Advantageous properties of halide perovskite quantum dots towards energy-efficient sustainable applications

As lead halide perovskite(LHP)semiconductors have shown tremendous promise in many application fields,and particularly made strong impact in the solar photovoltaic area,low dimensional quantum dot forms of these perovskites are showing the potential to make distinct marks in the fields of electronics,optoelectronics and photonics.The so-called perovskite quantum dots(PQDs)not only possess the most important features of LHP materials,i.e.,the unusual high defect tolerance,but also demonstrate clear quantum size effects,along with exhibiting desirable optoelectronic properties such as near perfect photoluminescent quantum yield,multiple exciton generation and slow hot-carrier cooling.Here,we review the advantageous properties of these nanoscale perovskites and survey the prospects for diverse applications which include lightemitting devices,solar cells,photocatalysts,lasers,detectors and memristors,emphasizing the distinct superiorities as well as the challenges.

Thermodynamics of charged AdS black hole surrounded by quintessence in restricted phase space

We study thermodynamics of charged AdS black hole surrounded by quintessence in a new formalism which is called the restricted phase space thermodynamics.This context is based on Visser’s holographic thermodynamics with a fixed antide Sitter radius and a variable Newton constant.The conjugate variables,central charge C and the chemical potential m,are introduced as a new pair of thermodynamic variables.We find that the iso-e-charge T-S curve becomes non-monotonic when Q<Q_(c).Correspondingly,the F-T curve exhibits a swallow tail structure.This behavior is considered as a van der Waals-like phase transition.As the value of b related to the energy density of Kiselev’s fluid becomes larger,the critical temperature T_(c)will decrease.Thus,the van derWaals-like phase transition will occur at lower temperature.There is always a non-quilibrium transition from a small unstable black hole to a large stable black hole state in the isocoltage T-S process.There exist a maximum and a Hawking-Page phase transition points in theμ-C plane.As the value of b related to Kiselev’s fluid becomes larger,the Hawking-Page phase transition will occur at lower temperature in the isovoltageμ-T process.For other values of the state parameterω,there also exists van der Waals-like phase transition.

Microscopic growth mechanism and edge states of monolayer 1T'-MoTe_(2)

Transition metal ditellurides(TMTDs)have versatile physical properties,including non-trivial topology,Weyl semimetal states and unique spin texture.Controlled growth of high-quality and large-scale monolayer TMTDs with preferred crystal phases is crucial for their applications.Here,we demonstrate the epitaxial growth of 1T'-MoTe_(2) on Au(111)and graphitized silicon carbide(Gr/SiC)by molecular beam epitaxy(MBE).We investigate the morphology of the grown1T'-MoTe_(2) at the atomic level by scanning tunnelling microscopy(STM)and reveal the corresponding microscopic growth mechanism.It is found that the unique ordered Te structures preferentially deposited on Au(111)regulate the growth of monolayer single crystal 1T'-MoTe_(2),while the Mo clusters were preferentially deposited on the Gr/SiC substrate,which impedes the ordered growth of monolayer MoTe_(2).We confirm that the size of single crystal 1T'-MoTe_(2) grown on Au(111)is nearly two orders of magnitude larger than that on Gr/SiC.By scanning tunnelling spectroscopy(STS),we observe that the STS spectrum of the monolayer 1T'-MoTe_(2) nano-island at the edge is different from that at the interior,which exhibits enhanced conductivity.

Systematic study of the synthesis of heavy and superheavy nuclei in 48Ca-induced fusion-evaporation reactions

