Optical holography is a promising technique to achieve a naked-eye 3D display.However,the narrow viewing angle and chromatic aberration are the two key issues that usually limit the holographic display performance.A r...Optical holography is a promising technique to achieve a naked-eye 3D display.However,the narrow viewing angle and chromatic aberration are the two key issues that usually limit the holographic display performance.A recent work proposes a novel way to circumvent these constraints by introducing a color liquid crystal grating into a timesequenced holography system.展开更多
In recent years,femtosecond(fs)-lasers have evolved into a versatile tool for high precision micromachining of transparent materials because nonlinear absorption in the focus can result in refractive index modificatio...In recent years,femtosecond(fs)-lasers have evolved into a versatile tool for high precision micromachining of transparent materials because nonlinear absorption in the focus can result in refractive index modifications or material disruptions.However,when high pulse energies or low numerical apertures are required,nonlinear side effects such as self-focusing,filamentation or white light generation can decrease the modification quality.In this paper,we apply simultaneous spatial and temporal focusing(SSTF)to overcome these limitations.The main advantage of SSTF is that the ultrashort pulse is only formed at the focal plane,thereby confining the intensity distribution strongly to the focal volume and suppressing detrimental nonlinear side effects.Thus,we investigate the optical breakdown within a water cell by pump-probe shadowgraphy,comparing conventional focusing and SSTF under equivalent focusing conditions.The plasma formation is well confined for low pulse energies,2 mJ,but higher pulse energies lead to the filamentation and break-up of the disruptions for conventional focusing,thereby decreasing the modification quality.In contrast,plasma induced by SSTF stays well confined to the focal plane,even for high pulse energies up to 8 mJ,preventing extended filaments,side branches or break-up of the disruptions.Furthermore,while conventional focusing leads to broadband supercontinuum generation,only marginal spectral broadening is observed using SSTF.These experimental findings are in excellent agreement with numerical simulations of the nonlinear pulse propagation and interaction processes.Therefore,SSTF appears to be a powerful tool to control the processing of transparent materials,e.g.,for precise ophthalmic fs-surgery.展开更多
Ultrathin metasurfaces have shown the capability to influence all aspects of light propagation.This has made them promising options for replacing conventional bulky imaging optics while adding advantageous optical pro...Ultrathin metasurfaces have shown the capability to influence all aspects of light propagation.This has made them promising options for replacing conventional bulky imaging optics while adding advantageous optical properties or functionalities.We demonstrate that such metasurfaces can also be applied for single-lens three-dimensional(3-D)imaging based on a specifically engineered point-spread function(PSF).Using Huygens’metasurfaces with high transmission,we design and realize a phase mask that implements a rotating PSF for 3-D imaging.We experimentally characterize the properties of the realized double-helix PSF,finding that it can uniquely encode object distances within a wide range.Furthermore,we experimentally demonstrate wide-field depth retrieval within a 3-D scene,showing the suitability of metasurfaces to realize optics for 3-D imaging,using just a single camera and lens system.展开更多
Since the advent of femtosecond lasers,performance improvements have constantly impacted on existing applications and enabled novel applications.However,one performance feature bearing the potential of a quantum leap ...Since the advent of femtosecond lasers,performance improvements have constantly impacted on existing applications and enabled novel applications.However,one performance feature bearing the potential of a quantum leap for high-field applications is still not available:the simultaneous emission of extremely high peak and average powers.Emerging applications such as laser particle acceleration require exactly this performance regime and,therefore,challenge laser technology at large.On the one hand,canonical bulk systems can provide pulse peak powers in the multi-terawatt to petawatt range,while on the other hand,advanced solid-state-laser concepts such as the thin disk,slab or fibre are well known for their high efficiency and their ability to emit high average powers in the kilowatt range with excellent beam quality.In this contribution,a compact laser system capable of simultaneously providing high peak and average powers with high wall-plug efficiency is proposed and analysed.The concept is based on the temporal coherent combination(pulse stacking)of a pulse train emitted from a high-repetition-rate femtosecond laser system in a passive enhancement cavity.Thus,the pulse energy is increased at the cost of the repetition rate while almost preserving the average power.The concept relies on a fast switching element for dumping the enhanced pulse out of the cavity.The switch constitutes the key challenge of our proposal.Addressing this challenge could,for the first time,allow the highly efficient dumping of joule-class pulses at megawatt average power levels and lead to unprecedented laser parameters.展开更多
