We investigate the localized surface plasmon(LSP) effect by Al nanorings on the AlGaN/GaN multiple quantum well(MQW) structure emitting at 365 nm. For this experiment, first, the size of Al nanorings is optimized to m...We investigate the localized surface plasmon(LSP) effect by Al nanorings on the AlGaN/GaN multiple quantum well(MQW) structure emitting at 365 nm. For this experiment, first, the size of Al nanorings is optimized to maximize the energy transfer(or coupling) between the LSP and MQW using the silica nanospheres. Then, the Al nanorings with an outer diameter of 385 nm, which exhibit a strong absorption peak in the near-ultraviolet region, are applied to the top surface of the AlGaN/GaN MQW. The photoluminescence(PL) intensity of the MQW structure with Al nanorings increased by 227% at 365 nm compared to that without Al nanorings.This improvement is mainly attributed to an enhanced radiative recombination rate in the MQWs through the energy-matched LSPs by the temperature-dependent PL and time-resolved PL analyses. The radiative lifetime was about two times shorter than that of the structure without Al nanorings at room temperature. In addition, the measured PL efficiency at room temperature of the structure with Al nanorings was 33%, while that of the structure without Al nanorings was 19%, implying that LSP-QW coupling together with the nanoring array pattern itself played important roles in the enhancement.展开更多
White light-emitting diodes(LEDs)are becoming an alternative general light source,with huge energy savings compared to conventional lighting.However,white LEDs using phosphor(s)suffer from unavoidable Stokes energy co...White light-emitting diodes(LEDs)are becoming an alternative general light source,with huge energy savings compared to conventional lighting.However,white LEDs using phosphor(s)suffer from unavoidable Stokes energy converting losses,higher manufacturing cost,and reduced thermal stability.Here,we demonstrate electrically driven,phosphor-free,white LEDs based on three-dimensional gallium nitride structures with double concentric truncated hexagonal pyramids.The electroluminescence spectra are stable with varying current.The origin of the emission wavelength is studied by cathodoluminescence and high-angle annular dark field scanning transmission electron microscopy experiments.Spatial variation of the carrier injection efficiency is also investigated by a comparative analysis between spatially resolved photoluminescence and electroluminescence.展开更多
基金National Research Foundation of Korea(NRF)(2016R1A3B 1908249)
文摘We investigate the localized surface plasmon(LSP) effect by Al nanorings on the AlGaN/GaN multiple quantum well(MQW) structure emitting at 365 nm. For this experiment, first, the size of Al nanorings is optimized to maximize the energy transfer(or coupling) between the LSP and MQW using the silica nanospheres. Then, the Al nanorings with an outer diameter of 385 nm, which exhibit a strong absorption peak in the near-ultraviolet region, are applied to the top surface of the AlGaN/GaN MQW. The photoluminescence(PL) intensity of the MQW structure with Al nanorings increased by 227% at 365 nm compared to that without Al nanorings.This improvement is mainly attributed to an enhanced radiative recombination rate in the MQWs through the energy-matched LSPs by the temperature-dependent PL and time-resolved PL analyses. The radiative lifetime was about two times shorter than that of the structure without Al nanorings at room temperature. In addition, the measured PL efficiency at room temperature of the structure with Al nanorings was 33%, while that of the structure without Al nanorings was 19%, implying that LSP-QW coupling together with the nanoring array pattern itself played important roles in the enhancement.
基金supported by the National Research Foundation(NRF-2013R1A2A1A01016914,NRF-2013R1A1A2011750)the Ministry of Education,the Industrial Strategic Technology Development Program(10041878)+1 种基金the Ministry of Knowledge Economy,the Climate Change Research Hub of KAIST(Grant No.N01150041)the GRC project of KAIST Institute for the NanoCentury.
文摘White light-emitting diodes(LEDs)are becoming an alternative general light source,with huge energy savings compared to conventional lighting.However,white LEDs using phosphor(s)suffer from unavoidable Stokes energy converting losses,higher manufacturing cost,and reduced thermal stability.Here,we demonstrate electrically driven,phosphor-free,white LEDs based on three-dimensional gallium nitride structures with double concentric truncated hexagonal pyramids.The electroluminescence spectra are stable with varying current.The origin of the emission wavelength is studied by cathodoluminescence and high-angle annular dark field scanning transmission electron microscopy experiments.Spatial variation of the carrier injection efficiency is also investigated by a comparative analysis between spatially resolved photoluminescence and electroluminescence.