We investigate the nonlocal transport modulated by Coulomb interactions in devices comprising two interacting Majorana wires,where both nanowires are in proximity to a mesoscopic superconducting(SC)island.Each Majoran...We investigate the nonlocal transport modulated by Coulomb interactions in devices comprising two interacting Majorana wires,where both nanowires are in proximity to a mesoscopic superconducting(SC)island.Each Majorana bound state(MBS)is coupled to one lead via a quantum dot with resonant levels.In this device,the nonlocal correlations can be induced in the absence of Majorana energy splitting.We find that the negative differential conductance and giant current noise cross correlation could be induced,due to the interplay between nonlocality of MBSs and dynamical Coulomb blockade effect.This feature may provide a signature for the existence of the MBSs.展开更多
In this work,for the first time,we have analyzed and compared the responses of polar mesosphere winter echoes(PMWE)and their summer counterpart,polar mesosphere summer echoes(PMSE),to high-frequency(HF)heating in term...In this work,for the first time,we have analyzed and compared the responses of polar mesosphere winter echoes(PMWE)and their summer counterpart,polar mesosphere summer echoes(PMSE),to high-frequency(HF)heating in terms of modulated characteristics(i.e.,backscatter intensity reduction,recovery,and overshoot).Both PMWE and PMSE observations were from the same site(Tromsφ,Norway;69.6°N,19.2°E)and radar(EISCAT[European Incoherent Scatter Scientific Association]very high frequency,224 MHz).The heating patterns of both PMWE and PMSE were found to be similar;however,PMSE was more greatly affected by HF heating.Polar mesosphere summer echoes showed recovery and overshoot more frequently than did PMWE.In addition,the mean recovery and overshoot of PMSE were greater than those of PMWE.The associated electron temperature enhancement was estimated for both PMWE and PMSE and showed that,compared with PMWE,the electron temperature enhancement was more significant in PMSE.The strong heating effects on PMSE may be due to the considerable increase in electron temperature.展开更多
When the GaAs/AlGaAs superlattice-based devices are used under irradiation environments, point defects may be created and ultimately deteriorate their electronic and transport properties. Thus, understanding the prope...When the GaAs/AlGaAs superlattice-based devices are used under irradiation environments, point defects may be created and ultimately deteriorate their electronic and transport properties. Thus, understanding the properties of point defects like vacancies and interstitials is essential for the successful application of semiconductor materials. In the present study, first-principles calculations are carried out to explore the stability of point defects in GaAs/Al_(0.5)Ga_(0.5)As superlattice and their effects on electronic properties. The results show that the interstitial defects and Frenkel pair defects are relatively difficult to form, while the antisite defects are favorably created generally. Besides, the existence of point defects generally modifies the electronic structure of GaAs/Al_(0.5)Ga_(0.5)As superlattice significantly, and most of the defective SL structures possess metallic characteristics. Considering the stability of point defects and carrier mobility of defective states,we propose an effective strategy that AlAs, GaAs, and AlGaantisite defects are introduced to improve the hole or electron mobility of GaAs/Al_(0.5)Ga_(0.5)As superlattice. The obtained results will contribute to the understanding of the radiation damage effects of the GaAs/AlGaAs superlattice, and provide a guidance for designing highly stable and durable semiconductor superlattice-based electronics and optoelectronics for extreme environment applications.展开更多
Semiconductor-based solar-driven water splitting technology is an environmentally friendly and cost-effective approach for the production of clean fuels.The overall solar-to-hydrogen efficiency of semiconductorbased p...Semiconductor-based solar-driven water splitting technology is an environmentally friendly and cost-effective approach for the production of clean fuels.The overall solar-to-hydrogen efficiency of semiconductorbased photo(electro)catalysts is jointly determined by factors,such as light absorption efficiency of the photo(electro)catalysts,internal separation efficiency of charge carriers,and injection efficiency of surface charges.However,the traditional improvement strategies,such as morphology control,functional layer modification,and band alignment engineering,still have certain limitations in enhancing the conversion efficiency of the photo(electro)catalytic water splitting.Recently,unconventional enhancement strategies based on surface plasmonic effects,piezoelectric effects,thermoelectric effects,and magnetic effects have provided unique pathways for improving the solar-to-hydrogen efficiency of photo(electro)catalysts.Therefore,this review outlines the fundamental concepts of these physical effects and elucidates their intrinsic mechanisms in enhancing the efficiency of photo(electro)catalysts for water splitting process through practical application examples.Ultimately,the future development of unconventional strategies for enhancing photo(electro)catalytic water splitting is envisioned.展开更多
The observations of Polar Mesosphere Summer Echoes (PMSE) were carried out using the sporadic data of EISCAT UHF radar during the summer season from 2004 to 2015. There were 25 h of PMSE echoes with EISCAT UHF radar. ...The observations of Polar Mesosphere Summer Echoes (PMSE) were carried out using the sporadic data of EISCAT UHF radar during the summer season from 2004 to 2015. There were 25 h of PMSE echoes with EISCAT UHF radar. PMSE echoes were mostly observed only during the early morning and fore-noon time. Moreover, the PMSE echoes are positively correlated with Lymanα radiation, but the correlation is non-significant. The occurrence of PMSE echoes in the early morning and fore-noon time and there positive correlation with Lymanαradiation suggests that solar radiations might be one important factor for PMSE echoes in this study. Very weak positive, but statistically non-significant correlation is found between PMSE occurrence rate and the local geomagneticK-indices. It is found that there is a matching between the variation in the occurrence rate of PMSE and noctilucent clouds (NLC) up to some extent and they are positively correlated. This positive correlation might support the earlier proposed idea about the role of ice particle size in producing PMSE echoes at higher frequencies.展开更多
