rtotal. The values of the optimized response of H*(10) lie between 0.8 and 1.4, corresponding to the energy ranges 0.01 eV-70 keV and 4-14 MeV, respectively. This occupies nearly eight out of the nine orders of the total energy range. Even though the optimized response of Rtotal is constrained between 0.89 and 1.1 in the energy range of 0.01 eV-20 MeV, it is suitable for obtaining the broad neutron spectrum of fluence with good accuracy. 展开更多
关键词 FNTD GEANT4 AI2O3/C Mg PERSONAL NEUTRON DOSE
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Characterization of microstructural features of Tamusu mudstone
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作者 Hongdan Yu Chen Lu +2 位作者 Weizhong Chen Diansen Yang Honghui Li 《Journal of Rock Mechanics and Geotechnical Engineering》 SCIE CSCD 2022年第6期1923-1932,共10页
Tamusu mudstone formation, located in the Alxa area in western Inner Mongolia, is considered a potential host formation for high-level radioactive waste(HLW) underground disposal in China. In this study, complementary... Tamusu mudstone formation, located in the Alxa area in western Inner Mongolia, is considered a potential host formation for high-level radioactive waste(HLW) underground disposal in China. In this study, complementary analyses with X-ray diffraction(XRD), field emission scanning electron microscopy(FE-SEM), mercury intrusion porosimetry(MIP), and N_(2) physisorption isotherm were conducted on the Tamusu mudstone to characterize its physical characteristics and microstructural features, such as mineral compositions and pore structure. Several minerals, including carbonates, feldspar, clays and analcime, were identified in Tamusu mudstone by XRD. Images from FE-SEM show that pores in the Tamusu mudstone were dominantly on nanometer scale and generally located within their mineral matrix or at the interface with non-porous minerals. The combination of the MIP and N_2 physisorption curves indicated that the Tamusu mudstone has diverse pore sizes, a porosity varying from 2.34% to 2.84%, and a total pore volume in the range of 0.0065—0.0222 cm^(3)/g with the average pore diameter ranging from 9.6 nm to 19.23 nm. The specific surface area measured by MIP(2.572—5.861 m^(2)/g) was generally higher than that by N_(2) physisorption(1.29—3.04 m^(2)/g), due to the pore network effect, pore shape(e.g. ink-bottle shape), or technique limits. The results related to pore information can be applied as an input in the future to model single-or multi-phase fluid flow and the transport of radionuclides in porous geomedium by migration and diffusion. 展开更多
关键词 Tamusu mudstone Pore structure Field emission scanning electron microscopy(FE-SEM) N_2 physisorption Mercury intrusion porosimetry(MIP)
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Optical spectroscopy study of damage evolution in 6H-SiC by H_(2)^(+)implantation
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作者 王勇 廖庆 +5 位作者 刘茗 郑鹏飞 高新宇 贾政 徐帅 李炳生 《Chinese Physics B》 SCIE EI CAS CSCD 2021年第5期75-80,共6页
Lattice defects induced by ion implantation into SiC have been widely investigated in the decades by various techniques.One of the non-destructive techniques suitable to study the lattice defects in SiC is the optical... Lattice defects induced by ion implantation into SiC have been widely investigated in the decades by various techniques.One of the non-destructive techniques suitable to study the lattice defects in SiC is the optical characterization.In this work,confocal Raman scattering spectroscopy and photoluminescence spectrum have been used to study the effects of 134-keV H_(2)^(+)implantation and thermal treatment in the microstructure of 6H-SiC single crystal.The radiation-induced changes in the microstructure were assessed by integrating Raman-scattering peaks intensity and considering the asymmetry of Raman-scattering peaks.The integrated intensities of Raman scattering spectroscopy and photoluminescence spectrum decrease with increasing the fluence.The recovery of the optical intensities depends on the combination of the implantation temperature and the annealing temperature with the thermal treatment from 700℃to 1100℃.The different characterizations of Raman scattering spectroscopy and photoluminescence spectrum are compared and discussed in this study. 展开更多
关键词 SIC H_(2)^(+)implantation Raman scattering spectroscopy photoluminescence spectrum
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Effect of PAHs on Routine Blood and Immunoglobulin Indices of Residents Living in Areas Polluted by Coking
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作者 ZHANG Ting ZHOU Xiao Lin +7 位作者 YANG Jin ZHANG Chao MENG Qian Qian XUE Zhen Wei LI Wei Bin AN Quan LIU Zhan Qi YANG Jia Qiao 《Biomedical and Environmental Sciences》 SCIE CAS CSCD 2020年第4期286-293,共8页
Incomplete combustion of bituminous coal will produce a large number of coke oven emissions(COEs).Polycyclic aromatic hydrocarbons(PAHs)account for the largest proportion of these COEs.PAHs enter the human body mainly... Incomplete combustion of bituminous coal will produce a large number of coke oven emissions(COEs).Polycyclic aromatic hydrocarbons(PAHs)account for the largest proportion of these COEs.PAHs enter the human body mainly through the respiratory tract,digestive tract,and skin[1],becoming hydroxyl PAHs(OH-PAHs)following their metabolism by the human body and are ultimately excreted mainly in urine. 展开更多
关键词 BLOOD metabolism URINE
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A novel material for passive NO_(x) adsorber:Ce-based BEA zeolite