In the 2015 review paper‘Petawatt Class Lasers Worldwide’a comprehensive overview of the current status of highpower facilities of>200 TW was presented.This was largely based on facility specifications,with some ...In the 2015 review paper‘Petawatt Class Lasers Worldwide’a comprehensive overview of the current status of highpower facilities of>200 TW was presented.This was largely based on facility specifications,with some description of their uses,for instance in fundamental ultra-high-intensity interactions,secondary source generation,and inertial confinement fusion(ICF).With the 2018 Nobel Prize in Physics being awarded to Professors Donna Strickland and Gerard Mourou for the development of the technique of chirped pulse amplification(CPA),which made these lasers possible,we celebrate by providing a comprehensive update of the current status of ultra-high-power lasers and demonstrate how the technology has developed.We are now in the era of multi-petawatt facilities coming online,with 100 PW lasers being proposed and even under construction.In addition to this there is a pull towards development of industrial and multi-disciplinary applications,which demands much higher repetition rates,delivering high-average powers with higher efficiencies and the use of alternative wavelengths:mid-IR facilities.So apart from a comprehensive update of the current global status,we want to look at what technologies are to be deployed to get to these new regimes,and some of the critical issues facing their development.展开更多
Aperiodic sinusoidal patterns that are cast by a GOBO(GOes Before Optics)projector are a powerful tool for optically measuring the surface topography of moving or deforming objects with very high speed and accuracy.We...Aperiodic sinusoidal patterns that are cast by a GOBO(GOes Before Optics)projector are a powerful tool for optically measuring the surface topography of moving or deforming objects with very high speed and accuracy.We optimised the first experimental setup that we were able to measure inflating car airbags at frame rates of more than 50 kHz while achieving a 3D point standard deviation of~500μm.Here,we theoretically investigate the method of GOBO projection of aperiodic sinusoidal fringes.In a simulation-based performance analysis,we examine the parameters that influence the accuracy of the measurement result and identify an optimal pattern design that yields the highest measurement accuracy.We compare the results with those that were obtained via GOBO projection of phase-shifted sinusoidal fringes.Finally,we experimentally verify the theoretical findings.We show that the proposed technique has several advantages over conventional fringe projection techniques,as the easy-to-build and cost-effective GOBO projector can provide a high radiant flux,allows high frame rates,and can be used over a wide spectral range.展开更多
Optical metasurfaces,which consist of subwavelength scale meta-atoms,represent a novel platform to manipulate the polarization and phase of light.The optical performance of metasurfaces heavily relies on the quality o...Optical metasurfaces,which consist of subwavelength scale meta-atoms,represent a novel platform to manipulate the polarization and phase of light.The optical performance of metasurfaces heavily relies on the quality of nanofabrication.Retrieving the Jones matrix of an imperfect metasurface optical element is highly desirable.We show that this can be realized by decomposing the generalized Jones matrix of a meta-atom into two parallel ones,which correspond to the ideal matrix and a phase retardation.To experimentally verify this concept,we designed and fabricated metasurface polarizers,which consist of geometric phase-controlled dielectric meta-atoms.By scanning the polarization states of the incident and transmitted light,we are able to extract the coefficients of the two parallel matrices of a metasurface polarizer.Based on the results of the Jones matrix decomposition,we also demonstrated polarization image encryption and spin-selective optical holography.The proposed Jones matrix retrieval protocol may have important applications in computational imaging,optical computing,optical communications,and so on.展开更多
Spatial engineering of the nonlinear susceptibility χ^((2)) in resonant metasurfaces offers a new degree of freedom in the design of the far-field response of second-harmonic generation(SHG). We demonstrate this by a...Spatial engineering of the nonlinear susceptibility χ^((2)) in resonant metasurfaces offers a new degree of freedom in the design of the far-field response of second-harmonic generation(SHG). We demonstrate this by applying electric field poling to lithium niobate(LN) thin films, which inverts the spontaneous polarization and thus the sign of χ^((2)). Metasurfaces fabricated in periodically poled LN films reveal the distinct influence of theχ^((2))-patterning on the spatial distribution of the second harmonic. This work is a first step toward far-field engineering of SHG in metasurfaces with electric field poling.展开更多