Two-dimensional(2D)thermoelectric(TE)materials have been widely developed;however,some 2D materials exhibit isotropic phonon,electron transport properties,and poor TE performance,which limit their application scope.Th...Two-dimensional(2D)thermoelectric(TE)materials have been widely developed;however,some 2D materials exhibit isotropic phonon,electron transport properties,and poor TE performance,which limit their application scope.Thus,exploring excellent anisotropic and ultrahigh-performance TE materials are very warranted.Herein,we first investigate the phonon thermal and TE properties of a novel 2D-connectivity ternary compound named Ga2I2S2.This paper comprehensively studies the phonon dispersion,phonon anharmonicity,lattice thermal conductivity,electronic structure,carrier mobility,Seebeck coefficient,electrical conductivity,and the dimensionless figure of merit(ZT)versus carrier concentration for 2D Ga_(2)I_(2)S_(2).We conclude that the in-plane lattice thermal conductivities of Ga_(2)I_(2)S_(2) at room temperature(300 K)are found to be 1.55 W mK^(−1) in the X-axis direction(xx-direction)and 3.82 W mK^(−1)in the Y-axis direction(yy-direction),which means its anisotropy ratio reaches 1.46.Simultaneously,the TE performance of p-type and n-type doping 2D Ga2I2S2 also shows significant anisotropy,giving rise to the ZT peak values of p-type doping in xx-and yy-directions being 0.81 and 1.99,respectively,and those of n-type doping reach ultrahigh values of 7.12 and 2.89 at 300 K,which are obviously higher than the reported values for p-type and n-type doping ternary compound Sn2BiX(ZT∼1.70 and∼2.45 at 300 K)(2020 Nano Energy 67104283).This work demonstrates that 2D Ga_(2)I_(2)S_(2) has high anisotropic TE conversion efficiency and can also be used as a new potential room-temperature TE material.展开更多
As an ideal material,bulk metallic glass(MG)has a wide range of applications because of its unique properties such as structural,functional and biomedical materials.However,it is difficult to predict the glass-forming...As an ideal material,bulk metallic glass(MG)has a wide range of applications because of its unique properties such as structural,functional and biomedical materials.However,it is difficult to predict the glass-forming ability(GFA)even given the criteria in theory and this problem greatly limits the application of bulk MG in industrial field.In this work,the proposed model uses the random forest classification method which is one of machine learning methods to solve the GFA prediction for binary metallic alloys.Compared with the previous SVM algorithm models of all features combinations,this new model is successfully constructed based on the random forest classification method with a new combination of features and it obtains better prediction results.Simultaneously,it further shows the degree of feature parameters influence on GFA.Finally,a normalized evaluation indicator of binary alloy for machine learning model performance is put forward for the first time.The result shows that the application of machine learning in MGs is valuable.展开更多
The effects of 400 keV helium ion irradiation dose and temperature on the microstructure of the Ti3SiC2 ceramic were systematically investigated by grazing incidence x-ray diffraction, scanning electron microscopy, an...The effects of 400 keV helium ion irradiation dose and temperature on the microstructure of the Ti3SiC2 ceramic were systematically investigated by grazing incidence x-ray diffraction, scanning electron microscopy, and transmission electron microscopy.The helium irradiation experiments were performed at both room temperature(RT) and 500℃ with a fluence up to 2.0 × 1017 He+/cm2 that resulted in a maximum damage of 9.6 displacements per atom.Our results demonstrate that He irradiations produce a large number of nanometer defects in Ti3SiC2 lattice and then cause the dissociation of Ti3SiC2 to TiC nano-grains with the increasing He fluence.Irradiation induced cell volume swelling of Ti3SiC2 at RT is slightly higher than that at 500℃, suggesting that Ti3SiC2 is more suitable for use in a high temperature environment.The temperature dependence of cell parameter evolution and the aggregation of He bubbles in Ti3SiC2 are different from those in Ti3AlC2.The formation of defects and He bubbles at the projected depth would induce the degradation of mechanical performance.展开更多
Oxygen ions(O;)were implanted into fused silica at a fixed fluence of 1×10^(17) ions/cm^(2) with different ion energies ranging from 10 ke V to 60 ke V.The surface roughness,optical properties,mechanical properti...Oxygen ions(O;)were implanted into fused silica at a fixed fluence of 1×10^(17) ions/cm^(2) with different ion energies ranging from 10 ke V to 60 ke V.The surface roughness,optical properties,mechanical properties and laser damage performance of fused silica were investigated to understand the effect of oxygen ion implantation on laser damage resistance of fused silica.The ion implantation accompanied with sputtering effect can passivate the sub-/surface defects to reduce the surface roughness and improve the surface quality slightly.The implanted oxygen ions can combine with the structural defects(ODCs and E′centers)to reduce the defect densities and compensate the loss of oxygen in fused silica surface under laser irradiation.Furthermore,oxygen ion implantation can reduce the Si-O-Si bond angle and densify the surface structure,thus introducing compressive stress in the surface to strengthen the surface of fused silica.Therefore,the laser induced damage threshold of fused silica increases and the damage growth coefficient decreases when ion energy up to30 ke V.However,at higher ion energy,the sputtering effect is weakened and implantation becomes dominant,which leads to the surface roughness increase slightly.In addition,excessive energy aggravates the breaking of Si-O bonds.At the same time,the density of structural defects increases and the compressive stress decreases.These will degrade the laser laser-damage resistance of fused silica.The results indicate that oxygen ion implantation with appropriate ion energy is helpful to improve the damage resistance capability of fused silica components.展开更多
The famous Kadomtsev-Petviashvili(KP)equation is a classical equation in soliton theory.A B?cklund transformation between the KP equation and the Schwarzian KP equation is demonstrated by means of the truncated Painle...The famous Kadomtsev-Petviashvili(KP)equation is a classical equation in soliton theory.A B?cklund transformation between the KP equation and the Schwarzian KP equation is demonstrated by means of the truncated Painlevéexpansion in this paper.One-parameter group transformations and one-parameter subgroup-invariant solutions for the extended KP equation are obtained.The consistent Riccati expansion(CRE)solvability of the KP equation is proved.Some interaction structures between soliton-cnoidal waves are obtained by CRE and several evolution graphs and density graphs are plotted.展开更多
We study a forced variable-coefficient extended Korteweg-de Vries(KdV)equation in fluid dynamics with respect to internal solitary wave.Bäcklund transformations of the forced variable-coefficient extended KdV equ...We study a forced variable-coefficient extended Korteweg-de Vries(KdV)equation in fluid dynamics with respect to internal solitary wave.Bäcklund transformations of the forced variable-coefficient extended KdV equation are demonstrated with the help of truncated Painlevéexpansion.When the variable coefficients are time-periodic,the wave function evolves periodically over time.Symmetry calculation shows that the forced variable-coefficient extended KdV equation is invariant under the Galilean transformations and the scaling transformations.One-parameter group transformations and one-parameter subgroup invariant solutions are presented.Cnoidal wave solutions and solitary wave solutions of the forced variable-coefficient extended KdV equation are obtained by means of function expansion method.The consistent Riccati expansion(CRE)solvability of the forced variable-coefficient extended KdV equation is proved by means of CRE.Interaction phenomenon between cnoidal waves and solitary waves can be observed.Besides,the interaction waveform changes with the parameters.When the variable parameters are functions of time,the interaction waveform will be not regular and smooth.展开更多
