We report the realization of a synthetic magnetic field for photons and polaritons in a honeycomb lattice of coupled semiconductor micropillars.A strong synthetic field is induced in both the s and p orbital bands by ...We report the realization of a synthetic magnetic field for photons and polaritons in a honeycomb lattice of coupled semiconductor micropillars.A strong synthetic field is induced in both the s and p orbital bands by engineering a uniaxial hopping gradient in the lattice,giving rise to the formation of Landau levels at the Dirac points.We provide direct evidence of the sublattice symmetry breaking of the lowest-order Landau level wavefunction,a distinctive feature of synthetic magnetic fields.Our realization implements helical edge states in the gap between n=0 and n=±1 Landau levels,experimentally demonstrating a novel way of engineering propagating edge states in photonic lattices.In light of recent advances in the enhancement of polariton–polariton nonlinearities,the Landau levels reported here are promising for the study of the interplay between pseudomagnetism and interactions in a photonic system.展开更多
The writings of the text on the last line,left column on the 4^th page and the text on lines 8^th,10^th,11^th and 16^th in the 4^th paragraph,left column and on lines from 1st to 8^th in the 1st paragraph,right column...The writings of the text on the last line,left column on the 4^th page and the text on lines 8^th,10^th,11^th and 16^th in the 4^th paragraph,left column and on lines from 1st to 8^th in the 1st paragraph,right column on the 5^th page,and the text on line 4^th in the 1^st paragraph,left column on the 9^th page,and Fig.3 and its caption on the 5^th page in the original version of this article were unfortunately incorrect.展开更多
Expanding the functionalities of plasmon-assisted lasers is essential for emergent applications in nanoscience and nanotechnology.Here,we report on a novel ability of plasmonic structures to induce dual-wavelength las...Expanding the functionalities of plasmon-assisted lasers is essential for emergent applications in nanoscience and nanotechnology.Here,we report on a novel ability of plasmonic structures to induce dual-wavelength lasing in the near-infrared region in a Yb^(3+) solid-state laser.By means of the effects of disordered plasmonic networks deposited on the surface of a Yb^(3+)-doped nonlinear RTP crystal,room-temperature dual-wavelength lasing,with a frequency difference between the lines in the THz range,is realized.The dual-wavelength laser is produced by the simultaneous activation of two lasing channels,namely,an electronic-and a phonon-terminated laser transition.The latter is enabled by the out-of-plane field components that are generated by the plasmonic structures,which excite specific Raman modes.Additionally,multiline radiation at three different wavelengths is demonstrated in the visible spectral region via two self-frequency conversion processes,which occur in the vicinities of the plasmonic structures.The results demonstrate the potential of plasmonic nanostructures for inducing drastic modifications in the operational mode of a solid-state laser and hold promise for applications in a variety of fields,including multiplexing,precise spectroscopies,and THz radiation generation via a simple and cost-effective procedure.展开更多
Though it is well recognized that the space between graphene cover and the metal substrate canact as a two-dimensional(2D)nanoreactor,several issues are still unresolved,including the role of the metal substrate,the m...Though it is well recognized that the space between graphene cover and the metal substrate canact as a two-dimensional(2D)nanoreactor,several issues are still unresolved,including the role of the metal substrate,the mechanisms ruling water intercalation and the identification ofsites at which water is decomposed.Here,we solve these issues by means of density functional theory and high-resolution electron energyloss spectroscopy experiments carried out on graphene grown on(111)-oriented Cu foils.Specifically,we observe decomposition of H2O atroom temperature with only H atoms forming bonds with graphene and with buried OH groups underneath the graphene cover.Ourtheoretical model discloses physicochemical mechanisms ruling the migration and decomposition of water on graphene/Cu.We discover thatthe edge of graphene can be easily saturated by H through decomposition of H2O,which allows H2O to migrate in the subsurface region from thedecoupled edge,where H2O decomposes at room temperature.Hydrogen atoms produced by the decomposition of H2O initially form a chemicalbond with graphene for the lower energy barrier compared with other routes.These findings are essential to exploit graphene/Cu interfaces incatalysis and in energy-related applications.展开更多
基金supported by the ERC grant Honeypol,the H2020-FETFLAG project PhoQus(820392)the QUANTERA project Interpol(ANR-QUAN-0003-05)+11 种基金the French National Research Agency project Quantum Fluids of Light(ANR-16-CE30-0021)the French government through the Programme Investissement d’Avenir(I-SITE ULNE/ANR-16-IDEX-0004 ULNE)managed by the Agence Nationale de la Recherchethe French RENATECH network,the Labex CEMPI(ANR-11-LABX-0007)the CPER Photonics for Society P4S and the Metropole Europeenne de Lille(MEL)via the project TFlightfinancial support from the FPI Scholarship No.BES-2015-074708the Spanish MINECO grant No.MAT2017-83722-Rsupported by funding from the ERC Starting Grant TopoColdsupported by JSPS KAKENHI Grant Number JP18H05857JST PRESTO Grant Number JPMJPR19L2JST CREST Grant Number JPMJCR19T1the RIKEN Incentive Research Projectthe Interdisciplinary Theoretical and Mathematical Sciences Program(iTHEMS)at RIKEN.