Rare earth-doped fibres are a diode-pumped,solid-state laser architecture that is highly scalable in average power.The performance of pulsed fibre laser systems is restricted due to nonlinear effects.Hence,fibre desig...Rare earth-doped fibres are a diode-pumped,solid-state laser architecture that is highly scalable in average power.The performance of pulsed fibre laser systems is restricted due to nonlinear effects.Hence,fibre designs that allow for very large mode areas at high average powers with diffraction-limited beam quality are of enormous interest.Ytterbium-doped,rod-type,large-pitch fibres(LPF)enable extreme fibre dimensions,i.e.,effective single-mode fibres with mode sizes exceeding 100 times the wavelength of the guided radiation,by exploiting the novel concept of delocalisation of higher-order transverse modes.The non-resonant nature of the operating principle makes LPF suitable for high power extraction.This design allows for an unparalleled level of performance in pulsed fibre lasers.展开更多
The process of high harmonic generation(HHG)enables the development of table-top sources of coherent extreme ultraviolet(XUV)light.Although these are now matured sources,they still mostly rely on bulk laser technology...The process of high harmonic generation(HHG)enables the development of table-top sources of coherent extreme ultraviolet(XUV)light.Although these are now matured sources,they still mostly rely on bulk laser technology that limits the attainable repetition rate to the low kilohertz regime.Moreover,many of the emerging applications of such light sources(e.g.,photoelectron spectroscopy and microscopy,coherent diffractive imaging,or frequency metrology in the XUV spectral region)require an increase in the repetition rate.Ideally,these sources are operated with a multi-MHz repetition rate and deliver a high photon flux simultaneously.So far,this regime has been solely addressed using passive enhancement cavities together with low energy and high repetition rate lasers.Here,a novel route with significantly reduced complexity(omitting the requirement of an external actively stabilized resonator)is demonstrated that achieves the previously mentioned demanding parameters.A krypton-filled Kagome photonic crystal fiber is used for efficient nonlinear compression of 9 μJ,250 fs pulses leading to,7 μJ,31 fs pulses at 10.7 MHz repetition rate.The compressed pulses are used for HHG in a gas jet.Particular attention is devoted to achieving phase-matched(transiently)generation yielding.10^(13) photons s^(-1)(.50 μW)at 27.7 eV.This new spatially coherent XUV source improved the photon flux by four orders of magnitude for direct multi-MHZ experiments,thus demonstrating the considerable potential of this source.展开更多
The development of high-power,broadband sources of coherent mid-infrared radiation is currently the subject of intense research that is driven by a substantial number of existing and continuously emerging applications...The development of high-power,broadband sources of coherent mid-infrared radiation is currently the subject of intense research that is driven by a substantial number of existing and continuously emerging applications in medical diagnostics,spectroscopy,microscopy,and fundamental science.One of the major,long-standing challenges in improving the performance of these applications has been the construction of compact,broadband mid-infrared radiation sources,which unify the properties of high brightness and spatial and temporal coherence.Due to the lack of such radiation sources,several emerging applications can be addressed only with infrared(IR)-beamlines in largescale synchrotron facilities,which are limited regarding user access and only partially fulfill these properties.Here,we present a table-top,broadband,coherent mid-infrared light source that provides brightness at an unprecedented level that supersedes that of synchrotrons in the wavelength range between 3.7 and 18μm by several orders of magnitude.This result is enabled by a high-power,few-cycle Tm-doped fiber laser system,which is employed as a pump at 1.9μm wavelength for intrapulse difference frequency generation(IPDFG).IPDFG intrinsically ensures the formation of carrierenvelope-phase stable pulses,which provide ideal prerequisites for state-of-the-art spectroscopy and microscopy.展开更多
Thermally induced refractive index gratings in Yb-doped fibers lead to transverse mode instability(TMI)above an average power threshold,which represents a severe problem for many applications.To obtain a deeper unders...Thermally induced refractive index gratings in Yb-doped fibers lead to transverse mode instability(TMI)above an average power threshold,which represents a severe problem for many applications.To obtain a deeper understanding of TMI,the evolution of the strength of the thermally induced refractive index grating with the average output power in a fiber amplifier is experimentally investigated for the first time.This investigation is performed by introducing a phase shift between the refractive index grating and modal interference pattern,which is obtained by applying a pump power variation to the fiber amplifier.It is demonstrated that the refractive index grating is sufficiently strong to enable modal energy coupling at powers that are significantly below the TMI threshold if the induced phase shift is sufficiently large.The experiments indicate that at higher powers,the refractive index grating becomes more sensitive to such phase shifts,which will ultimately trigger TMI.Furthermore,the experimental results demonstrate beam cleaning above the TMI threshold via the introduction of a positive phase shift.This finding paves the way for the development of a new class of mitigation strategies for TMI that are based on controlling the phase shift between the thermally induced refractive index grating and modal interference pattern.展开更多