In this work, the classic molecular dynamics simulations are employed to investigate the atomic structural modification of fused silica with defects as laser irradiation. The dynamics evolution of the atomic structure...In this work, the classic molecular dynamics simulations are employed to investigate the atomic structural modification of fused silica with defects as laser irradiation. The dynamics evolution of the atomic structure of fused silica is modeled during energy deposition. The structure parameters such as pair distribution functions(PDFs), bond angle distributions(BADs), and the coordination number are given. The calculated results reveal that fused silica undergoes significant changes in terms of Si-O, Si-Si, and O-O bond lengths, Si-O-Si and O-Si-O bond angles, and the Si and O coordination numbers during laser irradiation. The effects of different surface defects on the microstructure of fused silica are discussed too. The simulation results of molecular dynamics may help to understand the role of defects in the radiation effect of fused silica.展开更多
Quantum correlation plays a critical role in the maintenance of quantum information processing and nanometer device design.In the past two decades,several quantitative methods had been proposed to study the quantum co...Quantum correlation plays a critical role in the maintenance of quantum information processing and nanometer device design.In the past two decades,several quantitative methods had been proposed to study the quantum correlation of certain open quantum systems,including the geometry and entropy style discord methods.However,there are differences among these quantification methods,which promote a deep understanding of the quantum correlation.In this paper,a novel time-dependent three environmental open system model is established to study the quantum correlation.This system model interacts with two independent spin-environments(two spin-environments are connected to the other spin-environment)respectively.We have calculated and compared the changing properties of the quantum correlation under three kinds of geometry and two entropy discords,especially for the freezing phenomenon.At the same time,some original and novel changing behaviors of the quantum correlation under different timedependent parameters are studied,which is helpful to achieve the optimal revival of the quantum discord and the similar serrated form of the freezing phenomenon.Finally,it shows the controllability of the freezing correlation and the robustness of these methods by adjusting time-dependent parameters.This work provides a new way to control the quantum correlation and design nanospintronic devices.展开更多
For the first time,the effect of ions on complex conductivity and permittivity of dusty plasma at Polar Mesosphere Summer Echoes(PMSE)altitude is analyzed.Because of ions higher mass and smaller thermal velocity,gener...For the first time,the effect of ions on complex conductivity and permittivity of dusty plasma at Polar Mesosphere Summer Echoes(PMSE)altitude is analyzed.Because of ions higher mass and smaller thermal velocity,generally,their effects are not considered in the study of electromagnetic properties of dusty plasmas.In this study,we modified the equations of conductivity and permittivity by adding the effect of ions.In the PMSE altitude region between 80 and 90 km,a local reduction in electron density(i.e.,an electron biteout),is produced by electron absorption onto dust particles.The bite-out condition contains high dust density and smaller electron density.From simulation results in comparatively strong bite-out conditions,we found that the ion effects on conductivity become significant with smaller dust size,lower electron temperature,and lower neutral density.For comparatively weak bite-out conditions,the ion effects on conductivity become significant with larger dust size,higher electron temperature,and higher neutral density.On the other hand,for different dust sizes,electron temperatures and neutral density,the ion effects on complex permittivity become significant only in very strong bite-out conditions.Based on these simulation results,we conclude that,in the absence of electron bite-out conditions,the effect of ions on complex conductivity and permittivity is not significant and can be ignored.However,during bite-out conditions,the effect of ions becomes significant and cannot be ignored because it significantly changes the conductivity and permittivity of dusty plasmas.展开更多
<span style="font-family:Verdana;">Wearable electronic systems are able to monitor and measure multiple biophysical, biochemical signals to help researchers develop further understandings of human heal...<span style="font-family:Verdana;">Wearable electronic systems are able to monitor and measure multiple biophysical, biochemical signals to help researchers develop further understandings of human health and correlation between human performance and diseases. Driven by increasing demand for need in sports training, health monitoring and disease diagnose, bio-integrated systems are developing at a significant speed based on recent advances in material science, structure design and chemical techniques. A wide range of wearable systems are created and feature unique measuring targets, methods and soft, transparent, stretchable characters. This review summarizes the recent advances in wearable electronic technologies that also include material science, chemical science and electronic engineering. The introduction to basic wearable fundamentals covers </span><span style="font-family:Verdana;">subsequent consideration for materials, system integration and promising</span><span style="font-family:Verdana;"> platforms. Detailed classification towards their functions of physical, chemical detection is also mentioned. Strategies to achieve stretchability and promising material, AgNW, are fully discussed. This paper concludes with consideration of main challenging obstacles in this emerging filed and promises in materials that possess excellent potentials for predicted progress.</span>展开更多
Layered two-dimensional(2 D)materials have received tremendous attention due to their unique physical and chemical properties when downsized to single or few layers.Several types of layered materials,especially transi...Layered two-dimensional(2 D)materials have received tremendous attention due to their unique physical and chemical properties when downsized to single or few layers.Several types of layered materials,especially transition metal dichalcogenides(TMDs)have been demonstrated to be good electrode materials due to their interesting physical and chemical properties.Apart from TMDs,post-transition metal chalcogenides(PTMCs)recently have emerged as a family of important semiconducting materials for electrochemical studies.PTMCs are layered materials which are composed of post-transition metals raging from main group IIIA to group VA(Ga,In,Ge,Sn,Sb and Bi)and group VI chalcogen atoms(S,selenium(Se)and tellurium(Te)).Although a large number of literatures have reviewed the electrochemical and electrocatalytic applications of TMDs,less attention has been focused on PTMCs.In this review,we focus our attention on PTMCs with the aim to provide a summary to describe their fundamental electrochemical properties and electrocatalytic activity towards hydrogen evolution reaction(HER).The characteristic chemical compositions and crystal structures of PTMCs are firstly discussed,which are different from TMDs.Then,inherent electrochemistry of PTMCs is discussed to unveil the well-defined redox behaviors of PTMCs,which could potentially affect their efficiency when applied as electrode materials.Following,we focus our attention on electrocatalytic activity of PTMCs towards HER including novel synthetic strategies developed for the optimization of their HER activity.This review ends with the perspectives for the future research direction in the field of PTMC based electrocatalysts.展开更多