文摘We report the realization of a synthetic magnetic field for photons and polaritons in a honeycomb lattice of coupled semiconductor micropillars.A strong synthetic field is induced in both the s and p orbital bands by engineering a uniaxial hopping gradient in the lattice,giving rise to the formation of Landau levels at the Dirac points.We provide direct evidence of the sublattice symmetry breaking of the lowest-order Landau level wavefunction,a distinctive feature of synthetic magnetic fields.Our realization implements helical edge states in the gap between n=0 and n=±1 Landau levels,experimentally demonstrating a novel way of engineering propagating edge states in photonic lattices.In light of recent advances in the enhancement of polariton–polariton nonlinearities,the Landau levels reported here are promising for the study of the interplay between pseudomagnetism and interactions in a photonic system.
文摘The writings of the text on the last line,left column on the 4^th page and the text on lines 8^th,10^th,11^th and 16^th in the 4^th paragraph,left column and on lines from 1st to 8^th in the 1st paragraph,right column on the 5^th page,and the text on line 4^th in the 1^st paragraph,left column on the 9^th page,and Fig.3 and its caption on the 5^th page in the original version of this article were unfortunately incorrect.
基金support from the Spanish Government under project MAT2016-76106-RComunidad de Madrid under grant S2013/MIT-2740+4 种基金funding from the Spanish Government under projects MAT2016-75716-C2-1-R(AEI/FEDER,UE)TEC2014-55948-RGeneralitat de Catalunya under project 2017SGR755grant FPU13/02476 from the Spanish Ministry of Educationfinancial support from the Spanish Government,through The“Maria de Maeztu”Programme for Units of Excellence in R&D(MDM-2014-0377)”.
文摘Expanding the functionalities of plasmon-assisted lasers is essential for emergent applications in nanoscience and nanotechnology.Here,we report on a novel ability of plasmonic structures to induce dual-wavelength lasing in the near-infrared region in a Yb^(3+) solid-state laser.By means of the effects of disordered plasmonic networks deposited on the surface of a Yb^(3+)-doped nonlinear RTP crystal,room-temperature dual-wavelength lasing,with a frequency difference between the lines in the THz range,is realized.The dual-wavelength laser is produced by the simultaneous activation of two lasing channels,namely,an electronic-and a phonon-terminated laser transition.The latter is enabled by the out-of-plane field components that are generated by the plasmonic structures,which excite specific Raman modes.Additionally,multiline radiation at three different wavelengths is demonstrated in the visible spectral region via two self-frequency conversion processes,which occur in the vicinities of the plasmonic structures.The results demonstrate the potential of plasmonic nanostructures for inducing drastic modifications in the operational mode of a solid-state laser and hold promise for applications in a variety of fields,including multiplexing,precise spectroscopies,and THz radiation generation via a simple and cost-effective procedure.
基金This work was supported by the National Natural Science Foundation of China(Nos.21676232 and 21673206).A.P.thanks Danil W.Boukhvalov for scientific discussions and Vito Fabio for technical support for the HREELS experiments.D.F.acknowledges financial support from the Spanish Ministry of Economy and Competitiveness,through the Maria de Maeztu Programme for Units of Excellence in R&D(No.MDM-2014-0377)and MINECO project MAT2015-65356-C3-3-R.
文摘Though it is well recognized that the space between graphene cover and the metal substrate canact as a two-dimensional(2D)nanoreactor,several issues are still unresolved,including the role of the metal substrate,the mechanisms ruling water intercalation and the identification ofsites at which water is decomposed.Here,we solve these issues by means of density functional theory and high-resolution electron energyloss spectroscopy experiments carried out on graphene grown on(111)-oriented Cu foils.Specifically,we observe decomposition of H2O atroom temperature with only H atoms forming bonds with graphene and with buried OH groups underneath the graphene cover.Ourtheoretical model discloses physicochemical mechanisms ruling the migration and decomposition of water on graphene/Cu.We discover thatthe edge of graphene can be easily saturated by H through decomposition of H2O,which allows H2O to migrate in the subsurface region from thedecoupled edge,where H2O decomposes at room temperature.Hydrogen atoms produced by the decomposition of H2O initially form a chemicalbond with graphene for the lower energy barrier compared with other routes.These findings are essential to exploit graphene/Cu interfaces incatalysis and in energy-related applications.