Bright,coherent soft X-ray radiation is essential to a variety of applications in fundamental research and life sciences.To date,a high photon flux in this spectral region can only be delivered by synchrotrons,free-el...Bright,coherent soft X-ray radiation is essential to a variety of applications in fundamental research and life sciences.To date,a high photon flux in this spectral region can only be delivered by synchrotrons,free-electron lasers or high-order harmonic generation sources,which are driven by kHz-class repetition rate lasers with very high peak powers.Here,we establish a novel route toward powerful and easy-to-use SXR sources by presenting a compact experimentin which nonlinear pulse self-compression to the few-cycle regime is combined with phase-matched high-orderharmonic generation in a single,helium-illed antiresonant hollow-core fibre.This enables the first 100 kHz-classrepetition rate,table-top soft X-ray source that delivers an application-relevant flux of 2.8×10^6 photon s^-1 eV^-1 around 300 ev.The fibre integration of temporal pulse self-compression(leading to the formation of the necessarystrong-field waveforms)and pressure-controlled phase matching will allow compact,high-repetition-rate lasertechnology,including commercially available systems,to drive simple and cost-effective,coherent high-flux softX-ray sources.展开更多
Microscopy with extreme ultraviolet(EUV)radiation holds promise for high-resolution imaging with excellent material contrast,due to the short wavelength and numerous element-specific absorption edges available in this...Microscopy with extreme ultraviolet(EUV)radiation holds promise for high-resolution imaging with excellent material contrast,due to the short wavelength and numerous element-specific absorption edges available in this spectral range.At the same time,EUV radiation has significantly larger penetration depths than electrons.It thus enables a nano-scale view into complex three-dimensional structures that are important for material science,semiconductor metrology,and next-generation nano-devices.Here,we present high-resolution and material-specific microscopy at 13.5 nm wavelength.We combine a highly stable,high photon-flux,table-top EUV source with an interferometrically stabilized ptychography setup.By utilizing structured EUV illumination,we overcome the limitations of conventional EUV focusing optics and demonstrate high-resolution microscopy at a half-pitch lateral resolution of 16 nm.Moreover,we propose mixed-state orthogonal probe relaxation ptychography,enabling robust phase-contrast imaging over wide fields of view and long acquisition times.In this way,the complex transmission of an integrated circuit is precisely reconstructed,allowing for the classification of the material composition of mesoscopic semiconductor systems.展开更多
We propose a novel quantum nonlinear interferometer design that incorporates a passive parity-time(PT)-symmetric coupler sandwiched between two nonlinear sections where signal-idler photon pairs are generated.The PT s...We propose a novel quantum nonlinear interferometer design that incorporates a passive parity-time(PT)-symmetric coupler sandwiched between two nonlinear sections where signal-idler photon pairs are generated.The PT symmetry enables efficient coupling of the longer-wavelength idler photons and facilitates the sensing of losses in the second waveguide exposed to analyte under investigation,whose absorption can be inferred by measuring only the signal intensity at a shorter wavelength where efficient detectors are readily available.Remarkably,we identify a new phenomenon of sharp signal intensity fringe shift at critical idler loss values,which is distinct from the previously studied PT symmetry breaking.We discuss how such unconventional properties arising from quantum interference can provide a route to enhancing the sensing of analytes and facilitate broadband spectroscopy applications in integrated photonic platforms.展开更多
A comprehensive material study of different transparent conductive oxides (TCOs) is presented. The layers are deposited by pulsed direct current (DC) magnetron sputtering in an inline sputtering system. Indium tin...A comprehensive material study of different transparent conductive oxides (TCOs) is presented. The layers are deposited by pulsed direct current (DC) magnetron sputtering in an inline sputtering system. Indium tin oxide (ITO) films are studied in detail. The optimum pressure of 0.33 Pa (15Ar:202) produces a 300- nm thin film with a specific resistivity p of 2.2 × 10-6 Ωm and a visual transmittance of 81%. Alternatively, ZnO:A1 and ZnO:Ga layers with thicknesses of 200 and 250 nm are deposited with a minimum resistivity of 5.5× 10-6 and 6.8× 10-6Ωm, respectively. To compare the optical properties in the ultraviolet (UV) range, the optical spectra are modeled and the band gap is determined.展开更多
基金the National Key Technologies R&D Program of China(2022YFA1404301)the National Natural Science Foundation of China(12161141010).
文摘Optical holography is a promising technique to achieve a naked-eye 3D display.However,the narrow viewing angle and chromatic aberration are the two key issues that usually limit the holographic display performance.A recent work proposes a novel way to circumvent these constraints by introducing a color liquid crystal grating into a timesequenced holography system.
基金This study was supported by the Thuringian Ministry of Education,Science and Culture(OptiMi 2020-Graduate Research School‘Green Photonics’,B514-10061)the German Research Foundation(Leibniz program)the Carl Zeiss Foundation.