In this paper, a modified sub-gridding scheme that hybridizes the conventional finite-difference time-domain(FDTD)method and the unconditionally stable locally one-dimensional(LOD) FDTD is developed for analyzing ...In this paper, a modified sub-gridding scheme that hybridizes the conventional finite-difference time-domain(FDTD)method and the unconditionally stable locally one-dimensional(LOD) FDTD is developed for analyzing the periodic metallic nanoparticle arrays. The dispersion of the metal, caused by the evanescent wave propagating along the metal-dielectric interface, is expressed by the Drude model and solved with a generalized auxiliary differential equation(ADE) technique.In the sub-gridding scheme, the ADE–FDTD is applied to the global coarse grids while the ADE–LOD–FDTD is applied to the local fine grids. The time step sizes in the fine-grid region and coarse-grid region can be synchronized, and thus obviating the temporal interpolation of the fields in the time-marching process. Numerical examples about extraordinary optical transmission through the periodic metallic nanoparticle array are provided to show the accuracy and efficiency of the proposed method.展开更多
Quantum correlation shows a fascinating nature of quantum mechanics and plays an important role in some physics topics,especially in the field of quantum information.Quantum correlations of the composite system can be...Quantum correlation shows a fascinating nature of quantum mechanics and plays an important role in some physics topics,especially in the field of quantum information.Quantum correlations of the composite system can be quantified by resorting to geometric or entropy methods,and all these quantification methods exhibit the peculiar freezing phenomenon.The challenge is to find the characteristics of the quantum states that generate the freezing phenomenon,rather than only study the conditions which generate this phenomenon under a certain quantum system.In essence,this is a classification problem.Machine learning has become an effective method for researchers to study classification and feature generation.In this work,we prove that the machine learning can solve the problem of X form quantum states,which is a problem of physical significance.Subsequently,we apply the density-based spatial clustering of applications with noise(DBSCAN)algorithm and the decision tree to divide quantum states into two different groups.Our goal is to classify the quantum correlations of quantum states into two classes:one is the quantum correlation with freezing phenomenon for both Rènyi discord(α=2)and the geometric discord(Bures distance),the other is the quantum correlation of non-freezing phenomenon.The results demonstrate that the machine learning method has reasonable performance in quantum correlation research.展开更多
Polar mesosphere summer echoes(PMSEs)are very strong radar echoes in the polar mesopause in local summer.Here we present the frequency dependence of the volume reflectivity and the effect of energetic particle precipi...Polar mesosphere summer echoes(PMSEs)are very strong radar echoes in the polar mesopause in local summer.Here we present the frequency dependence of the volume reflectivity and the effect of energetic particle precipitation on modulated PMSEs by using PMSEs observations carried out by European Incoherent SCATter(EISCAT)heating equipment simultaneously with very high frequency(VHF)radar and ultra high frequency(UHF)radar on 12 July 2007.According to the experimental observations,the PMSEs occurrence rate at VHF was much higher than that at UHF,and the altitude of the PMSEs maximum observed at VHF was higher than that at UHF.Overlapping regions were observed by VHF radar between high energetic particle precipitation and the PMSEs.In addition,highfrequency heating had a very limited impact on PMSEs when the UHF electron density was enhanced because of energetic particle precipitation.In addition,an updated qualitative method was used to study the relationship between volume reflectivity and frequency.The volume reflectivity was found to be inversely proportional to the fourth power of radar frequency.The theoretical and experimental results provide a definitive data foundation for further analysis and investigation of the physical mechanism of PMSEs.展开更多
Nonlayered two-dimensional(2D)materials have attracted increasing attention,due to novel physical properties,unique surface structure,and high compatibility with microfabrication technique.However,owing to the inheren...Nonlayered two-dimensional(2D)materials have attracted increasing attention,due to novel physical properties,unique surface structure,and high compatibility with microfabrication technique.However,owing to the inherent strong covalent bonds,the direct synthesis of 2D planar structure from nonlayered materials,especially for the realization of large-size ultrathin 2D nonlayered materials,is still a huge challenge.Here,a general atomic substitution conversion strategy is proposed to synthesize large-size,ultrathin nonlayered 2D materials.Taking nonlayered CdS as a typical example,large-size ultrathin nonlayered CdS single-crystalline flakes are successfully achieved via a facile low-temperature chemical sulfurization method,where pre-grown layered CdI2 flakes are employed as the precursor via a simple hot plate assisted vertical vapor deposition method.The size and thickness of CdS flakes can be controlled by the CdI2 precursor.The growth mechanism is ascribed to the chemical substitution reaction from I to S atoms between CdI2 and CdS,which has been evidenced by experiments and theoretical calculations.The atomic substitution conversion strategy demonstrates that the existing 2D layered materials can serve as the precursor for difficult-to-synthesize nonlayered 2D materials,providing a bridge between layered and nonlayered materials,meanwhile realizing the fabrication of large-size ultrathin nonlayered 2D materials.展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.12074209 and 12274063)the Fundamental Research Funds for the Central Universities(Grant No.ZYGX2019J100)the Open Project of State Key Laboratory of Low-Dimensional Quantum Physics(Grant No.KF202008)。
文摘We investigate the nonlocal transport modulated by Coulomb interactions in devices comprising two interacting Majorana wires,where both nanowires are in proximity to a mesoscopic superconducting(SC)island.Each Majorana bound state(MBS)is coupled to one lead via a quantum dot with resonant levels.In this device,the nonlocal correlations can be induced in the absence of Majorana energy splitting.We find that the negative differential conductance and giant current noise cross correlation could be induced,due to the interplay between nonlocality of MBSs and dynamical Coulomb blockade effect.This feature may provide a signature for the existence of the MBSs.
