We performed detailed temperature-dependent optical measurements on optimally doped Ba0.6K0.4Fe2As2 single crystal, We examine the changes of the in-plane optical conductivity spectral weight in the normal state and t...We performed detailed temperature-dependent optical measurements on optimally doped Ba0.6K0.4Fe2As2 single crystal, We examine the changes of the in-plane optical conductivity spectral weight in the normal state and the evolution of the superconducting condensate in the superconducting state. In the normal state, the low-frequency spectral weight shows a metallic response with an arctan (T) dependence, indicating a T-linear scattering rate behavior for the carriers. A high energy spectral weight transfer associated with the Hund's coupling occurs from the low frequencies below 4000 cm^-1 5000 cm^-1 to higher frequencies up to at least 104 cm^-1. Its temperature dependence analysis suggests that the Hund's coupling strength is continuously enhanced as the temperature is reduced. In the superconducting state, the FGT sum rule is conserved according to the spectral weight estimation within the conduction bands, only about 40% of the conduction bands participates in the superconducting condensate indicating that Ba0.6K0.4Fe2As2 is in dirty limit.展开更多
The far-infrared optical reflectivity of an optimaUy doped Ba1-xKxFe2As2 (x = 0.4) single crystal is measured from room temperature down to 4 K. We study the temperature dependence of the in-plane infrared-active ph...The far-infrared optical reflectivity of an optimaUy doped Ba1-xKxFe2As2 (x = 0.4) single crystal is measured from room temperature down to 4 K. We study the temperature dependence of the in-plane infrared-active phonon at 251 em-1. This phonon exhibits a symmetric line shape in the optical conductivity, suggesting that the coupling between the phonon and the electronic background is weak. Upon cooling down, the frequency of this phonon continu- ously increases, following the conventional temperature dependence expected in the absence of a structural or magnetic transition. The intensity of this phonon is temperature independent within the measurement accuracy. These observa- tions indicate that the structural and magnetic phase transition might be completely suppressed by chemical doping in the optimally doped Bao.6Ko.4Fe2As2 compound.展开更多
基金Project supported by the National Basic Research Program of China(Grant Nos.2012CB821403,2011CBA00107,and 2012CB921302)the National Natural Science Foundation of China(Grant Nos.11374345,11104335,and 91121004)
文摘We performed detailed temperature-dependent optical measurements on optimally doped Ba0.6K0.4Fe2As2 single crystal, We examine the changes of the in-plane optical conductivity spectral weight in the normal state and the evolution of the superconducting condensate in the superconducting state. In the normal state, the low-frequency spectral weight shows a metallic response with an arctan (T) dependence, indicating a T-linear scattering rate behavior for the carriers. A high energy spectral weight transfer associated with the Hund's coupling occurs from the low frequencies below 4000 cm^-1 5000 cm^-1 to higher frequencies up to at least 104 cm^-1. Its temperature dependence analysis suggests that the Hund's coupling strength is continuously enhanced as the temperature is reduced. In the superconducting state, the FGT sum rule is conserved according to the spectral weight estimation within the conduction bands, only about 40% of the conduction bands participates in the superconducting condensate indicating that Ba0.6K0.4Fe2As2 is in dirty limit.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 11104335 and 91121004), the National Basic Research Program of China (Grant Nos. 2011CBA00107, 2012CB821400, and 2009CB929102), and the ANR, France (Grant No. BLAN07-1-183876 GAPSUPRA).
文摘The far-infrared optical reflectivity of an optimaUy doped Ba1-xKxFe2As2 (x = 0.4) single crystal is measured from room temperature down to 4 K. We study the temperature dependence of the in-plane infrared-active phonon at 251 em-1. This phonon exhibits a symmetric line shape in the optical conductivity, suggesting that the coupling between the phonon and the electronic background is weak. Upon cooling down, the frequency of this phonon continu- ously increases, following the conventional temperature dependence expected in the absence of a structural or magnetic transition. The intensity of this phonon is temperature independent within the measurement accuracy. These observa- tions indicate that the structural and magnetic phase transition might be completely suppressed by chemical doping in the optimally doped Bao.6Ko.4Fe2As2 compound.