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Exploration of the Current Situation and Mechanism Innovation of University Education Management under the New Situation
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作者 Yuanfei Xue Minna Sun 《Journal of Contemporary Educational Research》 2024年第10期220-226,共7页
In the new era,university education management should be oriented toward the cultivation of innovative talents and the construction of a comprehensive education system.It should develop capable and qualified higher-le... In the new era,university education management should be oriented toward the cultivation of innovative talents and the construction of a comprehensive education system.It should develop capable and qualified higher-level talents in response to the social demand for talent application,thereby enhancing the overall educational competitiveness of universities and driving deep reforms in educational activities.However,in current educational practice,efficient educational management often focuses on curriculum development and cultural education,with insufficient attention paid to the development of students’comprehensive literacy.The talent cultivation and education programs are not yet perfect.This article explores the current situation of university education management activities under the new situation and considers practical methods for innovating university education management mechanisms. 展开更多
关键词 University education management New situation Talent cultivation
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Research on Innovation of Fair Competition Review System in Shenzhen
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作者 WANG Yu LI Changsheng 《Management Studies》 2023年第4期202-214,共13页
The Shenzhen Fair Competition Review System has experienced internal review and cross-examination since its inception.However,it is still dominated by the self-review of policy-making organs,with a lack of effective c... The Shenzhen Fair Competition Review System has experienced internal review and cross-examination since its inception.However,it is still dominated by the self-review of policy-making organs,with a lack of effective control and restraint mechanisms.In addition,insufficient compensatory effect of the external review has led to weak effectiveness of social supervision.Shenzhen is currently the pilot of an independent fair competition review system.The Fair Competition Commission can be set up as an independent review body.Then,the operational mechanism should be improved and the constraints and incentives should be set up scientifically.Last but not the least,by strengthening the social supervision network for fair competition review,the legality and rationality of a wide range of local regulations,rules,and normative documents will be reviewed,thereby regulating the behavior of policy-making organs. 展开更多
关键词 independent review review agency restraint mechanisms
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Audio-Text Multimodal Speech Recognition via Dual-Tower Architecture for Mandarin Air Traffic Control Communications
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作者 Shuting Ge Jin Ren +3 位作者 Yihua Shi Yujun Zhang Shunzhi Yang Jinfeng Yang 《Computers, Materials & Continua》 SCIE EI 2024年第3期3215-3245,共31页
In air traffic control communications (ATCC), misunderstandings between pilots and controllers could result in fatal aviation accidents. Fortunately, advanced automatic speech recognition technology has emerged as a p... In air traffic control communications (ATCC), misunderstandings between pilots and controllers could result in fatal aviation accidents. Fortunately, advanced automatic speech recognition technology has emerged as a promising means of preventing miscommunications and enhancing aviation safety. However, most existing speech recognition methods merely incorporate external language models on the decoder side, leading to insufficient semantic alignment between speech and text modalities during the encoding phase. Furthermore, it is challenging to model acoustic context dependencies over long distances due to the longer speech sequences than text, especially for the extended ATCC data. To address these issues, we propose a speech-text multimodal dual-tower architecture for speech recognition. It employs cross-modal interactions to achieve close semantic alignment during the encoding stage and strengthen its capabilities in modeling auditory long-distance context dependencies. In addition, a two-stage training strategy is elaborately devised to derive semantics-aware acoustic representations effectively. The first stage focuses on pre-training the speech-text multimodal encoding module to enhance inter-modal semantic alignment and aural long-distance context dependencies. The second stage fine-tunes the entire