基金supported by the National Natural Science Foundation of China(No.62271113,62201529)the National Key Laboratory of Electromagnetic Environment(No.202102010)the Natural Science Foundation of Sichuan Province(No.2022NSFSC1848).
文摘In this work,for the first time,we have analyzed and compared the responses of polar mesosphere winter echoes(PMWE)and their summer counterpart,polar mesosphere summer echoes(PMSE),to high-frequency(HF)heating in terms of modulated characteristics(i.e.,backscatter intensity reduction,recovery,and overshoot).Both PMWE and PMSE observations were from the same site(Tromsφ,Norway;69.6°N,19.2°E)and radar(EISCAT[European Incoherent Scatter Scientific Association]very high frequency,224 MHz).The heating patterns of both PMWE and PMSE were found to be similar;however,PMSE was more greatly affected by HF heating.Polar mesosphere summer echoes showed recovery and overshoot more frequently than did PMWE.In addition,the mean recovery and overshoot of PMSE were greater than those of PMWE.The associated electron temperature enhancement was estimated for both PMWE and PMSE and showed that,compared with PMWE,the electron temperature enhancement was more significant in PMSE.The strong heating effects on PMSE may be due to the considerable increase in electron temperature.
基金Project supported by the NSAF Joint Foundation of China (Grant No. U1930120)the Key Natural Science Foundation of Gansu Province, China (Grant No. 20JR5RA211)the National Natural Science Foundation of China (Grant No. 11774044)。
文摘When the GaAs/AlGaAs superlattice-based devices are used under irradiation environments, point defects may be created and ultimately deteriorate their electronic and transport properties. Thus, understanding the properties of point defects like vacancies and interstitials is essential for the successful application of semiconductor materials. In the present study, first-principles calculations are carried out to explore the stability of point defects in GaAs/Al_(0.5)Ga_(0.5)As superlattice and their effects on electronic properties. The results show that the interstitial defects and Frenkel pair defects are relatively difficult to form, while the antisite defects are favorably created generally. Besides, the existence of point defects generally modifies the electronic structure of GaAs/Al_(0.5)Ga_(0.5)As superlattice significantly, and most of the defective SL structures possess metallic characteristics. Considering the stability of point defects and carrier mobility of defective states,we propose an effective strategy that AlAs, GaAs, and AlGaantisite defects are introduced to improve the hole or electron mobility of GaAs/Al_(0.5)Ga_(0.5)As superlattice. The obtained results will contribute to the understanding of the radiation damage effects of the GaAs/AlGaAs superlattice, and provide a guidance for designing highly stable and durable semiconductor superlattice-based electronics and optoelectronics for extreme environment applications.
基金Research start-up funding in Yangtze Delta Region Institute of UESTC,Grant/Award Numbers:U03220088,U03220089,U032200106,U032200107Young Leading Talents of Nantaihu Talent Program in Huzhou(2022)。
文摘Semiconductor-based solar-driven water splitting technology is an environmentally friendly and cost-effective approach for the production of clean fuels.The overall solar-to-hydrogen efficiency of semiconductorbased photo(electro)catalysts is jointly determined by factors,such as light absorption efficiency of the photo(electro)catalysts,internal separation efficiency of charge carriers,and injection efficiency of surface charges.However,the traditional improvement strategies,such as morphology control,functional layer modification,and band alignment engineering,still have certain limitations in enhancing the conversion efficiency of the photo(electro)catalytic water splitting.Recently,unconventional enhancement strategies based on surface plasmonic effects,piezoelectric effects,thermoelectric effects,and magnetic effects have provided unique pathways for improving the solar-to-hydrogen efficiency of photo(electro)catalysts.Therefore,this review outlines the fundamental concepts of these physical effects and elucidates their intrinsic mechanisms in enhancing the efficiency of photo(electro)catalysts for water splitting process through practical application examples.Ultimately,the future development of unconventional strategies for enhancing photo(electro)catalytic water splitting is envisioned.
基金supported by the National Natural Science Foundation of China (Grant nos. 41104097 and 41304119)Fundamental Research Funds for the Central Universities (Grant nos. ZYGX2015J039, ZYGX2015J037, and ZYGX2015J041)
文摘The observations of Polar Mesosphere Summer Echoes (PMSE) were carried out using the sporadic data of EISCAT UHF radar during the summer season from 2004 to 2015. There were 25 h of PMSE echoes with EISCAT UHF radar. PMSE echoes were mostly observed only during the early morning and fore-noon time. Moreover, the PMSE echoes are positively correlated with Lymanα radiation, but the correlation is non-significant. The occurrence of PMSE echoes in the early morning and fore-noon time and there positive correlation with Lymanαradiation suggests that solar radiations might be one important factor for PMSE echoes in this study. Very weak positive, but statistically non-significant correlation is found between PMSE occurrence rate and the local geomagneticK-indices. It is found that there is a matching between the variation in the occurrence rate of PMSE and noctilucent clouds (NLC) up to some extent and they are positively correlated. This positive correlation might support the earlier proposed idea about the role of ice particle size in producing PMSE echoes at higher frequencies.
基金support from the National Natural Science Foundation of China[51720105007,52076031,11602149,51806031,52176166]the Fundamental Research Funds for the Central Universities[DUT19RC(3)006]the computing resources from the Supercomputer Center of Dalian University of Technology and RWTH Aachen University under project 3357.