We systematically studied the evaporation residue cross sections of ^(48)Ca-induced reactions on lanthanide and actinide target nuclei under the Dinuclear System(DNS)model framework to check the reliability and applicability of the model.To produce new proton-rich Fl and Lv isotopes through hot fusion reactions in the superheavy element region with Z≥104,we utilized the reactions ^(48)Ca+^(236,238,239) Pu and ^(48)Ca+^(242,243,244,250) Cm.However,owing to the detection limit of available equipment(0.1 pb),only 283Fl and 287−289Lv,which have the maximum evaporation residue cross section values of 0.149,0.130,9.522,and 0.309 pb,respectively,can be produced.Furthermore,to produce neutron-deficient isotopes of actinides near the proton drip line with Z=93−100,we attempted to generate the new isotopes(224−227Pu,228−232,237Cm)using the reactions ^(48)Ca+180,182,183 W and ^(48)Ca+^(184,186,187,192) Os.The maximum evaporation residue cross section values are 0.07,0.06,0.26,and 0.30 nb for the former set of reactions,and 1.96 pb,5.73 pb,12.16 pb,19.39 pb,54.79 pb,and 6.45 nb for the latter,respectively.These results are expected to provide new information for the future synthesis of unknown neutron-deficient isotopes.

Controlling Entropic Uncertainty in the Presence of Quantum Memory by Non-Markovian Effects and Atom-Cavity Couplings

Based on the time-convolutionless master-equation approach, the entropic uncertainty in the presence of quantum memory is investigated for a two-atom system in two dissipative cavities. We find that the entropic uncertainty can be controlled by the non-Markovian effect and the atom-cavity coupling. The results show that increasing the atom-cavity coupling can enlarge the oscillating frequencies of the entropic uncertainty and can decrease the minimal value of the entropic uncertainty. Enhancing the non-Markovian effect can reduce the minimal value of the entropic uncertainty. In particular, if the atom-cavity coupling or the non-Markovian effect is very strong, the entropic uncertainty will be very dose to zero at certain time points, thus Bob can minimize his uncertainty about Alice＇s measurement outcomes,

Quantum speed limit time of a two-level atom under different quantum feedback control

We investigate the quantum speed limit time （QSLT） of a two-level atom under quantum-jump-based feedback control or homodyne-based feedback control. Our results show that the two different feedback control schemes have different influences on the evolutionary speed. By adjusting the feedback parameters, the quantum-jump-based feedback control can induce speedup of the atomic evolution from an excited state, but the homodyne-based feedback control cannot change the evolutionary speed. Additionally, the QSLT for the whole dynamical process is explored. Under the quantum-jump-based feedback control, the QSLT displays oscillatory behaviors, which implies multiple speed-up and speed-down processes during the evolution. While, the homodyne-based feedback control can accelerate the speed-up process and improve the uniform speed in the uniform evolution process.

Quantum discord of two-qutrit system under quantum-jump-based feedback control

This paper studies quantum discord of two qutrits coupled to their own environments independently and coupled to the same environment simultaneously under quantum-jump-based feedback control. Our results show that spontaneous emission, quantum feedback parameters, classical driving, initial state, and detection efficiency all affect the evolution of quantum discord in a two-qutrit system. We find that under the condition of designing proper quantum-jump-based feedback parameters, quantum discord can be protected and prepared. In the case where two qutrits are independently coupled to their own environments, classical driving, spontaneous emission, and low detection efficiency have negative effect on the protection of quantum discord. For different initial states, it is found that the evolution of quantum discord under the control of appropriate parameters is similar. In the case where two qutrits are simultaneously coupled to the same environment,the classical driving plays a positive role in the generation of quantum discord, but spontaneous emission and low detection efficiency have negative impact on the generation of quantum discord. Most importantly, we find that the steady discord depends on feedback parameters, classical driving, and detection efficiency, but not on the initial state.

Spontaneous emission of a moving atom in a waveguide of rectangular cross section

We study the spontaneous emission(SE) of an excited nonrelativistic two-level system(TLS) interacting with the vacuum in a waveguide of rectangular cross section. All TLS’s transitions and the center-of-mass motion of the TLS are taken into account. The SE rate and the carried frequency of the emitted photon for the TLS initially being at rest are obtained, it is found that in the first order of the mass M, the frequency of the emitted photon is smaller than the transition frequency of the TLS and the SE rate is smaller than the SE rate Γfof the TLS fixed in the same waveguide. The SE rate for the TLS initially being moving is obtained in the second order of the mass M. The SE rate is smaller than Γfbut it is dependent not only on the atomic mass but also on the initial momentum. The carried frequency of the emitted photon is decreased when it travels along the direction of the initial momentum, whereas it is increased when it travels in the opposite direction of the initial momentum.