文摘In recent years,femtosecond(fs)-lasers have evolved into a versatile tool for high precision micromachining of transparent materials because nonlinear absorption in the focus can result in refractive index modifications or material disruptions.However,when high pulse energies or low numerical apertures are required,nonlinear side effects such as self-focusing,filamentation or white light generation can decrease the modification quality.In this paper,we apply simultaneous spatial and temporal focusing(SSTF)to overcome these limitations.The main advantage of SSTF is that the ultrashort pulse is only formed at the focal plane,thereby confining the intensity distribution strongly to the focal volume and suppressing detrimental nonlinear side effects.Thus,we investigate the optical breakdown within a water cell by pump-probe shadowgraphy,comparing conventional focusing and SSTF under equivalent focusing conditions.The plasma formation is well confined for low pulse energies,2 mJ,but higher pulse energies lead to the filamentation and break-up of the disruptions for conventional focusing,thereby decreasing the modification quality.In contrast,plasma induced by SSTF stays well confined to the focal plane,even for high pulse energies up to 8 mJ,preventing extended filaments,side branches or break-up of the disruptions.Furthermore,while conventional focusing leads to broadband supercontinuum generation,only marginal spectral broadening is observed using SSTF.These experimental findings are in excellent agreement with numerical simulations of the nonlinear pulse propagation and interaction processes.Therefore,SSTF appears to be a powerful tool to control the processing of transparent materials,e.g.,for precise ophthalmic fs-surgery.
基金We thank Waltraud Gräf,Daniel Voigt,Michael Banasch,and Thomas Käsebier for help with the fabrication.Financial support by the German Research Foundation within the Emmy-Noether program and the SPP“Tailored Disorder”(STA 1426/1-1,STA 1426/2-1,PE 1524/10-2)is gratefully acknowledged.Part of this research was funded by the German Federal Ministry of Education and Research(BMBF)under the project identifiers 13N14147 and 03ZZ0434.
文摘Ultrathin metasurfaces have shown the capability to influence all aspects of light propagation.This has made them promising options for replacing conventional bulky imaging optics while adding advantageous optical properties or functionalities.We demonstrate that such metasurfaces can also be applied for single-lens three-dimensional(3-D)imaging based on a specifically engineered point-spread function(PSF).Using Huygens’metasurfaces with high transmission,we design and realize a phase mask that implements a rotating PSF for 3-D imaging.We experimentally characterize the properties of the realized double-helix PSF,finding that it can uniquely encode object distances within a wide range.Furthermore,we experimentally demonstrate wide-field depth retrieval within a 3-D scene,showing the suitability of metasurfaces to realize optics for 3-D imaging,using just a single camera and lens system.
基金This work has been partly supported by the German Federal Ministry of Education and Research(BMBF)under contract 13N12082‘NEXUS’,by the Thuringian Ministry of Education,Science and Culture(TMBWK)under contract 12037-515‘BURST’by the European Research Council under the ERC grant agreement no.[617173]‘ACOPS’+3 种基金by the Deutsche Forschungsgemeinschaft Cluster of Excellence‘Munich-Centre for Advanced Photonics’(munich-photonics.de).AK acknowledges financial support by the Helmholtz-Institute Jena.TE acknowledges financial support by the CarlZeiss-Stiftung.IP and SH acknowledge financial support by the BMBF under PhoNa-Photonische Nanomaterialien,contract number 03IS2101B.
文摘Since the advent of femtosecond lasers,performance improvements have constantly impacted on existing applications and enabled novel applications.However,one performance feature bearing the potential of a quantum leap for high-field applications is still not available:the simultaneous emission of extremely high peak and average powers.Emerging applications such as laser particle acceleration require exactly this performance regime and,therefore,challenge laser technology at large.On the one hand,canonical bulk systems can provide pulse peak powers in the multi-terawatt to petawatt range,while on the other hand,advanced solid-state-laser concepts such as the thin disk,slab or fibre are well known for their high efficiency and their ability to emit high average powers in the kilowatt range with excellent beam quality.In this contribution,a compact laser system capable of simultaneously providing high peak and average powers with high wall-plug efficiency is proposed and analysed.The concept is based on the temporal coherent combination(pulse stacking)of a pulse train emitted from a high-repetition-rate femtosecond laser system in a passive enhancement cavity.Thus,the pulse energy is increased at the cost of the repetition rate while almost preserving the average power.The concept relies on a fast switching element for dumping the enhanced pulse out of the cavity.The switch constitutes the key challenge of our proposal.Addressing this challenge could,for the first time,allow the highly efficient dumping of joule-class pulses at megawatt average power levels and lead to unprecedented laser parameters.
文摘In the 2015 review paper‘Petawatt Class Lasers Worldwide’a comprehensive overview of the current status of highpower facilities of>200 TW was presented.This was largely based on facility specifications,with some description of their uses,for instance in fundamental ultra-high-intensity interactions,secondary source generation,and inertial confinement fusion(ICF).With the 2018 Nobel Prize in Physics being awarded to Professors Donna Strickland and Gerard Mourou for the development of the technique of chirped pulse amplification(CPA),which made these lasers possible,we celebrate by providing a comprehensive update of the current status of ultra-high-power lasers and demonstrate how the technology has developed.We are now in the era of multi-petawatt facilities coming online,with 100 PW lasers being proposed and even under construction.In addition to this there is a pull towards development of industrial and multi-disciplinary applications,which demands much higher repetition rates,delivering high-average powers with higher efficiencies and the use of alternative wavelengths:mid-IR facilities.So apart from a comprehensive update of the current global status,we want to look at what technologies are to be deployed to get to these new regimes,and some of the critical issues facing their development.