network to bridge the input modality variation gap between the training and inference phases and boost generalization performance. Extensive experiments demonstrate the effectiveness of the proposed speech-text multimodal speech recognition method on the ATCC and AISHELL-1 datasets. It reduces the character error rate to 6.54% and 8.73%, respectively, and exhibits substantial performance gains of 28.76% and 23.82% compared with the best baseline model. The case studies indicate that the obtained semantics-aware acoustic representations aid in accurately recognizing terms with similar pronunciations but distinctive semantics. The research provides a novel modeling paradigm for semantics-aware speech recognition in air traffic control communications, which could contribute to the advancement of intelligent and efficient aviation safety management. 展开更多
关键词 Speech-text multimodal automatic speech recognition semantic alignment air traffic control communications dual-tower architecture
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Network Defense Decision-Making Based on Deep Reinforcement Learning and Dynamic Game Theory
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作者 Huang Wanwei Yuan Bo +2 位作者 Wang Sunan Ding Yi Li Yuhua 《China Communications》 SCIE CSCD 2024年第9期262-275,共14页
Existing researches on cyber attackdefense analysis have typically adopted stochastic game theory to model the problem for solutions,but the assumption of complete rationality is used in modeling,ignoring the informat... Existing researches on cyber attackdefense analysis have typically adopted stochastic game theory to model the problem for solutions,but the assumption of complete rationality is used in modeling,ignoring the information opacity in practical attack and defense scenarios,and the model and method lack accuracy.To such problem,we investigate network defense policy methods under finite rationality constraints and propose network defense policy selection algorithm based on deep reinforcement learning.Based on graph theoretical methods,we transform the decision-making problem into a path optimization problem,and use a compression method based on service node to map the network state.On this basis,we improve the A3C algorithm and design the DefenseA3C defense policy selection algorithm with online learning capability.The experimental results show that the model and method proposed in this paper can stably converge to a better network state after training,which is faster and more stable than the original A3C algorithm.Compared with the existing typical approaches,Defense-A3C is verified its advancement. 展开更多
关键词 A3C cyber attack-defense analysis deep reinforcement learning stochastic game theory
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Female Warriors in the MCU and Wuxia Films:A Comparative Study
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作者 YE Wan-hua 《Journal of Literature and Art Studies》 2024年第5期386-394,共9页
This essay offers a comprehensive comparative analysis of female warriors in the Marvel Cinematic Universe(MCU)and Wuxia films.Both genres portray powerful and empowered female characters who defy societal expectation... This essay offers a comprehensive comparative analysis of female warriors in the Marvel Cinematic Universe(MCU)and Wuxia films.Both genres portray powerful and empowered female characters who defy societal expectations and embody resilience,effectively challenging gender norms and promoting female empowerment.However,despite their strength,many of these women warriors face certain narrative factors,such as the male gaze and a predetermined fate,which can restrict their agency and curtail their full potential.And it is within the realm of Wuxia films that the captivating element of cross-dressing among female warriors emerges,providing a nuanced exploration of identity and the constraints imposed by society. 展开更多
关键词 female warriors Marvel Cinematic Universe Wuxia films strength and agency male gaze predetermined fate cross-dressing
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Study on the Influence of Food Packaging on the Psychology of Different Groups of Consumers
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作者 CHEN Dai-yao 《Journal of Literature and Art Studies》 2024年第4期306-309,共4页
With the vigorous development of consumer culture in today’s society,various types of food packaging also appear in front of consumers in different forms.There are very big differences in food packaging in terms of s... With the vigorous development of consumer culture in today’s society,various types of food packaging also appear in front of consumers in different forms.There are very big differences in food packaging in terms of shape,color,style and other aspects of information transmission,which have the most direct impact on the audience’s food consumption needs.Driven by the consumption-oriented society,food packaging has shown very obvious comprehensive characteristics,is significantly interdisciplinary,and has close connections with other disciplines.This article will analyze and sort out the impact of food packaging on consumer psychology from different perspectives. 展开更多