Remote Quantum-Information Concentration: Reversal of Ancilla-Free Phase-Covariant Telecloning

Telecloning and its reverse process, referred to as remote quantum-information concentration (RQIC), have been attracting considerable interest because of their potential applications in quantum-information processing. The previous RQIC protocols were focused on the reverse process of the optimal universal telecloning. We here study the reverse process of ancilla-free phase-covariant telecloning (AFPCT). It is shown that the quantum information originally distributed into two spatially separated qubits from a single qubit via the optimal AFPCT procedure can be remotely concentrated back to a single qubit with a certain probability by using an asymmetric W state as the quantum channel.

Phase effect on dynamics of quantum discord modulated by interaction between qubits

We study the effects of the interaction strength and the initial phase on the dynamics of quantum discord in a twoqubit system under both spontaneous emission and dephasing noisy channels. It is shown that the time evolution of quantum discord displays quicker oscillations with increasing inter-qubit interaction strength but the effect of the initial phase closely depends on the interaction between the qubits. Only for non-zero inter-qubit interaction cases, the evolution of quantum discord is affected by the initial phase and its oscillating amplitude increases with increasing initial phase. A comparison between evolutions of quantum discord and entanglement is also made.

Control of entanglement between two atoms by the Stark shift

Considering a quantum model consisting of two effective two-level atoms and a single-mode cavity, this paper investigates the entanglement dynamics between the two atoms, and studies the effect of the Stark shift on the entanglement. The results show that, on the one hand the atom-atom entanglement evolves periodically with time and the periods are affected by the Stark shift; on the other hand, the two atoms are not disentangled at any time when the Stark shift is considered, and for large values of the Stark shift parameter, the two atoms can remain in a stationary entangled state. In addition, for the initially partially entangled atomic state, the atom-atom entanglement can be greatly enhanced due to the presence of Stark shift. These properties show that the Stark shift can be used to control entanglement between two atoms.

Combined Effect of Classical Chaos and Quantum Resonance on Entanglement Dynamics

We use linear entropy of an exact quantum state to study the entanglement between internal electronic states and external motional states for a two-level atom held in an amplitude-modulated and tilted optical lattice. Starting from an unentangled initial state associated with the regular ＇island＇ of classical phase space, it is demonstrated that the quantum resonance leads to entanglement generation, the chaotic parameter region results in the increase of the generation speed, and the symmetries of the initial probability distribution determine the final degree of entanglement. The entangled initial states are associated with the classical ＇chaotic sea＇, which do not affect the final entanglement degree for the same initial symmetry. The results may be useful in engineering quantum dynamics for quantum information processing.

Quantum speed limit time of a non-Hermitian two-level system

We investigated the quantum speed limit time of a non-Hermitian two-level system for which gain and loss of energy or amplitude are present. Our results show that, with respect to two distinguishable states of the non-Hermitian system, the evolutionary time does not have a nonzero lower bound. The quantum evolution of the system can be effectively accelerated by adjusting the non-Hermitian parameter, as well as the quantum speed limit time can be arbitrarily small even be zero.

Symmetric Telecloning and Entanglement Distribution of Spin Quantum States

We propose a physical realization of symmetric telecloning machine for spin quantum states. The concept of area average fidelity is introduced to describe the telecloning quality. It is indicated that for certain input states this quantity may come to an enough high level to satisfy the need of quantum information processing. We also study the properties of entanglement distribution via the spin chain for arbitrary two-qubit entangled pure states as inputs and find that the decay ratio of entanglement for the output states is only determined by the parameters of spin chain and waiting time, independent of the initial input states.