基金supported by the German Federal Ministry of Education and Research(BMBF)under project number 03ZZ0436.
文摘Aperiodic sinusoidal patterns that are cast by a GOBO(GOes Before Optics)projector are a powerful tool for optically measuring the surface topography of moving or deforming objects with very high speed and accuracy.We optimised the first experimental setup that we were able to measure inflating car airbags at frame rates of more than 50 kHz while achieving a 3D point standard deviation of~500μm.Here,we theoretically investigate the method of GOBO projection of aperiodic sinusoidal fringes.In a simulation-based performance analysis,we examine the parameters that influence the accuracy of the measurement result and identify an optimal pattern design that yields the highest measurement accuracy.We compare the results with those that were obtained via GOBO projection of phase-shifted sinusoidal fringes.Finally,we experimentally verify the theoretical findings.We show that the proposed technique has several advantages over conventional fringe projection techniques,as the easy-to-build and cost-effective GOBO projector can provide a high radiant flux,allows high frame rates,and can be used over a wide spectral range.
基金supported by the National Key Technologies R&D Program of China (Grant No.2022YFA1404301)the Zhangjiang Laboratory,the National Natural Science Foundation of China (Grant Nos.91950114 and 12161141010)+2 种基金the Guangdong Provincial Innovation and Entrepreneurship Project (Grant No.2017ZT07C071)the Guangdong Provincial Key Laboratory Program (Grant No.2021B1212040001)the Natural Science Foundation of Shenzhen Innovation Commission (Grant No.JCYJ20200109140808088).
文摘Optical metasurfaces,which consist of subwavelength scale meta-atoms,represent a novel platform to manipulate the polarization and phase of light.The optical performance of metasurfaces heavily relies on the quality of nanofabrication.Retrieving the Jones matrix of an imperfect metasurface optical element is highly desirable.We show that this can be realized by decomposing the generalized Jones matrix of a meta-atom into two parallel ones,which correspond to the ideal matrix and a phase retardation.To experimentally verify this concept,we designed and fabricated metasurface polarizers,which consist of geometric phase-controlled dielectric meta-atoms.By scanning the polarization states of the incident and transmitted light,we are able to extract the coefficients of the two parallel matrices of a metasurface polarizer.Based on the results of the Jones matrix decomposition,we also demonstrated polarization image encryption and spin-selective optical holography.The proposed Jones matrix retrieval protocol may have important applications in computational imaging,optical computing,optical communications,and so on.
基金Freistaat Thüringen[Pro Excellence initiative(ACP2020),Quantum Hub Thuringia(2021 FGI 0043)]The European Union(METAFAST-899673-FETOPENH2020)+1 种基金Bundesministerium für Bildung und Forschung(13N14877,13N16108)Deutsche Forschungsgemeinschaft(407070005,CRC 1375 NOA 398816777,subprojects B2and C2,PE 1524/13-1,SE 2749/1-1,STA 1426/2-1)
文摘Spatial engineering of the nonlinear susceptibility χ^((2)) in resonant metasurfaces offers a new degree of freedom in the design of the far-field response of second-harmonic generation(SHG). We demonstrate this by applying electric field poling to lithium niobate(LN) thin films, which inverts the spontaneous polarization and thus the sign of χ^((2)). Metasurfaces fabricated in periodically poled LN films reveal the distinct influence of theχ^((2))-patterning on the spatial distribution of the second harmonic. This work is a first step toward far-field engineering of SHG in metasurfaces with electric field poling.
基金The research leading to these results received funding from the European Research Council under the European Union’s Seventh Framework Programme(FP7/2007-2013)/ERC Grant Agreement No.[240460]the Thuringian Ministry of Education,Science and Culture under contract PE203-2-1(MOFA)and contract B514-10061(Green Photonics).FJ acknowledges financial support from the Abbe School of Photonics.
文摘Rare earth-doped fibres are a diode-pumped,solid-state laser architecture that is highly scalable in average power.The performance of pulsed fibre laser systems is restricted due to nonlinear effects.Hence,fibre designs that allow for very large mode areas at high average powers with diffraction-limited beam quality are of enormous interest.Ytterbium-doped,rod-type,large-pitch fibres(LPF)enable extreme fibre dimensions,i.e.,effective single-mode fibres with mode sizes exceeding 100 times the wavelength of the guided radiation,by exploiting the novel concept of delocalisation of higher-order transverse modes.The non-resonant nature of the operating principle makes LPF suitable for high power extraction.This design allows for an unparalleled level of performance in pulsed fibre lasers.