关键词 packaging design food design consumer psychology
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Regulatory Issues and Countermeasures in International Financial Markets
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作者 Qi Lin 《Proceedings of Business and Economic Studies》 2024年第4期80-85,共6页
With the deepening of globalization,the development speed of capital markets is constantly accelerating,presenting a trend of globalization.At the same time,the emergence of multiple forms of trading platforms and div... With the deepening of globalization,the development speed of capital markets is constantly accelerating,presenting a trend of globalization.At the same time,the emergence of multiple forms of trading platforms and diversified financial products further highlights the competitive relationship between security exchanges and other trading platforms.While promoting the transformation of security exchange forms in various countries,it also prompts governments to re-examine the financial regulatory system of securities markets.In this situation,it is very important to research the international financial market and financial regulatory system.This article explores the regulatory issues and countermeasures in the international financial market,intending to promote the stability and healthy development of the international financial market. 展开更多
关键词 International financial markets SUPERVISION PROBLEM COUNTERMEASURE
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Path Analysis of High-Quality Development of Regional Economy The Role and Impact of Industrial Policies
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作者 Nan Zhou 《Proceedings of Business and Economic Studies》 2024年第2期198-204,共7页
With China’s economic development entering a new normal,high-quality regional economic development has become an important goal of current economic development.As one of the important means to promote high-quality de... With China’s economic development entering a new normal,high-quality regional economic development has become an important goal of current economic development.As one of the important means to promote high-quality development of the regional economy,industrial policies are increasingly receiving attention in terms of their role and impact.This article mainly conducts an in-depth analysis of the mechanism and impact path of industrial policies,exploring the role and impact of industrial policies in promoting high-quality regional economic development.Firstly,industrial policies play an important role in promoting high-quality regional economic development.Secondly,the impact path of industrial policies on the high-quality development of the regional economy mainly includes promoting industrial structure upgrading,promoting technological innovation,guiding resource allocation,and enhancing enterprise competitiveness.Therefore,it is necessary to increase research and practice on industrial policies,continuously optimize policy measures,and promote high-quality development of the regional economy. 展开更多
关键词 Industrial policy Regional economy High-quality development Path analysis
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Interactive Media Visual Interpretation of Traditional Chinese Graphics in Urban Public Spaces
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作者 Fu Zhang 《Journal of Electronic Research and Application》 2024年第3期42-46,共5页
This paper focuses on the application of interactive media technology in the visual interpretation of traditional graphic urban public spaces in China.Case studies and practical exploration show that interactive media... This paper focuses on the application of interactive media technology in the visual interpretation of traditional graphic urban public spaces in China.Case studies and practical exploration show that interactive media technologies such as projection mapping,interactive devices,virtual reality technology,etc.,have realized the diversity of traditional graphics display forms in urban public space.The rich interactive experience design enhances the sense of participation and experience of urban citizens and tourists and promotes the visual culture transmission of traditional Chinese graphics.The future urban public space exhibition is destined to continue to deepen the integration of technology and graphics,promote the visual communication of traditional Chinese graphics visual interpretation in urban public space,and promote sustainable innovation in cultural output in urban public space exhibitions around the world. 展开更多