文摘Two-dimensional(2D)thermoelectric(TE)materials have been widely developed;however,some 2D materials exhibit isotropic phonon,electron transport properties,and poor TE performance,which limit their application scope.Thus,exploring excellent anisotropic and ultrahigh-performance TE materials are very warranted.Herein,we first investigate the phonon thermal and TE properties of a novel 2D-connectivity ternary compound named Ga2I2S2.This paper comprehensively studies the phonon dispersion,phonon anharmonicity,lattice thermal conductivity,electronic structure,carrier mobility,Seebeck coefficient,electrical conductivity,and the dimensionless figure of merit(ZT)versus carrier concentration for 2D Ga_(2)I_(2)S_(2).We conclude that the in-plane lattice thermal conductivities of Ga_(2)I_(2)S_(2) at room temperature(300 K)are found to be 1.55 W mK^(−1) in the X-axis direction(xx-direction)and 3.82 W mK^(−1)in the Y-axis direction(yy-direction),which means its anisotropy ratio reaches 1.46.Simultaneously,the TE performance of p-type and n-type doping 2D Ga2I2S2 also shows significant anisotropy,giving rise to the ZT peak values of p-type doping in xx-and yy-directions being 0.81 and 1.99,respectively,and those of n-type doping reach ultrahigh values of 7.12 and 2.89 at 300 K,which are obviously higher than the reported values for p-type and n-type doping ternary compound Sn2BiX(ZT∼1.70 and∼2.45 at 300 K)(2020 Nano Energy 67104283).This work demonstrates that 2D Ga_(2)I_(2)S_(2) has high anisotropic TE conversion efficiency and can also be used as a new potential room-temperature TE material.
基金supported by the National Key R&D Program of China,Grant No.2018YFA0306703.
文摘As an ideal material,bulk metallic glass(MG)has a wide range of applications because of its unique properties such as structural,functional and biomedical materials.However,it is difficult to predict the glass-forming ability(GFA)even given the criteria in theory and this problem greatly limits the application of bulk MG in industrial field.In this work,the proposed model uses the random forest classification method which is one of machine learning methods to solve the GFA prediction for binary metallic alloys.Compared with the previous SVM algorithm models of all features combinations,this new model is successfully constructed based on the random forest classification method with a new combination of features and it obtains better prediction results.Simultaneously,it further shows the degree of feature parameters influence on GFA.Finally,a normalized evaluation indicator of binary alloy for machine learning model performance is put forward for the first time.The result shows that the application of machine learning in MGs is valuable.
基金Project supported by the President Foundation of the China Academy of Engineering Physics(Grant No.YZJJLX2018003)the National Natural Science Foundation of China(Grant No.21601168)
文摘The effects of 400 keV helium ion irradiation dose and temperature on the microstructure of the Ti3SiC2 ceramic were systematically investigated by grazing incidence x-ray diffraction, scanning electron microscopy, and transmission electron microscopy.The helium irradiation experiments were performed at both room temperature(RT) and 500℃ with a fluence up to 2.0 × 1017 He+/cm2 that resulted in a maximum damage of 9.6 displacements per atom.Our results demonstrate that He irradiations produce a large number of nanometer defects in Ti3SiC2 lattice and then cause the dissociation of Ti3SiC2 to TiC nano-grains with the increasing He fluence.Irradiation induced cell volume swelling of Ti3SiC2 at RT is slightly higher than that at 500℃, suggesting that Ti3SiC2 is more suitable for use in a high temperature environment.The temperature dependence of cell parameter evolution and the aggregation of He bubbles in Ti3SiC2 are different from those in Ti3AlC2.The formation of defects and He bubbles at the projected depth would induce the degradation of mechanical performance.
基金Project supported by the National Natural Science Foundation of China(Grant No.12105037)the Key Project of National Natural Science Foundation of China-China Academy of Engineering Physics Joint Foundation(Grant No.U1830204)。
文摘Oxygen ions(O;)were implanted into fused silica at a fixed fluence of 1×10^(17) ions/cm^(2) with different ion energies ranging from 10 ke V to 60 ke V.The surface roughness,optical properties,mechanical properties and laser damage performance of fused silica were investigated to understand the effect of oxygen ion implantation on laser damage resistance of fused silica.The ion implantation accompanied with sputtering effect can passivate the sub-/surface defects to reduce the surface roughness and improve the surface quality slightly.The implanted oxygen ions can combine with the structural defects(ODCs and E′centers)to reduce the defect densities and compensate the loss of oxygen in fused silica surface under laser irradiation.Furthermore,oxygen ion implantation can reduce the Si-O-Si bond angle and densify the surface structure,thus introducing compressive stress in the surface to strengthen the surface of fused silica.Therefore,the laser induced damage threshold of fused silica increases and the damage growth coefficient decreases when ion energy up to30 ke V.However,at higher ion energy,the sputtering effect is weakened and implantation becomes dominant,which leads to the surface roughness increase slightly.In addition,excessive energy aggravates the breaking of Si-O bonds.At the same time,the density of structural defects increases and the compressive stress decreases.These will degrade the laser laser-damage resistance of fused silica.The results indicate that oxygen ion implantation with appropriate ion energy is helpful to improve the damage resistance capability of fused silica components.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11775047,11775146,and 11865013)the Science and Technology Project Foundation of Zhongshan City,China(Grant No.2017B1016).
文摘The famous Kadomtsev-Petviashvili(KP)equation is a classical equation in soliton theory.A B?cklund transformation between the KP equation and the Schwarzian KP equation is demonstrated by means of the truncated Painlevéexpansion in this paper.One-parameter group transformations and one-parameter subgroup-invariant solutions for the extended KP equation are obtained.The consistent Riccati expansion(CRE)solvability of the KP equation is proved.Some interaction structures between soliton-cnoidal waves are obtained by CRE and several evolution graphs and density graphs are plotted.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11775047,11775146,and 11865013).