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作者 Yan Wu Jun Wang +7 位作者 Zexiang Chen Yi Zhu Minghui Yu Chen Wang Yanping Zhai Jianqiang Wang Gurong Shen Meiqing Shen 《Journal of Rare Earths》 SCIE EI CAS CSCD 2023年第8期1163-1170,I0002,共9页
Passive NO_(x) adsorbers(PNAs)were proposed to address the NO_(x) emissions during the cold start phase.Here we show a novel Ce-based BEA zeolite,as a noble-metal-free passive NO_(x)adsorber.The NO_(x) adsorption capa... Passive NO_(x) adsorbers(PNAs)were proposed to address the NO_(x) emissions during the cold start phase.Here we show a novel Ce-based BEA zeolite,as a noble-metal-free passive NO_(x)adsorber.The NO_(x) adsorption capacity of Ce/BEA reaches 36μmol/g in the feed gas close to realistic exhaust conditions,and the NO_(x) desorption temperature,which is around 290℃,is ideal for diesel exhaust after-treatment systems.Ce/BEA also behaves notable stability of high temperature CO exposure conditions.Multiple characterizations were performed to explore the NO_(x) adsorption chemistry of Ce/BEA.The Ce(Ⅳ)species in the BEA zeolite serves as the active center for NO_(x) adsorption.The bidentate nitrate species is responsible for the observed NO_(x) storage capacity,and the active oxygen around Ce(Ⅳ)plays a critical role in its formation.Considering the significantly better cost efficiency of Ce compared to Pd,Ce/BEA presents an enormous potential for the PNA applications and provides a novel formulation for the noblemetal choice of PNA materials. 展开更多
关键词 Passive NO_(x)adsorbers Ce/BEA Non-noble-metal Cold start Rare earths
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Vertebral plate regeneration induced by radiation-sterilized allogeneic bone sheets in sheep 被引量:7
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作者 唐欣 杨述华 +8 位作者 许伟华 李进 杨操 叶哲伟 傅德皓 李鲲 李宝兴 孙世荃 余从年 《Chinese Journal of Traumatology》 CAS 2007年第1期34-39,共6页
关键词 椎板切除术 关节疾病 脊椎 椎板成形术
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Effect of cumulative gamma irradiation on microstructure and corrosion behaviour of X65 low carbon steel 被引量:3
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作者 Canshuai Liu Jianqiu Wang +5 位作者 Zhiming Zhang En-Hou Han Wei Liu Dong Liang Zhongtian Yang Xingzhong Cao 《Journal of Materials Science & Technology》 SCIE EI CAS CSCD 2018年第11期2131-2139,共9页
X65 low carbon steel was exposed to Co-60 radiation source with 1.25 MeV gamma rays, and cumulatively absorbed gamma irradiation doses(1, 2, and 3 MGy) were obtained after different exposure time(333, 667, and 1000 h)... X65 low carbon steel was exposed to Co-60 radiation source with 1.25 MeV gamma rays, and cumulatively absorbed gamma irradiation doses(1, 2, and 3 MGy) were obtained after different exposure time(333, 667, and 1000 h). The effect of cumulative gamma irradiation on microstructure and corrosion behaviour of the carbon steel in unirradiated aerobic Beishan groundwater at 25?C was investigated by using positron annihilation, scanning vibrating electrode, and electrochemical techniques. Cumulative gamma irradiation increases vacancy intensity and decreases open circuit potential(OCP) of carbon steel. They indicate that the irradiated carbon steel is activated. Measured current density distribution above the irradiated carbon steel shows that cumulative gamma irradiation accelerates localized corrosion after 0.5 h of immersion. In contrast, the analysis of electrochemical impedance spectroscopy of the irradiated carbon steel indicates that localized corrosion is transformed into general corrosion after 12 h of immersion, which is also accelerated by cumulative gamma irradiation. 展开更多
关键词 GAMMA 腐蚀行为 微观结构 低碳钢 累积 电气化学 暴露时间 正电子
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Solution-processed lead-free bulk 0D Cs3Cu2I5 single crystal for indirect gamma-ray spectroscopy application 被引量:3
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作者 Qiang Xu Juan Wang +8 位作者 Qindong Zhang Xiao Ouyang Maheng Ye Weiting Xie Xuewen Yan Deyuan Li Xiaoping Ouyang Xiaobing Tang Xiaodong Zhang 《Photonics Research》 SCIE EI CAS CSCD 2021年第3期351-356,共6页
Bulk scintillators that are with high density,low cost,and fine pulse-height energy spectral resolution,and are nonhygroscopic and user friendly,are desired for high-energy gamma-ray spectroscopy application.Recently,... Bulk scintillators that are with high density,low cost,and fine pulse-height energy spectral resolution,and are nonhygroscopic and user friendly,are desired for high-energy gamma-ray spectroscopy application.Recently,low-cost solution-processed perovskite nanoscintillators have been demonstrated with outstanding performances for indirect low-energy X-ray detection;however,the stability and thickness are not suitable for high-energy gamma-ray detection.Here,we report scintillation performances of a low-cost solution-processed bulk 0D Cs3Cu2I5 single crystal.The self-trapped exciton emission results in a large Stokes shift (109 nm) that is reabsorption free.A broad X-ray excited emission matches well with the sensitivity of a silicon photodiode.The unique Cs+ surrounded isolated [Cu2I5]3-cluster scintillator provides ultra-stability in air and strong radiation hardness under high-dose gammaray exposure from a 60Co source.This solution-processed Cs3Cu2I5 scintillator is expected with low-cost and has detection performances comparable to commercial alkali-halide scintillator products. 展开更多
关键词 SPECTROSCOPY stability CRYSTAL
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