关键词 Motion graphic design Public space Interactive media technology
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Research on the Mechanism and Strategy of Equity Investment Driving the Transformation of New Material Innovation Achievements
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作者 Xiao Zhang 《Proceedings of Business and Economic Studies》 2024年第4期136-141,共6页
Under the wave of global technological revolution,the new materials industry is facing difficulties in innovation and transformation.Equity investment has become a key driving force due to its flexible mechanism,risk ... Under the wave of global technological revolution,the new materials industry is facing difficulties in innovation and transformation.Equity investment has become a key driving force due to its flexible mechanism,risk sharing,and deep participation.Based on introducing the current development status of China’s new materials industry,this article reveals the mechanism of equity investment in financial support,risk management,incentive constraints,and resource integration.The article proposes optimization strategies,such as building an information-sharing mechanism and a diversified investment fund system,to promote the high-quality development of the new materials industry driven by innovation and provide strategic guidance for policymakers,investors,and enterprises. 展开更多
关键词 New materials industry Transformation of innovative achievements Equity investment
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Research on the Influencing Factors of College Students’Learning Experience in Livestreaming Courses
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作者 CHEN Meifen ZHANG Fang 《Psychology Research》 2023年第8期350-356,共7页
The learning experience of online courses has always been a hot topic.As livestreaming courses are online courses with real-time interaction between instructors and students,its learning experience directly affects th... The learning experience of online courses has always been a hot topic.As livestreaming courses are online courses with real-time interaction between instructors and students,its learning experience directly affects the learning behavior and effect.The evaluation indicators related to online course learning experience were combined with the attitudes of scholars,enterprise practitioners,and learners in livestreaming courses.When the questionnaire was designed,the exploratory and confirmatory factors were analyzed,the Questionnaire on Learning Experience of College Students in Livestreaming Courses was developed to evaluate the learning experience of college students attending livestreaming courses.Last but not the least,based on the survey data,important factors affecting college students’learning experience in livestreaming courses,including course content,learning environment,course interaction,and learning incentives were discussed and analyzed;strategies to optimize the learning experience in livestreaming courses were proposed. 展开更多
关键词 college students livestreaming courses learning experience influencing factor
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Analysis of the Architectural Design Talent Development Direction by Investigating the Employment Status of Architectural Design Graduates
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作者 Cuicui Qin Lijuan Xie +3 位作者 Qiliang Yu Guanhong Chen Binquan Zhang Yani Gao 《Journal of Architectural Research and Development》 2023年第6期23-28,共6页
Based on a comprehensive investigation of the employment status of architectural design graduates at a certain university,this paper analyzes the correctness of the talent development direction of architectural design... Based on a comprehensive investigation of the employment status of architectural design graduates at a certain university,this paper analyzes the correctness of the talent development direction of architectural design in hopes of pro-viding a valuable reference for further teaching reform and strengthening school-enterprise collaboration.The research re-sults show that architectural design is the main choice of graduates,accounting for as high as 63%,and traditional architec-tural design skills continue to be in demand in the market.Employment in fields such as interior design,BIM design,and green architecture is also included.The distribution of job positions for graduates is mainly in the areas of scheme design assistants and construction drawing design,requiring software operation,communication,scheme design,and construction drawing skills.This paper also proposes talent development measures such as optimizing the curriculum,strengthening faculty construction,and deepening school-enterprise collaboration,in order to improve the quality of talent development and the competitiveness of graduates. 展开更多