文摘We study a forced variable-coefficient extended Korteweg-de Vries(KdV)equation in fluid dynamics with respect to internal solitary wave.Bäcklund transformations of the forced variable-coefficient extended KdV equation are demonstrated with the help of truncated Painlevéexpansion.When the variable coefficients are time-periodic,the wave function evolves periodically over time.Symmetry calculation shows that the forced variable-coefficient extended KdV equation is invariant under the Galilean transformations and the scaling transformations.One-parameter group transformations and one-parameter subgroup invariant solutions are presented.Cnoidal wave solutions and solitary wave solutions of the forced variable-coefficient extended KdV equation are obtained by means of function expansion method.The consistent Riccati expansion(CRE)solvability of the forced variable-coefficient extended KdV equation is proved by means of CRE.Interaction phenomenon between cnoidal waves and solitary waves can be observed.Besides,the interaction waveform changes with the parameters.When the variable parameters are functions of time,the interaction waveform will be not regular and smooth.
文摘In this work, the classic molecular dynamics simulations are employed to investigate the atomic structural modification of fused silica with defects as laser irradiation. The dynamics evolution of the atomic structure of fused silica is modeled during energy deposition. The structure parameters such as pair distribution functions(PDFs), bond angle distributions(BADs), and the coordination number are given. The calculated results reveal that fused silica undergoes significant changes in terms of Si-O, Si-Si, and O-O bond lengths, Si-O-Si and O-Si-O bond angles, and the Si and O coordination numbers during laser irradiation. The effects of different surface defects on the microstructure of fused silica are discussed too. The simulation results of molecular dynamics may help to understand the role of defects in the radiation effect of fused silica.
基金Scientific Research Starting Project of SWPU[Zheng,D.,No.0202002131604]Major Science and Technology Project of Sichuan Province[Zheng,D.,No.8ZDZX0143]+1 种基金Ministry of Education Collaborative Education Project of China[Zheng,D.,No.952]Fundamental Research Project[Zheng,D.,Nos.549,550].
文摘Quantum correlation plays a critical role in the maintenance of quantum information processing and nanometer device design.In the past two decades,several quantitative methods had been proposed to study the quantum correlation of certain open quantum systems,including the geometry and entropy style discord methods.However,there are differences among these quantification methods,which promote a deep understanding of the quantum correlation.In this paper,a novel time-dependent three environmental open system model is established to study the quantum correlation.This system model interacts with two independent spin-environments(two spin-environments are connected to the other spin-environment)respectively.We have calculated and compared the changing properties of the quantum correlation under three kinds of geometry and two entropy discords,especially for the freezing phenomenon.At the same time,some original and novel changing behaviors of the quantum correlation under different timedependent parameters are studied,which is helpful to achieve the optimal revival of the quantum discord and the similar serrated form of the freezing phenomenon.Finally,it shows the controllability of the freezing correlation and the robustness of these methods by adjusting time-dependent parameters.This work provides a new way to control the quantum correlation and design nanospintronic devices.
基金supported by the National Natural Science Foundation of China(No.61671116,61771096,11905026)National Key Research and Development Program of China(No.2019YFA0210202)Fundamental Research Funds for the Central Universities(No.ZYGX2019Z006,ZYGX2019J012).
文摘For the first time,the effect of ions on complex conductivity and permittivity of dusty plasma at Polar Mesosphere Summer Echoes(PMSE)altitude is analyzed.Because of ions higher mass and smaller thermal velocity,generally,their effects are not considered in the study of electromagnetic properties of dusty plasmas.In this study,we modified the equations of conductivity and permittivity by adding the effect of ions.In the PMSE altitude region between 80 and 90 km,a local reduction in electron density(i.e.,an electron biteout),is produced by electron absorption onto dust particles.The bite-out condition contains high dust density and smaller electron density.From simulation results in comparatively strong bite-out conditions,we found that the ion effects on conductivity become significant with smaller dust size,lower electron temperature,and lower neutral density.For comparatively weak bite-out conditions,the ion effects on conductivity become significant with larger dust size,higher electron temperature,and higher neutral density.On the other hand,for different dust sizes,electron temperatures and neutral density,the ion effects on complex permittivity become significant only in very strong bite-out conditions.Based on these simulation results,we conclude that,in the absence of electron bite-out conditions,the effect of ions on complex conductivity and permittivity is not significant and can be ignored.However,during bite-out conditions,the effect of ions becomes significant and cannot be ignored because it significantly changes the conductivity and permittivity of dusty plasmas.
文摘<span style="font-family:Verdana;">Wearable electronic systems are able to monitor and measure multiple biophysical, biochemical signals to help researchers develop further understandings of human health and correlation between human performance and diseases. Driven by increasing demand for need in sports training, health monitoring and disease diagnose, bio-integrated systems are developing at a significant speed based on recent advances in material science, structure design and chemical techniques. A wide range of wearable systems are created and feature unique measuring targets, methods and soft, transparent, stretchable characters. This review summarizes the recent advances in wearable electronic technologies that also include material science, chemical science and electronic engineering. The introduction to basic wearable fundamentals covers </span><span style="font-family:Verdana;">subsequent consideration for materials, system integration and promising</span><span style="font-family:Verdana;"> platforms. Detailed classification towards their functions of physical, chemical detection is also mentioned. Strategies to achieve stretchability and promising material, AgNW, are fully discussed. This paper concludes with consideration of main challenging obstacles in this emerging filed and promises in materials that possess excellent potentials for predicted progress.</span>
基金financial support from the National Natural Science Foundation of China(Grant No.11774044)。
文摘Layered two-dimensional(2 D)materials have received tremendous attention due to their unique physical and chemical properties when downsized to single or few layers.Several types of layered materials,especially transition metal dichalcogenides(TMDs)have been demonstrated to be good electrode materials due to their interesting physical and chemical properties.Apart from TMDs,post-transition metal chalcogenides(PTMCs)recently have emerged as a family of important semiconducting materials for electrochemical studies.PTMCs are layered materials which are composed of post-transition metals raging from main group IIIA to group VA(Ga,In,Ge,Sn,Sb and Bi)and group VI chalcogen atoms(S,selenium(Se)and tellurium(Te)).Although a large number of literatures have reviewed the electrochemical and electrocatalytic applications of TMDs,less attention has been focused on PTMCs.In this review,we focus our attention on PTMCs with the aim to provide a summary to describe their fundamental electrochemical properties and electrocatalytic activity towards hydrogen evolution reaction(HER).The characteristic chemical compositions and crystal structures of PTMCs are firstly discussed,which are different from TMDs.Then,inherent electrochemistry of PTMCs is discussed to unveil the well-defined redox behaviors of PTMCs,which could potentially affect their efficiency when applied as electrode materials.Following,we focus our attention on electrocatalytic activity of PTMCs towards HER including novel synthetic strategies developed for the optimization of their HER activity.This review ends with the perspectives for the future research direction in the field of PTMC based electrocatalysts.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61471105 and 61331007)
文摘In this paper, a modified sub-gridding scheme that hybridizes the conventional finite-difference time-domain(FDTD)method and the unconditionally stable locally one-dimensional(LOD) FDTD is developed for analyzing the periodic metallic nanoparticle arrays. The dispersion of the metal, caused by the evanescent wave propagating along the metal-dielectric interface, is expressed by the Drude model and solved with a generalized auxiliary differential equation(ADE) technique.In the sub-gridding scheme, the ADE–FDTD is applied to the global coarse grids while the ADE–LOD–FDTD is applied to the local fine grids. The time step sizes in the fine-grid region and coarse-grid region can be synchronized, and thus obviating the temporal interpolation of the fields in the time-marching process. Numerical examples about extraordinary optical transmission through the periodic metallic nanoparticle array are provided to show the accuracy and efficiency of the proposed method.