基金This work was partly supported by the German Federal Ministry of Education and Research(BMBF)the European Research Council under the European Union’s Seventh Framework Programme(FP7/2007-2013)/ERC Grant Agreement No.240460Arno Klenke and Jan Rothhardt acknowledge financial support by the Helmholtz-Institute Jena.
文摘The process of high harmonic generation(HHG)enables the development of table-top sources of coherent extreme ultraviolet(XUV)light.Although these are now matured sources,they still mostly rely on bulk laser technology that limits the attainable repetition rate to the low kilohertz regime.Moreover,many of the emerging applications of such light sources(e.g.,photoelectron spectroscopy and microscopy,coherent diffractive imaging,or frequency metrology in the XUV spectral region)require an increase in the repetition rate.Ideally,these sources are operated with a multi-MHz repetition rate and deliver a high photon flux simultaneously.So far,this regime has been solely addressed using passive enhancement cavities together with low energy and high repetition rate lasers.Here,a novel route with significantly reduced complexity(omitting the requirement of an external actively stabilized resonator)is demonstrated that achieves the previously mentioned demanding parameters.A krypton-filled Kagome photonic crystal fiber is used for efficient nonlinear compression of 9 μJ,250 fs pulses leading to,7 μJ,31 fs pulses at 10.7 MHz repetition rate.The compressed pulses are used for HHG in a gas jet.Particular attention is devoted to achieving phase-matched(transiently)generation yielding.10^(13) photons s^(-1)(.50 μW)at 27.7 eV.This new spatially coherent XUV source improved the photon flux by four orders of magnitude for direct multi-MHZ experiments,thus demonstrating the considerable potential of this source.
基金supported by the German Federal Ministry of Education and Research(BMBF)under contract“NUKLEUS”(13N13973)the United States AFOSR(FA9550-15-10041)+2 种基金the United States ARO(W911NF-12-1-0450 and W911NF-17-1-0501)support by the Helmholtz-Institute Jenasupport by the Carl Zeiss Stiftung.
文摘The development of high-power,broadband sources of coherent mid-infrared radiation is currently the subject of intense research that is driven by a substantial number of existing and continuously emerging applications in medical diagnostics,spectroscopy,microscopy,and fundamental science.One of the major,long-standing challenges in improving the performance of these applications has been the construction of compact,broadband mid-infrared radiation sources,which unify the properties of high brightness and spatial and temporal coherence.Due to the lack of such radiation sources,several emerging applications can be addressed only with infrared(IR)-beamlines in largescale synchrotron facilities,which are limited regarding user access and only partially fulfill these properties.Here,we present a table-top,broadband,coherent mid-infrared light source that provides brightness at an unprecedented level that supersedes that of synchrotrons in the wavelength range between 3.7 and 18μm by several orders of magnitude.This result is enabled by a high-power,few-cycle Tm-doped fiber laser system,which is employed as a pump at 1.9μm wavelength for intrapulse difference frequency generation(IPDFG).IPDFG intrinsically ensures the formation of carrierenvelope-phase stable pulses,which provide ideal prerequisites for state-of-the-art spectroscopy and microscopy.
基金supported by the German Research Foundation(DFG)within the International Research Training Group(IRTG)2101by the European Research Council under the ERC grant“ACOPS”,agreement no.617173+1 种基金by the Fraunhofer and Max Planck cooperation program within the project“PowerQuant”by the German Federal Ministry of Education and Research(BMBF),project no.PT-VDI,TEHFA Ⅱ.
文摘Thermally induced refractive index gratings in Yb-doped fibers lead to transverse mode instability(TMI)above an average power threshold,which represents a severe problem for many applications.To obtain a deeper understanding of TMI,the evolution of the strength of the thermally induced refractive index grating with the average output power in a fiber amplifier is experimentally investigated for the first time.This investigation is performed by introducing a phase shift between the refractive index grating and modal interference pattern,which is obtained by applying a pump power variation to the fiber amplifier.It is demonstrated that the refractive index grating is sufficiently strong to enable modal energy coupling at powers that are significantly below the TMI threshold if the induced phase shift is sufficiently large.The experiments indicate that at higher powers,the refractive index grating becomes more sensitive to such phase shifts,which will ultimately trigger TMI.Furthermore,the experimental results demonstrate beam cleaning above the TMI threshold via the introduction of a positive phase shift.This finding paves the way for the development of a new class of mitigation strategies for TMI that are based on controlling the phase shift between the thermally induced refractive index grating and modal interference pattern.