关键词 Employment Investigation Architectural Design Talents Development Teaching Reform
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Simulation Evaluation of Outdoor Noise Environment in Buildings
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作者 Cuicui Qin Qiliang Yu Wenyu Zou 《Journal of Architectural Research and Development》 2023年第6期55-60,共6页
Green campus design has become an essential strategy to enhance campus life and learning.However,noise pol-lution remains a troubling aspect that impacts teaching and learning processes,even causing harm to the health... Green campus design has become an essential strategy to enhance campus life and learning.However,noise pol-lution remains a troubling aspect that impacts teaching and learning processes,even causing harm to the health of students and teachers.Therefore,acoustic environment quality design is crucial.This article focuses on the expansion project of a school campus in Shenzhen.We simulated and analyzed the outdoor noise environment separately for the proposed teach-ing building,as well as the existing buildings like the dining hall,teaching building,and laboratory building.The results showed that the proposed teaching building was mainly affected by surrounding noise,with the worst outdoor noise being in classrooms adjacent to the teaching building in the south and the basketball court at the west of the classroom,with maximum noise values reaching 73 dB and 66 dB,respectively.In the future,these rooms should be renovated to achieve an excellent indoor soundproof environment. 展开更多
关键词 Green campus Outdoor noise Simulation analysis Acoustic environment
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Assessment and Optimization Strategies of Campus Sound Environment
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作者 Cuicui Qin Qiliang Yu Wei Zhang 《Journal of World Architecture》 2023年第6期51-56,共6页
A good sound environment is essential in creating a harmonious and peaceful campus,improving students’learning outcomes,promoting physical and mental health,and creating a green and healthy campus.This study investig... A good sound environment is essential in creating a harmonious and peaceful campus,improving students’learning outcomes,promoting physical and mental health,and creating a green and healthy campus.This study investigated the impact of new buildings on existing ones by optimizing the spacing between new buildings and the sound insulation structure of building enclosures.The results indicated that building 4 was affected by the noise from new building 1 and its surroundings,with a maximum outdoor daytime noise level reaching 69 dB,and the indoor background noise level in the least favorable classroom was 43.73 dB,less than 45 dB,which was within the acceptable range.It is recommended that the sound insulation design be improved in the planning of new teaching buildings.Besides,the surrounding traffic conditions should be improved,and the usage time of sports facilities should be scheduled appropriately to prevent the noise from sporting activities from affecting the classroom activities.The findings of this study provide valuable references for future architectural acoustics design and campus planning,contributing to the creation of peaceful and comfortable campus environments. 展开更多
关键词 Green campus Teaching building Noise control Acoustic optimization
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Femtosecond laser 3D printed micro objective lens for ultrathin fiber endoscope 被引量:3
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作者 Bozhe Li Changrui Liao +8 位作者 Zhihao Cai Jie Zhou Cong Zhao Liqing Jing Jiaqi Wang Cong Xiong Lei Xu Ying Wang Yiping Wang 《Fundamental Research》 CAS CSCD 2024年第1期123-130,共8页
The most important optical component in an optical fiber endoscope is its objective lens.To achieve a high imaging performance level,the development of an ultra-compact objective lens is thus the key to an ultra-thin ... The most important optical component in an optical fiber endoscope is its objective lens.To achieve a high imaging performance level,the development of an ultra-compact objective lens is thus the key to an ultra-thin optical fiber endoscope.In this work,we use femtosecond laser 3D printing to develop a series of micro objective lenses with different optical designs.The imaging resolution and field-of-view performances of these printed micro objective lenses are investigated via both simulations and experiments.For the first time,multiple micro objective lenses with different fields of view are printed on the end face of a single imaging optical fiber,thus realizing the perfect integration of an optical fiber and objective lenses.This work demonstrates the considerable potential of femtosecond laser 3D printing in the fabrication of micro-optical systems and provides a reliable solution for the development of an ultrathin fiber endoscope. 展开更多