Dynamical control of population and entanglement for open Λ-type atoms by engineering the environment

The exactly analytical solution for the dynamics of the dissipative Λ-type atom in the zero-temperature Lorentzian environment is presented. On this basis, we study the evolution of the population and entanglement. We find that the stable populations on the two lower levels of the Λ-type atom can be effectively adjusted by the combination of the relative decay rate and the environmental spectral frequency. However, for the initial Werner-like state, the stable entanglement between the two Λ-type atoms has very little tunability. Furthermore, the stable entanglement for the bilateral environment case is larger than that of the unilateral environmental case. A nonintuitive relation between the stable entanglement and stable population is found.

Controlling the electronic structure of SnO_2 nanowires by Mo-doping

Mo-doped SnO2 （MTO） nanowires are synthesized by an in-situ doping chemical vapour deposition method. Raman scattering spectra indicate that the lattice symmetry of MTO nanowires lowers with the increase of Mo doping, which implies that Mo ions do enter into the lattice of SnO2 nanowire. Ultraviolet-visible diffuse reflectance spectra show that the band gap of MTO nanowires decreases with the increase of Mo concentration. The photoluminescence emission of SnO2 nanowires around 580~nm at room temperature can also be controlled accurately by Mo-doping, and it is extremely sensitive to Mo ions and will disappear when the atomic ratio reaches 0.46%.

Quantum routing of few photons using a nonlinear cavity coupled to two chiral waveguides

We investigate few-photon scattering properties in two one-dimensional waveguides chirally coupled to a nonlinear cavity.The quantum states of scattered few photons are solved analytically via a real-space approach,and the solution indicates the few-photon reflection and transmission properties.When inputting two photons of equal energy to resonate with the cavity,the propagation characteristics of the two photons will be interesting,which is different from the previous anti-bunching effects with a quantum emitter.More importantly,when the total energy of the two incident photons equals the energy of a nonlinear cavity accommodating two photons,influence of the bound state will become larger to result in disappearance of antibunching effect.However,the bound state has no effect on probability of routing to another waveguide.

Dynamics of quantum discord in a two-qubit system under classical noise

We study the quantum discord dynamics of two noninteracting qubits that are, respectively, subject to classical noise. The results show that the dynamics of quantum discord are dependent on both the coupling between the qubits and classical noise, and the average switching rate of the classical noise. In the weak-coupling Markovian region, quantum discord exhibits exponent decay without revival, and can be well protected by increasing the average classical noise switching rate. While in the strong-coupling non-Markovian region, quantum discord reveals slowly decayed oscillations with quick revival by decreasing the average switching rate of the classical noise. Thus, our results provide a new method of protecting quantum discord in a two-qubit system by controlling the coupling between the qubits and classical noise, and the average switching rate of the classical noise.

Properties on the distant distribution of entanglement for arbitrary two-qubit pure states via noisy quantum channels

This paper investigates the change of entanglement for transmitting an arbitrarily entangled two-qubit pure state via one of three typical kinds of noisy quantum channels： amplitude damping quantum channel, phase damping quantum channel and depolarizing quantum channel. It finds, in all these three cases, that the output distant entanglement （measured by concurrence） reduces proportionately with respect to its initial amount, and the decaying ratio is determined only by the noisy characteristics of quantum channels and independent of the form of initial input state.

A practical two-way system of quantum key distribution with untrusted source

The most severe problem of a two-way ＂plug-and-play＂ （p ＆： p） quantum key distribution system is that the source can be controlled by the eavesdropper. This kind of source is defined as an ＂untrusted source＂. This paper discusses the effects of the fluctuation of internal transmittance on the final key generation rate and the transmission distance. The security of the standard BB84 protocol, one-decoy state protocol, and weak＋vacuum decoy state protocol, with untrusted sources and the fluctuation of internal transmittance are studied. It is shown that the one-decoy state is sensitive to the statistical fluctuation but weak＋vacuum decoy state is only slightly affected by the fluctuation. It is also shown that both the maximum secure transmission distance and final key generation rate are reduced when Alice＇s laboratory transmittance fluctuation is considered.