We report the controlled fabrication of nitrogen doped graphene(NG)nanoplates,which are uniformly decorated with iron nitride(Fe_(3)N)nanoparticles,via ball milling of mixtures of graphite and iron nitrates and the fo...We report the controlled fabrication of nitrogen doped graphene(NG)nanoplates,which are uniformly decorated with iron nitride(Fe_(3)N)nanoparticles,via ball milling of mixtures of graphite and iron nitrates and the following ammonia annealing.The obtained Fe_(3)N@NG composites demonstrate excellent electrocatalytic activity and durability for oxygen evolution reaction,both of which outperform those of the state-of-the-art iridium oxide catalysts.This may be attributed to nitrogen doping as well as the synergistic effect between Fe3N and graphene nanoplates.展开更多
基金supported by the Open Research Fund Program of State Environmental Protection Key Laboratory of Food Chain Pollution Control(FC2022YB05,FC2022YB03)National Key Research and Development Program of China(2022YFE0105800)+2 种基金Shandong Top Talent Special Foundation(0031504),Natural Science Foundation of Beijing Municipality(8222042)Huzhou Science and Technology Project(2023GZ60)Special Research Funds of Shandong Jianzhu University(X20077Z0101 and X20087Z0101).
文摘We report the controlled fabrication of nitrogen doped graphene(NG)nanoplates,which are uniformly decorated with iron nitride(Fe_(3)N)nanoparticles,via ball milling of mixtures of graphite and iron nitrates and the following ammonia annealing.The obtained Fe_(3)N@NG composites demonstrate excellent electrocatalytic activity and durability for oxygen evolution reaction,both of which outperform those of the state-of-the-art iridium oxide catalysts.This may be attributed to nitrogen doping as well as the synergistic effect between Fe3N and graphene nanoplates.