基金supported by the National Natural Science Foundation of China(61502082)National Key R&D Program of China,Grant No.(2018YFA0306703).
文摘Quantum correlation shows a fascinating nature of quantum mechanics and plays an important role in some physics topics,especially in the field of quantum information.Quantum correlations of the composite system can be quantified by resorting to geometric or entropy methods,and all these quantification methods exhibit the peculiar freezing phenomenon.The challenge is to find the characteristics of the quantum states that generate the freezing phenomenon,rather than only study the conditions which generate this phenomenon under a certain quantum system.In essence,this is a classification problem.Machine learning has become an effective method for researchers to study classification and feature generation.In this work,we prove that the machine learning can solve the problem of X form quantum states,which is a problem of physical significance.Subsequently,we apply the density-based spatial clustering of applications with noise(DBSCAN)algorithm and the decision tree to divide quantum states into two different groups.Our goal is to classify the quantum correlations of quantum states into two classes:one is the quantum correlation with freezing phenomenon for both Rènyi discord(α=2)and the geometric discord(Bures distance),the other is the quantum correlation of non-freezing phenomenon.The results demonstrate that the machine learning method has reasonable performance in quantum correlation research.
基金This research was funded by the Sichuan Science and Technology Program(no.2019YJ0188)the National Natural Science Foundation of China(nos.61671116,61771096,11905026)+2 种基金the National Key Research and Development Program of China(no.2019YFA0210202)Fundamental Research Funds for the Central Universities(nos.ZYGX2019Z006,ZYGX2019J012)We are grateful to the EISCAT Scientific Association for providing the PMSE experimental data(http://portal.eiscat.se/schedule/schedule.cgi).The EISCAT Scientific Association is supported by China(China Research Institute of Radio Wave Propagation),Finland(Suomen Akatemia of Finland),Japan(the National Institute of Polar Research of Japan and Institute for Space-Earth Environmental Research at Nagoya University),Norway(Norges Forskningsråd of Norway),Sweden(the Swedish Research Council),and the UK(the Natural Environment Research Council).We also acknowledge the China Scholarship Council.
文摘Polar mesosphere summer echoes(PMSEs)are very strong radar echoes in the polar mesopause in local summer.Here we present the frequency dependence of the volume reflectivity and the effect of energetic particle precipitation on modulated PMSEs by using PMSEs observations carried out by European Incoherent SCATter(EISCAT)heating equipment simultaneously with very high frequency(VHF)radar and ultra high frequency(UHF)radar on 12 July 2007.According to the experimental observations,the PMSEs occurrence rate at VHF was much higher than that at UHF,and the altitude of the PMSEs maximum observed at VHF was higher than that at UHF.Overlapping regions were observed by VHF radar between high energetic particle precipitation and the PMSEs.In addition,highfrequency heating had a very limited impact on PMSEs when the UHF electron density was enhanced because of energetic particle precipitation.In addition,an updated qualitative method was used to study the relationship between volume reflectivity and frequency.The volume reflectivity was found to be inversely proportional to the fourth power of radar frequency.The theoretical and experimental results provide a definitive data foundation for further analysis and investigation of the physical mechanism of PMSEs.
基金This work was supported by National Natural Science Foundation of China(21825103,11774044,52072059)the Hubei Provincial Natural Science Foundation of China(2019CFA002)+1 种基金the Fundamental Research Funds for the Central Universities(2019kfyXMBZ018 and 2020kfyXJJS050)We also thank the technical support from Analytical and Testing Center in Huazhong University of Science and Technology.
文摘Nonlayered two-dimensional(2D)materials have attracted increasing attention,due to novel physical properties,unique surface structure,and high compatibility with microfabrication technique.However,owing to the inherent strong covalent bonds,the direct synthesis of 2D planar structure from nonlayered materials,especially for the realization of large-size ultrathin 2D nonlayered materials,is still a huge challenge.Here,a general atomic substitution conversion strategy is proposed to synthesize large-size,ultrathin nonlayered 2D materials.Taking nonlayered CdS as a typical example,large-size ultrathin nonlayered CdS single-crystalline flakes are successfully achieved via a facile low-temperature chemical sulfurization method,where pre-grown layered CdI2 flakes are employed as the precursor via a simple hot plate assisted vertical vapor deposition method.The size and thickness of CdS flakes can be controlled by the CdI2 precursor.The growth mechanism is ascribed to the chemical substitution reaction from I to S atoms between CdI2 and CdS,which has been evidenced by experiments and theoretical calculations.The atomic substitution conversion strategy demonstrates that the existing 2D layered materials can serve as the precursor for difficult-to-synthesize nonlayered 2D materials,providing a bridge between layered and nonlayered materials,meanwhile realizing the fabrication of large-size ultrathin nonlayered 2D materials.