关键词 Femtosecond laser Two-photon polymerization 3D printing Micro objective lens Fiber endoscope
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Layered coordination polymer with two-dimensional covalent bismuth-organic networks:Semiconductor and lithium ion storage
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作者 Mu-Qing Li Yulin Cao +3 位作者 Lei Qin Hua Cheng Weimin Yang Zhouguang Lu 《Nano Research》 SCIE EI CSCD 2024年第3期2181-2185,共5页
Single crystals of a bismuth-based coordination polymer(CP)with carboxyl-thiol ligands,[Bi(C_(8)H_(2)O_(4)S_(2))(C2H8N)]n(Bi-DSBDC-DMA,DMBDC=2,5-disulfur-1,4-dicarboxylate,DMA=dimethylamine),have been successfully syn... Single crystals of a bismuth-based coordination polymer(CP)with carboxyl-thiol ligands,[Bi(C_(8)H_(2)O_(4)S_(2))(C2H8N)]n(Bi-DSBDC-DMA,DMBDC=2,5-disulfur-1,4-dicarboxylate,DMA=dimethylamine),have been successfully synthesized.X-ray diffraction analysis reveals that Bi-DSBDC-DMA possesses a layered structure,with two-dimensional(2D)Bi-DSBDC networks alternating with layers composed of dimethylamine ions.This material demonstrates semiconducting properties,featuring an optical bandgap of 2.2 eV and an electrical conductivity of 2×10^(-8) S/cm.Furthermore,electrodes based on this material exhibit a capacity of 250 mAh/g after 200 cycles for lithium-ion storage. 展开更多
关键词 BISMUTH layer coordination polymer(CP) SEMICONDUCTOR lithium ion storage
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Topologically engineering of π-conjugated macrocycles: Tunable emission and photochemical reaction toward multi-cyclic polymers
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作者 Yi Liu Peng Lei +8 位作者 Yang Feng Shiwei Fu Xiaoqing Liu Siqi Zhang Bin Tu Chen Chen Yifan Li Lei Wang Qing-Dao Zeng 《Chinese Chemical Letters》 SCIE CAS CSCD 2024年第10期233-240,共8页
The topology of conjugated macrocycles had significant impacts on their photo-physical and photochemical properties.Herein,a series ofπ-conjugated macrocycles with diverse topology were synthesized via intramolecular... The topology of conjugated macrocycles had significant impacts on their photo-physical and photochemical properties.Herein,a series ofπ-conjugated macrocycles with diverse topology were synthesized via intramolecular McMurry coupling.Their chemical structure and macrocyclic topology were unambiguously confirmed via NMR,MALDI-TOF mass spectra,crystal analysis and scanning tunneling microscopy(STM).Depending on the structural topology and structural rigidity,these cyclic compounds display obviously distinctive emission behavior and photochemical reactions in the solution and in the solid state.Monocyclic phenylene vinylene macrocycle(denoted as MST)exhibiting aggregation-induced emission behavior,was more vulnerable to photo-cyclization in solution and triplet sensitizer promoted photodimerization due to lower strain and more flourishing intramolecular motions.After UV light irradiation,relatively more flexible MST could yield the anti-dimer via triplet excimer on the HOPG surface confirmed by STM investigation.By contrast,highly constrained bicyclic analogue(named as DMTPE)with central tetraphenylethene core,displayed high emission quantum yields of 68%both in solution and in the solid state,and was relatively inert to photochemical reactions and yield syn-dimer on the surface via singlet excimer involved[2+2]photo-dimerization.Based on the solution-mediated photo-polymerization of MST moiety,multicyclic porous carbon-rich ribbon connected with four-membered ring was successfully constructed and validated via STM imaging. 展开更多
关键词 Conjugated macrocycle Scanning tunneling microscopy Aggregation-induced emission PHOTOCHEMISTRY Multicyclicribbon
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Z-scheme Bi_(4)O_(5)Br_(2)/NH_(2)-MIL-125(Ti)heterojunctions enable exceptional visible photocatalytic degradation of organic pollutant
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作者 Feng Huang Muhammad Humayun +6 位作者 Gang Li Ting-Ting Fan Wen-Lin Wang Yu-Lin Cao Anton Nikiforov Chun-Dong Wang Jing Wang 《Rare Metals》 SCIE EI CAS CSCD 2024年第7期3161-3172,共12页