基金The authors would like to thank Prof.Adrian Pfeiffer and Dr.Felix Kittig forfruitful discussions and help with the numerical methods.Furthermore,theauthors would like to thank Dr.Steffen Hadrich,Dr.Cesar Jauregui-Misas,andTobias Ulsperger for their help in the early stages of this work.This work wassupported by the European Research Council(ERC)under the EuropeanUnion's Horizon 2020 research and innovation programme(grant 835306,SALT)the Fraunhofer Cluster of Excellence Advanced Photon Sources(CAPS)+1 种基金the Helmholtz-Institute Jena,the U.S.Army Research Office(grant W911NF1910426)the U.S.Air Force Office of Scientific Research(grantFA9550-15-10041).
文摘Bright,coherent soft X-ray radiation is essential to a variety of applications in fundamental research and life sciences.To date,a high photon flux in this spectral region can only be delivered by synchrotrons,free-electron lasers or high-order harmonic generation sources,which are driven by kHz-class repetition rate lasers with very high peak powers.Here,we establish a novel route toward powerful and easy-to-use SXR sources by presenting a compact experimentin which nonlinear pulse self-compression to the few-cycle regime is combined with phase-matched high-orderharmonic generation in a single,helium-illed antiresonant hollow-core fibre.This enables the first 100 kHz-classrepetition rate,table-top soft X-ray source that delivers an application-relevant flux of 2.8×10^6 photon s^-1 eV^-1 around 300 ev.The fibre integration of temporal pulse self-compression(leading to the formation of the necessarystrong-field waveforms)and pressure-controlled phase matching will allow compact,high-repetition-rate lasertechnology,including commercially available systems,to drive simple and cost-effective,coherent high-flux softX-ray sources.
基金supported by the Federal State of Thuringia(2017 FGR 0076)the European Social Fund(ESF)+1 种基金the Thüringer Aufbaubank(TAB)for funding the junior research group HOROS(FKZ:2017 FGR 0076)the European Research Council(ERC)under the European Union’s Horizon 2020 research and innovation programm(grant agreement No.[835306],SALT)。
文摘Microscopy with extreme ultraviolet(EUV)radiation holds promise for high-resolution imaging with excellent material contrast,due to the short wavelength and numerous element-specific absorption edges available in this spectral range.At the same time,EUV radiation has significantly larger penetration depths than electrons.It thus enables a nano-scale view into complex three-dimensional structures that are important for material science,semiconductor metrology,and next-generation nano-devices.Here,we present high-resolution and material-specific microscopy at 13.5 nm wavelength.We combine a highly stable,high photon-flux,table-top EUV source with an interferometrically stabilized ptychography setup.By utilizing structured EUV illumination,we overcome the limitations of conventional EUV focusing optics and demonstrate high-resolution microscopy at a half-pitch lateral resolution of 16 nm.Moreover,we propose mixed-state orthogonal probe relaxation ptychography,enabling robust phase-contrast imaging over wide fields of view and long acquisition times.In this way,the complex transmission of an integrated circuit is precisely reconstructed,allowing for the classification of the material composition of mesoscopic semiconductor systems.
基金Australian Research Council(DP190100277)German Research Foundation(SE 2749/1-1)+1 种基金German Federal Ministry of Education and Research(13N14877)UA-DAAD exchange scheme(57559284)。
文摘We propose a novel quantum nonlinear interferometer design that incorporates a passive parity-time(PT)-symmetric coupler sandwiched between two nonlinear sections where signal-idler photon pairs are generated.The PT symmetry enables efficient coupling of the longer-wavelength idler photons and facilitates the sensing of losses in the second waveguide exposed to analyte under investigation,whose absorption can be inferred by measuring only the signal intensity at a shorter wavelength where efficient detectors are readily available.Remarkably,we identify a new phenomenon of sharp signal intensity fringe shift at critical idler loss values,which is distinct from the previously studied PT symmetry breaking.We discuss how such unconventional properties arising from quantum interference can provide a route to enhancing the sensing of analytes and facilitate broadband spectroscopy applications in integrated photonic platforms.
文摘A comprehensive material study of different transparent conductive oxides (TCOs) is presented. The layers are deposited by pulsed direct current (DC) magnetron sputtering in an inline sputtering system. Indium tin oxide (ITO) films are studied in detail. The optimum pressure of 0.33 Pa (15Ar:202) produces a 300- nm thin film with a specific resistivity p of 2.2 × 10-6 Ωm and a visual transmittance of 81%. Alternatively, ZnO:A1 and ZnO:Ga layers with thicknesses of 200 and 250 nm are deposited with a minimum resistivity of 5.5× 10-6 and 6.8× 10-6Ωm, respectively. To compare the optical properties in the ultraviolet (UV) range, the optical spectra are modeled and the band gap is determined.