One key strategy to enhance photocatalytic performance is to improve the transfer and separation efficiency of photogenerated carriers by building optimized heterojunctions.Herein,novel Bi_(4)O_5Br_(2)/NH_(2)-MIL-125(... One key strategy to enhance photocatalytic performance is to improve the transfer and separation efficiency of photogenerated carriers by building optimized heterojunctions.Herein,novel Bi_(4)O_5Br_(2)/NH_(2)-MIL-125(Ti)Z-scheme heterojunctions are fabricated and used as photocatalysts for organic pollutant photodegradation.The NH_(2)-MIL-125(Ti)nanosheets are exfoliated via a self-developed alkali solution stripping approach and then uniformly decorated on Bi_(4)O_(5)Br_(2).The as-prepared Bi_(4)O_(5)Br_(2)/NH_(2)-MIL-125(Ti)presents more than 90%degradation of various pollutants,outperforming the counterpart individual ones.The various characterization results suggest that the enhanced degradation rate is due to the more intimate face-to-face interfacial contact of the lamellar Z-scheme heterojunction materials,in which the migration path of carriers from the material's interior to the surface can be reduced,in turn enhancing migration efficiency and separation capability significantly.A possible photocatalytic reaction mechanism is proposed based on the photoelectric behaviors,radical trapping experiments and liquid chromatography mass spectrometry analysis.This work promotes the development of new photocatalytic materials for heterojunctions with face-to-face interfacial contacts,as well as the effective purification of wastewater in environmental remediation. 展开更多
关键词 Z-scheme heterojunctions Photocatalysis Alkaline solution stripping Bi_(4)O_(5)Br_(2) NH_(2)-MIL-125(Ti)
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Regulation Flexibility Assessment and Optimal Aggregation Strategy of Greenhouse Loads in Modern Agricultural Parks
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作者 Shiwei Xia Liuyang Cai +3 位作者 Mingze Tong Ting Wu Peng Li Xiang Gao 《Protection and Control of Modern Power Systems》 SCIE EI 2024年第3期98-111,共14页
With advances in modern agricultural parks,the rural energy structure has undergone profound change,leading to the emergence of an agricultural energy internet.This integrated system combines agricultural energy utili... With advances in modern agricultural parks,the rural energy structure has undergone profound change,leading to the emergence of an agricultural energy internet.This integrated system combines agricultural energy utilization,the information internet,and agricultural production.Accordingly,this study proposes a regulation flexibility assessment approach and optimal aggregation strategy of greenhouse loads(GHLs)for modern agricultural parks.First,taking into account the operational characteristics of typical GHLs,refined load demand models for lighting,humidification,and temperature-controlled loads are established.Secondly,the recursive least squares method-based parameter identification method is designed to accurately determine key GHL model parameters.Finally,based on the regulation flexibility of quantitatively evaluated GHLs,GHLs are optimally aggregated into multiple flexible aggregators considering minimal operational cost and greenhouse environmental constraints.The results indicate that the proposed regulation flexibility assessment approach and optimal aggregation strategy of GHLs can alleviate the peak regulation pressure on power grids by flexibly shifting the load demands of GHLs. 展开更多
关键词 Agricultural park greenhouse load parameter identification regulation flexibility optimal aggregation of GHLs
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Fe-Ni-F electrocatalyst for enhancing reaction kinetics of water oxidation
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作者 Yi Zhang Biao Wang +6 位作者 Chao Hu Muhammad Humayun Yaping Huang Yulin Cao Mosaad Negem Yigang Ding Chundong Wang 《Chinese Journal of Structural Chemistry》 SCIE CAS CSCD 2024年第2期60-65,共6页
Highly active and low-cost oxygen evolution reaction(OER)catalytic electrodes are extremely essential for exploration of green hydrogen via water splitting.Herein,an advanced Fe-Ni-F electrocatalyst is fabricated by a... Highly active and low-cost oxygen evolution reaction(OER)catalytic electrodes are extremely essential for exploration of green hydrogen via water splitting.Herein,an advanced Fe-Ni-F electrocatalyst is fabricated by a facile annealing strategy using ammonium fluoride,of which the structure feature is unveiled by XRD,FESEM,TEM,EDS,BET,and XPS measurements.The as-prepared Fe-Ni-F addresses a low overpotential of 277 mV and a small Tafel slope of 49 mV dec^(-1)at a current density of 10 mA cm^(-2),significantly outperforming other control samples as well as the state-of-the-art RuO_(2).The advanced nature of our Fe-Ni-F catalyst could also be further evidenced from the robust stability in KOH alkaline solution,showing as 5.41%degradation after 24 h continuous working.Upon analysis,it suggests that the decent catalytic activity should be attributed to the formed bimetallic(oxy)hydroxides because of the introduction of fluoride and the synergistic effect of iron and nickel towards oxygen generation.This work represents the potential of Fe-and/or Ni-based fluoride as efficient catalyst for low-energy consumption oxygen generation. 展开更多
关键词 FLUORIDE Oxygen evolution reaction Fe-Ni-F Reaction kinetics
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